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Nano Research 2024年第3期17卷 1837-1855页

作者： jialin wang Kai Zhao Changqing Ye Yanlin Song School of Materials Science and Engineering Suzhou University of Science and TechnologySuzhou 215009China Key Laboratory of Green Printing Institute of ChemistryChinese Academy of SciencesBeijing 100190China

The booming development of wearable devices has aroused increasing interests in flexible and stretchable devices.With mechanosensory functionality,these devices are highly desirable on account of their wide range of applications in electronic skin,personal healthcare,human–machine interfaces and beyond.However,they are mostly limited by single electrical signal feedback,restricting their diverse applications in visualized mechanical sensing.Inspired by the mechanochromism of structural color materials,interactively stretchable electronics with optical and electrical dual-signal feedbacks are recently emerged as novel sensory platforms,by combining both of their sensing mechanisms and characteristics.Herein,recent studies on interactively stretchable electronics based on structural color materials are reviewed.Following a brief introduction of their basic components(i.e.,stretchable electronics and mechanochromic structural color materials),two types of interactively stretchable electronics with respect to the nanostructures of mechanochromic materials are outlined,focusing primarily on their design considerations and fabrication strategies.Finally,the main challenges and future perspectives of these emerging devices are discussed.

关键词： stretchable electronics structural color materials interactive sensing mechanochromism dual-signal feedbacks

The Mn/Yb/Er triple-doped CeO_(2) nanozyme with enhanced oxidase-like activity for highly sensitive ratiometric detection of nitrite

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Chinese Chemical Letters 2024年第6期35卷 491-495页

作者： Simin Wei Yaqing Yang Junjie Li jialin wang Jinlu Tang Ningning wang Zhaohui Li College of Chemistry Institute of Analytical Chemistry for Life ScienceHenan Joint International Research Laboratory of Green Construction of Functional Molecules and their Bioanalytical ApplicationsZhengzhou UniversityZhengzhou 450001China School of Basic Medical Sciences Zhengzhou UniversityZhengzhou 450001China

Long-term excessive intake of nitrite(NO_(2)^(-))poses a great threat to human health,needing a simple and fast method to detect NO_(2)-in food.Herein,via a simple and feasible strategy,Mn/Yb/Er triple-doped CeO_(2) nanozyme(Mn/Yb/Er/CeO_(2))was synthesized for highly sensitive ratiometric detection of nitrite.By doping Mn,Yb,Er into CeO_(2) lattice structure,Mn/Yb/Er/CeO_(2) nanozyme showed enhanced oxidase-like activity,obtaining a higher density of oxygen vacancy and a higher ratio of Ce^(3+)to Ce~(4+)than that of CeO_(2).The 3,3,5,5-tetramethylbenzidine(TMB)can be effectively oxidized by Mn/Yb/Er/CeO_(2) to produce the oxidized TMB(ox TMB),showing a significant absorption signal at 652 nm.Additionally,nitrite can react with ox TMB to produce yellow diazotized ox TMB,which is accompanied by an elevated absorption signal at 445 nm and a decreased absorption signal at 652 nm.Thus,based on the oxidase-mimetic activity of Mn/Yb/Er/CeO_(2) and the diazotization reaction between NO_(2)^(-)and ox TMB,a ratiometric colorimetric assay was established for NO_(2)^(-)detection in food.Furthermore,by integrating Mn/Yb/Er/CeO_(2) with a smartphone,a colorimetric smartphone-sensing platform was successfully fabricated for visualization and quantitative detection of NO_(2)^(-).Notably,this two-detection mode showed excellent sensitivity,selectivity,reliability and practicability in monitoring the NO_(2)^(-)in real samples,impling its great potential for food safety.

关键词： Mn/Yb/Er/CeO_(2)nanozyme Oxidase-like activity Nitrite Ratiometric detection Two-detection mode

Continuous advantage learning for minimum-time trajectory planning of autonomous vehicles

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Science China(Information Sciences) 2024年第7期67卷 285-294页

作者： Zhuo LI Weiran WU jialin wang Gang wang Jian SUN School of Automation Beijing Institute of Technology Beijing Institute of Technology Chongqing Innovation Center China Academy of Launch Vehicle Technology Intelligent Game and Decision Laboratory

This paper investigates the minimum-time trajectory planning problem of an autonomous vehicle. To deal with unknown and uncertain dynamics of the vehicle, the trajectory planning problem is modeled as a Markov decision process with a continuous action space. To solve it, we propose a continuous advantage learning(CAL) algorithm based on the advantage-value equation, and adopt a stochastic policy in the form of multivariate Gaussian distribution to encourage exploration. A shared actor-critic architecture is designed to simultaneously approximate the stochastic policy and the value function, which greatly reduces the computation burden compared to general actor-critic methods. Moreover, the shared actor-critic is updated with a loss function built as mean square consistency error of the advantage-value equation, and the update step is performed several times at each time step to improve data efficiency. Simulations validate the effectiveness of the proposed CAL algorithm and its better performance than the soft actor-critic algorithm.

关键词： trajectory planning continuous advantage learning stochastic policy shared actor-critic

Research Progress of High Entropy Ceramic Materials

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Research and Application of Materials Science 2024年第1期6卷 16-22页

作者： Song WU Shikai LIU jialin wang Bibo HAN Shaoyi SHEN Zhigang YU Zhaobo ZHANG Xinhua ZHENG School of Materials Science and Engineering Henan University of TechnologyZhengzhouHenan450001China

High-entropy materials(HEMs)have better mechanical,thermal,and electrical properties than traditional materials due to their special"high entropy effect".They can also adjust the performance of high entropy ceramics by adjusting the proportion of raw materials,and have broad application prospects in many fields.This article provides a review of the high entropy effect,preparation methods,and main applications of high entropy ceramic materials,especially exploring relevant research on high entropy perovskite ceramics.It is expected to provide reference for the promotion of scientific research and the development of further large-scale applications of high-entropy ceramic materials.

关键词： High-entropy ceramic materials high entropy effect preparation method perovskite structure research prog

Performance Analysis and Prediction for a Free-Space Optical Communication System under Foggy Absorption

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Journal of Communications and Information Networks 2023年第3期8卷 231-238页

作者： jialin wang Guanjun Xu Xiaozong Yu Zhaohui Song Shanghai Key Laboratory of Multidimensional Information Processing East China Normal UniversityShanghai 200241China Space Information Research Institute Hangzhou Dianzi UniversityHangzhou 310018China State Key Laboratory of Integrated Services Networks Xidian UniversityXi’an 710071China

We analyzed the performance of a freespace optical(FSO)system in this study,considering the combined effects of atmospheric turbulence,fog absorption,and pointing errors.The impacts of atmospheric turbulence and foggy absorption were modeled using the Fisher-Snedecor F distribution and the Gamma distribution,respectively.Next,we derived the probability density function(PDF)and cumulative probability density function of the optical system under these combined effects.Based on these statistical findings,closed-form expressions for various system metrics,such as outage probability,average bit error rate(BER),and ergodic capacity,were derived.Furthermore,we used a deep neural network(DNN)to predict the ergodic capacity of the system,achieving reduced running time and improved accuracy.Finally,the accuracy of the prediction results was validated by comparing them with the analytical results.

关键词： FSO communication foggy absorption Fisher-Snedecor F-distribution pointing errors deep learning DNN

Piezoelectrically Mediated Reactions:From Catalytic Reactions to Organic Transformations

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Chinese Journal of Chemistry 2023年第1期41卷 111-128页

作者： Ziye Ren Yuhao Peng Hanliang He Chengqiang Ding jialin wang Zhao wang Zhengbiao Zhang State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSuzhou Key Laboratory of Macromolecular Design and Precision SynthesisCollege of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhouJiangsu 215123China Suzhou Medical College Soochow UniversitySuzhouJiangsu 215123China The Department of Orthopedic Surgery Dushu Lake Hospital Affiliated to Soochow UniversitySuzhouJiangsu 215123China State Key Laboratory of Radiation Medicine and Protection Soochow UniversitySuzhouJiangsu 215123China

Recently,piezocatalysis has attracted considerable attention as a new type of renewable mechanical energy conversion technology,which relies on the strain induced polarization of the piezoelectric material.This new technology has been extensively applied in the applications of water splitting,water remediation,gas purification and tumor therapy.Despite the rapid development in the piezo-catalysis,the utilization of piezoelectric materials for synthetic purpose is still under exploration.Piezoelectric means to promote or-ganic reactions expand the scope of piezoelectrically mediated reactions and show successes in both organic and polymer synthesis.Herein,we provide a comprehensive review on recent progress of piezoelectrically mediated reactions,catalytic mechanisms and applications in the last few years.The limitations and future directions of this area are also discussed.We believe this review will provide new insights into the underlying mechanism of piezoelectric mediated electron transfer process and guide the design of new chemistry.

关键词： Piezocatalysis Heterogeneous catalysis Mechanical energy Polymerization Organic synthesis Water spilling Tumor therapy Mechanoredox Piezoelectric material

A Note on the Signature Representations of the Symmetric Groups

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Algebra Colloquium 2021年第3期28卷 469-478页

作者： Kay Jin Lim jialin wang Division of Mathematical Sciences Nanyang Technological University SPMS-04-0121 Nanyang LinkSingapore 637371Singapore

For a partition λ and a prime p,we prove a necessary and sufficient condition for there to exist a composition δ such that δ can be obtained from λ after rearrangement and no partial sums of δ are divisible by p.... 详细信息

关键词： symmetric group Schur algebra modular Kostka number

Shape/size controlling syntheses, properties and applications of two-dimensional noble metal nanocrystals

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Frontiers of Chemical Science and Engineering 2016年第3期10卷 360-382页

作者： Baozhen An Mingjie Li jialin wang Chaoxu Li Bioengineering Department College of Chemical Engineering Qingdao University of Science & Technology Qingdao 266042 China CAS Key Laboratory of Bio-based Materials Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao 266101 China

Two dimensional （2D） nanocrystals of noble metals （e.g., Au, Ag, Pt） often have unique structural and environmental properties which make them useful for applications in electronics, optics, sensors and biomedi- cines. In recent years, there has been a focus on discovering the fundamental mechanisms which govern the synthesis of the diverse geometries of these 2D metal nanocrystals （e.g., shapes, thickness, and lateral sizes）. This has resulted in being able to better control the properties of these 2D structures for specific applications. In this review, a brief historical survey of the intrinsic anisotropic properties and quantum size effects of 2D noble metal nanocrystals is given and then a summary of synthetic approaches to control their shapes and sizes is presented. The unique properties and fascinating applica- tions of these nanocrystals are also discussed.

关键词： two-dimension noble metal nanocrystal surface plasmon controllable synthesis

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金属熔融直写成形工艺射流沉积稳定性分析

机械工程学报 2024年第1期60卷 119-126页

作者：戎文娟单忠德王宝雨王佳琳王永威北京科技大学机械工程学院北京100083 中国机械科学研究总院先进成形技术与装备全国重点实验室北京100083 南京航空航天大学机电学院南京210016

金属材料增材制造具有工艺流程短、柔性可设计等优点,可满足复杂结构件单件小批量个性化需求,在众多金属增材制造工艺方法中,金属熔融直写成形具有成本低、效率高等优势。射流稳定性是影响金属熔融直写成形质量和精度的关键因素。针对... 详细信息

金属材料增材制造具有工艺流程短、柔性可设计等优点,可满足复杂结构件单件小批量个性化需求,在众多金属增材制造工艺方法中,金属熔融直写成形具有成本低、效率高等优势。射流稳定性是影响金属熔融直写成形质量和精度的关键因素。针对直写成形射流特点,分类建立了液滴流、曲张流、平滑流、波动流4种典型射流状态模型,模拟并分析了射流的演化过程,获得了修正后的金属射流连续段长度公式,以及射流沉积稳定性调控的关键因素;基于金属射流单道沉积工艺试验,获得了不同射流状态沉积后轨迹均匀性的基板速度调控范围。射流状态模型建立和沉积轨迹均匀性调控范围的获取,为金属熔融直写工艺形性调控提供理论依据。

关键词：金属增材制造金属熔融直写成形金属射流射流稳定性

锌铝合金熔融三维直写成形尺寸建模与组织分析

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中南大学学报（自然科学版） 2024年第3期55卷 918-927页

作者：戎文娟单忠德王宝雨王佳琳王永威北京科技大学机械工程学院北京100083 中国机械科学研究总院先进成形技术与装备全国重点实验室北京100083 南京航空航天大学机电学院江苏南京210016

为了实现金属熔融三维直写工艺过程的控形控性,开展锌铝合金熔融三维直写成形尺寸建模与组织分析研究。首先,以锌铝合金熔融直写的最小控制单元单道成形为研究对象,采用多元非线性回归方法拟合成形道宽,将成形特征参数w作为响应变量,D和... 详细信息

为了实现金属熔融三维直写工艺过程的控形控性,开展锌铝合金熔融三维直写成形尺寸建模与组织分析研究。首先,以锌铝合金熔融直写的最小控制单元单道成形为研究对象,采用多元非线性回归方法拟合成形道宽,将成形特征参数w作为响应变量,D和H作为预测变量,进行回归分析;其次,建立不同工艺参数下单道成形尺寸参数模型,并对模型进行拟合度校验;最后,对单道成形流固耦合过程进行数值模拟,分析典型凝固组织,通过引入熔融直写成形重熔预备时间tr,预测计算成形中层间结合效果好的工艺参数。研究结果表明:在单道成形道宽预测模型中,喷嘴直径D是影响成形道宽的第一要素,其次是喷嘴距成形底板高度H;当成形轨迹宽度近似等于凝固层宽度时,这是成形下一层的最佳时间。

关键词：金属熔融直写金属增材制造 3D打印尺寸建模微观组织