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A review on electrocatalytic CO_(2) conversion via C-C and C-N coupling

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Carbon Energy 2024年第2期6卷 167-194页

作者： Zhuangzhi Zhang Sijun Li Zheng Zhang Zhou Chen Hua wang Xianguang Meng Wenquan Cui Xiwei Qi jiacheng wang Hebei Provincial Laboratory of Inorganic Nonmetallic Materials College of Materials Science and EngineeringNorth China University of Science and TechnologyTangshanChina Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationCollege of Chemistry and Chemical EngineeringSouthwest UniversityChongqingChina State Key Laboratory of New Textile Materials and Advanced Processing Technologies Hubei Key Laboratory of Biomass Fibers and Eco-Dyeing and FinishingCollege of Chemistry and Chemical EngineeringWuhan Textile UniversityWuhanChina College of Materials Xiamen UniversityXiamenChina Hebei Iron and Steel Laboratory TangshanChina Hebei Key Laboratory for Environment Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshanChina College of Metallurgy and Energy North China University of Science and TechnologyTangshanChina State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghaiChina Institute of Electrochemistry School of Materials Science and EngineeringTaizhou UniversityTaizhouChina

Electrochemical C-C and C-N coupling reactions with the conversion of abundant and inexpensive small molecules,such as CO_(2) and nitrogencontaining species,are considered a promising route for increasing the value of CO_(2) reduction products.The development of high-performance catalysts is the key to the both electrocatalytic reactions.In this review,we present a systematic summary of the reaction systems for electrocatalytic CO_(2) reduction,along with the coupling mechanisms of C-C and C-N bonds over outstanding electrocatalytic materials recently developed.The key intermediate species and reaction pathways related to the coupling as well as the catalyst-structure relationship will be also discussed,aiming to provide insights and guidance for designing efficient CO_(2) reduction systems.

关键词： C-C coupling C-N coupling CO_(2) conversion electrocatalysis urea synthesis

Recent advances in nickel-based catalysts in eCO_(2)RR for carbon neutrality

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Carbon Energy 2024年第2期6卷 61-91页

作者： Weikang Peng Fengfeng Li Shuyi Kong Chenxi Guo Haotian Wu jiacheng wang Yi Shen Xianguang Meng Mingxi Zhang Hebei Key Laboratory of Inorganic Nonmetallic Materials School of Materials Science and EngineeringNorth China University of Science and TechnologyTangshanHebeiChina Hebei Iron and Steel Laboratory North China University of Science and TechnologyTangshanChina State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghaiChina School of Materials Science and Engineering Taizhou UniversityZhejiangChina

The excessive use of nonrenewable energy has brought about serious greenhouse effect.Converting CO_(2) into high-value-added chemicals is undoubtedly the best choice to solve energy problems.Due to the excellent cost-effectiveness and dramatic catalytic performance,nickel-based catalysts have been considered as the most promising candidates for the electrocatalytic CO_(2) reduction reaction(eCO_(2)RR).In this work,the electrocatalytic reduction mechanism of CO_(2) over Ni-based materials is reviewed.The strategies to improve the eCO_(2)RR performance are emphasized.Moreover,the research on Ni-based materials for syngas generation is briefly summarized.Finally,the prospects of nickel-based materials in the eCO_(2)RR are provided with the hope of improving transition-metal-based electrocatalysts for eCO_(2)RR in the future.

关键词： carbon energy carbon neutrality CO_(2)reduction electrocatalysis nickel-based materials

Stall Evolution Mechanism of a Centrifugal Compressor with a Wide-Long Vaneless Diffuser

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Journal of Thermal Science 2024年第3期33卷 899-913页

作者： ZHANG Lei KANG jiacheng LANG Jinhua AN Guangyao ZHANG Qian wang Longyao wang Qifang Department of Power Engineering North China Electric Power UniversityBaoding071003China Hebei Key Laboratory of Low Carbon and High Efficiency Power Generation Technology North China Electric Power UniversityBaoding071003China

The rotating stall mechanism is of high importance for the stability of centrifugal compressors and thermal power cycles.The majority of research concerning this topic has concentrated on the initial stall phase.However,the evolution of stall cells in wide-long diffusers has not been comprehensively studied.In this paper,the causes of rotating stall in the wide-long diffuser and the three-dimensional evolution mechanism of stall cells during the stall process were thoroughly analyzed.During the stall induction phase,an annulus vortex structure was found in the reverse-flow zone near the hub side of the diffuser outlet,which was the initial form of stall cells.The whole evolution process of stall cells was divided into three phases as the flow rate decreased.During the initial stall phase,the dynamic equilibrium was built under effects of the impeller wake and the adverse pressure gradient.As a result,the number of stall cells was kept at seven and the size of stall cells remained constant.During the transition phase,the flow in the diffuser became unstable.Stall cells extended to the impeller outlet,and the effect of the wake flow was strengthened significantly.Stall cells started integrating and separating regularly.As a result,the number and propagation speed of stall cells varied periodically at a constant mass flow rate.During the deep stall phase,the size of stall cells remained unchanged,and the number of stall cells kept at one.This study has important practical guidance and engineering value for the high-efficiency design and safe operation of centrifugal compressors.

关键词： centrifugal compressor wide-long vaneless diffuser stall evolution mechanism wake flow

A multiple flame-retardant,early fire-warning,and highly sensitive thread-shaped all-fabric-based piezoresistive sensor

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Science China(Technological Sciences) 2024年第4期67卷 1151-1159页

作者： LI WeiBiao ZHANG Shuai MA ShuQi wang jiacheng wang Huan YANG QiRong SONG YongTao ZHU Jie North China Institute of Aerospace Engineering Langfang 065000China Langfang Fire and Rescue Division of Hebei Province Langfang 065000China School of Information Science and Engineering Xinjiang College of Science and TechnologyKorla 841000China

In the artificial intelligence age,multifunctional and intelligent fireproof fabric-based electronics are urgently needed.Herein,a novel thread-shaped all-fabric-based piezoresistive sensor(denoted as TAFPS)with properties such as flame retardancy,firewarning,and piezoresistivity is proposed,which is composed of an inner nickel-plated fabric electrode,a multifunctional double helix fabric,and an external flame-retardant encapsulation fabric.Owing to the multiple flame-retardant properties of glass fiber tubular fabric,aminated carbon nanotubes(ACNTs),and ammonium polyphosphate,the char residue of the TAFPS reaches40.3 wt%at 800℃.In addition,the heat-sensitive effect of ACNTs during combustion causes a rapid decrease in the TAFPS resistance,triggering the fire alarm system within 2 s.Additionally,benefiting from the force-sensitive behavior of the double helix layer and tightly wrapped pattern of the external heat-shrinkable tubular fabric,TAFPS demonstrated a high sensitivity of4.40 kPa^(-1)(0–5.81 k Pa)and good stability for 10000 s.Considering its excellent flame resistance,high sensitivity,and agreeable stability,the developed TAFPS can be integrated into fire suits to monitor the exercise training process and the external fire environment.This work offers a novel approach for fabricating all-fabric-based piezoresistive sensors in the future for fire prevention and fire alarms,with promising applications in fire protection,the Internet of Things,and smart apparel.

关键词： all-fabric piezoresistive sensor multiple flame retardancy agile fire-warning high sensitivity

Vertical 3D Nanostructures Boost Efficient Hydrogen Production Coupled with Glycerol Oxidation Under Alkaline Conditions

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Nano-Micro Letters 2023年第10期15卷 609-621页

作者： Shanlin Li Danmin Liu Guowei wang Peijie Ma Xunlu wang jiacheng wang Ruguang Ma Key Laboratory of Advanced Functional Materials Ministry of EducationFaculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124People’s Republic of China The State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050People’s Republic of China School of Materials Science and Engineering Suzhou University of Science and Technology99 Xuefu RoadSuzhou 215011People’s Republic of China School of Materials Science and Engineering Taizhou UniversityTaizhou 318000People’s Republic of China Hebei Provincial Key Laboratory of Inorganic Nonmetallic Materials College of Materials Science and EngineeringNorth China University of Science and TechnologyTanshang 063210People’s Republic of China

Hydrogen production from electrolytic water is an important sustainable technology to realize renewable energy conversion and carbon neutrality.However,it is limited by the high overpotential of oxygen evolution reaction(OER)at the anode.To reduce the operating voltage of electrolyzer,herein thermodynamically favorable glycerol oxidation reaction(GOR)is proposed to replace the OER.Moreover,vertical Ni O flakes and NiMoNH nanopillars are developed to boost the reaction kinetics of anodic GOR and cathodic hydrogen evolution,respectively.Meanwhile,excluding the explosion risk of mixed H_2/O_(2),a cheap organic membrane is used to replace the expensive anion exchange membrane in the electrolyzer.Impressively,the electrolyzer delivers a remarkable reduction of operation voltage by 280 mV,and exhibits good long-term stability.This work provides a new paradigm of hydrogen production with low cost and good feasibility.

关键词： Hydrogen evolution reaction Glycerol oxidation reaction Oxygen evolution reaction Flow cell Nanostructure

Anode Interfacial Issues in Solid-State Li Batteries:Mechanistic Understanding and Mitigating Strategies

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Energy & Environmental Materials 2023年第4期6卷 384-404页

作者： jiacheng wang Liquan Chen Hong Li Fan Wu Tianmu Lake Institute of Advanced Energy Storage Technologies Liyang 213300China Henry Royce Institute and Department of Materials School of Natural SciencesThe University of ManchesterManchester M139PLUK Yangtze River Delta Physics Research Center Liyang 213300China Beijing Advanced Innovation Center for Materials Genome Engineering Key Laboratory for Renewable EnergyBeijing Key Laboratory for New Energy Materials and DevicesInstitute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China Nano Science and Technology Institute University of Science and Technology of ChinaSuzhou 215123China

All-solid-state Li metal batteries(ASSLBs)using inorganic solid electrolyte(SE)are considered promising alternatives to conventional Li-ion batteries,offering improved safety and boosted energy density.While significant progress has been made on improving the ionic conductivity of SEs,the degradation and instability of Li metal/inorganic SE interfaces have become the critical challenges that limit the coulombic efficiency,power performance,and cycling stability of ASSLBs.Understanding the mechanisms of complex/dynamic interfacial phenomena is of great importance in addressing these issues.Herein,recent studies on identifying,understanding,and solving interfacial issues on anode side in ASSLBs are comprehensively reviewed.Typical issues at Li metal/SE interface include Li dendrite growth/propagation,SE cracking,physical contact loss,and electrochemical reactions,which lead to high interfacial resistance and cell failure.The causes of these issues relating to the chemical,physical,and mechanical properties of Li metal and SEs are systematically discussed.Furthermore,effective mitigating strategies are summarized and their effects on suppressing interfacial reactions,improving interfacial Li-ion transport,maintaining interfacial contact,and stabilizing Li plating/stripping are highlighted.The in-depth mechanistic understanding of interfacial issues and complete investigations on current solutions provide foundations and guidance for future research and development to realize practical application of high-performance ASSLB.

关键词： all-solid-state Li metal batteries anode interfacial issues interface protection and modification interfacial reaction and evolution li dendrite growth

A numerical study on tread wear and fatigue damage of railway wheels subjected to anti-slip control

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Friction 2023年第8期11卷 1470-1492页

作者： Yunfan YANG Liang LING jiacheng wang Wanming ZHAI State Key Laboratory of Traction Power Southwest Jiaotong UniversityChengdu 610031China

Tread wear and rolling contact fatigue (RCF) damage propagated on railway wheels are the two extremely important focal points as they can tremendously deteriorate wheel/rail interactions and hunting stability and destroy wheel surface materials, and subsequently, cut down the lifetime of the wheels. The on-board anti-slip controllers are of essence aiming to hold back the striking slipping of the powered wheelsets under low-adhesion wheel/rail conditions. This paper intends to investigate the impact of anti-slip control on wheel tread wear and fatigue damage under diverse wheel/rail friction conditions. To this end, a prediction model for wheel wear and fatigue damage evolution on account of a comprehensive vehicle–track interaction model is extended, where the wheel/rail non-Hertzian contact algorithm is used. Furthermore, the effect of frictional wear on the fatigue damage at wheel surface is considered. The simulation results indicate that the wheel/rail contact is full-slip under the low-adhesion conditions with braking effort. The wear amount under the low-adhesion conditions is observably higher than that under the dry condition. It is further suggested that the wheel tread is prone to suffering more serious wear and fatigue damage issues with a higher anti-slip control threshold compared to that with a lower one.

关键词： anti-slip control wheel/rail non-Hertzian contact adhesion condition wheel tread wear fatigue damage

LPR-Trie: A Fast IPv6 Routing Lookup Algorithm with Virtual Nodes

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China Communications 2022年第10期19卷 1-11页

作者： Wenlong Chen Diya Liu jiacheng wang Xiaolan Tang The College of Information Engineering Capital Normal UniversityBeijing 100048China

The number of IPv6 routes in todays backbone routers has grown rapidly,which has put tremendous pressure on route lookup and storage.Based on the analysis of IPv6 address prefix length and distribution characteristics,this paper proposes an IPv6 route lookup architecture called LPR-Trie.The core idea of the algorithm is to utilize more spaces and accelerate routing lookup.Moreover,we put forward the concept of virtual nodes,and leverage the link between virtual nodes and ordinary nodes to accelerate routing lookup.We provide the longest prefix routing entry(LPR)calculation algorithm to achieve the longest prefix match.The experimental results show that the virtual node mechanism increases the search speed up to 244%,and the virtual nodes have better stability by setting an appropriate keep-alive time according to the characteristics of actual traffic.This paper shows that our design improves the routing lookup speed and have better memory utilization.

关键词： IPv6 route lookup longest prefix match virtual node Trie

Model of Surface Texture for Honed Gear Considering Motion Path and Geometrical Shape of Abrasive Particle

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Chinese Journal of Mechanical Engineering 2023年第4期36卷 311-325页

作者： Yuhu Liu Xiaohui Huang Huajun Cao jiacheng wang Huapan Xiao College of Mechanical and Vehicle Engineering Chongqing UniversityChongqing 400044China State Key Laboratory of Mechanical Transmissions Chongqing UniversityChongqing 400044China

Gear power-honing is mainly applied to finish small and medium-sized automotive gears,especially in new energy vehicles.The distinctive curved surface texture greatly improves the noise emission and service life of honed gears.The surface texture for honed gear considering the motion path and geometrical shape of abrasive particles has not been investigated.In this paper,the kinematics of the gear honing process is analyzed,and the machining marks produced by the abrasive particles of honing wheel scratching abrasive particles against the workpiece gear are calculated.The tooth surface roughness is modeled considering abrasive particle shapes and material plastic pile-ups.This results in a mathematical model that characterizes the structure of the tooth surface and the orientation of the machining marks.Experiments were used to verify the model,with a maximum relative error of less than 10%when abrasive particles are spherical.Based on this model,the effects of process parameters on the speeds of discrete points on the tooth flank,orientations of machining marks and roughness are discussed.The results show that the shaft angle between the workpiece gear and the honing wheel and the speed of the honing wheel is the main process parameters affecting the surface texture.This research proposes a surface texture model for honed gear,which can provide a theoretical basis for optimizing process parameters for gear power-honing.

关键词： Hardened gear Gear power-honing Surface texture Roughness