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Viscosity and structure relationship with equimolar substitution of CaO with MgO in the CaO–MgO–Al_(2)O_(3)–SiO_(2)slag melts

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 70-79页

作者： yong Hou Shuo Zhang Jie Dang jia Guo Hanghang Zhou Xuewei Lü College of Materials Science and Engineering Chongqing UniversityChongqing 400044China Chongqing Key Laboratory of Vanadium-Titanium Metallurgy and New Materials Chongqing UniversityChongqing 400044China

Currently,the Al_(2)O_(3)content in the high-alumina slag systems within blast furnaces is generally limited to 16wt%–18.5wt%,making it challenging to overcome this *** most studies that concentrated on managing the MgO/Al_(2)O_(3)ratio or basicity,this paper explored the effect of equimolar substitution of MgO for CaO on the viscosity and structure of a high-alumina CaO-MgO-Al_(2)O_(3)-SiO_(2)slag system,providing theoretical guidance and data to facilitate the application of high-alumina *** results revealed that the viscosity first decreased and then increased with higher MgO substitution,reaching a minimum at 15mol%MgO *** transform infrared spectroscopy(FTIR)results found that the depths of the troughs representing[SiO_(4)]tetrahedra,[AlO_(4)]tetrahedra,and Si-O-Al bending became progressively deeper with increased MgO *** of the Raman spectra showed that the average number of bridging oxygens per Si atom and the X_(Q^(3))/X_(Q^(2))(X_(Q^(i))is the molar fraction of Q^(i) unit,and i is the number of bridging oxygens in a[SiO_(4)]tetrahedral unit)ratio increased from 2.30 and 1.02 to 2.52 and 2.14,respectively,indicating a progressive polymerization of the silicate structure.X-ray photoelectron spectroscopy(XPS)results highlighted that non-bridging oxygen content decreased from 77.97mol% to 63.41mol% with increasing MgO concentration,whereas bridging oxygen and free oxygen contents *** analysis demonstrated a gradual increase in the polymerization degree of the tetrahedral structure with the increase in MgO ***,bond strength is another important factor affecting the slag *** occurrence of a viscosity minimum can be attributed to the complex evolution of bond strengths of non-bridging oxygens generated during depolymerization of the[SiO_(4)]and[AlO_(4)]tetrahedral structures by CaO and MgO.

关键词： aluminosilicate viscosity structure spectroscopy

Deciphering the role of ultra-low-loaded rhodium in NiFe-MIL-53 for superior oxygen evolution reaction

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Journal of Energy Chemistry 2025年第1期100卷 77-86页

作者： Jinzhi jia Jinhua Zhang Kailu Guo Lanyue Zhang Gening Du Hao You Junfeng Huang Mudong Tu Hua Li yong Peng Wei Dou Cailing Xu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering School of Materials and Energy Lanzhou University College of Chemistry and Chemical Engineering Luoyang Normal University

Designing highly active and stable electrocatalysts of oxygen evolution reaction （OER） is one of the crucial *** this study,a novel OER electrocatalyst,NiFe-MIL-53 modified with ultra-low rhodium（Rh@NiFe-MIL-53）,is successfully prepared via the hydrothermal ***-situ Raman spectroscopy and electrochemical impedance spectroscopy reveal that the doped Rh accelerates the phase transformation of NiFe-MIL-53 and the in-situ formed Rh@NiFeOOH is the actual active *** importantly,the enhanced reversibility of electrochemical reconstruction between NiFeOOH and NiFe（OH）2after doping Rh is beneficial for improving the electrochemical stability of the catalyst.X-ray photoelectron spectroscopy spectra show the strong electronic interaction between single-atom Rh and Ni/Fe in Rh@***,theoretical calculations confirm that the integration of single-atom Rh into the NiFeOOH successfully reduces the band gap,regulates the d-band center （εd）,accelerates the charge transfer,and optimizes the adsorption behavior of oxygen-containing intermediates,thereby lowering the energy barrier of rate-determining ***,the optimized Rh@NiFe-MIL-53 exhibits excellent OER activity （240 mV） with a small Tafel slope of 48.2 mV dec-1and long-term durability (over1270 h at 10 m A cm-2and 110 h at 200 mA cm-2).This work presents a new perspective on designing highly efficient OER electrocatalysts.

关键词： NiFe-MIL-53 Rh Electrochemical reconstruction Catalytic mechanism Oxygen evolution reaction

Merging bound states in the continuum in an open acoustic resonator

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 124-131页

作者： Lujun Huang Bin jia Artem S.Pilipchuk Sibo Huang Chen Shen Almas F.Sadreev yong Li Andrey E.Miroshnichenko School of Physics and Electronic Sciences East China Normal University Institute of Acoustics Tongji University L.V.Kirensky Institute of Physics Department of Mechanical Engineering Rowan University School of Engineering and Technology University of New South Wales at Canberra

Bound states in the continuum （BICs） are perfectly localized resonances despite embedding in the continuum ***,an isolated BIC is very sensitive to the structure ***,we report merging acoustic BICs in a single open resonator,robust against the structure *** find that both symmetry-protected BIC and Friedrich-Wintgen BIC are sustained in a single coupled waveguide-resonator *** varying the height and length of the resonator,these two BICs move toward each other and merge into a single one at a critical *** to an individual BIC,the merged BIC is robust against fabrication error because its Q-factor is proportional to ΔL-4,whereΔL embodies the structure *** essence of this extraordinary phenomenon is perfectly explained by the two-and three-level approximations of the effective nonHermitian ***,we present direct experimental demonstrations of the moving and merging of BICs in a coupled 3D waveguide-resonator,which are evidenced by the vanishing of the linewidth of Fano resonance in the transmission *** results may find exciting applications in designing high-quality acoustic sources,sensors and filters.

关键词： acoustic resonances bound state in the continuum high-Q resonances

Tree species classification in an extensive forest area using airborne hyperspectral data under varying light conditions

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Journal of Forestry Research 2023年第5期34卷 1359-1377页

作者： Wen jia yong Pang Institute of Forest Resource Information Techniques Chinese Academy of ForestryBeijing 100091People’s Republic of China Key Laboratory of Forestry Remote Sensing and Information System National Forestry and Grassland AdministrationBeijing 100091People’s Republic of China

Although airborne hyperspectral data with detailed spatial and spectral information has demonstrated significant potential for tree species classification,it has not been widely used over large areas.A comprehensive process based on multi-flightline airborne hyperspectral data is lacking over large,forested areas influenced by both the effects of bidirectional reflectance distribution function(BRDF)and cloud shadow *** this study,hyperspectral data were collected over the Mengjiagang Forest Farm in Northeast China in the summer of 2017 using the Chinese Academy of Forestry's LiDAR,CCD,and hyperspectral systems(CAF-LiCHy).After BRDF correction and cloud shadow detection processing,a tree species classification workflow was developed for sunlit and cloud-shaded forest areas with input features of minimum noise fraction reduced bands,spectral vegetation indices,and texture *** indicate that BRDF-corrected sunlit hyperspectral data can provide a stable and high classification accuracy based on representative training ***-shaded pixels also have good spectral separability for species *** red-edge spectral information and ratio-based spectral indices with high importance scores are recommended as input features for species classification under varying light *** to the classification accuracies through field survey data at multiple spatial scales,it was found that species classification within an extensive forest area using airborne hyperspectral data under various illuminations can be successfully carried out using the effective radiometric consistency process and feature selection strategy.

关键词： Tree species classification BRDF effects Cloud shadow Airborne hyperspectral data Random forest

Structural designs and mechanism insights into electrocatalytic oxidation of 5-hydroxymethylfurfural

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Journal of Energy Chemistry 2025年第1期 792-814页

作者： Jing Lei Huijie Zhang jian Yang jia Ran Jiqiang Ning Haiyan Wang yong Hu Key Laboratory of the Ministry of Education for Advanced Catalysis Materials Department of Chemistry Zhejiang Normal University Jinhua Advanced Research Institute Department of Optical Science and Engineering Fudan University College of Chemistry and Materials Engineering Zhejiang A&F University

Biomass conversion offers an efficient approach to alleviate the energy and environmental *** oxidation of 5-hydroxymethylfurfural(HMF) has attracted tremendous attention in the latest few years for the mild synthesis conditions and high conversion efficiency to obtain 2,5-furan dicarboxylic acid(FDCA), but there still remain problems such as limited yield, short cycle life,and ambiguous reaction mechanism. Despite many reviews highlighting a variety of electrocatalysts for electrochemical oxidation of HMF, a detailed discussion of the structural modulation of catalyst and the underlying catalytic mechanism is still lacking. We herein provide a comprehensive summary of the recent development of electrochemical oxidation of HMF to FDCA, particularly focusing on the mechanism studies as well as the advanced strategies developed to regulate the structure and optimize the performance of the electrocatalysts, including heterointerface construction, defect engineering,single-atom engineering, and in situ reconstruction. Experimental characterization techniques and theoretical calculation methods for mechanism and active site studies are elaborated, and challenges and future directions of electrochemical oxidation of HMF are also prospected. This review will provide guidance for designing advanced catalysts and deepening the understanding of the reaction mechanism beneath electrochemical oxidation of HMF to FDCA.

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First Eigenvalue Monotonicity for the p-Laplace Operator under the Ricci Flow

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Acta Mathematica Sinica,English Series 2011年第8期27卷 1591-1598页

作者： jia yong WU Department of Mathematics Shanghai Maritime University Shanghai 201306 P. R. China

In this note, we discuss the monotonicity of the first eigenvalue of the p-Laplace operator （p ≥2） along the Ricci flow on closed Riemannian manifolds. We prove that the first eigenvalue of the p-Laplace operator is nondecreasing along the Ricci flow under some different curvature assumptions, and therefore extend some parts of Ma＇s results [Ann. Glob. ***,29,287-292（2006）]

关键词： Ricci flow first eigenvalue p-Laplace operator monotonicity

Extending Structures for Gel'fand-Dorfman Bialgebras

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Acta Mathematica Sinica,English Series 2024年第2期40卷 619-638页

作者： jia jia WEN Yan yong HONG School of Mathematics Hangzhou Normal UniversityHangzhou 311121P.R.China

Gel'fand-Dorfman bialgebra,which is both a Lie algebra and a Novikov algebra with some compatibility condition,appeared in the study of Hamiltonian pairs in completely integrable *** also emerged in the description of a class special Lie conformal algebras called quadratic Lie conformal *** this paper,we investigate the extending structures problem for Gel'fand-Dorfman bialgebras,which is equivalent to some extending structures problem of quadratic Lie conformal ***,given a Gel'fand-Dorfman bialgebra(A,o,[.,.]),this problem is how to describe and classify all Gel'fand-Dorfman bialgebra structures on a vector space E(A⊂E)such that(A,o,[.,.])is a subalgebra of E up to an isomorphism whose restriction on A is the identity *** by the theories of extending structures for Lie algebras and Novikov algebras,we construct an object gH2(V,A)to answer the extending structures problem by introducing the notion of a unified product for Gel'fand-Dorfman bialgebras,where V is a complement of A in *** particular,we investigate the special case when dim(V)=1 in detail.

关键词： Gel'fand-Dorfman bialgebra Lie conformal algebra Extending structures problem Novikovalgebra

Modified constriction particle swarm optimization algorithm

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Journal of Systems Engineering and Electronics 2015年第5期26卷 1107-1113页

作者： Zhe Zhang Limin jia yong Qin Traffic and Transportation School Beijing Jiaotong University State Key Laboratory of Rail Traffic Control and Safety Beijing Jiaotong University Beijing Research Center of Urban Traffic Information Sensing and Service Technologies Beijing Jiaotong University

To deal with the demerits of constriction particle swarm optimization(CPSO), such as relapsing into local optima, slow convergence velocity, a modified CPSO algorithm is proposed by improving the velocity update formula of CPSO. The random velocity operator from local optima to global optima is added into the velocity update formula of CPSO to accelerate the convergence speed of the particles to the global optima and reduce the likelihood of being trapped into local optima. Finally the convergence of the algorithm is verified by calculation examples.

关键词： particle swarm optimization random speed operator convergence global optima

SIMULATION OF THE TWO PHASE FLOW OF DROPLET IMPINGEMENT ON LIQUID FILM BY THE LATTICE BOLTZMANN METHOD

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Journal of Hydrodynamics 2012年第2期24卷 292-297页

作者： GUO jia-hong WANG Xiao-yong Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai Institute of Applied Mathematics andMechanicsShanghai UniversityShanghai 200072China

A Lattice Boltzmann Method （LBM） with two-distribution functions is employed for simulating the two-phase flow induced by a liquid droplet impinging onto the film of the same liquid on solid *** model is suitable for solution of twophase flow problem at high density and viscosity ratios of liquid to vapor and phase transition between liquid and its *** roles of the vapor flow,the density ratio of liquid to vapor and the surface tension of the droplet in the splashing formation are *** is concluded that the vapour flow induced by the droplet fall and splash in the whole impinging process may affect remarkably the splash *** the case of large density ratio of liquid to vapor a crown may engender after the droplet collides with the ***,for the case of small density ratio of liquid to vapor a ＂bell＂ like splash may be observed.

关键词： droplet impact film two-phase flow Lattice Boltzmann Method (LBM) numerical simulation