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Science China Chemistry 2024年第4期67卷 1187-1192页

作者： hao Zhang Xingcong Zhang Xilun Wang Qingdi sun hao Liu Hongbing ji Xiaohui He Key Laboratory of Bioinorganic and Synthetic Chemistry of Ministry of Education Fine Chemical Industry Research InstituteSchool of ChemistryIGCMESun Yat-sen UniversityGuangzhou 510275China Huizhou Research Institute Sun Yat-sen UniversityHuizhou 516081China State Key Laboratory Breeding Base of Green-Chemical Synthesis Technology Institute of Green Petroleum Processing and Light Hydrocarbon ConversionCollege of Chemical EngineeringZhejiang University of TechnologyHangzhou 310014China

Single-atom catalysts(SACs)are considered the best candidates for olefin hydroformylation due to their combined advantages of homogeneous and heterogeneous *** conventional organo-phosphine modification,Rh SAC is modified by introducing Ca,resulting in a significant increase in activity(maximum~5.7-fold)and ***,a volcano curve between Ca addition ratio and catalytic activity is *** Ca significantly increases activity by decreasing the energy barrier,but excessive Ca decreases activity due to hindering substrate adsorption and reaction.

关键词： hydroformylation bimetallic single-atom catalysts rhodium heterogeneous catalyst

Long non-coding RNA BANCR promotes pancreatic cancer lymphangiogenesis and lymphatic metastasis by regulating the HIF-1α/VEGF-C/VEGFR-3 pathway via miR-143-5p

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Genes & Diseases 2024年第4期11卷 57-60页

作者： Shaolong hao Yu ji Weixuan Pan hao sun Fang Nie Jonathan Ray Warren Yuchuan Ding Wei Han Department of General Surgery Beijing Luhe HospitalCapital Medical UniversityTongzhouBeijing 101149China Department of Central Laboratory Beijing Luhe HospitalCapital Medical UniversityTongzhouBeijing 101149China Department of Neurosurgery Wayne State University School of MedicineJohn D.Dingell VA Medical CenterDetroitMI 48201USA

Pancreatic cancer is one of the most aggressive malignant tumors of the digestive *** node metastasis(LNM),as the main way of invasion and metastasis,can occur in the early stage of pancreatic cancer and be considered... 详细信息

关键词： metastasis cancer invasion

Fermi Blazars in the Zwicky Transient Facility Survey:Properties of Large Optical Variations

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Research in Astronomy and Astrophysics 2024年第10期24卷 104-115页

作者： Si-Si sun Zhong-Xiang Wang Shun-hao ji Department of Astronomy School of Physics and AstronomyYunnan UniversityKunming 650091China Shanghai Astronomical Observatory Chinese Academy of SciencesShanghai 200030China

We analyze the optical light curve data,obtained with the Zwicky Transient Facility(ZTF)survey,for 47 γ-ray blazars monitored by the Large Area Telescope onboard the Fermi Gamma-ray Space Telescope(Fermi).These 47sources are selected because they are among the Fermi blazars with the largest optical variations in the ZTF *** color-magnitude variation patterns are seen in them,with one being redder-to-stable-when-brighter(RSWB;in 31 sources)and the other being stable when brighter(in 16 sources).The patterns fit with the results recently reported in several similar studies with different ***,we find that the colors in the stable state of the sources share similar values,for which(after being corrected for the Galactic extinction)most sources are in a range of 0.4–*** feature could be intrinsic and may be applied in,for example,study of the intragalactic *** also determine the turning points for the sources showing the RSWB pattern,after which the color changes saturate and become *** find a correlation between optical fluxes and γ-ray fluxes at the turning *** physical implications of the correlation remain to be investigated,probably better with a sample of high-qualityγ-ray flux measurements.

关键词： (galaxies:)BL Lacertae objects:general (galaxies:)quasars:general gamma-rays:galaxies

Restricted Arc-Connectivity of Harary Digraphs

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Journal of the Operations Research Society of China 2024年第2期12卷 540-547页

作者： Jun-hao Zhang ji-Xiang Meng College of Mathematics and System Science Xinjiang UniversityUrumqi 830046XinJiangChina

The h-restricted arc-connectivity of a digraph is an important parameter to measure fault-tolerance of interconnection *** paper determines that the h-restricted arc-connectivity of the Harary digraph D=G(n;1,2,.:,k)i... 详细信息

关键词： Restricted arc-connectivity λ_(h)(D) Super-λ_(h) λ_(h)-Atom λ_(h)-Superatom

NiO-Doped Fe_(2)O_(3)/MgO Properties for the Chemical Looping Oxidative Dehydrogenation of Ethane

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China Petroleum Processing & Petrochemical Technology 2024年第1期26卷 27-33页

作者： Liang hao Chen Junjie sun jie sun Hui Shenyang Ligong University Shenyang 110159China Fushun Ecology Environment Bureau Qingyuan County Branch Fushun 113399China

Ethane chemical looping oxidative dehydrogenation(CL-ODH)to ethylene is a new technology for ethylene ***_(2)O_(3)/MgO oxygen carrier was prepared using the co-precipitation *** influence of added NiO and its different loadings on Fe_(2)O_(3)/MgO were ***,a series of oxygen carriers were applied in the CL-ODH of the ethane cycle ***-Emmett-Teller(BET),X-ray diffractometry(XRD),X-ray photoelection spectroscopy(XPS),and H2-temperature programmed reduction(TPR)were used to characterize the physicochemical properties of these oxygen *** was confirmed that an interaction between NiO and Fe_(2)O_(3) occurred based on the XPS and H2-TPR *** on the CL-ODH activity performance tests conducted in a fixed-bed reactor,it was revealed that ethylene selectivity was significantly improved after NiO ***_(2)O_(3)-10%NiO/MgO showed the best activity performance with 93%ethane conversion and 50%ethylene selectivity at a reaction temperature of 650℃,atmospheric pressure,and space velocity of 7500 mL/(g·h).

关键词： chemical looping oxidative dehydrogenation oxygen carrier Fe_(2)O_(3)/MgO NiO

Distinct effect of preparation methods on reaction efficiency of Mn-Ce/Al2O3 catalysts in low-temperature NH3-SCR

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Journal of Rare Earths 2024年第10期42卷 1865-1872页

作者： Shijie hao Yandi Cai Wei Wei Yanan Lv jiawei ji Wei Tan jingfang sun Liwei jia Changjin Tang Lin Dong State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentJiangsu Key Laboratory of Vehicle Emissions ControlCenter of Modern AnalysisKey Laboratory of Mesoscopic Chemistry of MOESchool of Chemistry and Chemical EngineeringNanjing University Wuxi Weifu Environmental Catalysts Co. Ltd. School of Environment Nanjing Normal University

In this study,a series of Mn-Ce/Al2O3catalysts was prepared by different methods of depositionprecipitation（MnCeAl-DP）,impregnation（MnCeAl-IM） and citric acid（MnCeAl-CA）,and the distinct effect of preparation methods on NOxremoval performance at low temperature was *** show that MnCeAl-DP exhibits not only the best activity but also the highest resistance against SO2/*** the assistance of comprehensive characterizations from scanning electron microscopy（SEM）,Brunauer-Emmett-Teller（BET）,X-ray diffraction（XRD）,H2-temperature programmed reduction（H2-TPR）,NH3-te mperature programmed deso rption（NH3-TPD）,and X-ray photoelectron spectroscopy（XPS）,it is revealed that the MnCeAl-DP sample owns admired features of large surface area and pore volume,enriched Mn4+and chemisorbed oxygen species originating from enhanced interaction between MnOxand CeO2,as well as improved adsorption capacity to NH3and *** these factors contribute to activity *** in-situ DRIFTS studies reveal that the improvement of NH3-SCR performance over MnCeAI-DP is related to the formation of abundant nitrate species,which is beneficial to the "NH4NO3" reaction pathway and thus enhances low-temperature activity.

关键词： Fast SCR Low temperature Mn-Ce/Al2O3 catalysts NH3-SCR NH4NO3 Rare earths

Probabilistic seismic inversion based on physics-guided deep mixture density network

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Petroleum Science 2024年第3期21卷 1611-1631页

作者： Qian-hao sun Zhao-Yun Zong Xin Li National Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)Qingdao266580ShandongChina Laoshan Laboratory Qingdao266580ShandongChina CNOOC Research Institute Ltd. Beijing100028China

Deterministic inversion based on deep learning has been widely utilized in model parameters *** by logging data,seismic data,wavelet and modeling operator,deterministic inversion based on deep learning can establish nonlinear relationships between seismic data and model ***,seismic data lacks low-frequency and contains noise,which increases the non-uniqueness of the *** conventional inversion method based on deep learning can only establish the deterministic relationship between seismic data and parameters,and cannot quantify the uncertainty of *** order to quickly quantify the uncertainty,a physics-guided deep mixture density network(PG-DMDN)is established by combining the mixture density network(MDN)with the deep neural network(DNN).Compared with Bayesian neural network(BNN)and network dropout,PG-DMDN has lower computing cost and shorter training time.A low-frequency model is introduced in the training process of the network to help the network learn the nonlinear relationship between narrowband seismic data and low-frequency *** addition,the block constraints are added to the PG-DMDN framework to improve the horizontal continuity of the inversion *** illustrate the benefits of proposed method,the PG-DMDN is compared with existing semi-supervised inversion *** synthetic data examples of Marmousi II model are utilized to quantify the influence of forward modeling part,low-frequency model,noise and the pseudo-wells number on inversion results,and prove the feasibility and stability of the proposed *** addition,the robustness and generality of the proposed method are verified by the field seismic data.

关键词： Deep learning Probabilistic inversion Physics-guided Deep mixture density network

Customer Joining Behavior and Regulation Strategy in Visible Multi-Server Queues with Synchronous Vacations of Partial Servers

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Journal of Systems Science & Complexity 2024年第3期37卷 1209-1232页

作者： sun Wei WANG hao XIE Xumeng LI Shiyong School of Economics and Management Yanshan UniversityQinhuangdao 066004China

This paper studies customer joining behavior and system regulation strategy in nonexhaustive visible M/M/m queues with synchronous vacations of a part of the *** this part of the servers are idle,they take multiple vacations simultaneously(vacation period).Until there are customers waiting in the queue,they are reactivated and all servers are busy or idle(busy period).The authors call this part of the servers as“partial servers”.In view of the fully visible queue and the almost visible queue,the authors obtain customers’equilibrium joining threshold strategies and their socially optimal joining threshold strategies,respectively,and observe that customer joining behavior in equilibrium generally makes the system overcrowded,which makes the equilibrium social welfare lower than the optimal social *** regulation,interestingly,for optimizing social welfare,the system manager hopes not only customers arriving in vacation period pay attention to the number of partial servers,but also customers arriving in busy period should care about it rather than ***,arranging more servers for vacation does not necessarily lead to the decrease of social welfare on condition that the number of partial servers is close to *** for the information advantage of the fully visible case,it is not obvious for increasing social welfare and even unfavorable to servers’profit unless the number of partial servers is big ***,given the different composition of social welfare,there exists the optimal number of partial servers and the optimal arrival rate of customers for maximizing social welfare.

关键词： Customer behavior non-exhaustive service partial servers regulation strategy synchronous vacations visible queue

A New Random Sampling Method and Its Application in Improving Progressive BKZ Algorithm

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Journal of Systems Science & Complexity 2024年第5期37卷 2262-2292页

作者： sun Minghao WANG Shixiong CHEN hao QU Longjiang College of Sciences National University of Defense Technology Academy of Military Sciences College of Information Science and Technology/Cyber Security Jinan University

Random sampling algorithm was proposed firstly by Schnorr in 2003 to find short lattice vectors, as an alternative to enumeration. The follow-up developments in random sampling were mainly proposed by Fukase and Kashiwabara in 2015 and Aono and Nguyen in 2017. Although they extended the sampling space compared to Schnorr's work through the natural number representation, they did not show how to sample specifically in practice and what vectors should be sampled, in order to find short enough lattice vectors. In this paper, the authors firstly introduce a practical random sampling algorithm under some reasonable assumptions which can find short enough lattice vectors ***, as an application of this new random sampling algorithm, the authors show that it can improve the performance of progressive BKZ algorithm in practice. Finally, the authors solve the Darmstadt's Lattice Challenge and get a series of new records in the dimension from 500 to 825, using the improved progressive BKZ algorithm.

关键词： Darmstadt’s lattice challenge lattice lattice reduction algorithm post-quantum cryptography random sampling

Process synthesis for the separation of coal-to-ethanol products

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Chinese Journal of Chemical Engineering 2024年第5期69卷 263-278页

作者： Qingping Qu Daoyan Liu hao Lyu jinsheng sun School of Chemical Engineering and Technology Tianjin UniversityTianjin 300072China Sustainable Energy and Environment Thrust The Hong Kong University of Science and Technology(Guangzhou)Nansha 511400China

The coal-to-ethanol process,as the clean coal utilization,faces challenges from the energy-intensive distillation that separates multi-component effluents for pure *** to at least eight columns,the synthesis of the ethanol distillation system is impracticable for exhaustive comparison and difficult for conventional superstructure-based optimization as rigorous models are *** work adopts a superstructure-based framework,which combines the strategy that adaptively selects branches of the state-equipment network and the parallel stochastic algorithm for process ***-performance computing significantly reduces time consumption,and the adaptive strategy substantially lowers the complexity of the superstructure ***,parallel computing,elite search,population redistribution,and retention strategies for irrelevant parameters are used to improve the optimization efficiency *** optimization terminates after 3000 generations,providing a flowsheet solution that applies two non-sharp splitting options in its distillation *** a result,the 59-dimension superstructure-based optimization was solved efficiently via a differential evolution algorithm,and a high-quality solution with a 28.34%lower total annual cost than the benchmark was ***,the solution of the superstructure-based optimization is comparable to that obtained by optimizing a single specific configuration one by *** indicates that the superstructure-based optimization that combines the adaptive strategy can be a promising approach to handling the process synthesis of large-scale and complex chemical processes.

关键词： Coal-to-ethanol Process synthesis Superstructure-based optimization Differential evolution algorithm Distillation