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Gas–solid reactor optimization based on EMMS-DPM simulation and machine learning

Particuology 2024年第6期89卷 131-143页

作者： Haolei Zhang Aiqi zhu ji Xu wei Ge State Key Laboratory of Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China Innovation Academy for Green Manufacture Chinese Academy of SciencesBeijing 100190China

Design,scaling-up,and optimization of industrial reactors mainly depend on step-by-step experiments and engineering experience,which is usually time-consuming,high cost,and high *** numerical simulation can reproduce high resolution details of hydrodynamics,thermal transfer,and reaction process in reactors,it is still challenging for industrial reactors due to huge computational *** this study,by combining the numerical simulation and artificial intelligence(AI)technology of machine learning(ML),a method is proposed to efficiently predict and optimize the performance of industrial reactors.A gas–solid fluidization reactor for the methanol to olefins process is taken as an example.1500 cases under different conditions are simulated by the coarse-grain discrete particle method based on the Energy-Minimization Multi-Scale model,and thus,the reactor performance data set is *** develop an efficient reactor performance prediction model influenced by multiple factors,the ML method is established including the ensemble learning strategy and automatic hyperparameter optimization technique,which has better performance than the methods based on the artificial neural ***,the operating conditions for highest yield of ethylene and propylene or lowest pressure drop are searched with the particle swarm optimization algorithm due to its strength to solve non-linear optimization *** show that decreasing the methanol inflow rate and increasing the catalyst inventory can maximize the yield,while decreasing methanol the inflow rate and reducing the catalyst inventory can minimize the pressure *** two objectives are thus conflicting,and the practical operations need to be compromised under different circumstance.

关键词： Discrete particle method Artificial intelligence Machine learning Particle swarm optimization Industrial reactor optimization

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The effects of ultrasound frequency and power on the activation energy in Si-KOH reaction system

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Chinese Chemical Letters 2014年第4期25卷 617-620页

作者： Qing-Bin jiao Bayanheshig Xin Tan ji-wei zhu jian-Xiang Gao Changchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of Sciences University of Chinese Academy of Sciences ChAngchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of Sciences

The activation energy is the minimum amount of energy required to initiate a reaction. It is one of the important indexes for appraising a reaction. The chemical reaction rate is closely related to the value of activation energy, and reducing activation energy is propitious to promoting a chemical reaction. In the present paper, the relationship between the activation energy in Si-KOH reaction system and the ultrasound frequency and power has been discussed for the first time. The range of ultrasound frequency and power is 40-100kHz （interval by 20kHz） and 10-50W （interval by 10W）, respectively. The experimental clata indicate that the activation energy decreases with the increasing ultrasound power. Comparing with the activation energy without ultrasound irradiation, the results in our paper indicate that ultrasound irradiation could reduce the activation energy in Si-KOH reaction system and increase the reaction rate.

关键词： Si-KOH Etching rate Ultrasonic irradiation Activation energy

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Melting geodynamics reveals a subduction origin for the Purang ophiolite,Tibet,China

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Acta Geochimica 2024年第4期43卷 754-773页

作者： Tao Ruan Zhong-jie Bai wei-Guang zhu Shi-ji Zheng State Key Laboratory of Ore Deposit Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China University of Chinese Academy of Sciences Beijing 100049China

The debate regarding whether the Yarlung-Zangbo ophiolite(YZO)on the south of the Qinghai-Tibet Plateau,formed in a mid-ocean ridge(MOR)or a supra-subduction zone(SSZ)setting has remained *** we present petrological,mineralogical,and geochemical data associated with modeling melting geodynamics of the mantle peridotites from the Purang ophiolite in the western segment of the Yarlung-Zangbo Suture Zone(YZSZ)to explore its tectonic *** Purang lherzolites are characterized by the protogranular texture and have abyssal-peridotite-like mineral compositions,including low Cr^(#)(20-30)and TiO_(2) contents(<0.1wt%)in spinel,high Al_(2)O_(3)(2.9wt%-4.4wt%)and CaO(1.9wt%-3.7wt%)contents in orthopyroxene and LREE-depletion in *** of these lherzolites can be modeled by~11%dynamic melting of the DMM source with a small fraction of melt(~0.5%)entrapped within the source,a similar melting process to typical abyssal *** Purang harzburgites are characterized by the porphyroclastic texture and exhibit highly refractory mineral compositions such as high spinel Cr^(#)(40-68),low orthopyroxene Al_(2)O_(3)(<2.2wt%)and CaO(<1.1wt%)*** in these harzburgites are enriched in Sr(up to 6.0 ppm)and LREE[(Ce)N=0.02-0.4],but depleted in Ti(200 ppm,on average)and HREE[(Yb)N<2].Importantly,the more depleted samples tend to have higher clinopyroxene Sr and LREE *** observations indicate an open-system hydrous melting with a continuous influx of slab fluid at a subduction *** modeled results show that these harzburgites could be formed by 19%-23%hydrous melting with the supply rate of slab fluid at 0.1%-1%.The lower clinopyroxene V/Sc ratios in harzburgites than those in lherzolites suggest a high oxidation stage of the melting system of harzburgites,which is consistent with a hydrous melting environment for these *** is therefore concluded that the Purang ophiolite has experienced a transformat

关键词： Melting geodynamics SSZ peridotites MOR peridotites Clinopyroxene Purang ophiolite

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Infrared microspectroscopy beamline BL06B at SSRF

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Nuclear Science and Techniques 2024年第1期35卷 10-17页

作者： Te ji Hua-Chun zhu wei-wei Peng jie Wang Hong-wei Zhao Ai-Guo Li Min Chen Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210China

The infrared microspectroscopy beamline(BL06B) is a phase Ⅱ beamline project at the Shanghai Synchrotron Radiation Facility(SSRF). The construction and optical alignment of BL06B were completed by the end of 2020. By 2021, it became accessible to users. The synchrotron radiation infrared(SRIR) source included edge radiation(ER) and bending magnet radiation(BMR). The extracted angles in the horizontal and vertical directions were 40 and 20 mrad, respectively. The photon flux, spectral resolution, and focused spot size were measured at the BL06B endstation, and the experimental results were consistent with theoretical calculations. SRIR light has a small divergence angle, high brightness, and a wide wavelength range. As a source of IR microscopy, it can easily focus on a diffraction-limited spatial resolution with a high signal-to-noise ratio(SNR). The BL06B endstation can be applied in a wide range of research fields, including materials, chemistry, biology, geophysics, and pharmacology.

关键词： Synchrotron radiation Infrared beamline Infrared microspectroscopy

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Quality assessment of friction-stir-welded aluminum alloy welds via three-dimensional force signals

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Advances in Manufacturing 2024年第1期12卷 61-75页

作者： ji-Hong Dong Yi-Ming Huang jia-Lei zhu wei Guan Xu-Kai Ren Huan-wei Yu Lei Cui Beijing Institute of Petrochemical Technology Beijing102617People’s Republic of China Beijing Academy of Safety Engineering and Technology Beijing102617People’s Republic of China AVIC Manufacturing Technology Institute Beijing100024People’s Republic of China Tianjin Key Laboratory of Advanced Joining Technology School of Materials Science and EngineeringTianjin UniversityTianjin300350People’s Republic of China Shaoxing Special Equipment Testing Institute Shaoxing Key Laboratory of Special Equipment Intelligent Testing and EvaluationShaoxing312071ZhejiangPeople’s Republic of China

An online detection technology must be developed for realizing the real-time control of friction stir *** this study,the three-dimensional force exerted on a material during friction stir welding was collected synchronously and the relationship between the forces and welding quality was *** results indicated that the fluctuation period of the traverse force was equal to that of the lateral force during the stable welding *** phase difference between two horizontal forces wasπ/*** values of the horizontal forces increased with welding speed,whereas their amplitudes remained the *** proposed force model showed that the traverse and lateral forces conformed to an elliptical curve,and this result was consistent with the behavior of the measured *** variational mode decomposition was used to process the plunge *** intrinsic mode function that represented the real fluctuation in the plunge force varied at the same frequency as the spindle rotational *** tunnel defects occurred,the fluctuation period features were consistent with those obtained during normal welding,whereas the ratio parameter defined in this study increased significantly.

关键词： Friction stir welding(FSW) Three-dimensional force model Variational mode decomposition Tunnel defect

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A Second-Order Image Denoising Model for Contrast Preservation

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Communications on Applied Mathematics and Computation 2024年第2期6卷 1406-1427页

作者： wei zhu Department of Mathematics University of AlabamaBox 870350TuscaloosaAL35487USA

In this work,we propose a second-order model for image denoising by employing a novel potential function recently developed in zhu(J Sci Comput 88:46,2021)for the design of a regularization *** to this new second-order derivative based regularizer,the model is able to alleviate the staircase effect and preserve image *** augmented Lagrangian method(ALM)is utilized to minimize the associated functional and convergence analysis is established for the proposed *** experiments are presented to demonstrate the features of the proposed model.

关键词： Image denoising Variational model Image contrast Augmented Lagrangian method(ALM)

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Soft coarse-grained particle model for particle-fluid systems

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Particuology 2024年第1期84卷 178-193页

作者： Yanhao Ye ji Xu wei Ge State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing100049China Innovation Academy for Green Manufacture Chinese Academy of SciencesBeijing100190China

By modeling a group of neighboring real particles as a single coarse-grained particle(CGP),discrete particle method(DPM)is now capable of simulating industrial-scale particle-fluid ***,a systematic approach to determine the CGP properties and develop their interaction models is still lacking,which casts uncertainty on the predictivity of the *** this study,collisions between predefined particle groups are analyzed to construct kernel functions for modeling the CGPs and then the model parameters are determined by equating the statistical properties of the CGPs and the real particles in the physical process *** approach is implemented for homogeneous cooling of granular gas,then demonstrated effective in simulating experimental fluidized beds.

关键词： Coarse-grain(CG) Discrete particle method(DPM) Fluidized bed Multi-scale simulation

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Efficient wide-bandgap perovskite solar cells with open-circuit voltage deficit below 0.4 V via hole-selective interface engineering

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Science China Chemistry 2024年第6期67卷 2102-2110页

作者： Xiaoyu ji Shuo Zhang Furong Yu Huidong Zhang Liqing Zhan Yue Hu wei-Hong zhu Yongzhen Wu Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Shanghai Key Laboratory of Functional Materials ChemistryFrontiers Science Center for Materiobiology and Dynamic ChemistryInstitute of Fine ChemicalsSchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai200237China School of Chemistry University of EdinburghKing’s BuildingsEdinburghEH93FJUK

Wide-bandgap mixed-halide perovskite solar cells(WBG-PSCs)are promising top cells for efficient tandem photovoltaics to achieve high power conversion efficiency(PCE)at low ***,the open-circuit voltage(V_(OC))of WBG-PSCs is still unsatisfactory as the V_(OC)-deficit is generally larger than 0.45 ***,we report a buried interface engineering strategy that substantially improves the V_(OC)of WBG-PSCs by inserting amphiphilic molecular hole-selective materials featuring with a cyanovinyl phosphonic acid(CPA)anchoring group between the perovskite and *** assembly and redistribution of CPA-based amphiphilic molecules at the perovskite-substrate buried interface not only promotes the growth of a low-defect crystalline perovskite thin film,but also suppresses the photo-induced halide phase *** energy level alignment between wide-bandgap perovskite and the hole-selective layer is further improved by modulating the substituents on the triphenylamine donor moiety(methoxyls for MPA-CPA,methyls for Me PA-CPA,and bare TPA-CPA).Using a 1.68 e V bandgap perovskite,the Me PA-CPA-based devices achieved an unprecedentedly high V_(OC)of 1.29 V and PCE of 22.3%under standard AM 1.5 *** V_(OC)-deficit(<0.40 V)is the lowest value reported for *** work not only provides an effective approach to decreasing the V_(OC)-deficit of WBG-PSCs,but also confirms the importance of energy level alignment at the charge-selective layers in PSCs.

关键词： cyanovinyl phosphonic acid energy level alignment hole-selective material open-circuit voltage wide-bandgap perovskite

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Two Applications of the ■■-Hodge Theory

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Chinese Annals of Mathematics,Series B 2024年第1期45卷 137-150页

作者： Dingchang wei Shengmao zhu Center of Mathematical Sciences Zhejiang UniversityHangzhou 310027China Department of Mathematics Zhejiang Normal UniversityJinhua 321004ZhejiangChina

Using Hodge theory and Banach fixed point theorem,Liu and zhu developed a global method to deal with various problems in deformation *** this note,the authors generalize Liu-zhu's method to treat two deformation problems for non-Kahler *** apply the ■■-Hodge theory to construct a deformation formula for(p,q)-forms of compact complex manifold under deformations,which can be used to study the Hodge number of complex manifold under *** the second part of this note,by using the ■■-Hodge theory,they provide a simple proof of the unobstructed deformation theorem for the non-Kahler Calabi-Yau ■■-manifolds.

关键词： Complex structures Deformations (p,q)-Forms Non-Kahler Calabi-Yaumanifolds

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Intelligent extraction of road cracks based on vehicle laser point cloud and panoramic sequence images

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Journal of Road Engineering 2024年第1期4卷 69-79页

作者： Ming Guo Li zhu Ming Huang jie ji Xian Ren Yaxuan wei Chutian Gao School of Geomatics and Urban Spatial Informatics Beijing University of Civil Engineering and ArchitectureBeijing 102616China Engineering Research Centre of Representative Building and Architectural Heritage Database Ministry of EducationBeijing 100044China Key Laboratory of Modern Urban Surveying and Mapping National Administration of SurveyingBeijing 102616China School of Civil and Transportation Engineering Beijing University of Civil Engineering and ArchitectureBeijing 102616China

In light of the limited efficacy of conventional methods for identifying pavement cracks and the absence of comprehensive depth and location data in two-dimensional photographs,this study presents an intelligent strategy for extracting road *** methodology involves the integration of laser point cloud data obtained from a vehicle-mounted system and a panoramic sequence of *** study employs a vehicle-mounted LiDAR measurement system to acquire laser point cloud and panoramic sequence image data simultaneously.A convolutional neural network is utilized to extract cracks from the panoramic sequence *** extracted sequence image is then aligned with the laser point cloud,enabling the assignment of RGB information to the vehicle-mounted three dimensional(3D)point cloud and location information to the two dimensional(2D)panoramic ***,a threshold value is set based on the crack elevation change to extract the aligned roadway point *** three-dimensional data pertaining to the cracks can be *** experimental findings demonstrate that the use of convolutional neural networks has yielded noteworthy outcomes in the extraction of road *** utilization of point cloud and image alignment techniques enables the extraction of precise location data pertaining to road *** approach exhibits superior accuracy when compared to conventional ***,it facilitates rapid and accurate identification and localization of road cracks,thereby playing a crucial role in ensuring road maintenance and traffic ***,this technique finds extensive application in the domains of intelligent transportation and urbanization *** technology exhibits significant promise for use in the domains of intelligent transportation and city development.

关键词： Road crack extraction Vehicle laser point cloud Panoramic sequence images Convolutional neural network

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