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Study of the gas sources of the Ordovician gas reservoir in the Central-Eastern Ordos Basin

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Petroleum Science 2022年第3期19卷 949-962页

作者： ji-jun li Zi-Wei Song Chun-lin Zhang Shuang-Fang Lu Mei-jun Dong Shu-Ning Zhang jun jiang Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)QingdaoShandong266580China PetroChina Research Institute of Petroleum Exploration and Development Beijing100083China

The source of the natural gas in the Lower Paleozoic Ordovician strata in the Ordos Basin,China is a controversial *** the present study,the genesis and distribution characteristics of the Ordovician natural gas were qualitatively investigated based on the composition of the natural gas and the hydrocarbon isotopic ***,the kinetics of the carbon isotope were analyzed to determine the proportions of the gas in the Ordovician gas reservoir contributed from the Carboniferous-Permian and Ordovician *** results show the *** to the Upper Paleozoic natural gas,the Ordovician natural gas has a large dryness *** core areas where gypsum-salt rocks are developed,the gypsum-salt rocks completely isolate the gas *** weathering crust of the reservoir in the fifth member of the Majiagou Formation(Ma_(5)^(1+2))originates primarily from the Upper Paleozoic coal-measure source rocks,while the Ma_(5)^(5)and the pre-salt natural gas are mainly derived from the Ordovician source *** the areas where the gypsum-salt rocks are relatively well-developed,the gypsum-salt rocks isolate the gas source to some extent,the pre-salt gas reservoir is mainly derived from the Lower Paleozoic source rocks,and this contribution gradually increases with increasing *** the areas where the gypsum-salt rocks are not developed,the proportion of the contribution of the Upper and Lower Paleozoic source rocks to the gas source of the Ordovician gas reservoir is mainly controlled by the volume of gas generated and the other accumulation conditions,and it does not reflect the isolation effect of the gypsum-salt rocks on the gas *** Ordovician natural gas accumulation models in the central-eastern Ordos Basin can be divided into four types according to the differences in the gas sources.

关键词： Ordos Basin Majiagou Formation Carbon isotope kinetics Gypsum layer Gas source

Discovery of the choristodere Hyphalosaurus baitaigouensis from the Lower Cretaceous jiufotang Formation of western liaoning,China and its paleobiogeographic significance

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Journal of Palaeogeography 2024年第3期13卷 547-562页

作者： li-jun Zhang Shu-An ji Hai-Chun Zhang South China Sea Culture Museum Hainan Tropical Ocean University Key Laboratory of Stratigraphy and Paleontology Ministry of Natural Resources Institute of Geology Chinese Academy of Geological Sciences State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and Palaeontology and Center for Excellence in Life and Paleoenvironment Chinese Academy of Sciences

The water-living reptile genus Hyphalosaurus was previously discovered in the Lower Cretaceous Yixian Formation bearing the middle Jehol Biota in western liaoning, China. Two complete skeletons of Hyphalosaurus are reported for the first time from the jiufotang Formation bearing the late Jehol Biota at two sites in western liaoning. They show the typical characteristics of Hyphalosaurus baitaigouensis in terms of the contact between some cranial bones and the number of cervical and dorsal vertebrae, and therefore are assigned to H. baitaigouensis. This discovery extends the stratigraphic range of this species from the Yixian Formation to the overlying jiufotang Formation. This paper further briefly compares the main characteristics of the two skeletons, summarizes the temporal and spatial distribution of Hyphalosaurus, and discusses the palaeogeographic evolution of western liaoning at the middle and late Jehol Biota stages based on the aquatic habits of Hyphalosaurus and the geological background of western liaoning. The analytical results show that the volcanic downwarped lakes, with distinct geographical divisions in western liaoning during the deposition of the Yixian Formation, had not completely disappeared till the deposition of the jiufotang Formation. The palaeo-lake in the Fuxin-Yixian Basin underwent the process of generation, expansion and shrinkage during the depositional period of the Yixian Formation and finally merged into a large lake. The palaeo-Dalinghe River,which connected the main basins in western liaoning during the depositional period of the jiufotang Formation, was formed simultaneously.

关键词： Western liaoning Jehol biota jiufotang formation Hyphalosaurus baitaigouensis Palaeobiogeography

Stable stripe and vortex solitons in two-dimensional spin-orbit coupled Bose-Einstein condensates

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Communications in Theoretical Physics 2024年第6期76卷 26-33页

作者： Yuan Guo Muhammad Idrees ji lin Hui-jun li Institute of Nonlinear Physics and Department of Physics Zhejiang Normal UniversityJinhua 321004China Zhejiang Institute of Photoelectronics and Zhejiang Institute for Advanced light Source Zhejiang Normal UniversityJinhua 321004China

We present a flexible manipulation and control of solitons via Bose-Einstein *** the presence of Rashba spin-orbit coupling and repulsive interactions within a harmonic potential,our investigation reveals the numerical local solutions within the *** manipulating the strength of repulsive interactions and adjusting spin-orbit coupling while maintaining a zero-frequency rotation,diverse soliton structures emerge within the *** include plane-wave solitons,two distinct types of stripe solitons,and odd petal solitons with both single and double *** stability of these solitons is intricately dependent on the varying strength of spin-orbit ***,stripe solitons can maintain a stable existence within regions characterized by enhanced spin-orbit coupling while petal solitons are unable to sustain a stable existence under similar *** rotational frequency is introduced to the system,solitons undergo a transition from stripe solitons to a vortex array characterized by a sustained *** rotational directions of clockwise and counterclockwise are non-equivalent owing to spin-orbit *** a result,the properties of vortex solitons exhibit significant variation and are capable of maintaining a stable existence in the presence of repulsive interactions.

关键词： Bose-Einstein condensate spin-orbit coupling rotation frequency stripe solitons vortex array

SciCN:A Scientific Dataset for Chinese Named Entity Recognition

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Computers, Materials & Continua 2024年第3期78卷 4303-4315页

作者： jing Yang Bin ji Shasha li jun Ma jie Yu College of Computer National University of Defense TechnologyChangsha410073China

Named entity recognition(NER)is a fundamental task of information extraction(IE),and it has attracted considerable research attention in recent *** abundant annotated English NER datasets have significantly promoted the NER research in the English *** contrast,much fewer efforts are made to the Chinese NER research,especially in the scientific domain,due to the scarcity of Chinese NER *** alleviate this problem,we present aChinese scientificNER dataset–SciCN,which contains entity annotations of titles and abstracts derived from 3,500 scientific *** manually annotate a total of 62,059 entities,and these entities are classified into six *** to English scientific NER datasets,SciCN has a larger scale and is more diverse,for it not only contains more paper abstracts but these abstracts are derived from more research *** investigate the properties of SciCN and provide baselines for future research,we adapt a number of previous state-of-theart Chinese NER models to evaluate *** results show that SciCN is more challenging than other Chinese NER *** addition,previous studies have proven the effectiveness of using lexicons to enhance Chinese NER *** by this fact,we provide a scientific domain-specific *** results demonstrate that our lexicon delivers better performance gains than lexicons of other *** hope that the SciCN dataset and the lexicon will enable us to benchmark the NER task regarding the Chinese scientific domain and make progress for future *** dataset and lexicon are available at:https://***/yangjingla/***.

关键词： Named entity recognition dataset scientific information extraction lexicon

Span-based joint entity and relation extraction augmented with sequence tagging mechanism

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Science China(Information Sciences) 2024年第5期67卷 84-98页

作者： Bin ji Shasha li Hao XU jie YU jun MA Huijun liU jing YANG College of Computer National University of Defense Technology

Span-based joint extraction simultaneously conducts named entity recognition(NER) and relation extraction(RE) in a text span form. However, since previous span-based models rely on span-level classifications, they cannot benefit from token-level label information, which has been proven advantageous for the task. In this paper, we propose a sequence tagging augmented span-based network(STSN), a spanbased joint model that can make use of token-level label information. In STSN, we construct a core neural architecture by deep stacking multiple attention layers, each of which consists of three basic attention *** the one hand, the core architecture enables our model to learn token-level label information via the sequence tagging mechanism and then uses the information in the span-based joint extraction; on the other hand, it establishes a bi-directional information interaction between NER and RE. Experimental results on three benchmark datasets show that STSN consistently outperforms the strongest baselines in terms of F1,creating new state-of-the-art results.

关键词： joint extraction named entity recognition relation extraction span sequence tagging mechanism

Multiple exciton generation effect in photocatalytic overall water splitting

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Science China Chemistry 2024年第2期67卷 424-425页

作者： Xiaolei Guo ji-jun Zou Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin300072China

This highlight is based on recent research published in Nature Energy by li and co-workers [1] from Northwestern Polytechnology University, reporting an exceeding 100% internal quantum efficiency(IQE) in photocatalytic overall water splitting. This breakthrough promises a bright future for efficient photocatalyst design by utilizing the multiple exciton effect(MEG).

关键词： splitting effect utilizing

Recovery and in-situ reduction of precious metals by graphdiyne and graphdiyne oxide for antibacterial use

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Rare Metals 2024年第4期43卷 1747-1757页

作者： Ming-ji jiang Ya-Na Zhang ling-Shen Meng jing Kang Yong-jun li Alideertu Dong College of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot010021China Engineering Research Center of Dairy Quality and Safety Control Technology Ministry of EducationInner Mongolia UniversityHohhot010021China Department of Chemistry University of ZurichCH-8057ZurichSwitzerland Laboratory of Organic Solids and Beijing National Laboratory for Molecular Sciences Institute of ChemistryChinese Academy of SciencesBeijing100190China

Based on the in-situ self-reduction and chemical stability,graphdiyne(GDY)and graphdiyne oxide(GDYO)are used as trapping agents to investigate the ability for recovering Au^(3+),Ag^+,and Pd^(2+)under different pH values and interfering *** strong acidity at pH=1,these two agents demonstrate high select recovery towards the three precious metal ions,which could be insitu reduced to nanoparticles(NPs).In addition,superparamagnetic Fe_(3)O_(4)NPs are deposited on the surfaces of GDY and *** magnetic responses enable GDYFe_(3)O_(4)to recover precious metals conveniently and efficiently by the aid of an external magnetic *** study also confirms the antibacterial activity of the as-recovered NPs deposited on GDY and GDYO against Escherichia coli and Staphylococcus aureus(1×10^(5)colony-forming unit(CFU)·mL^(-1)),and the antibacterial rates are 100%.This strategy of recovering precious metals and subsequently reusing to combat pathogens will be of great significance for environmental remediation and biomedical applications.

关键词： Graphdiyne In-situ reduction Recovery Precious metals Antibacterial

In situ modification of heavy oil catalyzed by nanosized metal-organic framework at mild temperature and its mechanism

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Chinese Journal of Chemical Engineering 2024年第3期67卷 166-173页

作者： li Wang ji-Xiang Guo Rui-Ying Xiong Chen-Hao Gao Xiao-jun Zhang Dan Luo The Unconventional Oil and Gas Institute China University of Petroleum-BeijingBeijing 102200China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China

Two catalysts, nano-sized cobalt-metal-organic framework(Co-MOF) and nickel(Ni)-MOF, were successfully prepared by the modification method. Tetralin(C10H12) was used as the hydrogen donor for the catalytic cracking and hydrogenation modification study of the dehydrated crude oil from the Shengli Oilfield. The optimal reaction conditions were determined through orthogonal experiments, and the components of the crude oil and modified oil samples were analyzed. The results revealed that the nanoMOF catalysts were successfully prepared and exhibited high catalytic activity. They could catalyze the cracking of large molecules in heavy oil at mild temperatures(<300°C), leading to the decomposition of the hydrogen donor. When the mass fraction of the catalyst was 0.2%, the mass fraction of the hydrogen donor was 1%, and the reaction temperature was 280°C, the Ni-MOF showed the best catalytic viscosity reduction effect. It could reduce the viscosity of heavy oil at 50°C from 15761.9 m Pa.s to 1266.2 m Pa.s,with a viscosity reduction rate of 91.97%. The modification effect of Co-MOF was the next best, which could reduce the viscosity of heavy oil to 2500.1 m Pa.s with a viscosity reduction rate of 84.14%. Molecular dynamics simulations revealed a strong interaction force between the MOF surface and asphaltene molecules. In the process of heavy-oil catalytic hydrogenation, the nano-MOF catalyst exhibited high catalytic activity. On the one hand, the empty d orbitals outside the metal atoms in the catalyst could polarize the carbon atoms in the organic matter, accelerating the breaking of long chains. On the other hand, the metal atoms in the catalyst could bond with the carbon σ bonds, breaking the carbon-carbon bonds. This disrupted the structure of the recombined components in the crude oil, irreversibly reducing the viscosity of the heavy oil and improving its fluidity.

关键词： Nano-sized MOF Petroleum Viscosity reduction Catalyst Nanomaterials

Multifunctional AlPO_(4)reconstructed liMn_(2)O_(4)surface for electrochemical lithium extraction from brine

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Journal of Energy Chemistry 2024年第2期89卷 410-421,I0010页

作者： jun Gu linlin Chen Xiaowei li Guiling Luo linjing Fan Yanhong Chao Haiyan ji Wenshuai Zhu School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina School of Chemistry and Chemical Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina College of Science State Key Laboratory of Heavy Oil ProcessingChina University of Petroleum-BeijingBeijing 102249China School of the Environment and Safety Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina

liMn_(2)O_(4)(LMO)electrochemical lithium-ion pump has gained widespread attention due to its green,high efficiency,and low energy consumption in selectively extracting lithium from ***,collapse of crystal structure and loss of lithium extraction capacity caused by Mn dissolution loss limits its industrialized ***,a multifunctional coating was developed by depositing amorphous AlPO_(4)on the surface of LMO using sol-gel *** characterization and electrochemical performance test provided insights into the mechanism of li^(+)embedment and de-embedment and revealed that multifunctional AlPO_(4)can reconstruct the physical and chemical state of LMO surface to improve the interface hydrophilicity,promote the transport of li^(+),strengthen cycle ***,after 20 cycles,the capacity retention rate of 0.5AP-LMO reached 93.6%with only 0.147%Mn dissolution *** average li^(+)release capacity of 0.5AP-LMO//Ag system in simulated brine is 28.77 mg/(g h),which is 90.4%higher than ***,even in the more complex Zabuye real brine,0.5AP-LMO//Ag can still maintain excellent lithium extraction *** results indicate that the 0.5AP-LMO//Ag lithium-ion pump shows promising potential as a li^(+)selective extraction system.

关键词： liMn_(2)O_(4) Multifunctional AlPO_(4)coating li^(+)embedment and de-embedment mechanism Stability Hydrophilicity Various solution