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Identification and comparison of the local physicochemical structures of transition metal-based layered double hydroxides for high performance electrochemical oxygen evolution reactions

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Journal of Energy Chemistry 2023年第12期87卷 89-97,I0004页

作者： Min Sung Kim Bipin Lamichhane Ju-hyeon lee Jin-Gyu Bae jeong Yeon Heo hyeon jeong lee Shyam Kattel Ji Hoon lee School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea KNU Advanced Material Research Institute Kyungpook National UniversityDaegu 41566Republic of Korea Department of Materials Science and Engineering Ulsan National Institute of Science and TechnologyUlsan 44919Republic of Korea Department of Physics Florida A&M UniversityTallahasseeFlorida 32307United States

Layered double hydroxides(LDHs) have attracted considerable attention as a cost effective alternative to the precious iridium-and ruthenium-based electrocatalysts for an oxygen evolution reaction(OER),a bottleneck of water electrolysis for sustainable hydrogen *** their excellent OER performance,the structural and electronic properties of LDHs,particularly during the OER process,remain to be poorly *** this study,a series of LDH catalysts is investigated through in situ X-ray absorption fine structure analyses and density functional theory(DFT) *** experimental results reveal that the LDH catalyst with equal amounts of Ni and Fe(NF-LDH) exhibits the highest OER activity and catalytic life span when compared with its counterparts having equal amounts of Ni and Co(NC-LDH)and Ni only(Ni-LDH).The NF-LDH shows a markedly enhanced OER kinetics compared to the NC-LDH and the Ni-LDH,as proven by the lower overpotentials of 180,240,and 310 mV,respectively,and the Tafel slopes of 35.1,43.4,and 62.7 mV dec^(-1),*** DFT calculations demonstrate that the lowest overpotential of the NF-LDH is associated with the active sites located at the edge planes of NF-LDH in contrast to those located at the basal planes of Ni-LDH and *** current study pinpoints the active sites on various LDHs and presents strategies for optimizing the OER performance of the LDH catalysts.

关键词： Layered double hydroxides Oxygen evolution reaction In situ X-ray analyses Density functional theory Catalytic active sites

维普期刊数据库

Acute lower extremity arterial thrombosis after intraocular foreign body removal under general anesthesia: A case report and review of literature

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World Journal of Clinical Cases 2021年第27期9卷 8232-8241页

作者： Soeun Jeon jeong-Min Hong hyeon jeong lee Eunsoo Kim Hyunju lee Yesul Kim Hyun-Su Ri Jae Jung lee Department of Anesthesia and Pain Medicine Pusan National UniversitySchool of MedicineBusan 49241South Korea Biomedical Research Institute Pusan National University HospitalBusan 49241South Korea Department of Anesthesia and Pain Medicine Kyungpook National UniversitySchool of MedicineDaegu 41944South Korea Department of Ophthalmology College of MedicinePusan National UniversitySchool of MedicineYangsan 50612South Korea

BACKGROUND Surgery,which is a major risk factor for venous thrombosis,has rarely been considered a risk factor for arterial *** studies have suggested that venous and arterial thromboses share common risk factors and have a bidirectional ***,there is a growing interest in the risk of arterial thrombosis after *** report a case of acute bilateral lower extremity arterial thromboses that developed after a prolonged *** SUMMARY A 59-year-old man was hospitalized for intraocular foreign body removal *** was a heavy-drinking smoker and had untreated hypertension and varicose veins in both *** operation was unexpectedly prolonged,lasting 4 h and 45 *** after emergence from general anesthesia,the patient complained of extreme pain in both *** the surgical drape was removed,cyanosis was evident in both feet of the *** pulse was not palpable,and continuous-wave Doppler signals were inaudible in the bilateral dorsalis pedis and posterior tibial *** tomography angiography confirmed acute bilateral thrombotic occlusion of the popliteal arteries,proximal anterior tibial arteries,and tibioperoneal *** pulse returned in both lower limbs after 6 h of heparin *** patient was discharged on postoperative day 26 without any *** Acute lower extremity arterial thrombosis can occur after *** should pay particular attention to patients with risk factors for thrombosis.

关键词： Thromboembolism Thrombosis Arterial thrombosis Arterial occlusive diseases Peripheral occlusive artery disease Case report

Paradoxical carbon dioxide embolism during laparoscopic hepatectomy without intracardiac shunt:A case report

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World Journal of Clinical Cases 2022年第9期10卷 2908-2915页

作者： Soeun Jeon jeong-Min Hong hyeon jeong lee Yesul Kim Hyunjong Kang Boo-young Hwang Dowon lee Young-hoon Jung Department of Anesthesia and Pain Medicine Pusan National UniversitySchool of MedicineBusan 49241South Korea Biomedical Research Institute Pusan National University HospitalBusan 49241South Korea

BACKGROUND Laparoscopic hepatectomy has recently become popular because it results in less bleeding than open ***,CO_(2)embolism occurs more *** CO_(2)embolisms during laparoscopic surgery are self-resolving and non-symptomatic;however,severe CO_(2)embolism may cause hypotension,cyanosis,arrhythmia,and cardiovascular *** particular,paradoxical CO_(2)embolisms are highly likely to cause neurological *** report a case of paradoxical CO_(2)embolism found on transesophageal echocardiography(TEE)during laparoscopic hepatectomy,although the patient had no intracardiac *** SUMMARY A 71-year-old man was admitted for laparoscopic left *** left hepatic vein ligation,the inferior vena cava was accidentally *** observed a sudden drop in oxygen saturation to 85%,decrease in systolic blood pressure(SBP)below 90 mm Hg,and reduction in end-tidal CO_(2)to 24 mm Hg.A“mill-wheel”murmur was auscultated over the *** fraction of inspired oxygen was increased to 100%with 5 cm H2O of positive end-expiratory pressure(PEEP)and hyperventilation was *** infusion was increased to maintain SBP above 90 mm Hg.A TEE probe was inserted,revealing gas bubbles in the right side of the heart,left atrium,left ventricle,and ascending *** surgeon reduced the pneumoperitoneum pressure from 17 to 14 mm Hg and repaired the damaged vessel ***,the patient’s hemodynamic status *** patient was transferred to the intensive care unit,recovering well without *** TEE monitoring is important to quickly determine the presence and extent of embolism in patients undergoing laparoscopic hepatectomy.

关键词： Carbon dioxide Embolism Laparoscopy Pneumoperitoneum Transesophageal echocardiography Case report

Cystic Brunner's gland hamartoma in the duodenum:A case report

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World Journal of Gastroenterology 2009年第39期15卷 4980-4983页

作者： Beom Jin Park Min Ju Kim jeong hyeon lee Sung-Soo Park Deuk Jae Sung Sung Bum Cho Department of Radiology Korea UniversityCollege of MedicineAnam Hospital Department of Pathology Korea UniversityCollege of MedicineAnam Hospital Department of Surgery Korea UniversityCollege of MedicineAnam Hospital

Cystic Brunner's gland hamartoma in the duodenum is exceedingly rare,although microscopic examination may sometimes reveal a Brunner's gland hamartoma containing dilated ducts in the *** present a case of large cystic Brunner's gland hamartoma in the duodenum with a long stalk,which is described in light of multidetector-row computed tomography,magnetic resonance imaging,and a modified small bowel series,together with pathologic correlation and differential diagnosis.

关键词： Brunner's gland Hamartoma Duodenum Multidetector-row computed tomography Magnetic resonance imaging

Biliary phytobezoar resulting in intestinal obstruction

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World Journal of Gastroenterology 2013年第1期19卷 133-136页

作者： Yura Kim Beom Jin Park Min Ju Kim Deuk Jae Sung Dong-Sik Kim Young-Dong Yu jeong hyeon lee Department of Radiology College of MedicineKorea UniversityAnam HospitalSeoul 136-705South Korea Division of HBP Surgery and Liver Transplantation Department of SurgeryCollege of MedicineKorea UniversityAnam HospitalSeoul 136-705South Korea Department of Pathology College of MedicineKorea UniversityAnam HospitalSeoul 136-705South Korea

Phytobezoar is the most common type of *** is composed of indigestible vegetable matter and is usually found in the *** phytobezoar is extremely rare and difficult to diagnose *** pathogenesis is not clear,and there have been only a few reports of biliary bezoars associated with sphincteric impairmentat the ampulla of ***,we present a report of biliary bezoar that resulted in jejunal *** were unable to identifythe bezoar in the extrahepatic bile duct until it obstructed the small bowel *** our knowledge,this is the first report of small bowel obstruction resulting frommigration of a biliary bezoar.

关键词： Phytobezoar Biliary Intestinal obstruction Choledochoduodenal Fistula Multidetector-row computed tomography

Multimodal Metabolic Imaging Reveals Pigment Reduction and Lipid Accumulation in Metastatic Melanoma

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Biomedical Engineering Frontiers 2021年第1期2卷 1-17页

作者： hyeon jeong lee Zhicong Chen Marianne Collard Fukai Chen Jiaji G.Chen Muzhou Wu Rhoda M.Alani Ji-Xin Cheng Photonics Center Department of Electrical and Computer EngineeringDepartment of Biomedical EngineeringBoston UniversityBostonMA 02215USA Department of Dermatology Boston University School of MedicineBostonMA 02118USA

Objective and Impact *** signatures are needed for early diagnosis and improved treatment of metastatic *** high-resolution multimodal chemical imaging of human melanoma samples,we identify a metabolic reprogramming from pigmentation to lipid droplet(LD)accumulation in metastatic *** plasticity promotes cancer survival and metastasis,which promises to serve as a prognostic marker and/or therapeutic ***,identifying metabolic alterations has been challenged by difficulties in mapping localized metabolites with high spatial *** developed a multimodal stimulated Raman scattering and pump-probe imaging *** time-domain measurement and phasor analysis,our platform allows simultaneous mapping of lipids and pigments at a subcellular ***,we identify the sources of these metabolic signatures by tracking deuterium metabolites at a subcellular *** validation with mass spectrometry,a specific fatty acid desaturase pathway was *** identified metabolic reprogramming from a pigment-containing phenotype in low-grade melanoma to an LD-rich phenotype in metastatic *** LDs contain high levels of cholesteryl ester and unsaturated fatty *** fatty acid uptake,but not de novo lipogenesis,contributes to the LD-rich *** sapienate,mediated by FADS2,is identified as an essential fatty acid that promotes cancer *** such metabolic signatures effectively suppresses the migration capacity both in vitro and in *** multimodal spectroscopic imaging and lipidomic analysis,the current study reveals lipid accumulation,mediated by fatty acid uptake,as a metabolic signature that can be harnessed for early diagnosis and improved treatment of metastatic melanoma.

关键词： Lipid Metabolic diagnosis

Unconventional Regulatory Mechanism of Sterol Synthesis Unveiled by Stimulated Raman Imaging of Subcellular Metabolites

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Unconventional Regulatory Mechanism of Sterol Synthesis Unve...

Single-cell and spatial omics:exploring hypothalamic heterogeneity

第四届中国生物物理学会代谢生物学分会学术研讨会

作者： Yongqing Zhang Yihui Zhou Wen Fang Cunqi Ye Delong Zhang hyeon jeong lee

＜正＞Cholesterol is connected to multiple health problems. Although the biochemical pathway is well-understood, cholesterol, as a crucial metabolite, still has many disease-related mechanisms unclear, such as subcellular regulation of cholesterol synthesis. It presents a grand challenge for conventional characterization methods, such as biochemical assay or mass spectrometry, which have difficulties providing non-invasive, high-speed, and high-resolution measurement of metabolites in living cells. In contrast, stimulated Raman scattering （SRS）,

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Neural Regeneration Research 2025年第6期20卷 1525-1540页

作者： Muhammad Junaid Eun jeong lee Su Bin Lim Department of Biochemistry&Molecular Biology Ajou University School of MedicineSuwonSouth Korea Department of Biomedical Sciences Graduate School of Ajou UniversitySuwonSouth Korea Department of Brain Science Ajou University School of MedicineSuwonSouth Korea

Elucidating the complex dynamic cellular organization in the hypothalamus is critical for understanding its role in coordinating fundamental body functions. Over the past decade, single-cell and spatial omics technologies have significantly evolved, overcoming initial technical challenges in capturing and analyzing individual cells. These high-throughput omics technologies now offer a remarkable opportunity to comprehend the complex spatiotemporal patterns of transcriptional diversity and cell-type characteristics across the entire hypothalamus. Current single-cell and single-nucleus RNA sequencing methods comprehensively quantify gene expression by exploring distinct phenotypes across various subregions of the hypothalamus. However, single-cell/single-nucleus RNA sequencing requires isolating the cell/nuclei from the tissue, potentially resulting in the loss of spatial information concerning neuronal networks. Spatial transcriptomics methods, by bypassing the cell dissociation, can elucidate the intricate spatial organization of neural networks through their imaging and sequencing technologies. In this review, we highlight the applicative value of single-cell and spatial transcriptomics in exploring the complex molecular-genetic diversity of hypothalamic cell types, driven by recent high-throughput achievements.

关键词： cellular diversity hypothalamus multi-omics single-cell transcriptomics spatial transcriptomics

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Ru/NiMnB spherical cluster pillar for highly proficient green hydrogen electrocatalyst at high current density

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Journal of Energy Chemistry 2025年第1期100卷 397-408页

作者： Md Ahasan Habib Shusen Lin Mehedi Hasan Joni Sumiya Akter Dristy Rutuja Mandavkar Jae-Hun jeong Jihoon lee Department of Electronic Engineering College of Electronics and Information Kwangwoon University

Advanced OER/HER electrocatalytic alternatives are crucial for the wide adaptation of green hydrogen ***,Ru/NiMnB spherical cluster pillar （SCP）,denoted as Ru/NiMnB,is synthesized using a combination of electro-deposition and hydrothermal *** investigation of Ru doping in the NiMnB matrix revealed significant improvements in electrocatalytic *** Ru/NiMnB SCPs demonstrate superior OER/HER activity with low overpotentials of 150 and 103 mV at 50mA/cm2in 1 M KOH,making them highly competitive with state-of-the-art ***,the Ru/NiMnB SCPs exhibit a low 2-E cell voltage of 2.80 V at ultra-high current density of 2,000 m A/cm2in 1 M KOH,outperforming the standard benchmark electrodes of RuO2||Pt/C,thereby positioning Ru/NiMnB as one of the best bifunctional *** SCPs exhibit exceptional high-current characteristics,stability and corrosion resistance,as evidenced by continuous operation at 1,000 mA/cm2high-current density for over 150 h in 6 M KOH at elevated temperatures under harsh industrial *** a small amount of Ru incorporation significantly enhances the electrocatalytic performances of NiMnB,attributed to increased active sites and improved intrinsic properties such as conductivity,adsorption/desorption capability and reaction ***,Ru/NiMnB SCPs present a promising bi-functional electrode concept for efficient green H2production.

关键词： Advanced electrocatalyst High current Corrosion resistance Industrial requirement