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New Opportunities for Lanthanide Luminescence

Journal of Rare Earths 2007年第3期25卷 257-274页

作者： jean-claude G. Bünzli Steve Comby Anne-Sophie Chauvin Caroline D. B. Vandevyver Laboratory of Lanthanide Supramolecular Chemistry Ecole Polytechnique Fédérale de Lausanne BCH 1402 CH-1015 Lausanne Switzerland

Trivalent lanthanide ions display fascinating optical properties. The discovery of the corresponding elements and their first industrial uses were intimately linked to their optical properties. This relationship has been kept alive until today when many high-technology applications of lanthanide-containing materials such as energy-saving lighting devices, displays, optical fibers and amplifiers, lasers, responsive luminescent stains for biomedical analyses and in cellulo sensing and imaging, heavily rely on the brilliant and pure-color emission of lanthanide ions. In this review we first outlined the basics of lanthanide luminescence with emphasis on f-f transitions, the sensitization mechanisms, and the assessment of the luminescence efficiency of lanthanide-containing emissive molecular edifices. Emphasis was then put on two fast developing aspects of lanthanide luminescence： materials for telecommunications and light emitting diodes, and biomedical imaging and sensing. Recent advances in NIR-emitting materials for plastic amplifiers and waveguides were described, together with the main solutions brought by researchers to minimize non-radiative deactivation of excited states. The demonstration in 1999 that erbium tris（8-hydroxyquinolinate） displayed a bright green emission suitable for organic light emitting diodes （OLEDs） was followed by realizing that in OLEDs, 25% of the excitation energy leads to singlet states and 75% to triplet states. Since lanthanide ions are good triplet quenchers, they now also play a key role in the development of these lighting devices. Luminescence analyses of biological molecules are among the most sensitive analytical techniques known. The long lifetime of the lanthanide excited states allows time-resolved spectroscopy to be used, suppressing the sample autofluorescence and reaching very low detection limits. Not only visible lanthanide sensors are now ubiquitously provided in medical diagnosis and in cell imaging, but the feasibili

关键词： lanthanide luminescence sensitization near infrared telecommunications organic light emitting diode (OLED) time-resolved luminescence in cellulo sensing cell imaging rare earths

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A quantum cascade laser infrared spectrometer for CO_2 stable isotope analysis：Field implementation at a hydrocarbon contaminated site under bio-remediation

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Journal of Environmental Sciences 2016年第2期28卷 60-74页

作者： Christophe Guimbaud Cécile Noel Michel Chartier Valéry Catoire Michaela Blessing jean Christophe Gourry claude Robert Laboratoire de Physique et de Chimie de l'Environnement et de l'Espace (LPC2E) CNRS et Universite d'Orleans (UMR 7328)45071 Orleans cedex 2 France Bureau de Recherches Geologiques et Minieres (BRGM) 45060 Orleans cedex 2 France

Real-time methods to monitor stable isotope ratios of CO_2 are needed to identify biogeochemical origins of CO_2 emissions from the soil–air interface. An isotope ratio infra-red spectrometer（IRIS） has been developed to measure CO_2 mixing ratio with δ~13C isotopic signature, in addition to mixing ratios of other greenhouse gases（CH_4, N2_O）. The original aspects of the instrument as well as its precision and accuracy for the determination of the isotopic signature δ~13C of CO_2 are discussed. A first application to biodegradation of hydrocarbons is presented, tested on a hydrocarbon contaminated site under aerobic bio-treatment. CO_2 flux measurements using closed chamber method is combined with the determination of the isotopic signature δ~13C of the CO_2 emission to propose a non-intrusive method to monitor in situ biodegradation of hydrocarbons. In the contaminated area, high CO_2 emissions have been measured with an isotopic signature δ~13C suggesting that CO_2 comes from petroleum hydrocarbon *** first field implementation shows that rapid and accurate measurement of isotopic signature of CO_2 emissions is particularly useful in assessing the contribution of contaminant degradation to the measured CO_2 efflux and is promising as a monitoring tool for aerobic bio-treatment.

关键词： Isotope ratio infrared spectrometry Isotopic signature δ^(13)C of CO_2 Biodegradation monitoring Hydrocarbons BTEX

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Decomposition and decoupling analysis of carbon dioxide emissions in African countries during 1984–2014

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Journal of Environmental Sciences 2021年第4期33卷 85-98页

作者： Claudien Habimana Simbi Jianyi Lin Dewei Yang jean claude Ndayishimiye Yang Liu Huimei Li Lingxing Xu Weijing Ma Key Lab of Urban Environment and Health Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China School of Geographical Sciences Southwest UniversityChongqing 400715China Faculty of Geography University of MarburgMarburg 35032Germany

The potential for mitigating climate change is growing worldwide,with an increasing emphasis on reducing CO_(2)emissions and minimising the impact on the *** continent is faced with the unique challenge of climate change whilst coping with extreme poverty,explosive population growth and economic ***_(2)emission patterns in Africa are analysed in this study to understand primary CO_(2)sources and underlying driving forces *** are examined using gravity model,logarithmic mean divisia index and Tapio's decoupling indicator of CO_(2)emissions from economic development in 20 selected African countries during *** reveal that CO_(2)emissions increased by 2.11%(453.73 million ton)over the research *** centre for African CO_(2)emissions had shifted towards the northeast *** and economic growth were primary driving forces of CO_(2)*** structure and emission efficiency effects partially offset the growth of CO_(2)*** economic growth effect was an offset factor in central African countries and Zimbabwe due to political instability and economic *** structure and emission efficiency were insufficient to decouple economic development from CO_(2)emissions and relieve the pressure of population explosion on CO_(2)emissions in ***,future efforts in reducing CO_(2)emissions should focus on scaleup energy-efficient technologies,renewable energy update,emission pricing and long-term green development towards sustainable development goals by 2030.

关键词： CO_(2)emissions Decoupling Driving forces Logarithmic mean divisia index method Patterns Africa

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Urbanization reduces resource use efficiency of phytoplankton community by altering the environment and decreasing biodiversity

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Journal of Environmental Sciences 2022年第2期34卷 140-151页

作者： Yigang Yang Huihuang Chen Mamun Abdullah Al jean claude Ndayishimiye Jun R Yang Alain Isabwe Anqi Luo Jun Yang Aquatic EcoHealth Group Fujian Key Laboratory of Watershed EcologyKey Laboratory of Urban Environment and HealthInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China Engineering Research Center of Ecology and Agricultural Use of Wetland(Ministry of Education) College of AgricultureYangtze UniversityJingzhou 434025China

Urbanization often exerts multiple effects on aquatic and terrestrial organisms,including changes in biodiversity,species composition and ecosystem ***,the impacts of urbanization on river phytoplankton in subtropical urbanizing watersheds remain largely ***,we explored the effects of urbanization on phytoplankton community structure(i.e.,biomass,community composition and diversity)and function(i.e.,resource use efficiency)in a subtropical river at watershed scale in southeast China over 6 years.A total of 318 phytoplankton species belonging into 120 genera and 7 phyla were identified from 108 *** biomass showed an increasing trend with increasing urbanization *** phytoplankton community shifted from Chlorophyta dominance in rural upstream waters to Bacillariophyta dominance in urbanized downstream ***,phytoplankton diversity and resource use efficiency(RUE=phytoplankton biomass/total phosphorus)were significantly decreased with increasing urbanization level from upstream to *** RUE exhibited a significant positive correlation with species richness,but a negative correlation with phytoplankton *** variation in environmental factors(turbidity,total nitrogen,NH_(4)^(+)-N,total phosphorus,PO_(4)^(3-)-P and percentage urbanized area)was significantly correlated with phytoplankton diversity and ***,our results revealed the influence of urbanization on phytoplankton community structure and ecosystem function was due to its altering the environmental ***,human-driven urbanization may play crucial roles in shaping the structure and function of phytoplankton communities in subtropical rivers,and the mechanism of this process can provide important information for freshwater sustainable uses,watershed management and conservation.

关键词： Plankton Community functioning Subtropical river Urbanization gradient Land use Watershed ecology

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Micromorphological description of vernacular cob process and comparison with rammed earth

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Frontiers of Architectural Research 2020年第1期9卷 203-215页

作者： Erwan Hamard Cécilia Cammas Blandine Lemercier Bogdan Cazacliu jean-claude Morel IFSTTAR MASTGPEMF-44344BouguenaisFrance INRAP UMR 5140AgroParisTechF-78850Thiverval-GrignonFrance UMR SAS AGROCAMPUS OUESTINRAF-35042RennesFrance Faculty of Engineering Environment and ComputingCentre for the Built and Natural EnvironmentCoventry UniversityCoventryCV15FBUK

Past builders have developed very low-embodied energy construction techniques optimizing the use of local building *** techniques are a source of inspiration for modern sustainable ***,this know-how was orally transmitted and was lost as earth construction fell into disuse during the 20th century in European *** absence of written documents makes necessary to use an archaeological approach in order to rediscover these construction *** analysis of thin sections collacted in earth building walls was used for the first time to describe cob construction technique and highlighted several typical pedofeatures allowing to clearly identifying this ***,a first comparison of the cob and rammed earth micromorphological features permitted to identify two key factors to distinguish these two techniques,the manufacturing state(solid or plastic)and the organization of the material in the wall.

关键词： Cob Rammed earth Micromorphology Architectural heritage Pedology

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Lanthanide-doped nanoscintillators

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Light(Science & Applications) 2022年第10期11卷 2264-2266页

作者： jean-claude Georges Bünzli institute of Chemical Sciences and Engineering Swiss Federal Institute of TechnologyLausanne(EPFL)LausanneSwitzerland Department of Biomedical Engineering Southern University of Science and Technology(SUSTech)ShenzhenChina

Lanthanide-doped nanoscintillators are taking the lead in several important fields including radiation detection,biomedicine,both at the level of diagnosis and therapy,and information encoding.

关键词： diagnosis Lanthanide ill

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Basic deep eutectic solvents as reactant, template and solvents for ultra-fast preparation of transition metal oxide nanomaterials

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Chinese Chemical Letters 2020年第6期31卷 1584-1587页

作者： Jia Chen Mohammad Chand Ali Ruirui Liu jean claude Munyemana Zhan Li Honglin Zhai Hongdeng Qiu CAS Key Laboratory of Chemistry of Northwestern Plant Resources and Key Laboratory for Natural Medicine of Gansu Province Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000.China University of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100039China Department of Chemistry Lanzhou UniversityLanzhou 730000.China

Developing a new type of deep eutectic solvents(DESs)is indispensable for expanding their application in various ***,we report a series of new highly basic ***-IR,quantitative 1 H NMR,MD simulation and physical properties show that these basic liquids are made up of hydroxide acceptor of alkali metal hydroxides in which the hydrogen bonding interactions coordinate the *** DESs can be played three roles as new solvents,template and reactant for facile and ultra-fast preparation of transition metal oxide nanomaterials such as NiCo2 O4,MnCo2 O4,NiMn2 O4,CoCu2 O4 and Co3 O4 under mild *** work shows one of the low energy-intensive methods for nanomaterial *** initial findings of basic deep eutectic solvents provide a potential applicability around the systematic development of transition metal oxide nanosheets.

关键词： Basic deep eutectic solvents Hydrogen-bonding acceptors Hydrogen-bonding donors Transition metal oxide Nanomaterials

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ON MAXWELL EQUATIONS WITH THE TRANSPARENT BOUNDARY CONDITION

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Journal of Computational Mathematics 2008年第3期26卷 284-296页

作者： Zhiming Chen jean-claude Nédélec LSEC ICMSEC Academy of Mathematics and Systems Science Chinese Academy of Sciences Beijing 100080 China Centre de Mathématiques Appliquées Ecole Polytechnique 91228 Palaiseau Cedex France

In this paper we show the well-posedness and stability of the Maxwell scattering problem with the transparent boundary condition. The proof depends on the well-posedness of the time-harmonic Maxwell scattering problem... 详细信息

关键词： Electromagnetic scattering Well-posedness Stability

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金属注射成形烧结工艺的试验与数值模拟

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机械工程学报 2008年第8期44卷 157-163页

作者：宋久鹏 BARRIERE Thierry 柳葆生 GELIN jean-claude 西南交通大学应用力学与工程系成都610031 法国Femto-ST研究所应用力学实验室

采用粘塑性理论建立烧结过程的本构模型,以316L不锈钢粉末注射成形产品为例,设计出烧结过程中重力作用下弯曲梁试验和膨胀计中的自由烧结试验,分别用于标定本构模型中的粘度模量和烧结应力。通过用户子程序,在有限元求解器Abaqus^(?)上... 详细信息

采用粘塑性理论建立烧结过程的本构模型,以316L不锈钢粉末注射成形产品为例,设计出烧结过程中重力作用下弯曲梁试验和膨胀计中的自由烧结试验,分别用于标定本构模型中的粘度模量和烧结应力。通过用户子程序,在有限元求解器Abaqus^(?)上实现数值模拟,预测产品在烧结过程中的收缩和变形。考虑了重力、摩擦以及注射阶段粉末与粘结剂的偏析效应对于烧结工艺的影响,数值模拟结果与试验结果一致。

关键词：金属注射成形烧结粘塑性有限元法

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The synergy between the payloads on the ASO-S mission

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Research in Astronomy and Astrophysics 2019年第11期19卷 115-126页

作者： jean-claude Vial Institut d’Astrophysique Spatiale University Paris-Sud

This paper addresses the improved science resulting from joint observations performed by the different instruments onboard the Advanced Space-based Solar Observatory(ASO-S)mission along with ancillary instruments on missions flying at the same *** first describes the three major instruments along with their stated *** it presents some basic science issues concerning jointly observed flares,coronal mass ejections(CMEs)and eruptive prominences(EPs).Each physical candidate(magnetic reconnection,instability,hard X-ray emission and magnetic coronal field topology)is discussed in terms of its signature and identification with ASO-S *** importance of Lyαdetection and non-LTE modeling is *** instrumental and science challenges are briefly discussed.

关键词： techniques imagery,polarimetry-Sun eruptions,flares,coronal mass ejections

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