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Surface modification of tungsten oxide by oxygen vacancies for hydrogen adsorption

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Journal of Materials Science & Technology 2022年第22期117卷 23-35页

作者： q.Zhang F.W.Tang Z.Zhao Z.r.Nie X.Y.Song Faculty of Materials and Manufacturing Key Laboratory of Advanced Functional MaterialsMinistry of Education of ChinaBeijing University of TechnologyBeijing 100124China

A model for describing the adsorption process of hydrogen on surface of tungsten oxide was proposed based on the first-principle calculations. Multiple factors such as type of active surface, adsorption site and distribution of oxygen vacancies were considered to evaluate the hydrogen adsorption capability of tungsten oxide. The adsorption Gibbs free energies, electronic structures and bonding characteristics under various conditions were examined to reveal the influence of oxygen vacancies on the surface. It is found that the capability of hydrogen adsorption of tungsten oxide can be significantly enhanced by adjusting the oxygen vacancy on the outermost layer of certain active surfaces. The modeling predicts that the surface structure stability and gas adsorption ability of tungsten oxide can be simultaneously improved through the formation of W–H bonds. The proposed strategy for moderating surface provides a new approach to obtain excellent gas-sensitive metal oxide materials.

关键词： Metal oxide Gas-sensitive material Surface adsorption Oxygen vacancy First-principles calculation

Amplitude analysis of the decays D^(0)→π^(+)π^(−)π^(+)π^(−)and D^(0)→π^(+)π^(−)π^(0)π^(0)

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Chinese Physics C 2024年第8期48卷 6-33页

作者： M.Ablikim M.N.Achasov P.Adlarson O.Afedulidis X.C.Ai r.Aliberti A.Amoroso q.An Y.Bai O.Bakina I.Balossino Y.Ban H.-r.Bao V.Batozskaya K.Begzsuren N.Berger M.Berlowski M.Bertani D.Bettoni F.Bianchi E.Bianco A.Bortone I.Boyko r.A.Briere A.Brueggemann H.Cai X.Cai A.Calcaterra G.F.Cao N.Cao S.A.Cetin J.F.Chang W.L.Chang G.r.Che G.Chelkov C.Chen C.H.Chen Chao Chen G.Chen H.S.Chen M.L.Chen S.J.Chen S.L.Chen S.M.Chen T.Chen X.r.Chen X.T.Chen Y.B.Chen Y.q.Chen Z.J.Chen Z.Y.Chen S.K.Choi X.Chu G.Cibinetto F.Cossio J.J.Cui H.L.Dai J.P.Dai A.Dbeyssi r.E.de Boer D.Dedovich C.q.Deng Z.Y.Deng A.Denig I.Denysenko M.Destefanis F.De Mori B.Fang S.S.Fang W.X.Fang Y.Fang Y.q.Fang r.Farinelli L.Fava F.Feldbauer G.Felici C.q.Feng J.H.Feng Y.T.Feng K.Fischer M.Fritsch C.D.Fu J.L.Fu Y.W.Fu H.Gao Y.N.Gao Yang Gao S.Garbolino I.Garzia P.T.Ge Z.W.Ge C.Geng E.M.Gersabeck B.Ding X.X.Ding Y.Ding Y.Ding J.Dong L.Y.Dong M.Y.Dong X.Dong M.C.Du S.X.Du Z.H.Duan P.Egorov Y.H.Fan J.Fang JA.Gilman K.Goetzen L.Gong W.X.Gong W.Gradl S.Gramigna M.Greco M.H.Gu Y.T.Gu C.Y.Guan Z.L.Guan A.q.Guo L.B.Guo M.J.Guo r.P.Guo Y.P.Guo A.Guskov J.Gutierrez K.L.Han T.T.Han X.q.Hao F.A.Harris K.K.He K.L.He F.H.Heinsius C.H.Heinz Y.K.Heng C.Herold T.Holtmann P.C.Hong G.Y.Hou X.T.Hou Y.r.Hou Z.L.Hou B.Y.Hu H.M.Hu J.F.Hu T.Hu Y.Hu G.S.Huang K.X.Huang L.q.Huang X.T.Huang Y.P.Huang T.Hussain F.H\"olzken N.H\"usken N.in der Wiesche M.Irshad J.Jackson S.Janchiv J.H.jeong q.Ji q.P.Ji W.Ji X.B.Ji X.L.Ji Y.Y.Ji X.q.Jia Z.K.Jia D.Jiang H.B.Jiang P.C.Jiang S.S.Jiang T.J.Jiang X.S.Jiang Y.Jiang J.B.Jiao J.K.Jiao Z.Jiao S.Jin Y.Jin M.q.Jing X.M.Jing T.Johansson S.Kabana N.Kalantar-Nayestanaki X.L.Kang X.S.Kang M.Kavatsyuk B.C.Ke V.Khachatryan A.Khoukaz r.Kiuchi O.B.Kolcu B.Kopf M.Kuessner X.Kui A.Kupsc W.K\"uhn J.J.Lane P.Larin L.Lavezzi T.T.Lei Z.H.Lei H.Leithoff M.Lellmann T.Lenz C.Li C.Li C.H.Li Cheng Li D.M.Li F.Li G.Li H.Li H.B.Li H.J.Li H.N.Li Hui Li J.r.Li J.S.Li K.Li L.J.Li L.K.Li Lei Li M.H.Li P.r.Li q.M.Li q.X.Li r.Li S.X.Li T.Li W.D.Li W.G.Li X.Li X.H.Li X.L.Li X.Y.Li Y Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Beihang University Beijing 100191China Bochum ruhr-University D-44780 BochumGermany Budker Institute of Nuclear Physics SB rAS(BINP) Novosibirsk 630090Russia Carnegie Mellon University PittsburghPennsylvania 15213USA Central China Normal University Wuhan 430079China Central South University Changsha 410083China China Center of Advanced Science and Technology Beijing 100190China China University of Geosciences Wuhan 430074China Chung-Ang University Seoul06974Republic of Korea COMSATS University Islamabad Lahore CampusDefence RoadOff Raiwind Road54000 LahorePakistan Fudan University Shanghai 200433China GSI Helmholtzcentre for Heavy Ion research GmbH D-64291 DarmstadtGermany Guangxi Normal University Guilin 541004China Guangxi University Nanning 530004China Hangzhou Normal University Hangzhou 310036China Hebei University Baoding 071002China Helmholtz Institute Mainz Staudinger Weg 18D-55099 MainzGermany Henan Normal University Xinxiang 453007China Henan University Kaifeng 475004China Henan University of Science and Technology Luoyang 471003China Henan University of Technology Zhengzhou 450001China Huangshan College Huangshan 245000China Hunan Normal University Changsha 410081China Hunan University Changsha 410082China Indian Institute of Technology Madras Chennai 600036India Indiana University BloomingtonIndiana 47405USA INFN Laboratori Nazionali di Frascati INFN Laboratori Nazionali di FrascatiI-00044FrascatiItaly INFN Laboratori Nazionali di Frascati INFN Sezione di PerugiaI-06100PerugiaItaly INFN Laboratori Nazionali di Frascati University of PerugiaI-06100PerugiaItaly INFN Sezione di Ferrara INFN Sezione di FerraraI-44122FerraraItaly INFN Sezione di Ferrara University of FerraraI-44122FerraraItaly Inner Mongolia University Hohhot 010021China Institute of Modern Physics Lanzhou 730000China Institute of Physics and Technology Peace Avenue 54BUlaanbaatar 13330Mongolia Instituto de A

Using e^(+)e^(−)annihilation data corresponding to an integrated luminosity of 2.93 fb^(−1)taken at the center-of-mass energy√s=3.773 GeV with the BESIII detector,a joint amplitude analysis is performed on the decays D^(0)→π^(+)π^(−)π^(+)π^(−)and D^(0)→π^(+)π^(−)π^(0)π^(0)(non-η).The fit fractions of individual components are obtained,and large interferences among the dominant components of the decays D^(0)→a_(1)(1260)π,D^(0)→π(1300)π,D^(0)→ρ(770)ρ(770),and D^(0)→2(ππ)_(S)are observed in both *** the obtained amplitude model,the CP-even fractions of D^(0)→π^(+)π^(−)π^(+)π^(−)and D^(0)→π^(+)π^(−)π^(0)π^(0)(non-η)are determined to be(75.2±1.1_(stat).±1.5_(syst.))%and(68.9±1.5_(stat).±2.4_(syst.))%,*** branching fractions of D^(0)→π^(+)π^(−)π^(+)π^(−)and D^(0)→π^(+)π^(−)π^(0)π^(0)(non-η)are measured to be(0.688±0.010_(stat.)±0.010_(syst.))%and(0.951±0.025_(stat.)±0.021_(syst.))%,*** amplitude analysis provides an important model for the binning strategy in measuring the strong phase parameters of D^(0)→4πwhen used to determine the CKM angleγ(ϕ_(3))via the B^(−)→DK^(−)decay.

关键词： BESIII D^(0)meson decays amplitude analysis CP-even fraction

EFFECT OF CErIUM ION IMPLANTATION ON THE AqUEOUS COrrOSION BEHAVIOr OF ZIrCONIUM

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Acta Metallurgica Sinica(English Letters) 2004年第6期17卷 812-816页

作者： D.q.Peng X.D.Bai q.G.Zhou X.W.Chen r.H.Yu X.Y.Liu DepartmentofMaterialsScienceandEngineering TsinghuaUniversityBeijing100084ChinaManuscriptreceived9September2003

In order to study the influence of cerium ion implantation on the aqueous corrosion behavior of zirconium, specimens were implanted by cerium ions with a dosage range from 1×1016 to 1×1017 ions/cm2 at about 150℃, using MEVVA source at an acceler ative voltage of 40kV. The valence of the surface layer was analyzed by X-ray photo- electron spectroscopy (XPS); Three-sweep potentiodynamic polarization measurement was employed to value the aqueous corrosion resistance of zirconium in a 0.5mol/L H2SO4 solution. It was found that a remarkable decline in the aqueous corrosion behavior of zirconium implanted with cerium ions compared with that of the as-received zirconium. Finally, the mechanism of the corrosion resistance decline of the cerium-implanted zirconium is discussed.

关键词： zirconium corrosion resistance cerium ion implantation potentio- dynamic polarization X-ray photoelectron spectroscopy (XPS)

Effects of chemical pressure on diluted magneticsemiconductor(Ba,K)(Zn,Mn)_2As_2

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Chinese Physics B 2019年第5期28卷 288-292页

作者： Y Peng S Yu G q Zhao W M Li J F Zhao L P Cao X C Wang q q Liu S J Zhang r Z Yu Z Deng X H Zhu C q Jin College of Materials Science & Engineering Sichuan University Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences School of Physics University of Chinese Academy of Sciences Collaborative Innovation Center of quantum Matter

Chemical pressure induced by iso-valent doping has been widely employed to tune physical properties of materials. In this work, we report effects of chemical pressure by substitution of Sb or P into As on a recently discovered diluted magnetic semiconductor(Ba,K)(Zn,Mn)_2 As_2, which has the record of reliable Curie temperature of 230 K due to independent charge and spin doping. Sb and P are substituted into As-site to produce negative and positive chemical pressures, respectively.X-ray diffraction results demonstrate the successful chemical solution of dopants. Magnetic properties of both K-underdoped and K-optimal-doped samples are effectively tuned by Sb-and P-doping. The Hall effect measurements do not show decrease in carrier concentrations upon Sb-and P-doping. Impressively, magnetoresistance is significantly improved from7% to 27% by only 10% P-doping, successfully extending potential application of(Ba,K)(Zn,Mn)_2 As_2.

关键词： chemical pressure (Ba,K)(Zn,Mn)2As2 diluted magnetic semiconductor iso-valent doping

Gnetifolin K, a New Stilbene Diglucoside from Gnetum parvifolium

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Chinese Chemical Letters 1997年第6期8卷 509-510页

作者： Xu, q Lin, M CHINESE ACAD MED SCI INST MAT MEDBEIJING 100050PEOPLES R CHINA BEIJING UNION MED COLL BEIJING 100050PEOPLES R CHINA

A new stilbene diglucoside, gnetifolin K, was isolated from the lianas of Gnetum parvifolium. Its structure was established as isorhapotigenin-3,4'-di-O-beta-D-glucoside on the basis of spectral and chemical evidence.

关键词： Gnetifolin K a New Stilbene Diglucoside from Gnetum parvifolium

Molecular Arrangement of a Bolaamphiphilic Anthrancene Derivative in Langmuir-Blodgett Film

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Chinese Chemical Letters 2001年第12期12卷 1105-1108页

作者： Lu, q Liu, MH Chinese Acad Sci Lab Colloid & Interface Sci Ctr Mol Sci Inst Chem Beijing 100080 Peoples R China

This paper reports the molecular assembly in the LB film of a novel bolaamphiphilic anthracene derivative (BISANS) in comparison with that of one-headed amphiphilic anthracene derivative (ANS). While ANS formed a stretched monolayer at the air/water interface, BISANS underwent aggregation to form crystal film on the water surface. Both of the H-aggregates and J-aggregates exist in the transferred LB films of bolaamphiphilic BISANS, only J-aggregates formed in the LB film of ANS.

关键词： bolaamphiphile air/water interface stretched monolayer

Bosonic discrete supersymmetry for quasi-two-dimensional optical arrays

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Photonics research 2019年第11期7卷 1240-1243页

作者： q.Zhong S.Nelson M.Khajavikhan D.N.Christodoulides r.El-Ganainy Department of Physics Michigan Technological UniversityHoughtonMichigan 49931USA Henes Center for quantum Phenomena Michigan Technological UniversityHoughtonMichigan 49931USA College of Optics&Photonics-CrEOL University of Central FloridaOrlandoFlorida 32816USA

We apply the notion of discrete supersymmetry based on matrix factorization to quantum systems consisting of coupled bosonic oscillators to construct isospectral bosonic quantum networks. By using the algebra that arises due to the indistinguishability of bosonic particles, we write down the Schr?dinger equations for these oscillators in the different boson-number sectors. By doing so, we obtain, for every partner quantum network, a system of coupled differential equations that can be emulated by classical light propagation in optical waveguide *** mathematical scheme allows us to build quasi-two-dimensional optical arrays that are either isospectral or share only a subset of their spectrum after deliberately omitting some chosen eigenstates from the spectrum. As an example, we use this technique(which we call bosonic discrete supersymmetry or BD-SUSY) to design two optical, silica-based waveguide arrays consisting of six and three elements, respectively, with overlapping eigenspectrum.

关键词： spectrum. symmetry quasi

SEPArATION　CHArACTErISTICS　OF　THE　HYDrOCYCLONE　WITH　A　CENTrAL　CONE　AND　ANNULAr　TEETH

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中国有色金属学会会刊：英文版 1996年第4期6卷 11-15页

作者： Chu, LY Chen, WM Luo, q NOrTHEASTErN UNIV DEPT MINERAL ENGN SHENYANG 110006 PEOPLES R CHINA SICHUAN UNION UNIV DEPT CHEM PROC MACHINERY CHENGDU 610065 PEOPLES R CHINA

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关键词： ydrocyclone central cone annular teeth separation sharpness classification efficiency separation characteristics

New Alkaloids from the rhizomes of Goniothalamus Griffithii

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Chinese Chemical Letters 1998年第11期9卷 0-0,0-0页

作者： Zhang Y.J. Kong M. Chen r.Y. Yu D.q. Institute of Materia Medica Chinese Academy of Medical Sciences Peking Union Medical College Beijing 100050 China

Three new alkaloids, griffithdionc 1, griffiazanone A 2 and griffiazanone B 3 were isolated from the rhizomes of Goniothalamus griffithii Hook. F. el. Thoms. Their structures were elucidated by analysis the spectral data (Ir, UV, MS, 1 H and 13C NMr, HMBC, NOE experiment).The absolute configuration of griffithazanone A 2 was determined by Mosher's methods.

关键词： Goniothalamus griffithii phenanthrene lactam alkaloids griffithdione griffiazadioneA and griffiazadione B