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An Improved Repetitive-Control System Using a Complex-Coefficient Filter

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IEEE/CAA Journal of Automatica Sinica 2025年第1期12卷 282-284页

作者： Qicheng Mei jinhua She Fei Long Yanjun Shen the College of Electrical Engineering and New Energy China Three Gorges University the Hubei Provincial Key Laboratory for Operation and Control of Cascaded Hydropower Station the School of Engineering Tokyo University of Technology

Dear Editor,This letter presents an improved repetitive controller(IRC) that uses a complex-coefficient filter to enhance the tracking performance of a system for periodic signals. Compared with the low-pass filter used in the conventional repetitive controller(CRC), the complex-coefficient filter causes less change in the phase and amplitude of a signal at the frequencies of the periodic signal, especially at the fundamental frequency, when the two filters have the same cutofffrequency.

关键词： Low pass filters

Mn/S diatomic sites in C3N4 to enhance O2 activation for photocatalytic elimination of emerging pollutants

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Journal of Environmental Sciences 2025年第3期149卷 512-523页

作者： Chengji Sui Zixuan Nie Xiaobin Xie Yifeng Wang Lingshuai Kong Shou-Qing Ni jinhua Zhan Key Laboratory for Colloid&Interface Chemistry of Education Ministry School of Chemistry and Chemical EngineeringShandong UniversityJinan 250100China Institute of Eco-Environmental Forensics School of Environmental Science and EngineeringShandong UniversityQingdao 266237China

Oxygen activation leading to the generation of reactive oxygen species(ROS)is essential for photocatalytic environmental *** limited efficiency of O_(2)adsorption and reductive activation significantly limits the production of ROS when employing C_(3)N_(4)for the degradation of emerging *** with metal single atoms may lead to unsatisfactory efficiency,due to the recombination of photogenerated electron-hole ***,Mn and S single atoms were introduced into C_(3)N_(4),resulting in the excellent photocatalytic ***/S-C_(3)N_(4)achieved 100%removal of bisphenol A,with a rate constant 11 times that of pristine C_(3)N_(4).According to the experimental results and theoretical simulations,Satoms restrict holes,facilitating the photo-generated carriers’***-atom Mn acts as the O_(2)adsorption site,enhancing the adsorption and activation of O_(2),resulting the generation of *** study presents a novel approach for developing highly effective photocatalysts that follows a new mechanism to eliminate organic pollutants from water.

关键词： Photocatalytic degradation O_(2)activation Reactive oxygen species Emerging pollutants Single-atom catalyst

Multifunctional Nacre‑Like Nanocomposite Papers for Electromagnetic Interference Shielding via Heterocyclic Aramid/MXene Template‑Assisted In‑Situ Polypyrrole Assembly

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Nano-Micro Letters 2025年第3期17卷 37-54页

作者： jinhua Xiong Xu Zhao Zonglin Liu He Chen Qian Yan Huanxin Lian Yunxiang Chen Qingyu Peng Xiaodong He National Key Laboratory of Science and Technology On Advanced Composites in Special Environments Center for Composite Materials and StructuresHarbin Institute of TechnologyHarbin 150080People’s Republic of China

Robust, ultra-flexible, and multifunctional MXene-basedelectromagnetic interference (EMI) shielding nanocomposite filmsexhibit enormous potential for applications in artificial intelligence,wireless telecommunication, and portable/wearable electronic *** this work, a nacre-inspired multifunctional heterocyclic aramid(HA)/MXene@polypyrrole (PPy) (HMP) nanocomposite paper withlarge-scale, high strength, super toughness, and excellent tolerance tocomplex conditions is fabricated through the strategy of HA/MXenehydrogel template-assisted in-situ assembly of PPy. Benefiting from the"brick-and-mortar" layered structure and the strong hydrogen-bondinginteractions among MXene, HA, and PPy, the paper exhibits remarkable mechanical performances, including high tensile strength (309.7 MPa),outstanding toughness (57.6 MJ m−3), exceptional foldability, and structural stability against ultrasonication. By using the template effect ofHA/MXene to guide the assembly of conductive polymers, the synthesized paper obtains excellent electronic conductivity. More importantly,the highly continuous conductive path enables the nanocomposite paper to achieve a splendid EMI shielding effectiveness (EMI SE) of 54.1 dBat an ultra-thin thickness (25.4 μm) and a high specific EMI SE of 17,204.7 dB cm2g−1. In addition, the papers also have excellent applicationsin electromagnetic protection, electro-/photothermal de-icing, thermal therapy, and fire safety. These findings broaden the ideas for developinghigh-performance and multifunctional MXene-based films with enormous application potential in EMI shielding and thermal management.

关键词： MXene Remarkable mechanical properties Heterocyclic aramid Electromagnetic interference shielding Polypyrrole Multifunctionality

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Deciphering the role of ultra-low-loaded rhodium in NiFe-MIL-53 for superior oxygen evolution reaction

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Journal of Energy Chemistry 2025年第1期100卷 77-86页

作者： Jinzhi Jia jinhua Zhang Kailu Guo Lanyue Zhang Gening Du Hao You Junfeng Huang Mudong Tu Hua Li Yong Peng Wei Dou Cailing Xu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringSchool of Materials and EnergyLanzhou UniversityLanzhou 730000GansuChina College of Chemistry and Chemical Engineering Luoyang Normal UniversityLuoyang 471934HenanChina

Designing highly active and stable electrocatalysts of oxygen evolution reaction(OER)is one of the crucial *** this study,a novel OER electrocatalyst,NiFe-MIL-53 modified with ultra-low rhodium(Rh@NiFe-MIL-53),is successfully prepared via the hydrothermal ***-situ Raman spectroscopy and electrochemical impedance spectroscopy reveal that the doped Rh accelerates the phase transformation of NiFe-MIL-53 and the in-situ formed Rh@NiFeOOH is the actual active *** importantly,the enhanced reversibility of electrochemical reconstruction between NiFeOOH and NiFe(OH)_(2)after doping Rh is beneficial for improving the electrochemical stability of the catalyst.X-ray photoelectron spectroscopy spectra show the strong electronic interaction between single-atom Rh and Ni/Fe in Rh@***,theoretical calculations confirm that the integration of single-atom Rh into the NiFeOOH successfully reduces the band gap,regulates the d-band center(εd),accelerates the charge transfer,and optimizes the adsorption behavior of oxygen-containing intermediates,thereby lowering the energy barrier of rate-determining ***,the optimized Rh@NiFe-MIL-53 exhibits excellent OER activity(240 mV)with a small Tafel slope of 48.2 mV dec^(-1)and long-term durability(over1270 h at 10 m A cm^(-2)and 110 h at 200 mA cm^(-2)).This work presents a new perspective on designing highly efficient OER electrocatalysts.

关键词： NiFe-MIL-53 Rh Electrochemical reconstruction Catalytic mechanism Oxygen evolution reaction

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Distribution of Human Papillomavirus (HPV) Infection in Women of Appropriate Age in Beiliu City and Recommendations for Public Health Intervention

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Natural Science 2025年第1期17卷 1-6页

作者： Haiquan Li jinhua Wei Huan Zhao Department of Laboratory Beiliu Maternal and Child Health Hospital Yulin China Department of Laboratory Longan Maternal and Child Health Hospital Nanning China Department of Laboratory Chongzuo Maternal and Child Health Hospital Chongzuo China

Objective: This study aims to analyze the distribution of positive human papillomavirus (HPV) infections among women of appropriate age in Beiliu City during cervical cancer screening in 2024, providing data support for subsequent public health interventions. Methods: A retrospective analysis was conducted on the HPV test results from January 1, 2024, to November 30, 2024, at Beiliu Maternal and Child Health Hospital. We statistically analyzed the positive rates of different HPV genotypes and the co-infection status of multiple genotypes. Results: A total of 7558 individuals were tested, with 1103 positive cases identified, resulting in a positivity rate of 14.59%. Among these, HPV type 52 had the highest positive rate, accounting for 18.47%. The co-infection analysis showed that there were 788 cases with single genotype positivity, 236 with double genotype positivity, and 58 with triple genotype positivity, while cases with multiple genotypes simultaneously positive were relatively rare. Conclusion: The HPV infection rate among women of appropriate age in Beiliu City is relatively high, especially for high-risk HPV types. To reduce the future incidence of cervical cancer, it is recommended to enhance health education and vaccination efforts for this population.

关键词： HPV Infection Cervical Cancer Screening Positive Distribution Women of Appropriate Age Public Health

An enhanced equivalent input disturbance approach to current control of PMSM with periodic and aperiodic disturbances

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Science China(Information Sciences) 2025年第03期68卷 272-285页

作者： Tao YANG Youwu DU Bo LI Weihua CAO Chuanke ZHANG jinhua SHE School of Electrical & Information Jiangsu University of Technology School of Automation China University of Geosciences School of Engineering Tokyo University of Technology

The current-loop control of a permanent magnet synchronous motor(PMSM) system suffers from periodic and aperiodic disturbances, which result in current ripples and degrade control performance. This paper presents an enhanced equivalent-input-disturbance(EID) approach to reject periodic and aperiodic disturbances in the current loop of a *** additional quasi-resonant compensators(QRCs) are integrated into a conventional EID estimator with a low-pass filter(LPF) to handle the disturbances. The configuration of an enhanced EID(EEID)-based control system for PMSM current loop is explained. An analysis in the frequency domain shows the mechanism of the presented method for rejecting periodic and aperiodic disturbances simultaneously. It reveals that the sensitivity reduction of the system for aperiodic disturbances is mainly determined by the bandwidth of the LPF and that for periodic disturbances is determined by the parameters of the *** stability of the system is analyzed using the Nyquist stability criterion. The design algorithm for system parameters is provided. Compared to the conventional EID approach, the proposed method provides an additional degree of freedom to deal with periodic disturbances. The design of the QRCs is independent of each other, which makes the proposed method flexible and easy to implement. The effectiveness and the superiority of the EEID approach are validated by simulation results of a PMSM system.

关键词： equivalent input disturbance (EID) disturbance rejection permanent magnet synchronous motor (PMSM) periodic and aperiodic disturbances quasi-resonant compensator

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Multi-Objective Optimization Method for Performance Prediction Loss Model of Centrifugal Compressors

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Journal of Thermal Science 2025年第02期 590-606页

作者： ZHANG Lei FENG Xueheng YUAN Wei CHEN Ruilin ZHANG Qian LI Hongyang AN Guangyao LANG jinhua Department of Power Engineering North China Electric Power University Hebei Key Laboratory of Low Carbon and High Efficiency Power Generation Technology North China Electric Power University Baoding Key Laboratory of Low Carbon and High Efficiency Power Generation Technology North China Electric Power University

The selection of loss models has a significant effect on the one-dimensional mean streamline analysis for obtaining the performance of centrifugal *** this study,a set of optimized loss models is proposed based on the classical loss models suggested by Aungier,Coppage,and *** proportions and variation laws of losses predicted by the three sets of models are discussed on the NASA Low-Speed-Centrifugal-Compressor(LSCC) under the mass flow of 22 kg/s to 36 kg/*** results indicate that the weights of Skin friction loss,Diffusion loss,Disk friction loss,Clearance loss,Blade loading loss,Recirculation loss,and Vaneless diffuser loss are greater than 10%,which is dominant for performance ***,these losses are considered in the composition of new loss *** addition,the multi-objective optimization method with the Genetic Algorithm(GA) is applied to the correction of loss coefficients to obtain the final optimization loss *** with the experimental data,the maximum relative error of adiabatic the three classical models is 7.22%,while the maximum relative error calculated by optimized loss models is 1.22%,which is reduced by 6%.Similarly,compared with the original model,the maximum relative error of the total pressure ratio is also *** a result,the present optimized models provide more reliable performance prediction in both tendency and accuracy than the classical loss models.

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InNi alloy-induced interface effect promoting the parallel electron transfer: improved photothermal catalytic CO2 hydrogenation

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Science China Chemistry 2025年

作者： Haoyu Zhang Yuhang Li Yu Nie Xinyu Dou Haodong Ji Xin Tan jinhua Ye Tao Yu School of Chemical Engineering and Technology Tianjin University Eco-environment and Resource Efficiency Research Laboratory School of Environment and Energy Peking University Shenzhen Graduate School School of Environmental Science and Engineering Tianjin University Advanced Catalytic Materials Research Center School of Materials Science and Engineering Tianjin University Research Center for Solar Driven Carbon Neutrality Hebei University

Photothermal catalytic CO2hydrogenation is an effective means of utilizing carbon ***,it is severely limited in terms of kinetics and ***,it is necessary to meticulously design catalysts to solve this ***,a sandwich structured NiO@InNi/In2O3is designed to intrinsically regulate the direction of photogenerated carriers transfer,resulting in a CO yield of 42.97 mmol g-1h-1(1290.3μmol h-1) with a selectivity near to 100%.InNi alloy favors the collection of photogenerated carriers by the parallel way and enhancement of the adsorption and activation of *** grown on the surface of InNi alloy not only improves the adsorption of H2and provides sufficient H+for the reaction,but also makes InNi alloy more stable during the reaction *** photothermal effect caused by In2O3accelerates the transfer of photogenerated carriers and increases the surface temperature of the catalyst,thereby synergistically promoting the reaction from a kinetic *** work ameliorates the kinetic and thermodynamic limitations of the photothermal catalytic CO2hydrogenation process through rationally designing the electron transfer direction of the sandwich structured catalysts to parallel way.

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Bulk photovoltaic effect in two-dimensional ferroelectric α-In2Se3

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Science China(Information Sciences) 2025年第2期68卷 285-292页

作者： Huiting WANG Shuaiqin WU Yan CHEN Qianru ZHAO jinhua ZENG Ruotong YIN Yuqing ZHENG Chang LIU Shukui ZHANG Tie LIN Hong SHEN Xiangjian MENG Jun GE Xudong WANG Junhao CHU Jianlu WANG State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of Sciences University of Chinese Academy of Sciences Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and Perception Institute of OptoelectronicsFudan University Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences Frontier Institute of Chip and System Fudan University

Non-centrosymmetric material systems can generate spontaneous photocurrent without a p-n junction under uniform illumination, which is known as the bulk photovoltaic effect（BPVE）. It has garnered significant attention for its application potential in the fields of energy harvesting and photoelectric detection. In this study, we report the BPVE observed in twodimensional ferroelectric α-In2Se3multilayer flakes. The reversal in spontaneous photocurrent polarity is observed and associated with the out-of-plane ferroelectric polarization direction. The spontaneous photocurrent originating from the shift current is also polarization-sensitive. The amplitude of spontaneous photocurrent is further increased by one order of magnitude through vacuum annealing. Our results provide a further application potential for new-generation photodetectors based on BPVE with low power consumption and multi-dimensional optoelectronic detection.

关键词： bulk photovoltaic effect 2D ferroelectrics 3R $\alpha$-In$_2$Se$_3$ shift current self-powered photodetection

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