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Dielectric-ion-conductive ZnNb2O6 layer enabling rapid desolvation and diffusion for dendrite-free Zn metal batteries

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Journal of Energy Chemistry 2025年第1期100卷 693-701页

作者： Haifeng Yang Jian Wang Panpan zhang Xiaomin Cheng Qinghua Guan jing Dong Bixian Chen Lujie Jia jing zhang Yongzheng zhang Yunjian Liu Hongzhen Lin School of Materials Science and Engineering Jiangsu University i-Lab & CAS Key Laboratory of Nanophotonic Materials and Devices Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Helmholtz Institute Ulm (HIU) Karlsruhe Institute of Technology (KIT) School of Materials Science and Engineering Xi'an University of Technology State Key Laboratory of Chemical Engineering East China University of Science and Technology

Rechargeable aqueous zinc-metal batteries （AZMBs） are promising candidates for large-scale energy storage systems due to their low cost and high ***,their performance and sustainability are significantly hindered by the sluggish desolvation kinetics at the electrode/electrolyte interface and the corresponding hydrogen evolution reaction where active water molecules tightly participate in the Zn（H2O）62+solvation ***,learnt from self-generated solid electrolyte interphase （SEI） in anodes,the dielectric but ion-conductive zinc niobate nanoparticles artificial layer is constructed on metallic Zn surface （ZNB@Zn）,acting as a rapid desolvation *** zincophilic and dielectric-conductive properties of ZNB layer accelerate interfacial desolvation/diffusion and suppress surface corrosion or dendrite formation,achieving uniform Zn plating/stripping behavior,as confirmed by electronic/optical microscopies and interface spectroscopical measurements together with theoretical ***,the as-prepared ZNB@Zn electrode exhibits excellent cycling stability of over 2000 h and robust reversibility （99.54%） even under high current density and depth of discharge ***,the assembled ZNB@Zn-based full cell displays high capacity-retention rate of 80.21%after 3000 cycles at 5 A g-1and outstanding rate performance up to 10 A *** large-areal pouch cell is stabilized for hundreds of cycles,highlighting the bright prospects of the dielectric but ion-conductive layer in further application of AZMBs.

关键词： Zn metal battery Dielectric artificial layer Rapid ion diffusion Zincophilic diffusion Active water inhibition

The interaction between KIF21A and KANK1 regulates dendritic morphology and synapse plasticity in neurons

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Neural Regeneration Research 2025年第1期20卷 209-223页

作者： Shi-Yan Sun Lingyun Nie jing zhang Xue Fang Hongmei Luo Chuanhai Fu Zhiyi Wei Ai-Hui Tang Hefei National Research Center for Physical Sciences at the Microscale CAS Key Laboratory of Brain Function and DiseaseMinistry of Education Key Laboratory for Membrane-less Organelles and Cellular DynamicsDivision of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefeiAnhui ProvinceChina CAS Center for Excellence in Molecular Cell Sciences Division of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Department of Neurobiology School of Life SciencesSouthern University of Science and TechnologyShenzhenGuangdong ProvinceChina Brain Research Center Southern University of Science and TechnologyShenzhenGuangdong ProvinceChina

Morphological alterations in dendritic spines have been linked to changes in functional communication between neurons that affect learning and ***-4 KIF21A helps organize the microtubule-actin network at the cell cortex by interacting with KANK1;however,whether KIF21A modulates dendritic structure and function in neurons remains *** this study,we found that KIF21A was distributed in a subset of dendritic spines,and that these KIF21A-positive spines were larger and more structurally plastic than KIF21A-negative ***,the interaction between KIF21A and KANK1 was found to be critical for dendritic spine morphogenesis and synaptic *** of either KIF21A or KANK1 inhibited dendritic spine morphogenesis and dendritic branching,and these deficits were fully rescued by coexpressing full-length KIF21A or KANK1,but not by proteins with mutations disrupting direct binding between KIF21A and KANK1 or binding between KANK1 and *** down KIF21A in the hippocampus of rats inhibited the amplitudes of long-term potentiation induced by high-frequency stimulation and negatively impacted the animals’cognitive *** together,our findings demonstrate the function of KIF21A in modulating spine morphology and provide insight into its role in synaptic function.

关键词： actin cytoskeleton dendrite KANK1 KIF21A microtubule spine morphology spine synaptic plasticity talin1

汉语作为方法:从早期文字记录看汉语诗学的当代价值

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河北学刊 2025年第1期45卷 67-73页

作者：张晶刘璇中国传媒大学辽宁师范大学文学院

汉语兼具“文”与“言”的双重属性,与以“言”为主的印欧语相区别。语法与逻辑的同根同源使印欧语在理论表述中陷入了概念与经验的争执,而汉语贯通形而上与形而下的特质使汉语表述本身即构成一种方法。作为“道”之文的载体,中国早期... 详细信息

汉语兼具“文”与“言”的双重属性,与以“言”为主的印欧语相区别。语法与逻辑的同根同源使印欧语在理论表述中陷入了概念与经验的争执,而汉语贯通形而上与形而下的特质使汉语表述本身即构成一种方法。作为“道”之文的载体,中国早期记录及其文法结构提供了关键信息,甲骨卜辞的体例制式为“易”类文献的结构提供了可追溯的原型,也为探索“论出于易”对汉语诗学功能的塑造提供了重要线索。其中,干支配伍的宇宙纪日为“以时系事”的话语表述提供了超线性时空结构;“正反对贞”以对言的形式表现语义的动态平衡与赋形必变的道理;“主题+阐释”的体例结构以逐层累积的文本层次为断言的疑难提供了积极的方案。汉语文法能够在表述判断的同时保持对“变”的关切,这为建构既能规范描述艺术经验又能直面人类自身处境的理论话语提供了时代价值。

关键词：汉语早期文字记录文法结构汉语诗学当代价值

雾收集用单向导湿针织物涂层摩擦制备及性能研究

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丝绸 2025年第1期62卷 49页

作者：张静广靖陈诚新疆大学特色纺织品与清洁染整技术重点实验室新疆智能与绿色纺织重点实验室

随着人口爆炸、工业和高新产业发展的持续，工厂和居民对清洁用水需求日益增加，水雾收集器件不断涌现，而现有水雾收集器件多采用飞秒激光刻蚀等方式达到符合要求的浸润性表面，对设备要求较高。本文基于简便的室温自发胶凝作用，温和... 详细信息

随着人口爆炸、工业和高新产业发展的持续，工厂和居民对清洁用水需求日益增加，水雾收集器件不断涌现，而现有水雾收集器件多采用飞秒激光刻蚀等方式达到符合要求的浸润性表面，对设备要求较高。本文基于简便的室温自发胶凝作用，温和构建凝胶聚合物基质，通过引入反应组分以控制胶凝成形期间的微观形貌与表面能分布，经室温修饰形成超疏水聚合物复合材料。以针织物为基底、摩擦为手段构制Janus针织物涂层，利用其润湿不对称性实现单向导湿，进而在捕雾集水的同时减缓水蒸发以提升应用效率，达到低成本且高效的雾收集。

关键词：雾收集单向导湿针织物涂层摩擦制备 Janus

Pulp health and calcific healing of a complicated crown–root fracture with additional root fracture in a maxillary incisor: A case report

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World Journal of Clinical Cases 2025年第3期13卷 42-49页

作者： Na Li Yue-Yue Ren Ying Tang Qi Yang Tian-Tian Meng Song Li jing zhang Stomatological Hospital and College Anhui Medical UniversityHefei 230032Anhui ProvinceChina Department of Endodontics The Affiliated Stomatological Hospital of Xuzhou Medical UniversityXuzhou 221000Jiangsu ProvinceChina

BACKGROUND Complicated crown–root fracture (CRF) involves severe injury to the crown, root,and pulp, and may be accompanied by multiple root fractures. The loss of a toothhas lifelong consequences for children and teenagers, but the maintenance of pulphealth and the calcific healing of multiple root fractures are rarely reported in *** SUMMARY This case reports healing of a permanent tooth with complicated crown–root andadditional root fractures, in which pulp health was maintained. A 10-year-old girlfell and fractured the root of her maxillary left central incisor at the cervical *** the coronal fragment was repositioned, the tooth was splinted until thetooth was no longer mobile, 2 years later. Eight years after treatment, the toothhas remained asymptomatic with vital pulp and localized gingival ***-beam computed tomography revealed not only calcified healing of the CRFbut also spontaneous healing in an additional undiagnosed root fracture. Thefracture line on the enamel could not be healed by hard tissue and formed agroove in the cervical crown. It was speculated that the groove was related to thelocalized gingival *** This case provides a clinical perspective of the treatment of a tooth with acomplicated CRF and an additional root fracture.

关键词： Complicated crown-root fracture Multiple root fracture Spontaneous healing Cone-beam computed tomography Long-term follow-up Case report

Knowledge Learning With Crowdsourcing:A Brief Review and Systematic Perspective

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IEEE/CAA Journal of Automatica Sinica 2022年第5期9卷 749-762页

作者： jing zhang IEEE School of Computer Science and Engineering Nanjing University of Science and TechnologyNanjing 210094China

Big data have the characteristics of enormous volume,high velocity,diversity,value-sparsity,and uncertainty,which lead the knowledge learning from them full of *** the emergence of crowdsourcing,versatile information can be obtained on-demand so that the wisdom of crowds is easily involved to facilitate the knowledge learning *** the past thirteen years,researchers in the AI community made great efforts to remove the obstacles in the field of learning from *** concentrated survey paper comprehensively reviews the technical progress in crowdsourcing learning from a systematic perspective that includes three dimensions of data,models,and learning *** addition to reviewing existing important work,the paper places a particular emphasis on providing some promising blueprints on each dimension as well as discussing the lessons learned from our past research work,which will light up the way for new researchers and encourage them to pursue new contributions.

关键词： Crowdsourcing data fusion learning from crowds learning paradigms learning with uncertainty

Nano high-entropy oxide cathode with enhanced stability for direct borohydride fuel cells

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Journal of Energy Chemistry 2025年第1期 309-316页

作者： Lei zhang Lingfeng Kuang Lianke zhang Wen Chu Haiying Qin jing zhang Junjing He Hualiang Ni Hongzhong Chi New Energy Materials Research Center College of Materials and Environmental Engineering Hangzhou Dianzi University School of Materials Science and Engineering Zhejiang University Key Laboratory of MEMS of Ministry of Education School of Integrated Circuits Southeast University

High-entropy materials have become high-activity electrocatalysis owing to their high-entropy effect and multiple active ***,we synthesize a series of carbon-supported nano high-entropy oxides（HEOs/C）,specifically （PtFeCoNiCu）O/C,using a carbothermal shock （CTS） method for application as a cathode catalyst in direct borohydride fuel cells （DBFCs）.The microstructure of the prepared catalysts was characterized by X-ray photoelectron spectroscopy,X-ray absorption fine structure,and transmission electron *** prepared （PtFeCoNiCu）O/C,with particle sizes ranging from 2 to 4 nm,demonstrates 3.94 transferred electrons towards the oxygen reduction reaction in an alkaline environment,resulting in a minimal H2O2yield of 2.6%.Additionally,it exhibits a Tafel slope of 61 mV dec-1,surpassing that of commercial Pt/C (82 mV dec-1).Furthermore,after 40,000 cycles of cyclic voltammetry（CV） testing,the half-wave potential of （PtFeCoNiCu）O/C shows a positive shift of 3 mV,with no notable decline in the limiting current *** （PtFeCoNiCu）O/C is used as a cathode catalyst in DBFCs,the DBFC achieves a maximum power density of 441 mW cm-2at 60°C and sustains a cell voltage of approximately 0.73 V after 52 h at 30°*** findings confirm that HEO/C is a promising cathode catalyst for DBFCs.

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A hybrid artificial photosynthesis system with molecular catalysts covalently linked onto TiO2 as electron relay for efficient photocatalytic hydrogen evolution

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Journal of Materials Science & Technology 2020年第15期47卷 147-152页

作者： Jie zhang Gehong zhang jing zhang School of Civil and Architecture Engineering Xi'an Technological UniversityXi'an710021China

Efficient charge carrier transfer from light harvesters to catalysts greatly determines the photocatalytic activity in an artificial photosynthesis(AP) system for solar hydrogen *** this study,an AP system composed of xanthene dye as light harvester and cobaloxime molecular complex as catalyst,with TiO2 as electron relay,was designed for photocatalytic hydrogen evolution under visible light(λ>420 nm).It was demonstrated that with cobaloxime molecule covalently linked onto the TiO2 electron relay,the resulting hybrid AP system exhibited much increased photocatalytic activity as compared to that without *** greatly increased photocatalytic activity should be due to the efficient electron transfer from xanthene dye as light harvester and cobaloxime molecular complex as catalyst,shuttled by the TiO2 electron relay,for the following water reduction *** present study demonstrates a facile and feasible strategy to guide the design of high performance AP systems through the electron relay shuttled and promoted cha rge transfer process.

关键词： Artificial photosynthesis Molecular catalysts Electron relay Photocatalytic hydrogen evolution

A Dugdale-Barenblatt model for elliptical orifice problem with asymmetric cracks in one-dimensional orthorhombic quasicrystals

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Applied Mathematics and Mechanics(English Edition) 2023年第9期44卷 1533-1546页

作者： jing zhang Guanting LIU College of Mathematics Science Inner Mongolia Normal UniversityHuhhot 010022China

By means of Muskhelishvili’s method and the technique of generalized conformal mapping,the physical plane problems are transformed into regular mathematical problems in quasicrystals(QCs).The analytical solution to an elliptical orifice problem with asymmetric cracks in one-dimensional(1D)orthorhombic QCs is *** using the Dugdale-Barenblatt model,the plastic simulation at the crack tip of the elliptical orifice with asymmetric cracks in 1D orthorhombic QCs is ***,the size of the atomic cohesive force zone is determined precisely,and the size of the atomic cohesive force zone around the crack tip of an elliptical orifice with a single crack or two symmetric cracks is obtained.

关键词： one-dimensional(1D)orthorhombic quasicrystal(QC) Dugdale-Barenblatt model atomic cohesive force zone crack