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Multidimensional hollow SiO_(2)/C nanofibers modified by magnetic nanocrystals for electromagnetic energy conversion and lithium battery storage

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Nano Research 2024年第8期17卷 7301-7314页

作者： Chen Han Qi Zheng Juncheng jin Jiajia Zhang Wen-Qiang Cao Kun xiang Min Zhang Mao-Sheng Cao Anhui Provincial Laboratory of Biomimetic Sensor and Detecting Technology College of Materials and Chemical EngineeringWest Anhui UniversityLu’an 237012China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Department of Physics Beijing Technology and Business UniversityBeijing 100048China

Multifunctional materials are powerful tools to support the advancement of energy conversion *** with prominent electromagnetic and electrochemical properties can realize the conversion of electromagnetic energy and solve the subsequent storage ***,an electrospinning-thermal reduction method is employed to construct ultrafine nickel nanoparticle modified porous SiO_(2)/C(Ni-SiO_(2)/C)hollow nanofibers as promising materials for applications in both electromagnetic wave absorption(EMA)and lithium-ion ***,when used as an EMA material,the reflection loss(RL)of Ni-SiO_(2)/C can reach−47.8 dB at 15.8 GHz with a matching thickness of 2.2 *** excellent microwave absorption performance can be attributed to the enhanced conduction loss,polarization relaxation,synergistic magnetic loss,and preferred impedance matching,which result from multi-component magnetic/dielectric synergy and the unique interconnected multidimensional hollow ***,the electronic conductivity and electrochemical activity of the samples are significantly enhanced due to the uniform distribution of ultrafine Ni nanoparticles in the amorphous SiO_(2)/C ***,the hierarchical hollow porous structure provides sufficient free space for volume change during lithiation/delithiation ***,the Ni-SiO_(2)/C nanocomposite exhibits a high reversible capacity of 917.6 mAh·g^(−1)at 0.1 A·g^(−1).At a high current density of 2 A·g^(−1),a capacity of 563.9 mAh·g^(−1)can be maintained after 300 *** energy conversion-storage device is designed to store waste electromagnetic energy in the form of useful electrical *** work inspires the development of high-performance bifunctional materials.

关键词： Ni-SiO_(2)/C nanofiber electromagnetic absorption lithium-ion storage electrospinning multidimensional structure

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Lattice-distorted Pt wrinkled nanoparticles for highly effective hydrogen electrocatalysis

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Nano Research 2024年第5期17卷 3819-3826页

作者： Xue Li xiang Han Zhenrui Yang Shun Wang Yun Yang Juan Wang Jiadong Chen Zhongwei Chen Huile jin Wenzhou Key Lab of Advanced Energy Storage and Conversion Zhejiang Province Key Lab of Leather EngineeringCollege of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China Institute of New Materials and Industry Technology College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China Department of Chemical Engineering Waterloo Institute for NanotechnologyUniversity of WaterlooWaterlooOntario N2L 3G1Canada

Modulating Pt surfaces through the introduction of lattice distortion emerges as immensely effective strategy that enhances the kinetics of alkaline hydrogen evolution and oxidation *** this study,we fabricated lattice-distorted Pt wrinkled nanoparticles(LD-Pt WNPs)for efficient hydrogen *** LD-Pt WNPs not only outperform the Pt/C benchmark in hydrogen oxidation reaction,achieving an excellent mass-specific current of 968.5 mA·mg_(Pt)^(-1)(9 times that of Pt/C),but also demonstrate outstanding hydrogen evolution reaction activity with a small overpotential of 58.0 *** experiments and density functional theory calculations reveal that lattice defects introduce an abundance of unsaturated coordination atoms while modifying the d-band center of *** dual effect optimizes the binding strength of crucial H and OH intermediates,leading to a significant reduction in the energy barrier of the reaction bottleneck,commonly known as the Volmer *** work unveils a fresh viewpoint on projecting and developing high efficiency electrocatalysts through defect engineering.

关键词： distortion nanoparticle hydrogen evolution reaction defect engineering hydrogen oxidation reaction

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氨氮与镉单一和复合作用对沉水植物穗花狐尾藻和轮叶黑藻光合能力的影响

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环境科学 2006年第10期27卷 1974-1978页

作者：许秋瑾金相灿王兴民陈书琴颜昌宙中国环境科学研究院湖泊研究中心北京100012

在水-土环境中,单一物质引起的污染很少,绝大多数污染是多种污染物质共存所造成的.利用碘量法测定溶解氧,研究了氨氮与镉单一和复合作用对沉水植物穗花狐尾藻和轮叶黑藻光合能力的影响.结果显示,氨氮浓度在4.0 mg.L-1时,对轮叶黑藻有较... 详细信息

在水-土环境中,单一物质引起的污染很少,绝大多数污染是多种污染物质共存所造成的.利用碘量法测定溶解氧,研究了氨氮与镉单一和复合作用对沉水植物穗花狐尾藻和轮叶黑藻光合能力的影响.结果显示,氨氮浓度在4.0 mg.L-1时,对轮叶黑藻有较强的胁迫作用,表现为光合作用的产氧量与呼吸作用的耗氧量均下降,而此浓度对穗花狐尾藻没有表现出胁迫作用;当镉处理浓度为0.2 mg.L-1时,镉对2种沉水植物都表现出明显的胁迫效应,且对轮叶黑藻的胁迫作用更强;当镉与氨氮复合作用时,对轮叶黑藻产生联合毒害作用,但对穗花狐尾藻毒害作用较轻,可能原因是穗花狐尾藻所含的粗纤维比轮叶黑藻少,细胞壁上能结合重金属的位点较少,所以吸附的镉相应减少,毒性较小.实验结果表明在进行湖泊水生植物修复时,相对于轮叶黑藻,穗花狐尾藻更适合作为生态恢复的先锋物种.

关键词：氨氮镉穗花狐尾藻轮叶黑藻光合作用呼吸作用

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STING-mediated IL-6 Inhibits OATP1B1 Expression via the TCF4 Signaling Pathway in Cholestasis

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Journal of Clinical and Translational Hepatology 2024年第8期12卷 701-712页

作者： Yan Guo Hongjia Zhang Nan Zhao Ying Peng Dongya Shen Yubin Chen Xiaoxun Zhang can-E Tang jin Chai Department of Endocrinology Xiangya HospitalCentral South UniversityChangshaHunanChina Department of Gastroenterology Institute of Digestive Diseases of PLACholestatic Liver Diseases Center and Center for Metabolic Associated Fatty Liver DiseaseThe First Affiliated Hospital(Southwest Hospital)to Third Military Medical University(Army Medical University)ChongqingChina Department of Clinical Pharmacology Xiangya HospitalCentral South UniversityChangshaHunanChina Department of Cardiac Surgery Xiangya HospitalCentral South UniversityChangshaHunanChina National Clinical Research Center for Geriatric Disorders Xiangya HospitalCentral South UniversityChangshaHunanChina

Background and Aims Organic anion-transporting polypeptides(OATPs)play a crucial role in the transport of bile acids and *** our previous study,interleukin 6(IL-6)reduced OATP1B3 levels in cholestatic ***,it remains unclear whether IL-6 inhibits OATP1B1 expression in cholestatic *** study aimed to investigate whether IL-6 can inhibit OATP1B1 expression and explore the underlying *** The effect of stimulator of interferon genes(STING)signaling on inflammatory factors was investigated in a cholestatic mouse model using RT-qPCR and enzyme-linked immunosorbent *** assess the impact of inflammatory factors on OATP1B1 expression in hepatocellular carcinoma,we analyzed OATP1B1 expression by RT-qPCR and Western Blot after treating PLC/PRF/5 cells with TNF-α,IL-1β,and *** elucidate the mechanism by which IL-6 inhibits OATP1B1 expression,we examined the expression of the OATP1B1 regulator TCF4 in PLC/PRF/5 and HepG2 cells using RT-qPCR and Western *** interaction mechanism betweenβ-catenin/TCF4 and OATP1B1 was investigated by knocking downβ-catenin/TCF4 through siRNA *** The STING inhibitor decreased inflammatory factor levels in the cholestatic mouse model,with IL-6 exhibiting the most potent inhibitory effect on ***-6 downregulatedβ-catenin/TCF4,leading to decreased OATP1B1 ***-downβ-catenin/TCF4 counteracted theβ-catenin/TCF4-mediated repression of *** STING-mediated IL-6 up-regulation may inhibit OATP1B1,leading to reduced transport of bile acids and bilirubin by *** may contribute to altered pharmacokinetics in patients with diseases associated with increased IL-6 production.

关键词： Inflammation Bile acid Bilirubin Cholestasis STING IL-6 β-catenin TCF4

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Fine-tuning the activation behaviors of ternary modular cabazitaxel prodrugs for efficient and on-target oral anti-cancer therapy

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Asian Journal of Pharmaceutical Sciences 2024年第2期19卷 188-203页

作者： Mingyang Zhang Yifan Miao can Zhao Tong Liu Xiyan Wang Zixuan Wang Wenxin Zhong Zhonggui He Chutong Tian jin Sun Department of Pharmaceutics Wuya College of InnovationShenyang Pharmaceutical UniversityShenyang 110016China Key Laboratory of Advanced Drug Delivery Systems of Zhejiang Province Hangzhou 310058China Joint International Research Laboratory of Intelligent Drug Delivery Systems Ministry of EducationShenyang 110016China Liaoning Provincial Institute of Drug Inspection and Testing Shenyang 110036China

The disulfide bond plays a crucial role in the design of anti-tumor prodrugs due to its exceptional tumor-specific redox responsiveness. However, premature breaking of disulfide bonds is triggered by small amounts of reducing substances (e.g., ascorbic acid, glutathione, uric acid and tea polyphenols) in the systemic circulation. This may lead to toxicity, particularly in oral prodrugs that require more frequent and high-dose treatments. Fine-tuning the activation kinetics of these prodrugs is a promising prospect for more efficient on-target cancer therapies. In this study, disulfide, steric disulfide, and ester bonds were used to bridge cabazitaxel (CTX) to an intestinal lymph vessel-directed triglyceride (TG) module. Then, synthetic prodrugs were efficiently incorporated into self-nanoemulsifying drug delivery system (corn oil and Maisine CC were used as the oil phase and Cremophor EL as the surfactant). All three prodrugs had excellent gastric stability and intestinal permeability. The oral bioavailability of the disulfide bond-based prodrugs (CTX-(C)S-(C)S-TG and CTX-S-S-TG) was 11.5- and 19.1-fold higher than that of the CTX solution, respectively, demonstrating good oral delivery efficiency. However, the excessive reduction sensitivity of the disulfide bond resulted in lower plasma stability and safety of CTX-S-S-TG than that of CTX-(C)S-(C)S-TG. Moreover, introducing steric hindrance into disulfide bonds could also modulate drug release and cytotoxicity, significantly improving the anti-tumor activity even compared to that of intravenous CTX solution at half dosage while minimizing off-target adverse effects. Our findings provide insights into the design and fine-tuning of different disulfide bond-based linkers, which may help identify oral prodrugs with more potent therapeutic efficacy and safety for cancer therapy.

关键词： Steric disulfide bond Triglyceride-like pr odrugs Cabazitaxel Lymphatic transport Oral chemotherapy

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Remaining useful life prediction for train bearing based on an ILSTM network with adaptive hyperparameter optimization

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Transportation Safety and Environment 2024年第2期6卷 75-86页

作者： Deqiang He jingren Yan Zhenzhen jin Xueyan Zou Sheng Shan Zaiyu xiang Jian Miao State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi Key Laboratory of Manufacturing System&Advanced Manufacturing Tec hnologySc hool of Mec hanical EngineeringGuangxi Univ ersityNanning 530004GuangxiChina Zhuzhou CRRC Times Electric Co. Ltd.Zhuzhou 412001HunanChina

Remaining useful life(RUL)prediction for bearing is a significant part of the maintenance of urban rail transit *** RUL is closely linked to the reliability and safety of train running,but the current prediction accuracy makes it difficult to meet the re-quirements of high reliability *** at the problem,a prediction model based on an improved long short-term memory(ILSTM)network is ***,the variational mode decomposition is used to process the signal,the intrinsic mode function with stronger representation ability is determined according to energy entropy and the degradation feature data is constructed com-bined with the time domain ***,to improve learning ability,a rectified linear unit(ReLU)is applied to activate a fully connected layer lying after the long short-term memory(LSTM)network,and the hidden state outputs of the layer are weighted by attention *** Harris Hawks optimization algorithm is introduced to adaptively set the hyperparameters to improve the performance of the ***,the ILSTM is applied to predict bearing *** experimental cases,the better perfor-mance in bearing RUL prediction and the effectiveness of each improving measures of the model are validated,and its superiority of hyperparameters setting is demonstrated.

关键词： train bearing remaining useful life prediction long short-term memory(LSTM) attention mechanism Harris Hawks op-timization(HHO)

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人工湿地处理农业径流的研究进展

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生态学报 2007年第6期27卷 2627-2635页

作者：卢少勇张彭义余刚金相灿清华大学环境科学与工程系中国环境科学研究院湖泊生态环境创新基地国家环境保护湖泊污染控制重点实验室北京100012

人工湿地(CW)是独特的土壤-植物-微生物-动物系统。按水流方式分为表面流湿地(FWS)和潜流湿地(SFW)。FWS投资低,但占地大,低温地区冬季运行需要独特的考虑。SFW的保温保水效果好,卫生条件较好,但投资高,易堵塞。SFW分为水平潜流湿地(HF... 详细信息

人工湿地(CW)是独特的土壤-植物-微生物-动物系统。按水流方式分为表面流湿地(FWS)和潜流湿地(SFW)。FWS投资低,但占地大,低温地区冬季运行需要独特的考虑。SFW的保温保水效果好,卫生条件较好,但投资高,易堵塞。SFW分为水平潜流湿地(HF)和垂直潜流湿地(VF)。HF床供氧较差,适于去除SS和BOD,但NH3-N的去除较差。VF床供氧好,占地小,适于硝化和去除BOD,但对SS的去除不如HF床,而且构建费高,易堵塞。FWS按系统中的主体植物的不同分为大型自由漂浮植物湿地、大型沉水植物湿地和大型挺水植物湿地。农业径流(AR)由农田排水、灌溉余水、村落污水、畜禽养殖污水和部分雨水径流组成。其污水源具有面广、量大、分散、间歇的峰值和高无机沉淀物负荷的特点。中国大多数农村经济基础薄弱,管理水平不高。农村中的低洼地、低产田和公共用地均可作为生态环境保护用地。农村的污水收集系统欠完善。传统污水处理技术处理AR时难度大、维护管理复杂、投资和运行费高。而CW的耐冲击负荷能力强、投资低、运行费低、维护管理简便,但占地较大。因此CW适合于有地可用的农村的AR的处理。小结了1982年起CW技术在AR处理中的研究和应用。已有研究结合AR的水质、水量规律及农村的特点,进行了CW的设计与工艺改进。对氮、磷、有机物、农药和杀虫剂等污染物的去除效果有较多的研究。关于CW的运行、维护和管理的研究有沉积物积累、水量平衡、去除效果的衡量、植物收割和费用分析。CW的运行效果的衡量应当基于进出水负荷量而非基于进出水浓度。总之CW在AR污染控制中具有良好的应用前景。CW经合理设计和管理后有望实现“零费用运行”或者“盈利性运行”。

关键词：人工湿地农业径流

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水流模拟断面中硝基苯的迁移转化规律

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环境科学研究 2008年第1期21卷 78-84页

作者：陈刚金相灿姜霞吕宪俊山东科技大学化学与环境工程学院山东青岛266510 中国环境科学研究院湖泊生态环境创新基地北京100012

采用实验室模拟装置研究了4,10和20℃条件下,封闭、开放状态和不同环境因素影响下硝基苯污染水团流经模拟断面前后,硝基苯在上覆水与沉积物中的迁移转化规律.结果表明:封闭、开放状态模拟断面上覆水和沉积物中硝基苯迁移分配受温度变化... 详细信息

采用实验室模拟装置研究了4,10和20℃条件下,封闭、开放状态和不同环境因素影响下硝基苯污染水团流经模拟断面前后,硝基苯在上覆水与沉积物中的迁移转化规律.结果表明:封闭、开放状态模拟断面上覆水和沉积物中硝基苯迁移分配受温度变化影响显著;开放状态下,上覆水、沉积物中硝基苯变化量均低于封闭状态.挥发不但影响硝基苯在沉积物-上覆水间的迁移分配,而且能促进沉积物中硝基苯的解吸;光照对模拟断面硝基苯迁移转化无影响.对于相同的沉积物和上覆水,影响模拟断面系统中硝基苯迁移、分配的因素依次为温度、挥发和光照.分析实验结果和材料推测,硝基苯在该实验条件下不存在降解转化.

关键词：模拟断面硝基苯迁移转化影响因素

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连续淹水培养条件下沉积物和土壤的氮素矿化过程

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土壤通报 2006年第5期37卷 909-915页

作者：金相灿崔哲王圣瑞中国环境科学研究院湖泊生态环境创新基地北京100012

在淹水条件下,采用连续培养法研究了后海沉积物(HH)、环科院沉积物(HK)和土壤(TR)的氮素矿化过程。结果表明:三个处理矿化趋势基本相同,都是培养前期矿化量迅速升高并达到峰值,之后逐渐降低,最后回到培养前的氨氮含量水平。两种沉积物... 详细信息

在淹水条件下,采用连续培养法研究了后海沉积物(HH)、环科院沉积物(HK)和土壤(TR)的氮素矿化过程。结果表明:三个处理矿化趋势基本相同,都是培养前期矿化量迅速升高并达到峰值,之后逐渐降低,最后回到培养前的氨氮含量水平。两种沉积物的矿化高峰出现时间在培养的第4天,要早于TR的第7天;污染严重HH的矿化最大累积量远大于污染较轻的HK和TR。培养过程中各处理各层次有机质、总氮和固定态铵含量都表现为降低趋势。说明培养过程中,开始占主导地位的氨化微生物被其它土壤微生物所代替,这些微生物大量繁殖,生物固持作用逐渐强于矿化作用,造成矿化氮和固定态铵含量迅速下降。

关键词：连续淹水培养沉积物土壤氮素矿化

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Effect of low-degree astigmatism on the objective visual quality

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International Journal of Ophthalmology(English edition) 2024年第6期17卷 1086-1093页

作者： Ling-Ying Ye Shu-Feng Li jing-jing Zuo jin Li Hui-xiang Ma National Clinical Research Center for Ocular Diseases Eye HospitalWenzhou Medical UniversityWenzhou 325027Zhejiang ProvinceChina

AIM:To evaluate the effect of low-degree astigmatism on objective visual quality through the Optical Quality Analysis System(OQAS).METHODS:This study enrolled 46 participants(aged 23 to 30y,90 eyes)with normal or corrected-to-normal *** cylindrical lenses(0,0.5,0.75,1.0,and 1.25 D)were placed at the axial direction(180°,45°,90°,and 135°)in front of the eyes with the best correction to form 16 types of regular low-degree *** was used to detect the objective visual quality,recorded as the objective scattering index(OSI),OQAS values at contrasts of 100%,20%,and 9%predictive visual acuity(OV100%,OV20%,and OV9%),modulation transfer function cut-off(MTFcut-off)and Strehl ratio(SR).The mixed effect linear model was used to compare objective visual quality differences between groups and examine associations between astigmatic magnitude and objective visual quality ***:Apparent negative relationships between the magnitude of low astigmatism and objective visual quality were *** increase of OSI per degree of astigmatism at 180°,45°,90°,and 135°axis were 0.38(95%CI:0.35,0.42),0.50(95%CI:0.46,0.53),0.49(95%CI:0.45,0.54)and 0.37(95%CI:0.34,0.41),*** decrease of MTFcut-off per degree of astigmatism at 180°,45°,90°,and 135°axis were-10.30(95%CI:-11.43,-9.16),-12.73(95%CI:-13.62,-11.86),-12.75(95%CI:-13.79,-11.70),and-9.97(95%CI:-10.92,-9.03),*** the same astigmatism degree,OSI at 45°and 90°axis were higher than that at 0°and 135°axis,while MTFcut-off were ***:Low astigmatism of only 0.50 D can significantly reduce the objective visual quality.

关键词： low-degree astigmatism objective visual quality Optical Quality Analysis System

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