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Effect of Ti Additions on Mechanical and Thermodynamic Properties of W-Ti Alloys: A First-principles Study

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 246-257页

作者： zhang jian NIE Wei HUANG jin ZHU Ke LIU Ruxia zhang Ruizhi LUO Guoqiang shen Qiang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Institute for Carbon Neutrality University of Science and Technology BeijingBeijing 100083China

The mechanical and thermodynamic properties of W-Ti alloys(including W_(15)Ti_(1),W_(14)Ti_(2),W_(12)Ti_(4) and W_(8)Ti_(8) alloys)were investigated by the first-principles approach based on density functional *** results indicate that W-Ti alloys except W_(8)Ti_(8) are thermodynamically *** modulus and hardness of W-Ti alloys are smaller than those of pure tungsten and gradually decrease with increasing Ti ***,their B/G ratios and Poisson's ratios exceed those of pure tungsten,suggesting that the introduction of Ti decreases the mechanical strength while enhancing the ductility of W-Ti *** thermal expansion coefficients for W-Ti alloys all surpass those of pure tungsten,indicating that the introduction of titanium exacerbates the thermal expansion behavior of W-Ti ***,elevated pressure has the capacity to suppress the thermal expansion tendencies in titanium-doped tungsten *** study offers theoretical insights for the design of nuclear materials by exploring the mechanical and thermodynamic properties of W-Ti alloys.

关键词： first-principles mechanical properties thermodynamic properties tungsten-titanium alloys

The cGAS-STING-interferon regulatory factor 7 pathway regulates neuroinflammation in Parkinson's disease

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Neural Regeneration Research 2025年第8期20卷 2361-2372页

作者： shengyang Zhou Ting Li Wei zhang jian Wu Hui Hong Wei Quan Xinyu Qiao Chun Cui Chenmeng Qiao Weijiang Zhao Yanqin shen Laboratory of Neurodegenerative and Neuroinjury Diseases Wuxi Medicine SchoolJiangnan UniversityWuxiJiangsu ProvinceChina

Interferon regulatory factor 7 plays a crucial role in the innate immune ***,whether interferon regulatory factor 7-mediated signaling contributes to Parkinson's disease remains *** we report that interferon regulatory factor 7 is markedly up-regulated in a 1-methyl-4-phenyl-1,2,3,6-tetrahydropyridine-induced mouse model of Parkinson's disease and co-localizes with microglial *** the selective cyclic guanosine monophosphate adenosine monophosphate synthase inhibitor RU.521 and the stimulator of interferon genes inhibitor H151 effectively suppressed interferon regulatory factor 7 activation in BV2 microglia exposed to 1-methyl-4-phenylpyridinium and inhibited transformation of mouse BV2 microglia into the neurotoxic M1 *** addition,si RNA-mediated knockdown of interferon regulatory factor 7 expression in BV2 microglia reduced the expression of inducible nitric oxide synthase,tumor necrosis factorα,CD16,CD32,and CD86 and increased the expression of the anti-inflammatory markers ARG1 and *** together,our findings indicate that the cyclic guanosine monophosphate adenosine monophosphate synthase-stimulator of interferon genes-interferon regulatory factor 7 pathway plays a crucial role in the pathogenesis of Parkinson's disease.

关键词： cyclic guanosine monophosphate adenosine monophosphate synthase H151 interferon regulatory factor 7 M1 phenotype neurodegenerative disease neuroinflammation Parkinson’s disease RU521 STING type I interferon

Negative PO3-implanted bionic ion transport channels for promoting Li-S battery

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Science China Chemistry 2025年

作者： Wenhuan Huang Shun Wang Xuehan Hou Yanan zhang Xingxing zhang Yaoxiao Zhao Xilang jin Huabin zhang Fei Wang jian zhang Key Laboratory of Chemical Additives for China National Light Industry College of Chemistry and Chemical EngineeringShaanxi University of Science and Technology School of Materials and Chemical Engineering Xi'an Technological University Chemistry Program Physical Science and Engineering Division King Abdullah University of Science and Technology State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences

Lithium-sulfur （Li-S） battery,as a promising next-generation high-energy-density battery,suffers from lithium polysulfides（LPSs） shuttle and Li dendrites *** crystalline framework-based membranes as separator can effectively absorb and restrain LPSs but without precise structural design principal exploration and mechanism ***,bio-inspired 1D oriented lithium-ion transport channels with molecular negatively charged PO3（-1） have been developed in hybrid tetrazole frameworks for promoting the transmission of Li+*** theoretical calculations and in situ spectroscopy demonstrated the higher binding energy and inhibited diffusion of LPSs in *** assembled PP@PO3Janus separator in Li-S coin cell delivered a high initial capacity of 1410.9 mAh g-1at 0.1 C and a low attenuation rate of 0.038%per cycle over 500 cycles at 5 ***,the high capacities of 862,542 and 409 mAh g-1based on high-sulfur-loading cathodes of 2.6,3.8 and 5.0 mg cm-2at0.5 C were achieved,***,the punch battery of PO3@PP separator with S-cathode of 1.2 mg cm-2has been developed for demonstrating its potentials commercial application,which displays impressive capacity of 873.4 mAh g-1with the retention of～78.9%over 50 cycles.

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Maintaining moderate levels of hypochlorous acid promotes neural stem cell proliferation and differentiation in the recovery phase of stroke

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Neural Regeneration Research 2025年第3期20卷 845-857页

作者： lin-Yan Huang Yi-De zhang Jie Chen Hai-Di Fan Wan Wang Bin Wang Ju-Yun Ma Peng-Peng Li Hai-Wei Pu Xin-Yian Guo jian-Gang shen Su-Hua Qi School of Medical Technology Xuzhou Key Laboratory of Laboratory DiagnosticsXuzhou Medical UniversityXuzhouJiangsu ProvinceChina School of Pharmacy Xuzhou Medical UniversityXuzhouJiangsu ProvinceChina Department of Laboratory Medicine Branch Hospital of Huai’an First People’s HospitalHuai’anJiangsu ProvinceChina Department of Laboratory Medicine the Affiliated Hospital of Xuzhou Medical UniversityXuzhouJiangsu ProvinceChina School of Chinese Medicine The University of Hong KongHong Kong Special Administrative RegionChina

It has been shown clinically that continuous removal of ischemia/reperfusion-induced reactive oxygen species is not conducive to the recovery of late ***,previous studies have shown that excessive increases in hypochlorous acid after stroke can cause severe damage to brain *** previous studies have found that a small amount of hypochlorous acid still exists in the later stage of stroke,but its specific role and mechanism are currently *** simulate stroke in vivo,a middle cerebral artery occlusion rat model was established,with an oxygen-glucose deprivation/reoxygenation model established in vitro to mimic *** found that in the early stage(within 24 hours)of ischemic stroke,neutrophils produced a large amount of hypochlorous acid,while in the recovery phase(10 days after stroke),microglia were activated and produced a small amount of hypochlorous ***,in acute stroke in rats,hypochlorous acid production was prevented using a hypochlorous acid scavenger,taurine,or myeloperoxidase inhibitor,4-aminobenzoic acid *** results showed that high levels of hypochlorous acid(200μM)induced neuronal apoptosis after oxygen/glucose deprivation/***,in the recovery phase of the middle cerebral artery occlusion model,a moderate level of hypochlorous acid promoted the proliferation and differentiation of neural stem cells into neurons and *** suggests that hypochlorous acid plays different roles at different phases of cerebral ischemia/reperfusion *** levels of hypochlorous acid(5 and 100μM)promoted nuclear translocation ofβ-*** transfection of single-site mutation plasmids,we found that hypochlorous acid induced chlorination of theβ-catenin tyrosine 30 residue,which promoted nuclear ***,our study indicates that maintaining low levels of hypochlorous acid plays a key role in the recovery of neurological function.

关键词： cell differentiation cerebral ischemia/reperfusion injury chlorination hypochlorous acid microglia neural stem cell neurogenesis nuclear translocation stroke β-catenin

Boosting aqueous nickel-zinc battery stability with bimetallic ion-integrated 1D metal-organic nanowires

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Science China Chemistry 2025年

作者： Yihao Chen jin Liang Yichun Su Guoyin Zhu Hengyue Xu Hongye Ding Guangxun zhang Dianheng Yu Zizhou shen Yizhou zhang Wei Huang Huan Pang School of Chemistry and Chemical Engineering Yangzhou University Key Laboratory of Flexible Electronics (KLoFE) & Institute of Advanced Materials (IAM) School of Flexible Electronics (Future Technologies) Nanjing Tech University (NanjingTech) Institute of Advanced Materials and Flexible Electronics (IAMFE) School of Chemistry and Materials Science Nanjing University of Information Science & Technology Department of Chemistry Tsinghua University State Key Laboratory of Coordination Chemistry Nanjing University

Limited by low conductivity,designing cathode materials with excellent electron transfer efficiency for high-performance nickel-zinc batteries （NZBs） remains *** this study,a series of bimetallic metal-organic nanowires were fabricated by doping M ions in NiNTA,resulting in NiMNTA (M=Mg2+,Mn2+,Co2+,Zn2+,Ag+),and NixCo6-xNTA （x=1,2,3,4,5）.The proportions and types of metal ions can be modified without altering the initial coordination structure.X-ray absorption fine structure spectroscopy （XAFS） revealed that only M–O bonds,not metal bonds,were present in the *** performance of Ni2Co4NTA as the cathode for aqueous NZBs was significantly improved,achieving the maximum energy density of 279.17Wh kg-1with the high cycle stability （retention rate of 72.0%after 1,000 cycles）.The flexible Ni2Co4NTA//Zn@carbon cloth battery employing gel electrolyte also exhibits the excellent Coulombic efficiency of 96%after 350 *** approach shows considerable potential for designing one-dimensional materials with bimetallic modifications,providing new strategies for developing cathode materials for NZBs with high specific capacity and cycle stability.

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Non-noble metal-based catalysts for acetylene semihydrogenation:from thermocatalysis to sustainable catalysis

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Science China Chemistry 2023年第7期66卷 1963-1974页

作者： Lei zhang jin lin Zhenpeng Liu jian zhang Research&Development Institute of Northwestern Polytechnical University in shenzhen School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710129China State Key Laboratory of Solidification Processing and School of Materials Science and Engineering Northwestern Polytechnical UniversityXi’an 710072China

Selective semihydrogenation of acetylene in raw olefin streams to ethylene is a key industrial reaction to produce polymer-grade feeds for the manufacture of corresponding *** currently used process in industry is the thermocatalytic acetylene semihydrogenation with pressurized hydrogen and Pd-based catalysts at relatively high *** high cost of Pd urgently desires the design of non-noble metal-based ***,non-noble metal-based catalysts commonly require much higher reaction temperatures than Pd-based catalysts because of their poor intrinsic ***,aiming at increasing economic efficiency and sustainability,various strategies are explored for developing non-noble metal-based catalysts for thermocatalytic and green acetylene semihydrogenation *** this review,we systematically summarize the recent advances in catalytic technology from thermocatalysis to sustainable alternatives,as well as corresponding regulation strategies for designing high-performance non-noble metal-based *** crucial factors affecting catalytic performance are discussed,and the fundamental structure-performance correlation of catalysts is ***,we emphasize current challenging issues and future perspectives for acetylene *** review will not only promote the rapid exploration of non-noble metal-based catalysts for acetylene semihydrogenation,but also advance the development of sustainable processes like electrocatalysis and photocatalysis.

关键词： acetylene semihydrogenation non-noble metal-based catalysts thermocatalysis sustainable catalysis

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A method for observing tridimensional morphology of sulfide inclusions by non-aqueous solution electrolytic etching

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Journal of Iron and Steel Research International 2019年第3期26卷 275-284页

作者： Dong zhang ping shen jian-bo Xie jin-min An Zong-ze Huang jian-xun Fu State Key Laboratory of Advanced Special Steel Shanghai Key Laboratory of Advanced Ferrous Metallurgy School of Materials Science and Engineering Shanghai University Shanghai 200072 China State Key Laboratory of Development and Application Technology of Automotive Steel (Baosteel Group) Shanghai 20190 China

Three-dimensional investigation of sulfides is required in order to improve the mechanical properties of steel by controlling the sulfides in the steel.A method including its principles and device is introduced for the investigation of threedimensional morphology of *** method is suitable for gear steel,free cutting steel,non-quenched steel,tempered steel(ws≥0.02 wt.%),*** influences of current density,time,and temperature on the exposure degree of sulfide inclusions were investigated by using 16MnCrS5 *** best parameters of electrolytic etching of sulfur steel,as found by experimentation,are as follows:current density,37.5-52.5 mA/cm2;time,30-35 min;and temperature,—10 to 0℃.Under these conditions,the three-dimensional morphology of sulfide inclusions in sulfur-bearing steel can be exposed effectively.

关键词： Sulfide Non-aqueous electrolyte Electrolytic etching Three-dimensional morphology

Response of snow hydrological processes to a changing climate during 1961 to 2016 in the headwater of Irtysh River Basin, Chinese Altai Mountains

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Journal of Mountain Science 2017年第11期14卷 2295-2310页

作者： zhang Wei KANG Shi-chang shen Yong-ping HE jian-qiao CHEN An-an State Key Laboratory of Cryospheric Sciences Northwest Institute of Eco-Environment and Resources Chinese Academy of Sciences Chinese Academy of Sciences Center for Excellence in Tibetan Plateau Earth Sciences University of Chinese Academy of Sciences

With changing climatic conditions and snow cover regime, regional hydrological cycle for a snowy basin will change and further available surface water resources will be redistributed. Assessing snow meltwater effect on runoff is the key to water safety, under climate warming and fast social-economic developing status. In this study, stable isotopic technology was utilized to analyze the snow meltwater effect on regional hydrological processes, and to declare the response of snow hydrology to climate change and snow cover regime, together with longterm meteorological and hydrological observations, in the headwater of Irtysh River, Chinese Altai Mountains during 1961-2015. The average δ^(18) O values of rainfall, snowfall, meltwater, groundwater and river water for 2014–2015 hydrological year were-10.9‰,-22.3‰,-21.7‰,-15.7‰ and-16.0‰, *** results from stable isotopes, snow melting observation and remote sensing indicated that the meltwater effect on hydrological processes in Kayiertesi River Basin mainly occurred during snowmelt supplying period from April to June. The contribution of meltwater to runoff reached 58.1% during this period, but rainfall, meltwater and groundwater supplied 49.1%, 36.9% and 14.0% of water resource to annual runoff, respectively. With rising air temperature and increasing snowfall in cold season, the snow water equivalent(SWE) had an increasing trend but the snow cover duration declined by about one month including 13-day delay of the first day and 17-day advancement of the end day during 1961–2016. Increase in SWE provided more available water resource. However, variations in snow cover timing had resulted in redistribution of surface water resource, represented by an increase of discharge percentage in April and May, and a decline in Juneand July. This trend of snow hydrology will render a deficit of water resource in June and July when the water resource demand is high for agricultural irrigation and industrial manufacture.

关键词： Irtysh River Basin Chinese AltaiMountains Snow hydrology Isotope Climate change

Effect of Mg-treatment on transformation of oxide inclusions in X80 pipeline steel

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Journal of Iron and Steel Research International 2024年第11期31卷 2802-2814页

作者： ping shen Hao zhang Kang Xu Shuai Liu jin-xing jiang jian-xun Fu Center for Advanced Solidification Technology(CAST) State Key Laboratory of Advanced Special SteelShanghai UniversityShanghai200444China Nanjing Iron and Steel Co. Ltd.Nanjing210000JiangsuChina

In order to investigate the modification behavior and regularity of inclusions in X80 pipeline steel by Mg-treatment, the comparative industrial experiments of Mg-treatment and Ca-treatment in X80 pipeline steel were carried out. Mg and Ca were added to the steel in the form of cored wire after RH (Ruhrstahl-Hereaeus vacuum degassing) process. After adding Ca-containing cored wire, the inclusions were transformed into CaO–Al_(2)O_(3) in the steel. With the progress of smelting, the cleanliness of molten steel became worse, and the equivalent diameter of inclusions was at a higher level. Mg-treatment had a good effect on the modification of inclusions. After Mg-containing cored wire was added to the steel, Al_(2)O_(3) and CaO–Al_(2)O_(3) in the steel were transformed into MgO, MgO·Al_(2)O_(3), and CaO–MgO–Al_(2)O_(3) inclusions, which were basically spherical. The initial precipitated MgO became the core of other inclusions in the steel, which promotes the precipitation of MgO·Al_(2)O_(3). After Mg-treatment, almost no unmodified calcium aluminate inclusions existed in the hot rolled plate, and the cleanliness of the steel was improved. The effect of Ca and Mg on the transformation of inclusions in pipeline steel was studied by thermodynamic calculation, the result of which is consistent with the experimental results.

关键词： Pipeline steel Mg-treatment Ca-treatment Calcium aluminate MgO·Al_(2)O_(3)