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Hydrogen-bonded organic framework modified separator for simultaneously enhancing the safety and electrochemical performance of Ni-rich lithium-ion battery

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Journal of Energy Chemistry 2024年第9期96卷 72-78页

作者： Chengyu Han Yu Cao Ming yang Yuhan Wang Di Tang Shaojie Zhang Yiran jia Yiming Zhang Hern Kim fusheng Pan Zhongyi jiang Jie Sun Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Science and Technology on Power Sources Laboratory Tianjin Institute of Power SourcesTianjin 300384China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China Quzhou Institute for Innovation in Resource Chemical Engineering Quzhou 324000ZhejiangChina Department of Energy Science and Technology Director Environmental Waste Recycle InstituteYongin 17058Republic of Korea School of Chemistry and Chemical Engineering Hainan UniversityHaikou 570228HainanChina

Nickel-rich layered oxide cathode(LiNi_(x)Co_(y)Mn_(1−x−y)O_(2),x>0.5,NCM)shows substantial potential for applications in longer-range electrical ***,the rapid capacity decay and serious safety concerns impede its practical *** work provides a hydrogen-bonded organic framework(HOF)modification strategy to simultaneously improve the electrochemical performance,thermal stability and incombustibility of *** cyanurate(MCA),as a low-cost and reliable flame-retardant HOF,was implemented in the separator modification layer,which can prevent the battery short circuit even at a high *** addition,the supermolecule properties of MCA provide unique physical and chemical microenvironment for regulating ion-transport behavior in *** MCA coating layer enabled the nickel-rich layered oxide cathode with a high-capacity retention of 90.3%after 300 cycles at 1.0 ***,the usage of MCA in lithium-ion batteries(LIBs)affords a simple,low-cost and efficient strategy to improve the security and service life of nickel-rich layered cathodes.

关键词： Hydrogen-bonded organic framework Modified separator Ni-richlayered oxide cathode Thermal runaway Li^(+)transference number

Accelerated design of high-performance Mg-Mn-based magnesium alloys based on novel bayesian optimization

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Journal of magnesium and Alloys 2024年第2期12卷 750-766页

作者： Xiaoxi Mi Lili Dai Xuerui Jing jia She Bjørn Holmedal Aitao Tang fusheng Pan College of materials Science and Engineering Chongqing UniversityChongqing 400044China Southwest Technology and Engineering Research Institute Chongqing 400039China national Engineering Research Center for magnesium Alloys Chongqing UniversityChongqing 400044China Department of materials Science and Engineering Norwegian University of Science and Technology(NTNU)Trondheim 7051Norway

magnesium(Mg),being the lightest structural metal,holds immense potential for widespread applications in various *** development of high-performance and cost-effective Mg alloys is crucial to further advancing their commercial *** the rapid advancement of machine learning(ML)technology in recent years,the“data-driven''approach for alloy design has provided new perspectives and opportunities for enhancing the performance of Mg *** paper introduces a novel regression-based Bayesian optimization active learning model(RBOALM)for the development of high-performance Mg-Mn-based wrought *** employs active learning to automatically explore optimal alloy compositions and process parameters within predefined ranges,facilitating the discovery of superior alloy *** model further integrates pre-established regression models as surrogate functions in Bayesian optimization,significantly enhancing the precision of the design *** RBOALM,several new high-performance alloys have been successfully designed and ***,after mechanical property testing of the designed alloys,the Mg-2.1Zn-2.0Mn-0.5Sn-0.1Ca alloy demonstrates exceptional mechanical properties,including an ultimate tensile strength of 406 MPa,a yield strength of 287 MPa,and a 23%fracture ***,the Mg-2.7Mn-0.5Al-0.1Ca alloy exhibits an ultimate tensile strength of 211 MPa,coupled with a remarkable 41%fracture elongation.

关键词： Mg-Mn-based alloys High-performance Alloy design machine learning Bayesian optimization

超声辅助水酶法提取花生油脂工艺研究及油脂品质分析

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河南工业大学学报（自然科学版） 2024年第2期45卷 11-18页

作者：董艺帆贾赛阳杨鸣陈复生段晓杰布冠好杨趁仙朱婷伟河南工业大学粮油食品学院河南郑州450001

为了实现花生油脂的高效提取和利用,采用超声辅助水酶法提取花生油脂,研究超声功率、作用时间、作用温度、料液比及酶用量对花生油脂提取率的影响,采用响应面试验优化提取工艺,并分析花生油脂的脂肪酸组成、酸价、过氧化值和抗氧化能力... 详细信息

为了实现花生油脂的高效提取和利用,采用超声辅助水酶法提取花生油脂,研究超声功率、作用时间、作用温度、料液比及酶用量对花生油脂提取率的影响,采用响应面试验优化提取工艺,并分析花生油脂的脂肪酸组成、酸价、过氧化值和抗氧化能力。结果表明:花生油脂的最优提取工艺条件为料液比1∶5 g/mL、纤维素酶用量1.0%、超声功率247 W、作用时间41 min、作用温度51℃,此条件下的油脂提取率为92.64%±0.73%;从提取的花生油脂中共检出8种脂肪酸,其中油酸含量最高,为40.44%±0.57%,亚油酸含量为36.97%±0.05%;花生油脂的酸价为(0.38±0.04)mg/g,过氧化值为(0.15±0.00)g/100 g,DPPH和ABTS自由基清除率分别为64.82%±2.51%、82.56%±6.47%。超声辅助水酶法有效缩短了提取时间,降低了酶用量,并且制备的花生油脂中不饱和脂肪酸含量高,具有良好的抗氧化能力。

关键词：花生油脂水酶法超声脂肪酸抗氧化能力

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Microstructures and mechanical properties of titanium-reinforced magnesium matrix composites: Review and perspective

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Journal of magnesium and Alloys 2022年第9期10卷 2311-2333页

作者： Hong yang Xianhua Chen Guangsheng Huang jiangfeng Song jia She jun Tan Kaihong Zheng Yiming Jin Bin jiang fusheng Pan national Engineering Research Center for magnesium Alloys Chongqing UniversityChongqing 400044China College of materials Science and Engineering Chongqing UniversityChongqing 400044China Institute of New materials Guangdong Academy of SciencesGuangzhou 510650China Southwest Technology and Engineering Research Institute Chongqing 400039China

Currently, many gratifying signs of progress have been made in magnesium(Mg) matrix composites(MMCs) by virtue of their high mechanical properties both at room and elevated temperatures. Although the commonly used reinforcements in MMCs are ceramic particles,they often provide improved yield and ultimate stresses by a significant loss in ductility. Therefore, hard metallic phases were introduced as alternative candidates for the manufacturing of MMCs, especially titanium(Ti). It has a high melting point, high Young’s modulus, high plasticity, low level of mutual solubility with Mg matrix, and closer thermal expansion coefficient to that of Mg metal than that of ceramic particles. It is highly preferable to provide both high ultimate stress and ductility in Mg matrix. However, many critical challenges for the fabrication of Ti-reinforced MMCs remain, such as Ti’s homogeneity, low recovery rate, and the optimization of interfacial bonding strength between Mg and Ti, etc. Meanwhile, different fabrication methods have various effects on the microstructures, mechanical properties, and the interfacial strength of Ti-reinforced MMCs. Hence, this review placed emphasis on the microstructural characteristics and mechanical properties of Ti-reinforced MMCs fabricated by different techniques. The influencing factors that govern the strengthening mechanisms were systematically compared and discussed. Future research trends, key issues, and prospects were also proposed to develop Ti-reinforced MMCs.

关键词： magnesium matrix composites Ti Microstructures Mechanical properties Fabrication techniques

Rational design, synthesis and prospect of biodegradable magnesium alloy vascular stents

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Journal of magnesium and Alloys 2023年第9期11卷 3012-3037页

作者： Senwei Wang Chengao Du Xin Shen Xiong Wu Sihui Ouyang jun Tan jia She Aitao Tang Xianhua Chen fusheng Pan College of materials Science and Engineering Chongqing UniversityChongqingChina national Engineering Research Center for Mg Alloys Chongqing UniversityChongqingChina Beijing Amsinomed Medical Co LtdBeijingChina

Biodegradable magnesium(Mg) alloys are expected to be promising materials for cardiovascular stents(CVS), which can avoid the longterm clinical problems of current CVS, such as in-stent restenosis, late stent thrombosis, etc. Mg alloy stents exhibit superior biocompatibility and tunable biodegradability, compared with conventional permanent metallic stents. However, the poor formability and non-uniform corrosion of Mg alloy stents hinder their clinical application of CVS. This review focuses on the development of Mg alloys for CVS in recent *** to the results of bibliometric analysis, we analyzed different biodegradable Mg alloy systems. Moreover, the structural design strategies for Mg alloy stents that can reduce the stress concentration, as well as the surface modification methods to control the corrosion behavior and biological performance of Mg alloy stents are also highlighted. At last, this review systematically discussed the potential directions and challenges of biodegradable magnesium stents(BMgS) in cardiovascular fields.

关键词： Mg alloy micro-tube Biodegradable Mg stent Alloying design Structural design Functional properties

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管道内检测腐蚀数据概率分布规律研究及应用

油气田地面工程 2024年第7期43卷 70-76页

作者：闻亚星贾福生刘鹏程王锋陈金忠马义来中国特种设备检测研究院中国石油天然气股份有限公司塔里木油田分公司

腐蚀伴随着管道整个生命周期,管道腐蚀速率评估是管道剩余寿命评估的重要部分,为了提高管道剩余寿命评价的准确性,为制定合理的检测维修周期提供支撑,以某条管道连续两轮漏磁内检测腐蚀数据为基础,并采用最大似然估计法将腐蚀速率与几... 详细信息

腐蚀伴随着管道整个生命周期,管道腐蚀速率评估是管道剩余寿命评估的重要部分,为了提高管道剩余寿命评价的准确性,为制定合理的检测维修周期提供支撑,以某条管道连续两轮漏磁内检测腐蚀数据为基础,并采用最大似然估计法将腐蚀速率与几种常见的概率分布模型进行拟合,通过K-S检验和p-p散点图方法的比较分析,深入研究了该管道径向和轴向腐蚀速率的概率分布规律,发现该管道径向和轴向腐蚀速率的最优分布规律为广义极值分布规律。在此基础上建立了基于概率分布规律的管道剩余寿命评估模型,选取该概率分布模型95%分位数的腐蚀速率作为管道剩余寿命的评估腐蚀速率。分析采用局部腐蚀速率评价方法、最大腐蚀速率评价方法、概率分布腐蚀速率评价方法时5年内需要维修点的数量,结果表明:采用概率分布腐蚀速率评价方法需维修点数量介于局部腐蚀速率评价法和最大腐蚀速率评价法之间,可在一定程度上避免过度维修和维修不及时。

关键词：油气管道内检测概率分布腐蚀速率剩余寿命

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柑橘感染褐斑病过程中BAG1的作用

园艺学报 2024年第5期51卷 956-970页

作者：周慧珍张嘉胡军华李白雪曹立余歆王福生邹修平周彦西南大学柑桔研究所国家柑桔工程技术研究中心重庆400712

本研究旨在探究柑橘BAG1参与褐斑病菌(Alternaria alternata)侵染的调控机制。从‘秤砣红橘’(Citrus tangerina *** Tanaka)、‘宫本温州蜜柑’(*** macf)、‘爱媛38’杂柑(*** Blanco)和‘金秋砂糖橘’(*** Blanco)叶片中扩增BAG1基因... 详细信息

本研究旨在探究柑橘BAG1参与褐斑病菌(Alternaria alternata)侵染的调控机制。从‘秤砣红橘’(Citrus tangerina *** Tanaka)、‘宫本温州蜜柑’(*** macf)、‘爱媛38’杂柑(*** Blanco)和‘金秋砂糖橘’(*** Blanco)叶片中扩增BAG1基因。BAG1蛋白相对保守,均具有Ubiquitin泛素结构域和BAG结构域,‘爱媛38’的BAG结构域存在3个新的氨基酸变动,导致侧链基团变动。上游启动子序列显示4个柑橘品种均包含相同的激素和胁迫相关顺式作用元件。系统分析显示4个柑橘品种与宽皮柑橘类BAG1蛋白聚为一支,相似度最高,与甜橙类、柚类亲缘关系较远。qRT-PCR显示在褐斑病菌THJ菌株侵染的抗、感品种上BAG1的表达差异显著。BAG1受外源Me JA、ABA和SA诱导上调表达。烟草亚细胞定位显示BAG1存在于细胞核和细胞膜中。BAG1沉默能够增强对***的抗性,过表达对***的抗性降低。表明BAG1通过参与活性氧激发和ABA、JA或SA信号途径,参与柑橘对褐斑病菌的调控。

关键词：柑橘 BAG1 褐斑病菌感病基因活性氧

面向6G的高速太赫兹无线通信系统与关键技术验证

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无线电通信技术 2024年第1期50卷 34-40页

作者：董博宇冯叶青李国强贾俊连张俊文付杰尉迟楠朱伏生复旦大学电磁波信息科学教育部重点实验室上海200433 广东省新一代通信与网络创新研究院广东广州510663

太赫兹通信以其可提供更高速、更大容量和更安全的数据传输的独特优势,在未来6G中成为重要的关键技术之一。基于固态电子的太赫兹通信系统存在带宽受限、频谱响应不平坦等问题,需要先进的信号形式结合灵活高效的处理方法来提升系统性能... 详细信息

太赫兹通信以其可提供更高速、更大容量和更安全的数据传输的独特优势,在未来6G中成为重要的关键技术之一。基于固态电子的太赫兹通信系统存在带宽受限、频谱响应不平坦等问题,需要先进的信号形式结合灵活高效的处理方法来提升系统性能。搭建了基于固态电子的G波段太赫兹无线通信系统,通过采用比特-功率加载的离散多音(Bit and Power Loading-Discrete Multitone, BPL-DM)调制技术,实现了对系统频谱资源的有效利用;通过对通信速率的灵活调整、自适应削波和基于三阶多项式的后均衡技术,解决了峰值功率约束带来的挑战,提升了整体传输性能,实现了在195 GHz中心频率下,单通道130 Gbit/s的通信线路速率。基于以上技术,为进一步提升系统容量,搭建了4×4的多输入多输出(Multiple-Input Multiple-Output, MIMO)太赫兹通信系统,总线路速率超过399 Gbit/s。

关键词：太赫兹无线通信多输入多输出离散多音调制比特-功率加载自适应削波

Effect of Al on microstructure and mechanical properties of as-extruded Mg–1Mn alloy sheet

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Progress in natural Science:materials International 2020年第3期30卷 402-409页

作者： Shida ma Aitao Tang Peng Peng Geng Zhang Zhengwen Yu jia She fusheng Pan material Science and Engineering College Chongqing University School of Stomatology Zunyi Medical University national Engineering Research Center for magnesium Alloy Chongqing University

The effect of Al addition on microstructure and mechanical properties of hot extruded Mg–1 Mn alloy sheet was investigated. The results revealed that the dynamic recrystallization was promoted by increasing Al content. The ultimate tensile strength and yield strength of the alloy increased with the increase of Al content. The Mg–9 Al–1 Mn alloy exhibited the highest strength, with tensile strength of 308 MPa, 307 MPa, 319 MPa, yield strength of 199 MPa, 207 MPa, 220 MPa and the elongation of 20.9%, 20.1%, 19.2% in 0°, 45°, 90°, *** high strength was mainly attributed to the formation of fine dynamically recrystallized grains and large amounts of the second phase. The strengthening mechanism of the alloys was explained.

关键词： magnesium alloy Microstructure Mechanical properties Mg–Al–Mn