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A COLUMN RECURRENCE ALGORITHM FOR SOLVING LINEAR LEAST SQUARES PROBLEM

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journal of Computational Mathematics 1996年第4期14卷 301-310页

作者： j.x. zhao(Department of Mathematics, Nanjing University, Nanjing China) NANjING UNIV DEPT MATHNANJING 210008PEOPLES R CHINA

A new column recurrence algorithm based on the classical Greville method and modified Huang update is proposed for computing generalized inverse matrix and least squares solution. The numerical results have shown the ... 详细信息

关键词： Math A COLUMN RECURRENCE ALGORITHM FOR SOLVING LINEAR LEAST SQUARES PROBLEM ABS

ON THE A/D TYPE TWIN BOUNDARY IN 18R MARTENSITE OF A Cu-Zn-Al ALLOY

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Acta Metallurgica Sinica(English Letters) 1997年第5期10卷 425-429页

作者： Zhang, j.x. Zheng, Y.F. Cai, W. zhao, L.C. Harbin Inst of Technology Harbin China

The A/D type twin boundary in a Cu-Zn-Al shape memory alloy appears curved under TEM and shows irregularly serrated steps under HREM. Crystallographic analysis shows that the macroscopic curve results from non-self-accommodation of the boundary, the deviation from exact twin orientation and a preferential orientation for lower boundary energy.

关键词： Aluminum alloys Copper alloys Crystallography Electron microscopy Martensite Zinc alloys

High-temperature-tolerant flexible supercapacitors: Gel polymer electrolytes and electrode materials

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journal of Energy Chemistry 2025年第1期100卷 426-457页

作者： Chong Peng xinyi Huang Mingwei zhao Shuling Liao Quanhong Yang Nianjun Yang Siyu Yu School of Chemistry & Chemical Engineering Southwest University Nanoyang Group Tianjin Key Laboratory of Advanced Carbon and Electrochemical Energy Storage School of Chemical Engineering and Technology and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) Tianjin University Department of Chemistry & IMO-IMOMEC Hasselt University

The development of flexible supercapacitors(FSCs) capable of operating at high temperatures is crucial for expanding the application areas and operating conditions of supercapacitors. Gel polymer electrolytes and electrode materials stand as two key components that significantly impact the efficacy of hightemperature-tolerant FSCs(HT-FSCs). They should not only exhibit high electrochemical performance and excellent flexibility, but also withstand intense thermal stress. Considerable efforts have been devoted to enhancing their thermal stability while maintaining high electrochemical and mechanical performance. In this review, the fundamentals of HT-FSCs are outlined. A comprehensive overview of state-of-the-art progress and achievements in HT-FSCs, with a focus on thermally stable gel polymer electrolytes and electrode materials is provided. Finally, challenges and future perspectives regarding HT-FSCs are discussed, alongside strategies for elevating operational temperatures and *** review offers both theoretical foundations and practical guidelines for designing and manufacturing HT-FSCs, further promoting their widespread adoption across diverse fields.

关键词： Flexible supercapacitors High-temperature tolerance Gel polymer electrolytes Electrode materials

Mechanical Properties and Defective Effects of 316LN Stainless Steel by First-Principles Simulations

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journal of Materials Science & Technology 2011年第11期27卷 1029-1033页

作者： x.Q. Li j.j. zhao j.C. xu x. Liu Key Laboratory of Materials Modification by Laser Ion and Electron Beams Ministry of Education Dalian University of Technology Dalian 116024 China College of Advanced Science and Technology Dalian University of Technology Dalian 116024 China School of Chemical Engineering Dalian University of Technology Dalian 116024 China

In current International Thermonuclear Experimental Reactor （ITER） design, the 316LN austenitic stainless steel （316LN SS） is used for first-wall/blanket structures. Thus, it is necessary to study the fundamental mechanical properties and irradiation effect of 316LN SS. A random solid solution model of Fe-Cr-Ni-Mn- Mo-Si alloy is used for describing 310LN S$. Using first-principles approaches, the elastic constants and ideal strength of the alloy were calculated. Such alloy exhibits good ductile behavior according to the theoretical values of Cauchy pressure and ratio of bulk modulus and shear modulus. Within the 256-atom supercell, inclusion of single vacancy defect further enhances the ductility of the alloy, and the existence of interstitial （Fe, H, He） atoms enhances the Young＇s modulus.

关键词： Stainless steel Mechanical properties Vacancy Interstitial

Low-cost and fluoride-free synthesis of MFI zeolite nanosheets with enhanced stability for benzene alkylation with ethanol

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journal of Energy Chemistry 2025年第1期100卷 458-468页

作者： Peng Zhu Cun Liu Yiren Yu Guoshu Gao Yumeng zhao xiongfu Zhang Guodong Liu Guohui Yang State Key Laboratory of Fine Chemicals School of Chemical Engineering Dalian University of Technology State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences

Zeolite nanosheets with a short b-axis thickness are highly desirable in lots of catalytic reactions due to their reduced diffusion resistance. Nevertheless, conventional synthesis methods usually require expensive structure-directing agents(SDAs), pricey raw materials, and eco-unfriendly fluorine-containing additives. Here, we contributed a cost-effective and fluoride-free synthesis method for synthesizing high-quality MFI zeolite nanosheets through a Silicalite-1(Sil-1) seed suspension and urea cooperative strategy, only with inexpensive colloidal silica as the Si source. Our approach was effective for synthesizing both Sil-1 and aluminum-containing ZSM-5 nanosheets. By optimizing key synthesis parameters,including seed aging time, seed quantity, and urea concentration, we achieved precise control over the crystal face aspect ratio and b-axis thickness. We also revealed a non-classical oriented nanosheet growth mechanism, where Sil-1 seeds induced the formation of quasi-ordered precursor particles, and the(010)crystal planes of these particles facilitated urea adsorption, thereby promoting c-axis-oriented *** obtained ZSM-5 nanosheets exhibited exceptional catalytic performance in the benzene alkylation with ethanol, maintaining stability for over 500 h, which is 5 times longer than traditional ZSM-5 catalysts. Furthermore, large-scale production of ZSM-5 nanosheets was successfully carried out in a 3 L highpressure autoclave, yielding samples consistent with those from laboratory-scale synthesis. This work marks a significant step forward in the sustainable and efficient production of MFI nanosheets using inexpensive and environmentally friendly raw materials, offering the broad applicability in catalysis.

关键词： MFI zeolite ZSM-5 Nanosheets Scale-up synthesis Aromatic alkylation

Flexible molecules dedicate to release strain of inverted inorganic perovskite solar cell

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journal of Energy Chemistry 2025年第1期100卷 87-93页

作者： Hongrui Sun Sanlong Wang Pengyang Wang Yali Liu Shanshan Qi Biao Shi Ying zhao xiaodan Zhang Institute of Photoelectronic Thin Film Devices and Technology Renewable Energy Conversion and Storage Center State Key Laboratory of Photovoltaic Materials and CellsNankai University Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin Haihe Laboratory of Sustainable Chemical Transformations Engineering Research Center of Thin Film Photoelectronic Technology of Ministry of Education Collaborative Innovation Center of Chemical Science and Engineering (Tianjin)

The tensile strain in inorganic perovskite films induced by thermal annealing is one of the primary factors contributing to the inefficiency and instability of inorganic perovskite solar cells （IPSCs）,which reduces the defect formation ***,a flexible molecule 5-maleimidovaleric acid （5-MVA） was introduced as a strain buffer to release the residual strain of *** anhydride and carboxyl groups in 5-MVA interact strongly with the uncoordinated Pb2+through Lewis acid-base reaction,thus tightly“pull”the perovskite *** in-between soft carbon chain increased the structural flexibility of CsPbI2.85Br0.15perovskite materials,which effectively relieved the intrinsic internal strain of CsPbI2.85Br0.15,resisted the corrosion of external strain,and also reduced the formation of defects such as VIand *** addition,the introduction of 5-MVA improved crystal quality,passivated residual defects,and narrowed energy level ***,power conversion efficiency （PCE） of NiOxbased inverted IPSCs increased from 19.25% to 20.82% with the open-circuit voltage enhanced from 1.164 V to 1.230 *** release of strain also improved the stability of CsPbI2.85Br0.15perovskite films and devices.

关键词： Inverted inorganic perovskite solar cells Flexible molecules Strain release Crystallization Energy barrier High PCE

Single-cell omics: experimental workflow, data analyses and applications

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Science China Life Sciences 2025年第1期68卷 5-102页

作者： Fengying Sun Haoyan Li Dongqing Sun Shaliu Fu Lei Gu xin Shao Qinqin Wang xin Dong Bin Duan Feiyang xing jun Wu Minmin xiao Fangqing zhao jing-Dong j.Han Qi Liu xiaohui Fan Chen Li Chenfei Wang Tieliu Shi Department of Clinical Laboratory the Affiliated Wuhu Hospital of East China Normal University (The Second People's Hospital of Wuhu City) Pharmaceutical Informatics Institute College of Pharmaceutical SciencesZhejiang University Key Laboratory of Spine and Spinal Cord Injury Repair and Regeneration (Tongji University) Ministry of EducationOrthopaedic DepartmentTongji HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Frontier Science Center for Stem Cells School of Life Sciences and TechnologyTongji University Translational Medical Center for Stem Cell Therapy and Institute for Regenerative Medicine Shanghai East HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Research Institute of Intelligent Computing Zhejiang Lab Shanghai Research Institute for Intelligent Autonomous Systems Center for Single-cell Omics School of Public HealthShanghai Jiao Tong University School of Medicine National Key Laboratory of Chinese Medicine Modernization Innovation Center of Yangtze River DeltaZhejiang University Center for Bioinformatics and Computational Biology Shanghai Key Laboratory of Regulatory Biologythe Institute of Biomedical Sciences and School of Life SciencesEast China Normal University Beijing Institutes of Life Science Chinese Academy of Sciences Peking-Tsinghua Center for Life Sciences Academy for Advanced Interdisciplinary StudiesCenter for Quantitative Biology (CQB)Peking University Zhejiang Key Laboratory of Precision Diagnosis and Therapy for Major Gynecological Diseases Women's HospitalZhejiang University School of Medicine Key Laboratory of Advanced Theory and Application in Statistics and Data Science-MOE School of StatisticsEast China Normal University

Cells are the fundamental units of biological systems and exhibit unique development trajectories and molecular features. Our exploration of how the genomes orchestrate the formation and maintenance of each cell, and control the cellular phenotypes of various organismsis, is both captivating and intricate. Since the inception of the first single-cell RNA technology, technologies related to single-cell sequencing have experienced rapid advancements in recent years. These technologies have expanded horizontally to include single-cell genome, epigenome,proteome, and metabolome, while vertically, they have progressed to integrate multiple omics data and incorporate additional information such as spatial sc RNA-seq and CRISPR screening. Single-cell omics represent a groundbreaking advancement in the biomedical field,offering profound insights into the understanding of complex diseases, including cancers. Here, we comprehensively summarize recent advances in single-cell omics technologies, with a specific focus on the methodology section. This overview aims to guide researchers in selecting appropriate methods for single-cell sequencing and related data analysis.

关键词： single-cell sequencing genome epigenome proteomics metabolomics multimodal spatial transcriptomics CRISPR screening

Machine learning guided automatic recognition of crystal boundaries in bainitic/martensitic alloy and relationship between boundary types and ductile-to-brittle transition behavior

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journal of Materials Science & Technology 2021年第25期84卷 49-58页

作者： x.C.Li j.x.zhao j.H.Cong R.D.K.Misra x.M.Wang x.L.Wang C.j.Shang Collaborative Innovation Center of Steel Technology University of Science and Technology BeijingBeijing 100083China Department of Metallurgical Materials and Biomedical EngineeringUniversity of Texas at El Paso500 W.University AvenueEl PasoTX 79968USA

Gradient boosting decision tree(GBDT)machine learning(ML)method was adopted for the first time to automatically recognize and conduct quantitative statistical analysis of boundaries in bainitic microstructure using electron back-scatter diffraction(EBSD)*** spite of lack of large sets of EBSD data,we were successful in achieving the desired accuracy and accomplishing the objective of recognizing the *** with a low model accuracy ofxis-angle pair as characteristic features,the accuracy of the model was significantly enhanced to about 88%when the Euler angle was converted to overall misorientation angle(OMA)and specific misorientation angle(SMA)and considered as important *** this model,the recall score of prior austenite grain(PAG)boundary was~93%,high angle packet boundary(OMA>40°)was~97%,and block boundary was~96%.The derived outcomes of ML were used to obtain insights into the ductile-to-brittle transition(DBTT)***,ML modeling approach suggested that DBTT was not determined by the density of high angle grain boundaries,but significantly influenced by the density of PAG and packet *** study underscores that ML has a great potential in detailed recognition of complex multi-hierarchical microstructure such as bainite and martensite and relates to material performance.

关键词： Machine learning Feature engineering Automatic recognition Lath structure Crystallography

FORMATION OF SILICONIZED LAYER ON TiAl-BASED ALLOY AND THE OxIDATION RESISTANCE

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Acta Metallurgica Sinica(English Letters) 2003年第6期16卷 466-472页

作者： W.Liang x.x.Ma x.G.zhao j.Zhang D.x.Zou SchoolofMaterialsScienceandEngineering TaiyuanUniversityofTechnologyTaiyuan030024China CentralIron＆SteelResearchInstitute Beijing100081China

The Ti-48Al alloy was pack siliconized with 15%Si+85%Al2O3. The microstructure of the siliconized coating on the TiAl-based alloy was analyzed and its effect on oxidation resistance was investigated. The specimens before and after cycle oxidation were examined by xRD and SEM equipped with xEDS. The results showed that the coating is composed of a thin Al2O3 outer layer and a composite inner layer of Ti5Si3 with an appropriate amount of Al2O3 dispersed in. Cycle oxidation tests showed that the high temperature oxidation resistance of TiAl-based alloy was greatly improved by forming such composite coating. No spaliation and crack happened and the weight gain was very small after cycle oxidation at 900℃ for 314h.

关键词： TiAl-based alloy microstructure composite coating high tem-perature oxidation