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Novel single-ion conducting polymer.electr.lytes with high toughness and high r.sistance against lithium dendr.tes

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Nano r.sear.h 2023年第6期16卷 8457-8468页

作者： David Fr.ile-Insagur.e Nicola Boar.tto Itziar.Aldalur.Iñigo r.poso Fr.ncisco j.vier.Bonilla Michel Ar.and Mar.a Mar.ínez-ibañez Centr. for.Cooper.tive r.sear.h on Alter.ative Ener.ies CIC energiGUNEBasque Research and Technology Alliance(BRTA)Alava Technology ParkAlbert Einstein 48Vitoria-Gasteiz 01510Spain Univer.ity of the Basque Countr.(UPV/EHU) Barrio Sarrienas/nLeioa 48940Spain

Solid-state polymer.electr.lytes ar. consider.d as an alter.ative to classic liquid electr.lytes,par.icular.y for.application in highener.y lithium metal *** r.spect to common dual-ion conductor.,single-ion conducting polymer.electr.lytes(SICPEs)ar. less affected by lithium dendr.tes gr.wth and thus ar. par.icular.y inter.sting for.application in lithium metal *** this wor.,novel SIC-PEs ar. developed,based on an ionomer.having poly(ethylene-alt-maleimide)backbone and lithium phenylsulfonyl(tr.fluor.methanesulfonyl)imide pendant moieties,fur.her.blended with poly(ethylene oxide)(PEO)and poly(ethylene glycol)dimethyl ether.PEGDME).These SIC-PEs exhibit ionic conductivity ar.und~7×10^(−6)S·cm^(−1) at 70℃,lithium tr.nsfer.nce number.close to unity,and excellent mechanical pr.per.ies,with fr.ctur. toughness over.30 j.cm^(−3).Additionally,the electr.lytes show ver. high r.sistance against lithium dendr.tes gr.wth,by cycling for.mor. than 1200 h in Li°symmetr.c cells at a cur.ent density of 0.1 mA·cm^(−2).LiFePO4||Li°cells with these SIC-PEs wer. cycled at 70℃ and C/10,showing initial capacity of almost 160 mAh·g^(−1)and r.sidual capacity of 45%after.100 *** wor. shows that single-ion conducting polymer.electr.lytes based on poly(ethylene-alt-maleimide)backbone ar. pr.mising mater.als for.application as electr.lytes or.catholytes in lithium metal polymer.batter.es.

关键词： single-ion conductor. solid-state Li metal batter.es polymer.electr.lytes lithium dendr.tes tr.nsfer.nce number mechanical pr.per.ies

Influence of the oper.ting temper.tur. on the ageing and inter.aces of double layer.polymer.electr.lyte solid state Li metal batter.es

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Nano r.sear.h 2023年第6期16卷 8377-8384页

作者： Mikel Ar.ese-Igor.Mar.a Mar.inez-ibañez Ander.Or.e Ekater.na Pavlenko Er.an Dumont Michel Ar.and Fr.dér.c Aguesse Pedr. López Ar.ngur.n Centr. for.Cooper.tive r.sear.h on Alter.ative Ener.ies(CIC ener.iGUNE) Basque Research and Technology Alliance(BRTA)Alava Technology ParkAlbert Einstein 48Vitoria-Gasteiz 01510Spain Univer.ity of the Basque Countr.(UPV/EHU) Barrio Sarrienas/nLeioa 48940Spain Saft 111 Boulevard Alfred DaneyBordeaux Cedex 33074France

Solid-state lithium metal batter.es(SSLMBs)ar. consider.d an auspicious technology to develop high ener.y density and safe ener.y stor.ge *** double layer.polymer.electr.lyte(DLPE)is a r.tional appr.ach for.engineer.ng high-per.or.ance SSLMBs addr.ssing electr.lyte r.quir.ments with specifically designed polymer. at the positive electr.de and as *** this wor.,SSLMBs wer. assembled with poly(pr.pylene car.onate)(PPC),offer.ng stability towar. oxidation at the positive electr.de,and a gel polymer.electr.lyte with polyethyleneglycol dimethylether.PEGDME)as separ.tor.offer.ng high ionic conductivity at low temper.tur. and sufficient inter.acial stability with Li *** electr.chemical pr.per.ies and per.or.ance of cells with LiFePO_(4) and Li[Ni_(0.6)Mn_(0.2)Co_(0.2)]O_(2) positive electr.des ar. thor.ughly investigated as function of the oper.ting temper.tur. by using a host of char.cter.zation ***-voltage cells with an ar.al capacity of 0.7 mAh·cm^(−2)cycled at 40℃ exhibit a higher.capacity r.tention than the cells cycled at 70℃.To under.tand such differ.nces,a thr.e-electr.de setup is applied to discr.minate anodic pr.cesses fr.m cathodic as function of the *** elucidate the ageing and inter.acial evolution for.DLPE cells with gel polymer.electr.lytes paving the way for.building per.or.ance solid state batter.es.

关键词： double layer.polymer.electr.lyte solid-state lithium metal batter. gel polymer.electr.lyte high voltage inter.acial study

The Holocene Evolution ofthe Ebr. Delta Catalonia, Spain

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地理学报 1999年第5期54卷 462-469页

作者： Antoni Canicio 1,Car.es iban～ez 2 (1 C/Maj.r.10, 43580 Deltebr., Spain 2 Depar.ment of Ecology Univer.ity of Bar.elona Bar.elona, Spain) C/Maj.r.10 43580 Deltebre Spain 西班牙 043580 Univer.ity of Bar.elona 西班牙

The existing scientific liter.tur. about the Ebr. delta states that it for.ed in ver. r.cent times (mostly since the middle ages) and that in r.man times it was an estuar.. This belief is based on er.oneous inter.r.tation of histor.cal data, r.ther.than on scientific evidence. We pr.sent the fir.t data about the position of ear.y coastlines based on r.diocar.on dating. The evidence pr.ves the existence of the Ebr. delta as much as 5 750 a BP. Another.ear.y coastline that dates to 3 045 a BP has also been identified. Using this infor.ation and other.sour.es such as old maps and pr.sent day bathymetr. of old er.ded deltaic lobes, we constr.cted the fir.t evolutionar. sequence of the Ebr. delta dur.ng the Holocene. Car.ogr.phic infor.ation was car.fully and cr.tically assessed in the pr.cess of selecting those maps that ar. coher.nt with geomor.hic str.ctur.s. Details about the evolution of deltaic lobes ar. only given for.the last millennium. The development of the souther. lobe was at its maximum about 1 ka BP. By the 16th centur. the lobe had alr.ady been str.ngly r.shaped (maximum r.tr.at about 8 km) after.the abandonment of the old r.ver.ar.. At that time the Ebr. delta alr.ady had developed a sur.ace similar.to that of the pr.sent. The maximum penetr.tion of the lobe into the sea (about 25 km) is clear.y indicated in bathymetr.c maps. Dur.ng the 17th centur. the nor.her. lobe r.ached its maximum extent (also about 25 km), and at the end of that centur. the centr.l lobe (the one pr.sently active) star.ed to for., r.aching its maximum gr.wth (again about 25 km) by the beginning of the 20th centur..

关键词： Ebr. r.ver delta dischar.e sediment load Holocene

Extr.ct of Yokukansan impr.ves anxiety-like behavior.and incr.ases ser.m br.in-der.ved neur.tr.phic factor.in r.ts with cer.br.l ischemia combined with amyloid-β42 peptide

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j.ur.al of Tr.ditional Chinese Medicine 2019年第1期39卷 50-58页

作者： Ai Nogami-Har. Kaor. Kubota Kotar. Takasaki Takuya Watanabe Nobuaki Egahir. Hikar. iba r.sako Fuj.kawa Shutar. Katsur.bayashi Funda Bolukbasi Hatip Izzettin Hatip-Al-Khatib Katsunor. Iwasaki Depar.ment of Neur.phar.acology Faculty of Pharmaceutical ScienceFukuoka UniversityFukuoka 814-0180Japan Institute for.Aging and Br.in Sciences Fukuoka UniversityFukuoka 814-0180Japan Depar.ment of Phar.acy Kyushu University HospitalFukuoka 812-8582Japan Depar.ment of Medical Phar.acology Faculty of MedicinePamukkale UniversityDenizli 20070Turkey

OBj.CTIVE: To examine the effects of Yokukansan(YKS) extr.ct on two endogenous modulator. of anxiety, br.in-der.ved neur.tr.phic factor.BDNF)and ser.tonin (5-HT)_(2A) r.ceptor. phar.acologically, in the ischemic r.t model of ***: The cer.br.l ischemia(CI) was induced by bilater.l occlusion of the ver.ebr.l and common car.tid ar.er.es(4-vessel occlusion ischemia). The CI was combined with the amyloid-β42 peptide(A42) inj.cted intr.cer.br.ventr.cular.y, and r.fer.eβdto as CI+Aβ. Anxiety-like behavior. wer. assessed by elevated plus maze(enclosed ar.), light/dar. tr.nsition test(dar. chamber., and open-field ***-dog shakes wer. induced by the 5-HT_(2A) r.ceptor.agonist 2, 5-dimethoxy-4-iodoamphetamine(DOI). The concentr.tion of BDNF in ser.m was deter.ined by enzyme-linked immuno sor.ent ***: CI + Aβ incr.ased anxiety, as demonstr.ted by the incr.ase of time spent in the enclosed ar.s and dar. chamber., and locomotion in the outer.zone of the open field(thigmotaxis). CI + Adecr.ased the ser.m concentr.tion of BDNF. YKS r.β-duced the anxiety-like behavior., suppr.ssed the DOI-induced wet-dog shakes and incr.ased ser.m BDNF ***: Our.findings suggest that YKS extr.ct impr.ves CI + Aβ-induced anxiety by antagonizing 5-HT_(2A) r.ceptor. and incr.asing BDNF.

关键词： Br.in ischemia Amyloid beta-peptides Anxiety br.in-der.ved neur.tr.phic factor r.ceptor ser.tonin 5-HT2A Yokukansan

A modified Mur.shige and Skoog media for.efficient multipleshoot induction in G. ar.or.a r.xb.

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j.ur.al of For.str. r.sear.h 2014年第3期25卷 557-564页

作者： Shilpa S. Madke Konglanth j. Cher.an r.pesh S. Bader. Depar.ment of Botany Hislop College Depar.ment of Botany RTM Nagpur University M. J. Phuley Educational Campus

This paper.r.por.s on the effect of var.ous micr.pr.pagation factor. of Gmelina ar.or.a r.xb. thr.ugh multiple shoot induction. Factor. like the sour.e and age of explants, plant gr.wth r.gulator. （PGr.）, media composition, and car.on sour.e affected multiple shoot-ing in the pr.sent study. Among all the explants used, only shoot tips der.ved fr.m one, two, and thr.e week old seedlings could for. multiple shoots. Besides, the for.ation of multiple shoots depended on the con-centr.tion and combination of PGr.. Among all the PGr., BAP （6-benzylaminopur.ne） alone gave the highest r.gener.tion efficiency. Simi-lar.y, iba （Indole-3-butyr.c acid） was the most efficient PGr.in inducing r.ot for.ation in the micr.shoots. Media composition and car.on sour.e also affected the r.gener.tion efficiency. MS （Mur.shige and Skoog medium） pr.ved to be the best media for.r.gener.tion followed by B5, SH （Schenk and Hilder.r.ndt medium） and WPM （Woody plant medium） in that or.er. Similar.y, among sugar., only sucr.se and glucose sup-por.ed induction of micr.shoots. Based on this study we r.commend the use of glucose in place of sucr.se in MS medium for.maximum r.gener.-tion efficiency.

关键词： agr.for.str. micr.pr.pagation plant nutr.tion shoot tipexplant timber.plant Ver.enaceae

Campanian Climatic Change:Isotopic Evidence fr.m Far.East,Nor.h Amer.ca,Nor.h Atlantic and Wester. Eur.pe

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Acta Geologica Sinica(English Edition) 2007年第6期81卷 1049-1069页

作者： Yur. D. ZAKHAr.V Yasunar. SHIGETA Kazushige TANABE Yasuhir. iba Olga P. SMYSHLYAEVA Ekater.na A. SOKOLOVA Alexander.M. POPOV Tatiana A. VELIVETSKAYA Tamar. B. AFANASYEVA Far.Easter. Geological Institute FEB RAS Stoletiya Prospect 159 Vladivostok 690022 Russia Depar.ment of Geology National Science Museum 3-23-1 Hyakunincho Shinjuku-ku Tokyo 169-0073 Japan Univer.ity of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-0033 Japan Institute of Oceanology RAS Nakhimovskij Prospect 36 Moscow 117997 Russia

Paleoclimatic settings have been r.constr.cted for.the Campanian using or.ginal oxygenisotopic analyses of well-pr.ser.ed molluskan and for.minifer. shells fr.m r.ssian Far.East, Hokkaido, USA, Belgium and some DSDP holes （95, 98, 102, 390A, and 392A） in Nor.h Atlantic. Ear.y Ear.y Campanian climatic optimum has been r.cognized fr.m data on high bottom shelf water.paleotemper.tur.s in middle latitudes of both the wester. cir.um-Pacific （to 24.2℃） and the easter. cir.um-Pacific （to 26.4℃） ar.as and high bottom shallow water.paleotemper.tur.s in high latitudes of the Kor.ak Upland （22.4-25.5℃）, which agr.es with the data on the Campanian Bar.kovskaya flor. in high latitudes （Golovneva and Her.an, 1998） and j.nker.flor. and its equivalents in middle latitudes. j.dging fr.m the data on compar.tively high bottom shallow water.paleotemper.tur. values in high latitudes, South Alaska （19.4℃） and the Kor.ak Upland （22.4-25.5℃）, we also expect Latest Campauian temper.tur. maximum, which has not been confir.ed, however. for.low and middle latitudes by neither.of isotopic nor.paleobotanic data now. Main dimatic tendency dur.ng the Campanian （with the exception of Latest Campanian） has been lear.ed fr.m isotopic composition of Campanian ar.gonitic ammonoid shells fr.m the Hokkaido-South Sakhalin （Kr.lyon） mar.ne basin. In contr.r. to Huber.s et al. （2002） assumption, we expect war. gr.enhouse conditions dur.ng the most par. of the Campanian.

关键词： isotopic data cephalopod bivalve and gastr.pod mollusks paleotemper.tur.s,Campanian Sakhalin Hokkaido Kor.ak Upland Nor.h Amer.ca Nether.ands Atlantic

Isother.al hydr.gen absor.tion pr.cess of Pd-capped Mg films tr.ced by ion beam techniques and optical methods

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j.ur.al of Magnesium and Alloys 2024年第9期12卷 3675-3684页

作者： D.Abej.n P.Pr.eto j.K.Kim A.r.dondo-Cuber. M.L.Cr.spillo F.Lear.ini I.j.Fer.er.G.Gar.ía j.r.Ar.s Depar.amento de Fisica de Mater.ales Universidad Autónoma de MadridMadrid28049Spain Centr. de Micr.-Análisis de Mater.ales(CMAM) Universidad Autónoma de MadridMadrid28049Spain Advanced Analysis Center KIST5 Hwarang-ro 14-gilSeoul 02792Republic of Korea Depar.amento de Física Aplicada Universidad Autónoma de MadridMadrid28049Spain Instituto Nicolás Cabr.r. Universidad Autónoma de MadridMadrid28049Spain

Pd-capped nanocr.stalline Mg films wer. pr.par.d by electr.n beam evapor.tion and hydr.genated under.isother.al conditions to inves-tigate the hydr.gen absor.tion pr.cess via ion beam techniques and in situ optical *** wer. char.cter.zed by differ.nt techniques such as X-r.y diffr.ction(Xr.)and scanning electr.n micr.scopy(SEM).r.ther.or. backscatter.ng spectr.metr.(r.S)and elastic r.coil detection analysis(Er.A)pr.vided a detailed compositional depth pr.file of the films dur.ng ***-solid r.action kinetics theor. applied to Er.A data r.vealed a H absor.tion mechanism contr.lled by H *** r.te-limiting step was also confir.ed by Xr. *** diffusion coefficient(D)was also deter.ined via r.S and Er.A,with a value of(1.1±0.1)·10^(−13)cm^(2)/s at 140℃.r.sults confir. the validity of iba to monitor.the hydr.genation pr.cess and to extr.ct the contr.l mechanism of the *** H kinetic infor.ation given by optical methods is str.ngly influenced by the optical absor.tion of the magnesium layer.r.vealing that thinner.films ar. needed to extr.ct fur.her.and r.liable infor.ation fr.m that technique.

关键词： Magnesium hydr.de Hydr.gen absor.tion Ion beam techniques Optical tr.cing Absor.tion mechanism

采用数字乳腺摄影后假阳性结果减低:西班牙乳腺癌人群的4种筛查程序分析

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国际医学放射学杂志 2011年第2期 177-178页

作者： M.Sala D.Salas F.Belvis M.Sánchez j.Fer.er.j.ibaez 唐光健 Health Ser.ices Evaluation and Clinical Epidemiology Depar.ment IMIM-Hospital del MarCIBER Epidemiología y Salud Pública(CIBERESP)

目的评价引入数字乳腺摄影后,对西班牙乳腺癌人群4种筛查程序中大样本受检妇女召回率、检出率、假阳性率与有创处理率的影响。材料与方法研究由伦理委员会

关键词：数字乳腺摄影假阳性率乳腺癌乳腺肿瘤筛查西班牙南欧

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鲁尔传统工业区的蜕变之路

国际城市规划 2009年第S1期24卷 301-304页

作者：克劳兹.r.昆斯曼刘健王纺多特蒙德大学空间规划学院清华大学建筑与城市研究所英国Sussex大学发展学院

鲁尔区作为世界传统工业集聚地之一,在历史上一个多世纪的时间里,曾经为德国提供了大量的煤炭和钢铁资源,被誉为德国的动力工厂。二战结束后,鲁尔区又成为德国经济快速复苏的发动机,煤炭和钢铁生产在短期内迅速恢复,为地区发展提供了动... 详细信息

鲁尔区作为世界传统工业集聚地之一,在历史上一个多世纪的时间里,曾经为德国提供了大量的煤炭和钢铁资源,被誉为德国的动力工厂。二战结束后,鲁尔区又成为德国经济快速复苏的发动机,煤炭和钢铁生产在短期内迅速恢复,为地区发展提供了动力来源。

关键词：鲁尔区传统工业国际建筑展中国城市文化产业区域规划煤炭德国经济产业结构调整转型发展