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Journal of Rare Earths 2014年第12期32卷 1101-1108页

作者： Alexander A.Maleev Anatoly P.Pushkarev Vasily A.Ilichev Mikhail A.Lopatin Maxim A.Samsonov Georgy K.Fukin Georgy L.Pakhomov Vladislav V.Travkin ivan d.grishin Mikhail N.Bochkarev G.A.Razuvaev Institute of Organometallic Chemistry Russian Academy of Sciences Tropinina str.49 603950 Nizhny Novgorod Russia department of Organic Chemistry Nizhny Novgorod State University 23 Gagarin Avenue 603950 Nizhny Novgorod Russia Institute for Physics of Microstructures Russian Academy of Sciences 7 ul.Akademicheskaya 603950 Nizhny Novgorod Russia

The monophthalocyanine complexes of samarium and terbium containing axial 2-mercaptobenzothiazole（Pc Sm（MBT）（1））, 2-（2-benzoxazol-2-yl） phenolate（Pc Tb（OON）（2）） or 2-（2-benzothiazol-2-yl）phenolate（Pc Tb（SON）（3）） ligands were synthesized and identified by elemental, LdI-TOF and X-ray（for 1） ***（PL） and electroluminescence（EL） spectra of the compounds contained only emission bands of phthalocyanine and axial ligands but did not contain the bands of f-f *** was found that among the complexes 1, 2, 3 the latter had highest photoconductivity（~10–7 S/cm） and photovoltaic *** organic photovoltaic device（OPV） of configuration of ITO/3/C60/Alq3/Al revealed open-circuit voltage（VOC） of 0.24 V and short current density（ISC） of 0.3 μA/cm2 under illumination by a xenon lamp at 17 m W/cm2.

关键词： phthalocyanine samarium terbium luminescence photovoltaic OLEd rare earths

New luminescent 10-oxybenzoquinolate complexes of rare earth metals

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Journal of Rare Earths 2023年第8期41卷 1135-1143,I0001页

作者： Tatyana V.Balashova Svetlana K.Polyakova Vasily A.Ilichev Andrey A.Kukinov Roman V.Rumyantcev Georgy K.Fukin ivan d.grishin Artem N.Yablonskiy Alexander F.Shestakov Mikhail N.Bochkarev G.A.Razuvaev Institute of Organometallic Chemistry of Russian Academy of Sciences Tropinina Street49603950Nizhny NovgorodRussian Federation Nizhny Novgorod State University Gagarina Avenue 23/2603950Nizhny NovgorodRussian Federation Institute for Physics of Microstructures of Russian Academy of Sciences Akademicheskaya Street 7603950Nizhny NovgorodRussian Federation Institute of Problems of Chemical Physics of Russian Academy of Sciences Academician Semenov Avenue1ChernogolovkaMoscow Region142432Russian Federation

A series of Sc,Y,Ce,Pr,Nd,Sm,Eu,Gd,Tb,Ho,Er,Tm and Yb complexes with oxybenzoquinoline ligands(BQ) was synthesized by the reactions of 10-hydroxybenzo[h]quinoline with cyclopentadienides or tris(trimethylsilyl)amides of rare earth *** structure,as well as the photo-and electroluminescent(PL,EL) properties of these complexes in solutions and solid state were *** solutions,complexes of sodium and lanthanides exhibit double peaked ligand-centered PL of enol and keto forms of BQ with a quantum yield of 1%-8%.In the solid state the complexes of Sm,Eu,Ho,Nd,Er,and Yb along with the ligand-centered PL also exhibit a moderate-intensity metal-centered PL which is characteristic of the corresponding Ln^(3+) ***(BQ)_(3) complex shows bright green EL which has intensity comparable to the best results observed for scandium complexes with other organic ligands.

关键词： Lanthanides Photoluminescence(PL) Electroluminescence(EL) 10-hydroxybenzo[h]quinoline X-ray structure Organic light-emitting diodes(OLEds)

Boron-containing compounds as labels,drugs,and theranostic agents for diabetes and its complications

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World Journal of diabetes 2024年第6期15卷 1060-1069页

作者： Marvin A Soriano-Ursúa R ivan Cordova-Chávez Eunice d Farfan-García George Kabalka department of Physiology Escuela Superior de MedicinaInstituto Politécnico NacionalCiudad de México 11340Mexico department of Physiology Instituto Politécnico NacionalMexico City 11340Mexico department of Biochemistry Instituto Politécnico NacionalMexico City 11340Mexico department of Chemistry The University of TennesseeKnoxvilleTN 37996United States

diabetes is a disease with a high global *** strategies have failed to limit the advancement and impact of the *** early diagnosis and treatment will require the development of new *** this sense,boroncontaining compounds have been reported as agents with the ability to reduce glycemia and *** have also been used for labeling and measuring carbohydrates and other molecules linked to the initial stages of diabetes and its *** addition,certain boron compounds bind to molecules related to diabetes development and their biological activity in the regulation of elevated ***,it should be noted that some boron compounds appear to exert beneficial effects on diabetes complications such as accelerating wound healing while ameliorating pain in diabetic patients.

关键词： Boron Carbohydrates Metabolism diabetes Boronodipyrromethene

Three-dimensional Convection in an Inclined Porous Layer Subjected to a Vertical Temperature Gradient

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Fluid dynamics & Materials Processing 2024年第9期20卷 1957-1970页

作者： ivan Shubenkov Tatyana Lyubimova Evgeny Sadilov Computational Fluid dynamics Laboratory Institute of Continuous Media Mechanics UB RASPerm614068Russia Theoretical Physics department Perm State UniversityPerm614990Russia

In this paper,we study the onset and development of three-dimensional convection in a tilted porous layer saturated with a *** layer is subjected to a gravitational field and a strictly vertical temperature ***,problems of thermal convection in tilted porous media saturated with a liquid are studied by assuming constant different temperatures at the boundaries of the layer,which prevent these systems from supporting conductive(non-convective)*** boundary conditions considered in the present work allow a conductive state and are representative of typical geological *** an earlier work,we carried out a linear stability analysis of the conductive *** was shown that at any layer tilt angles,the most dangerous type of disturbances are longitudinal ***,a non-zero velocity component exists in *** the present work,threedimensional non-linear convection regimes are *** original three-dimensional problem is reduced to two-dimensional one with an analytical expression for the velocity z-component v_(z)=v_(z)(x,y).It is shown that the critical Rayleigh number values obtained through numerical solutions of the obtained 2d problem by a finite difference method for different layer inclination angles,are in a good agreement with those predicted by the linear *** number of convective rolls realized in nonlinear calculations also fits the linear theory predictions for a given cavity *** carried out at low supercriticalities show that a direct bifurcation takes *** increasing supercriticality,no transitions to other convective regimes are *** situation studied in this problem can be observed in oil-bearing rock formations under the influence of a geothermal temperature gradient,where the ensuing fluid convection can affect the distribution of oil throughout the layer.

关键词： Thermal convection inclined layer porous media vertical temperature gradient

Polariton lasing in Mie-resonant perovskite nanocavity

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Opto-Electronic Advances 2024年第4期7卷 27-42页

作者： Mikhail A.Masharin daria Khmelevskaia Valeriy I.Kondratiev daria I.Markina Anton d.Utyushev dmitriy M.dolgintsev Alexey d.dmitriev Vanik A.Shahnazaryan Anatoly P.Pushkarev Furkan Isik ivan V.Iorsh ivan A.Shelykh Hilmi V.demir Anton K.Samusev Sergey V.Makarov UNAM-Institute of Materials Science and Nanotechnology National Nanotechnology Research CenterDepartment of Electrical and Electronics EngineeringDepartment of PhysicsBilkent UniversityAnkara 06800Turkey ITMO University School of Physics and EngineeringSt.Petersburg 197101Russia Abrikosov Center for Theoretical Physics MIPTDolgoprudnyiMoscow Region 141701Russia LUMINOUS!Center of Excellence for Semiconductor Lighting and displays School of Electrical and Electronic EngineeringSchool of Physical and Mathematical SciencesSchool of Materials Science and EngineeringNanyang Technological UniversitySingapore 639798Singapore department of Physics Engineering Physics and AstronomyQueen’s UniversityKingstonOntario K7L 3N6Canada Science Institute University of IcelandDunhagi 3IS-107ReykjavikIceland Experimentelle Physik 2 Technische Universität DortmundDortmund 44227Germany Qingdao Innovation and development Center Harbin Engineering UniversityQingdao 266000China

deeply subwavelength lasers(or nanolasers)are highly demanded for compact on-chip bioimaging and sensing at the *** of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting *** we ex-ploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr3 nanoparticle to achieve coherent emission at the visible wavelength of around 0.53μm from its ultra-small(≈0.007μm3 or≈λ3/20)semiconductor *** polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct com-parison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material *** a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy(≈35 meV),re-fractive index(>2.5 at low temperature),and luminescence quantum yield of CsPbBr3,but also by the optimization of po-laritons condensation on the Mie resonances with quality factors improved by the metallic ***,the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr3,which govern polaritons condensation *** chemically synthesized colloidal CsPbBr3 nanolasers can be potentially de-posited on arbitrary surfaces,which makes them a versatile tool for integration with various on-chip systems.

关键词： nanolaser perovskite polariton Mie resonance exciton-polariton

Pelvic fractures in blunt trauma patients:A comparative study

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World Journal of Orthopedics 2024年第5期15卷 418-434页

作者： Alexander A Fokin Joanna Wycech Knight Madison E Tharp Kyler C Brinton Phoebe K Gallagher Justin Fengyuan Xie Russell d Weisz ivan Puente Trauma and Critical Care Services Delray Medical CenterDelray BeachFL 33484United States Charles E Schmidt College of Medicine Department of SurgeryFlorida Atlantic UniversityBoca RatonFL 33431United States Trauma and Critical Care Services Broward Health Medical CenterFort LauderdaleFL 33316United States Charles E Schmidt College of Medicine Florida Atlantic UniversityBoca RatonFL 33431United States Herbert Wertheim College of Medicine Department of SurgeryFlorida International UniversityMiamiFL 33199United States

BACKGROUNd Pelvic fractures(PF)with concomitant injuries are on the rise due to an increase of high-energy *** of the elderly population with age related comorbidities further complicates the *** organ injuries are kindred with PF due to the proximity to pelvic *** of contrast blush(CB)on computed tomography in patients with PF is considered a sign of active bleeding,however,its clinical significance and association with outcomes is *** To analyze polytrauma patients with PF with a focus on the geriatric population,co-injuries and the value of contrast *** This retrospective cohort study included 558 patients with PF admitted to level 1 trauma center(01/2017-01/2023).Analyzed variables included:Age,sex,mechanism of injury(MOI),injury severity score(ISS),Glasgow coma scale(GCS),abbreviated injury scale(AIS),co-injuries,transfusion requirements,pelvic angiography,embolization,laparotomy,orthopedic pelvic surgery,intensive care unit and hospital lengths of stay,discharge disposition and *** study compared geriatric and non-geriatric patients,patients with and without CB and abdominal *** score matching was implemented in comparison *** PF comprised 4%of all trauma admissions.89 patients had CB.286(52%)patients had concomitant injuries including 93(17%)patients with abdominal *** patients compared to non-geriatric had more falls as MOI,lower ISS and AIS pelvis,higher GCS,less abdominal co-injuries,similar CB and angio-embolization rates,less orthopedic pelvic surgeries,shorter lengths of stay and higher *** propensity matching,orthopedic pelvic surgery rates remained lower(8%vs 19%,Pd mortality higher(13%vs 4%,Pd to without CB had more pelvic angiography(71%vs 12%,P<0.001),hi

关键词： Pelvic fractures Geriatric trauma patients Abdominal co-injuries Contrast blush Contrast extravasation Angioembolization Polytrauma patients Surgical interventions Blunt trauma External and internal fixation for pelvic stabilization

From bibliometric analysis: 3d printing design strategies and battery applications with a focus on zinc‐ion batteries

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SmartMat 2024年第1期5卷 59-82页

作者： Xuan Gao Kejiang Liu Chang Su Wei Zhang Yuhang dai ivan P.Parkin Claire J.Carmalt Guanjie He Christopher Ingold Laboratory Department of ChemistryUniversity College LondonLondonUK Electrochemical Innovation Lab(EIL) Department of Chemical EngineeringUniversity College LondonLondonUK department of Physics Hong Kong Baptist UniversityHong KongChina Nanyang Technopreneurship Center Nanyang Technological UniversitySingaporeSingapore

Three‐dimensional(3d)printing has the potential to revolutionize the way energy storage devices are designed and *** this paper,we explore the use of 3d printing in the design and production of energy storage devices,especially zinc‐ion batteries(ZIBs)and examine its potential advantages over traditional manufacturing methods.3d printing could significantly improve the customization of ZIBs,making it a promising strategy for the future of energy *** particular,3d printing allows for the creation of complex,customized geometries,and designs that can optimize the energy density,power density,and overall performance of ***,we discuss and compare the impact of 3d printing design strategies based on different configurations of film,interdigitation,and framework on energy storage devices with a focus on ***,3d printing enables the rapid prototyping and production of batteries,reducing leading times and costs compared with traditional manufacturing ***,there are also challenges and limitations to consider,such as the need for further development of suitable 3d printing materials and processes for energy storage applications.

关键词： 3d printing battery commercialization bibliometric analysis electrode configurations zinc‐ion battery

Mid-term outcomes of a kinematically designed cruciate retaining total knee arthroplasty

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World Journal of Orthopedics 2024年第2期15卷 118-128页

作者： Jonathan L Katzman Akram A Habibi Muhammad A Haider Casey Cardillo ivan Fernandez-Madrid Morteza Meftah Ran Schwarzkopf department of Orthopedic Surgery Division of Adult Reconstructive SurgeryNYU Langone Orthopedic HospitalNYU Langone HealthNew YorkNY 10010United States

BACKGROUNd Advances in implant material and design have allowed for improvements in total knee arthroplasty(TKA)outcomes.A cruciate retaining(CR)TKA provides the least constraint of TKA designs by preserving the native posterior cruciate *** research exists that has examined clinical outcomes or patient reported outcome measures(PROMs)of a large cohort of patients undergoing a CR TKA utilizing a kinematically designed *** was hypothesized that the studied CR Knee System would demonstrate favorable outcomes and a clinically significant improvement in pain and functional *** To assess both short-term and mid-term clinical outcomes and PROMs of a novel CR TKA *** A retrospective,multi-surgeon study identified 255 knees undergoing a TKA utilizing a kinematically designed CR Knee System(JOURNEY™II CR;Smith and Nephew,Inc.,Memphis,TN)at an urban,academic medical institution between March 2015 and July 2021 with a minimum of two-years of clinical follow-up with an orthopedic *** demographics,surgical information,clinical outcomes,and PROMs data were collected via query of electronic medical *** PROMs collected in the present study included the Knee Injury and Osteoarthritis Outcome Score for Joint Replacement(KOOS JR)and Patient-Reported Outcomes Measurement Information System(PROMIS■)*** significance of improvements in mean PROM scores from preoperative scores to scores collected at six months and two-years postoperatively was analyzed using Independent Samples *** Of the 255 patients,65.5%were female,43.8%were White,and patients had an average age of 60.6 *** osteoarthritis(96.9%)was the most common primary *** mean surgical time was 105.3 minutes and mean length of stay was 2.1 d with most patients discharged home(92.5%).There were 18 emergency department(Ed)visits within 90 d of surgery resulting in a 90 d Ed visit rate of 7.1%,including a 2.4%orthopedic-related Ed visit ra

关键词： Total knee arthroplasty Cruciate retaining Kinematic design Survivorship Bearing material Prosthetic design Clinical outcomes Patient-reported outcome measures

Variational Approach to 2d and 3d Heat Conduction Modeling

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Journal of Applied Mathematics and Physics 2024年第4期12卷 1383-1400页

作者： Slavko Đurić ivan Aranđelović Milan Milotić Faculty of Traffic Engineering University of East Sarajevo Doboj Bosnia and Herzegovina Faculty of Mechanical Engineering University of Belgrade Belgrade Republic of Serbia

The paper proposes an approximate solution to the classical (parabolic) multidimensional 2d and 3d heat conduction equation for a 5 × 5 cm aluminium plate and a 5 × 5 × 5 cm aluminum cube. An approximate solution of the generalized (hyperbolic) 2d and 3d equation for the considered plate and cube is also proposed. Approximate solutions were obtained by applying calculus of variations and Euler-Lagrange equations. In order to verify the correctness of the proposed approximate solutions, they were compared with the exact solutions of parabolic and hyperbolic equations. The paper also presents the research on the influence of time parameters τ as well as the relaxation times τ ∗ to the variation of the profile of the temperature field for the considered aluminum plate and cube.

关键词： Classical Equation of Heat Conduction Generalized Equation of Heat Conduction Calculus of Variations Approximate Solution

3d micro-devices for enhancing the lateral resolution in optical microscopy

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Light(Advanced Manufacturing) 2024年第2期5卷 50-63页

作者： Gordon Zyla Goran Maconi Anton Nolvi Jan Marx dimitra Ladika Ari Salmi Vasileia Melissinaki ivan Kassamakov Maria Farsari Institute of Electronic Structure and Laser Foundation for Research and Technology-HellasHeraklionGreece Electronics Research Laboratory Department of PhysicsUniversity of HelsinkiHelsinkiFinland Applied Laser Technologies Ruhr University BochumBochumGermany

Although optical microscopy is a widely used technique across various multidisciplinary fields for inspecting small-scale objects,surfaces or organisms,it faces a significant limitation:the lateral resolution of optical microscopes is fundamentally constrained by light *** micro-spheres,however,offer a promising solution to this issue as they are capable of significantly enhancing lateral resolution through extraordinary phenomena,such as a photonic *** upon the potential of dielectric micro-spheres,this paper introduces a novel approach for fabricating 3d micro-devices designed to enhance lateral resolution in optical *** proposed 3d micro-device comprises a modified coverslip and a micro-sphere,facilitating easy handling and integration into any existing optical *** manufacture the device,two advanced femtosecond laser techniques are employed:femtosecond laser ablation and multi-photon *** laser ablation was employed to create a micro-hole in the coverslip,which allows light to be focused through this ***-photon lithography was used to fabricate a micro-sphere with a diameter of 20μm,along with a cantilever that positions the above the processed micro-hole and connect it with the *** this context,advanced processing strategies for multi-photon lithography to produce a micro-sphere with superior surface roughness and almost perfect geometry(λ/8)from a Zr-based hybrid photoresist are *** performance of the micro-device was evaluated using Mirau-type coherence scanning interferometry in conjunction with white light illumination at a central wavelength of 600 nm and a calibration grid(Λ=0.28μm,h>50 nm).Here,the 3d micro-device proved to be capable of enhancing lateral resolution beyond the limits achievable with conventional lenses or microscope objectives when used in ***,it maintained the high axial resolution characteristic of Mirau-type coherenc

关键词： Photonic nanojet Multi-photon lithography Optical microscopy Micro-optics Multi-photon grayscale lithography Extreme manufacturing