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Room Temperature Synthesis of Vertically Aligned Amorphous Ultrathin NiCo-LDH Nanosheets Bifunctional Flexible Supercapacitor Electrodes

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Energy & Environmental Materials 2024年第2期7卷 277-286页

作者： Kwadwo Asare Owusu Zhaoyang Wang Ali Saad Felix Ofori Boakye muhammad Asim Mushtaq muhammad Tahir Ghulam Yasin Dongqing Liu Zhengchun Peng Xingke Cai Institute for Advanced Study Shenzhen UniversityShenzhen 518060China College of Physics and Optoelectronics Shenzhen University3688 Nanhai BoulevardNanshan DistrictShenzhen 518060China School of Chemistry and Materials Science Hubei Engineering UniversityNo.272 Traffic AvenueXiaogan 432000China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyNo.122 Luoshi RoadWuhan 430070China Key Laboratory of Green Printing CAS Research Centre for Excellence in Molecular ScienceInstitute of Chemistry Chinese Academy of Sciences(ICCAS)Beijing 100190China College of Mechatronics and Control Engineering Shenzhen University3688 Nanhai BoulevardNanshan DistrictShenzhen 518050China

Developing a simple scalable method to fabricate electrodes with high capacity and wide voltage range is desired for the real use of electrochemical ***,we synthesized amorphous NiCo-LDH nanosheets vertically aligned on activated carbon cloth substrate,which was in situ transformed from Co-metal-organic framework materials nano-columns by a simple ion exchange process at room *** to the amorphous and vertically aligned ultrathin structure of NiCo-LDH,the NiCo-LDH/activated carbon cloth composites present high areal capacities of 3770 and 1480 mF cm^(-2)as cathode and anode at 2 mA cm^(-2),and 79.5%and 80%capacity have been preserved at 50 mA cm^(-2).In the meantime,they all showed excellent cycling performance with negligible change after>10000 *** fabricating them into an asymmetric supercapacitor,the device achieves high energy densities(5.61 mWh cm^(-2)and 0.352 mW cm^(-3)).This work provides an innovative strategy for simplifying the design of supercapacitors as well as providing a new understanding of improving the rate capabilities/cycling stability of NiCo-LDH materials.

关键词： amorphous nanosheets aqueous supercapacitor high volumetric/areal energy density NiCo-LDH room temperature synthesis

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Recent Advances in Deuteration Reactions

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Chinese Journal of Chemistry 2024年第10期42卷 1145-1156页

作者： Hao Li muhammad Shabbir Wu Li Aiwen Lei Institutefor Advanced Studies(IAS) Collegeof Chemistry and Molecular SciencesWuhan UniversityWuhanHubei 430072China

The deuteration of organic compounds has attracted more attentions in recent years for the potential applications in new drug discovery and synthetic *** this purpose,many efficient deuterium labeling methodologies have been developed,including hydrogen isotope exchange(HIE),reductive deuteration,and dehalogenative deuteration that allow for the synthesis of selectively deuterated *** the last few years,great breakthroughs in selective isotope labeling have been achieved and the interest in new methodologies for the deuteration of organic molecules is *** this review,we summarized the recent developments in the selective deuteration of organic molecules since *** types of key processes in deuterium incorporation reactions,including H/D exchange,reductive deuteration and dehalogenative deuteration,are introduced and discussed.

关键词： Deuterated compounds H/D exchange Reductive deuterations Dehalogenative deuterations Deuterium C-Hactivation Synthetic methods

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Moiré superlattices arising from growth induced by screw dislocations in layered materials

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Chinese Physics B 2024年第7期33卷 72-77页

作者：田伏钰 muhammad Faizan 贺欣孙远慧张立军 State Key Laboratory of Integrated Optoelectronics Key Laboratory of Automobile Materials of MOE and College of Materials Science and Engineering Jilin UniversityChangchun 130012China Suzhou Laboratory Suzhou 215123China

Moiré superlattices(MSLs) are modulated structures produced from homogeneous or heterogeneous two-dimensional layers stacked with a twist angle and/or lattice mismatch. Enriching the methods for fabricating MSL and realizing the unique emergent properties are key challenges in its investigation. Here we recommend that the spiral dislocation driven growth is another optional method for the preparation of high quality MSL samples. The spiral structure stabilizes the constant out-of-plane lattice distance, causing the variations in electronic and optical properties. Taking SnS_(2) MSL as an example, we find prominent properties including large band gap reduction(~ 0.4 e V) and enhanced optical activity. Firstprinciples calculations reveal that these unusual properties can be ascribed to the locally enhanced interlayer interaction associated with the Moiré potential modulation. We believe that the spiral dislocation driven growth would be a powerful method to expand the MSL family and broaden their scope of application.

关键词： Moirésuperlattices interlayer interaction spiral dislocation layered materials

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Stable stripe and vortex solitons in two-dimensional spin-orbit coupled Bose-Einstein condensates

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Communications in Theoretical Physics 2024年第6期76卷 26-33页

作者： Yuan Guo muhammad Idrees Ji Lin Hui-jun Li Institute of Nonlinear Physics and Department of Physics Zhejiang Normal UniversityJinhua 321004China Zhejiang Institute of Photoelectronics and Zhejiang Institute for Advanced Light Source Zhejiang Normal UniversityJinhua 321004China

We present a flexible manipulation and control of solitons via Bose-Einstein *** the presence of Rashba spin-orbit coupling and repulsive interactions within a harmonic potential,our investigation reveals the numerical local solutions within the *** manipulating the strength of repulsive interactions and adjusting spin-orbit coupling while maintaining a zero-frequency rotation,diverse soliton structures emerge within the *** include plane-wave solitons,two distinct types of stripe solitons,and odd petal solitons with both single and double *** stability of these solitons is intricately dependent on the varying strength of spin-orbit ***,stripe solitons can maintain a stable existence within regions characterized by enhanced spin-orbit coupling while petal solitons are unable to sustain a stable existence under similar *** rotational frequency is introduced to the system,solitons undergo a transition from stripe solitons to a vortex array characterized by a sustained *** rotational directions of clockwise and counterclockwise are non-equivalent owing to spin-orbit *** a result,the properties of vortex solitons exhibit significant variation and are capable of maintaining a stable existence in the presence of repulsive interactions.

关键词： Bose-Einstein condensate spin-orbit coupling rotation frequency stripe solitons vortex array

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Improved Proximal Policy Optimization Algorithm for Sequential Security-constrained Optimal Power Flow Based on Expert Knowledge and Safety Layer

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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 742-753页

作者： Yanbo Chen Qintao Du Honghai Liu Liangcheng Cheng muhammad Shahzad Younis State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources and School of Electrical&Electronic Engineering North China Electric Power UniversityBeijing 102206China School of Engineering Xining UniversityXining 810008Chinaand Key Laboratory of Smart Operation of New Energy Power SystemMinistry of EducationQinghai UniversityXining 810016China China Electric Power Research Institute Nanjing 210003China National University of Sciences and Technology Islamabad44000Pakistan

In recent years,reinforcement learning(RL)has emerged as a solution for model-free dynamic programming problem that cannot be effectively solved by traditional optimization *** has gradually been applied in the fields such as economic dispatch of power systems due to its strong selflearning and self-optimizing ***,existing economic scheduling methods based on RL ignore security risks that the agent may bring during exploration,which poses a risk of issuing instructions that threaten the safe operation of power ***,we propose an improved proximal policy optimization algorithm for sequential security-constrained optimal power flow(SCOPF)based on expert knowledge and safety layer to determine active power dispatch strategy,voltage optimization scheme of the units,and charging/discharging dispatch of energy storage *** expert experience is introduced to improve the ability to enforce constraints such as power balance in training process while guiding agent to effectively improve the utilization rate of renewable ***,to avoid line overload,we add a safety layer at the end of the policy network by introducing transmission constraints to avoid dangerous actions and tackle sequential SCOPF *** results on an improved IEEE 118-bus system verify the effectiveness of the proposed algorithm.

关键词： Sequential security-constrained optimal power flow(SCOPF) expert experience safety layer renewable energy safe reinforcement learning

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Aberrant adult neurogenesis in intractable epilepsy:can GABAergic progenitor transplantation normalize this process?

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Neural Regeneration Research 2024年第7期19卷 1419-1420页

作者： muhammad N.Arshad Janice R.Naegele Department of Biology Wesleyan UniversityMiddletownCTUSA Department of Neuroscience Tufts University School of MedicineBostonMAUSA

Temporal lobe epilepsy(TLE) is a common type of focal epilepsy characterized by seizure foci within the temporal *** surgical resection of the foci is an established and effective approach for controlling seizures,both temporal lobes cannot be removed,due to their prominent roles in learning and ***,seizures induce changes to the temporal lobes that contribute to hyperexcitability,including mossy fiber sprouting,astrogliosis.

关键词： epilepsy progenitor seizures

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A Survey of Edge Caching:Key Issues and Challenges

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Tsinghua Science and Technology 2024年第3期29卷 818-842页

作者： Hanwen Li Mingtao Sun Fan Xia Xiaolong Xu muhammad Bilal School of Computer Science Nanjing University of Information Science and TechnologyNanjing 210044China Shandong Provincial University Laboratory for Protected Horticulture Weifang University of Science and TechnologyWeifang 262700China Reading Academy Nanjing University of Information Science and TechnologyNanjing 210044China School of Software Nanjing University of Information Science and TechnologyNanjing 210044China Department of Computer Engineering Hankuk University of Foreign StudiesYongin-si 17035Republic of Korea

With the rapid development of mobile communication technology and intelligent applications,the quantity of mobile devices and data traffic in networks have been growing exponentially,which poses a great burden to networks and brings huge challenge to servicing user *** caching,which utilizes the storage and computation resources of the edge to bring resources closer to end users,is a promising way to relieve network burden and enhance user *** this paper,we aim to survey the edge caching techniques from a comprehensive and systematic *** first present an overview of edge caching,summarizing the three key issues regarding edge caching,i.e.,where,what,and how to cache,and then introducing several significant caching *** then carry out a detailed and in-depth elaboration on these three issues,which correspond to caching locations,caching objects,and caching strategies,*** particular,we innovate on the issue“what to cache”,interpreting it as the classification of the“caching objects”,which can be further classified into content cache,data cache,and service ***,we discuss several open issues and challenges of edge caching to inspire future investigations in this research area.

关键词： edge caching edge computing caching location caching object caching strategy 5G networkarchitecture Internet of Things(IoT)

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Development of anti-corrosive coating on AZ31 Mg alloy modified by MOF/LDH/PEO hybrids

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Journal of Magnesium and Alloys 2024年第2期12卷 586-607页

作者： muhammad Ali Khan Ananda Repycha Safira Mohammad Aadil Mosab Kaseem Corrosion and Electrochemistry Laboratory Department of Nanotechnology and Advanced Materials EngineeringSejong UniversitySeoul 05006Republic of Korea

The self-assembly of hybrid inorganic-organic materials on stationary platforms plays a critical role in improving their structural stability and wide *** this work,a novel two-step hydrothermal approach is proposed for synthesizing stable and advanced hybrid coatings on metal-oxide platforms through the surface modification of layered double hydroxide(LDH)films using novel metal-organic frameworks(MOFs).Initially,Mg-Al LDH nanocontainers,grown on a magnesium oxide layer produced through plasma electrolytic oxidation(PEO)of AZ31 Mg alloy substrate,were intercalated with cobalt via an oxidation route,providing the metallic coordination center for the MOF *** the subsequent step,a pioneering technique is introduced,utilizing tryptophan as the organic linker for the first time at a pH of *** self-assembly of cobalt-tryptophan complex,driven by the strong bonding between electrophilic sites of monomers and nucleophilic sites,facilitated the formation of a MOF network having a cloud-like structure on the surface of MgAl LDH's *** resulting MOF-LDH encapsulation containers demonstrate exceptional electrochemical stability when exposed to a 3.5 wt.%NaCl solution,surpassing the performance of PEO and pure LDH *** enhanced stability is attributed to the development of a dense top layer and a stable composition within the self-assembled MOF,effectively sealing flaws and preventing the infiltration of corrosive ions into the underlying metallic *** formation mechanism of MOFs on LDH galleries is investigated using density functional theory calculations.

关键词： Mg alloy Layered double hydroxide Metal-organic frameworks Corrosion DFT

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Comparative analysis of SIMILAR to RCD ONE(SRO)family from tetraploid cotton species and their diploid progenitors depict their significance in cotton growth and development

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Journal of Cotton Research 2024年第1期7卷 45-57页

作者： SHABAN muhammad TABASSUM Riaz RANA Iqrar Ahmad ATIF Rana muhammad AZMAT muhammad Abubakkar IQBAL Zubair MAJEED Sajid AZHAR muhammad Tehseen Department of Plant Breeding and Genetics University of Agriculture FaisalabadSub-Campus BurewalaVehari 61010Pakistan Department of Chemistry and Biochemistry University of AgricultureFaisalabad 38400Pakistan Centre of Agricultural Biochemistry and Biotechnology University of AgricultureFaisalabad 38400Pakistan Department of Plant Breeding and Genetics University of AgricultureFaisalabad 38400Pakistan Precision Agriculture and Analytics Lab National Centre in Big Data and Cloud ComputingCentre for Advanced Studies in Agriculture and Food SecurityUniversity of Agriculture FaisalabadFaisalabad 38400Pakistan Department of Plant Pathology University of CaliforniaDavisCA 95616USA State Key Laboratory of Cotton Biology Institute of Cotton ResearchChinese Academy of Agricultural SciencesAnyangHenan 455000China Federal Seed Certification and Registration Department Ministry of National Food Security and ResearchIslamabad 44090Pakistan School of Agriculture Sciences Zhengzhou UniversityZhengzhou 450000China

Background SRO(Similar to RCD1)genes family is largely recognized for their importance in the growth,develop-ment,and in responding to environmental ***,genome-wide identification and functional characteri-zation of SRO genes from cotton species have not been reported so *** A total of 36 SRO genes were identified from four cotton *** analysis divided these genes into three groups with distinct *** and chromosomal distribution analysis indicated uneven distribu-tion of GaSRO,GrSRO,GhSRO,and GbSRO genes on A2,D5 genomes,Gh-At,Gh-Dt,Gb-At,and Gb-Dt subgenomes,*** duplication analysis revealed the presence of six duplicated gene pairs among GhSRO *** promoter analysis,several elements responsive to the growth,development and hormones were found in GhSRO genes,implying gene induction during cotton growth and *** miRNAs responsive to plant growth and abiotic stress were predicted to target 12 GhSRO ***-specific expression profiling demonstrated the roles of GhSRO genes in one or more *** addition,specific expression pattern of some GhSRO genes dur-ing ovule development depicted their involvement in these developmental *** The data presented in this report laid a foundation for understanding the classification and functions of SRO genes in cotton.

关键词： Cotton SRO miRNAs Gene duplications Gene expression Ovule development

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Experimental Study on Heat Storage Properties Comparison of Paraffin/Metal Foams Phase Change Material Composites

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Journal of Thermal Science 2024年第2期33卷 469-478页

作者： Waqar AHMED Abid HUSSAIN Hanzla SHAHID Imran ALI Hafiz muhammad ALI Department of Mechanical Engineering University of Engineering and TechnologyTaxila47080Pakistan Department of Mechanical Engineering Institute of Space TechnologyIslamabadPakistan Department of Mechanical Mechatronics and Manufacturing EngineeringUniversity of Engineering and Technology LahoreFaisalabad CampusPunjabPakistan Mechanical Engineering Department King Fahd University of Petroleum and MineralsDhahran31261Saudi Arabia Interdisciplinary Research Center for Renewable Energy and Power Systems(IRC-REPS) King Fahd University of Petroleum and MineralsDhahran31261Saudi Arabia

Heat storage properties of phase change materials(PCMs) are essential characteristics that perform a key role in thermal heat energy storage *** thermal properties of PCMs can be improved by developing metal foam/PCM *** addition of metal foam in PCMs has a significant effect on the thermal characteristics of *** this paper,the heat storage properties of two different metal foam/PCM composites were experimentally *** behavior of paraffin in metal foam(copper and iron-nickel)/paraffin composites concerning pure paraffin at a constant heat flux of 1000 W/m^(2) in three directions simultaneously(x,y,and z) was *** was infiltrated into copper and iron-nickel foams to develop composite materials which resulted in enhancing the thermal conductivity of the paraffin.A comparative analysis is made on the heat storage properties of paraffin in copper and iron-nickel foams/paraffin *** temperature distribution during the phase transition process is experimentally *** comparison indicates that temperature uniformity in copper foam/paraffin composite is better than in iron-nickel foam/paraffin composite and pure paraffin at the same heat *** results show that at heat flux of 1000 W/m^(2),the heat storage time for copper foam/paraffin composite is 20.63% of that of iron-nickel foam/paraffin composite.

关键词： heat storage capacity paraffin/metal foam composite temperature uniformity heat storage rate phase transition process

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