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Research progress in synthesis and catalysis of polyoxometalates

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Progress in Natural Science:Materials International 2005年第5期15卷 385-394页

作者： GONG Yun1, HU Changwen1* and LIANG Hong2.1. Department of Chemistry, School of Science, the institute for Chemical physics,{2. institute of Technology,{2. 100081, china 2. Chemical Industry Press,{2. 10002., china) Sch. of Sci Inst. for Chem. Phys. Beijing Inst. of Technol. Beijing 100081 China Chem. Indust. Press Beijing 100029 China

Recent progress in the synthetic chemistry and catalysis of polyoxometalates (POMs) is reviewed. The novel POMs and their derivatives emerging in nearly three years (2.02.2.04) are introduced, including POMs with novel structure, POMs-organic hybrid compounds and host-guest complexes. Our review is focused on the elaboration of POMs' supramolecular chemistry.

关键词： polyoxometalates hybrid host-guest structure supramolecule catalysis.

Persistent anomalous flows over the subtropical western Pacific insummer

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Chinese Science Bulletin 1998年第8期43卷 672-675页

作者： ZHUANG Shiyu\+1 and JI Liren\+2.1. National Meteorological Centre, china Meteorological Administration, beijing 100081, china 2. LASG, institute of Atmospheric physics, Chinese Academy of Sciences, beijing 100080, china National Meteorological Ccntre China Meteomlcgical Administration Beijing China LASG Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China

The distribution of global persistent anomalies shows that the subtropical western Pacific is a key region with high_frequency occurrence of persistent anomalies. Analyses of streamfunction anomalies, OLR anomalies etc. suggest that the convective heating related to Indian monsoon might be responsible for the development of WPA. The results of numerical experiment by two linear barotropic models support the observation.

关键词： persistent anomalies subtropical high Indian monsoon anomalous forcing.

Pattern phenomena in an rf discharge dusty plasma system

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Science china(physics,Mechanics & Astronomy) 2006年第5期49卷 588-596页

作者： HUANG Feng1,2. YE Maofu2.& WANG Long2.1. College of Science, china Agricultural University, beijing 100083, china 2. institute of physics, Chinese Academy of Sciences, beijing 100080, china College of Science China Agricultural University Beijing China institute of physics Chinese Academy of Sciences Beijing China

Various dust patterns are observed in an rf discharge dusty plasma system. According to the dust growth process from small to large in size, the formation of different dust patterns can be divided into two stages: the small-particle stage (or dust cloud stage), and the large-particle stage (or dust crystal stage). The evolution relations between different dust patterns with gas pressure changing are investigated. Dust voids, dust acoustic waves and strong turbulence modes are presented at the small-particle stage. The self-organized dust lattices and dust clusters are investigated at the large-particle stage. The static structure of a dust lattice is characterized by means of the pair correlation function. Dust clusters formed by particles with different numbers and the regular evolution of the clusters with gas pressure are also investigated. The packing sequences of dust clusters are verified through two-dimensional confined molecular dynamics simulations.

关键词： dusty plasma dust patterns

Compression behavior of Zr_(41)Ti_(14)Cu_(12.5)Ni_(10)Be_(2..5) bulk metallic glass up to 2. GPa

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Science china(physics,Mechanics & Astronomy) 2005年第3期48卷 319-324页

作者： LI Gong 1, 2., ZHAN Zaiji 2., LIU Jing 3 , YUN Jinku 1 , SUN Liling 2., LIU Riping 1 , ZHANG Jun 2.& WANG Wenkui 1, 2.1. Key Laboratory of Metastable Materials Science and Technology, Yanshan University, qinhuangdao 066004, china 2. Center for Condensed Matter physics,{2. of physics, Chinese Academy of Sciences, beijing 100080, china 3. BSRF,{2. of High Energy physics, Chinese Academy of Sciences, beijing 100039, china Key Laboratory of Metastable Materials Science and Technology Yanshan University Qinhuangdao China Center for Condensed Matter physics Institute of Physics Chinese Academy of Sciences Beijing China BSRF Institute of High Energy Physics Chinese Academy of Sciences Beijing China

The compression of a Zr41Ti14Cu12.5Ni10Be2..5 bulk metallic glass (BMG) is investigated at room temperature up to 2. GPa using in-situ high pressure energy dispersive X-ray diffraction with a synchrotron radiation source. The pressure-induced structural relaxation is exhibited. It is found that below about 8 GPa, the existence of excess free volume contributes to the rapid structural relaxation, which gives rise to the rapid volumetric change, and the structural relaxation results in the structural stiffness under higher pressure.

关键词： bulk metallic glass, high pressure, structural relaxation, synchrotron radiation.

Mathematical stencil and its application in finite difference approximation to the Poisson equation

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Science china Mathematics 2005年第10期48卷 1421-1429页

作者： FENG Hui~1 ZHANG Baolin~(1,2. & LIU Yang~1 1. Department of Mathematics,Wuhan University,Wuhan 430072.china 2. Laboratory of Computational physics,{2. of Applied physics and Computational Mathematics,beijing 100088. china Department of Mathematics Wuhan University Wuhan China Laboratory of Computational physics Institute of Applied Physics and Computational Mathematics Beijing China

The concept of mathematical stencil and the strategy of stencil elimination for solving the finite difference equation is presented, and then a new type of the iteration algorithm is established for the Poisson equation. The new algorithm has not only the obvious property of parallelism, but also faster convergence rate than that of the classical Jacobi iteration. Numerical experiments show that the time for the new algorithm is less than that of Jacobi and Gauss-Seidel methods to obtain the same precision, and the computational velocity increases obviously when the new iterative method, instead of Jacobi method, is applied to polish operation in multi-grid method, furthermore, the polynomial acceleration method is still applicable to the new iterative method.

关键词： mathematical stencil, stencil elimination, Poisson equation, finite difference, iterative algorithm,parallelism.

The geometrical structure, electronic structure and magnetism of bimetallic Au_nM_2.(n=1, 2. M=Y, Zr, Nb, Mo, Tc, Ru, Rh, Pd) clusters

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Science china(physics,Mechanics & Astronomy) 2009年第7期52卷 1011-1020页

作者： GU Juan1,2. WANG ShanYing2.& GOU BingCong1 1 Department of physics, beijing{2. of Technology, beijing 100081, china 2.Department of physics, Tsinghua University, beijing 100084, china Department of physics Beijing Institute of Technology Beijing China Department of physics Tsinghua University Beijing China

The geometrical structure, stability, magnetism, and electronic structure of bimetallic clusters AuM2.and Au2.2. where M are 4d transition metal elements, are investigated systematically by using the first-principles method based on density functional theory. The calculation results show that there is a large amount of low-energy isomers with the very similar structure. AuM2.and Au2.2.clusters display dramatic magnetism. The magnetic moment of the 4d element is either enhanced or weakened with respect to the bulk value, which is largely dependent on the orbital exchange-splitting.

关键词： density functional theory first-principles cluster electronic structure magnetism

Research progress in the inner surface modification of metal tubes by plasma processing

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Progress in Natural Science:Materials International 2006年第11期16卷 1119-1126页

作者： ZHANG Guling~ 1,2.**, WU Xingfang~1, GU Weichao~2. CHEN Guangliang~2. FENG Wenran~2. NIU Erwu~2. LI Li~2. L Guohua~2. CHEN Huan~2. FAN Songhua~2. LIU Chizi~2.and YANG Size~2.1. School of Material Science and Engineering, University of Science and Technology beijing, beijing 100083,{2. 2. beijing National Laboratory for Condensed Matter physics, institute of physics, Chinese Academy of Sciences, beijing 100080,{2.) School of Material Science and Engineering University of Science and Technology Beijing Beijing 100083 China beijing National Laboratory for Condensed Matter physics Institute of Physics Chinese Academy of Sciences Beijing 100080 China

The recent progress in inner surface hardening of tubes by plasma processing is summerized. Several techniques of inner surface plasma source ion implantation and deposition are introduced, and their advantages and disadvantages are discussed. The basic principles, technical features and new progress of inner surface plasma source ion implantation methods for metal tubes, which were developed in our laboratory, are described in detail. And perspectives of the future technical development for inner surface ion implantation of tubes are presented.

关键词： PSII metal tubes inner surface surface modification.

The lepton flavor violating signal of the extra gauge boson Z′in photon-photon collision at the ILC

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Science china(physics,Mechanics & Astronomy) 2010年第11期53卷 1992-1997页

作者： LIU GuoLi 1,2.1 physics Department,Zhengzhou University,Zhengzhou 450001,china 2.Kavli{2. for Theoretical physics china,Chinese Academy of Sciences,beijing 100190,china physics Department Zhengzhou University Zhengzhou China Kavli institute for Theoretical physics{2. Chinese Academy of Sciences Beijing China

The hitherto unconstrained lepton flavor mixings,induced by the new gauge boson Z ,which are the prediction of many new physics models,such as topcolor-assisted technicolor (TC2. models and flavor-universal TC2.models,may lead to the lepton flavor violating productions of τμˉ,τeˉ and μeˉ in photon-photon collision at the proposed International Linear Collider (ILC).Through a comparative analysis of these processes,we find that the better channel to probe the new physics models is the production of τμˉ or τeˉ which occurs at a much higher rate than μeˉ production due to the large mixing angle and the large flavor changing coupling,and may reach the detectable level of the ILC for a large part of the parameter *** the rates predicted by the Standard Model are far below the detectable level,these processes may serve as a sensitive probe for such new physics models.

关键词： new gauge boson Z lepton flavor violating processes photon-photon

β-delayed proton decays near the proton drip line

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Science china(physics,Mechanics & Astronomy) 2005年第3期48卷 257-267页

作者： XU Shuwei 1 , LI Zhankui 1 , XIE Yuanxiang 1 , HUANG Wenxue 1 , SHU Nengchuan 2., CHEN Yongshou 2., XU Furong 3 , WANG Kun 4 , PAN qiangyan 1 , WANG Xudong 1 , YU Yong 1 & XING Yebing 1 1. institute of Modern physics, Chinese Academy of Sciences, Lanzhou 730000,{2. 2. Nuclear physics Department,{2. institute of Atomic Energy, beijing 102.13,{2. 3. Department of Technical physics, Peking University, beijing 100871,{2. 4. Shanghai institute for Nuclear Research, Shanghai 2.1800,{2. institute of Modern physics Chinese Academy of Sciences Lanzhou China Nuclear physics Department China Institute of Atomic Energy Beijing China Department of Technical physics Peking University Beijing China Shanghai institute for Nuclear Research Shanghai China

We briefly reviewed the experimental study on a-delayed proton decays near the proton drip line published by our group during the period of 1996―2.04, namely the first observation of the a-delayed proton decays of 9 new nuclides in the rare-earth region and the new measurements of a-delayed proton decays of 5 nuclides in the mass ～90 region near the N = Z line with the aid of the “p-?” coincidence in combination with a He-jet tape transport system. In the meantime some important experimental technique details were supplemented. The experimental results, including the half -lives, spins, parities, deformations and production reaction cross sections for the 14 nuclei were summarized and compared with the current nuclear-model predictions, and then the following points were represented. (1) The experimental half-lives for 85Mo and 92.h as well as the predicted “waiting point” nuclei 89Ru and 93Pd are 5―10 times longer than the theoretical predictions given by M?ller et al. using a macroscopic-microscopic model. It considerably influences the predictions of the abundances of the nuclides produced in the rp-process. (2. The current-model predictions are not consistent with the experimental assignments of the spins and parities for the proton drip-line nuclei 142.o and 12.Pm. However, the nuclear potential energy surface (PES) calculated by using a Woods- Saxon-Strutinsky method reproduced the experimental results. (3) The Alice code overestimated the production reaction cross sections of the studied 9 rare-earth nuclei by one order of magnitude or two, while HIVAP code overestimated them by one order of magnitude approximately.

关键词： proton drip line, β-delayed proton decay, He-jet tape transport system, "p-γ" coincidence, spin, parity, deformation, production reaction cross section.