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Engineering hierarchical quaternary superstructure of an integrated MOF-derived electrode for boosting urea electrooxidation assisted water electrolysis

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Green Energy & Environment 2024年第4期9卷 695-701页

作者： Jianjun Tian Changsheng Cao Yingchun He Muhammad imran khan Xin-Tao Wu Qi-Long Zhu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences(CAS)Fuzhou350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China University of Chinese Academy of Sciences Beijing100049China Research Institute of Sciences and Engineering(RISE) University of SharjahSharjah27272United Arab Emirates

Controllable design of the catalytic electrodes with hierarchical superstructures is expected to improve their electrochemical ***,a self-supported integrated electrode(NiCo-ZLDH/NF)with a unique hierarchical quaternary superstructure was fabricated through a self-sacrificing template strategy from the metal–organic framework(Co-ZIF-67)nanoplate arrays,which features an intriguing well-defined hierarchy when taking the unit cells of the NiCo-based layered double hydroxide(NiCo-LDH)as the primary structure,the ultrathin LDH nanoneedles as the secondary structure,the mesoscale hollow plates of the LDH nanoneedle arrays as the tertiary structure,and the macroscale three-dimensional frames of the plate arrays as the quaternary ***,the distinctive structure of NiCo-ZLDH/NF can not only accelerate both mass and charge transfer,but also expose plentiful accessible active sites with high intrinsic activity,endowing it with an excellent electrochemical performance for urea oxidation reaction(UOR).Specially,it only required the low potentials of 1.335,1.368 and 1.388 V to deliver the current densities of 10,100 and 200 mA cm^(-2),respectively,much superior to those for typical *** NiCo-ZLDH/NF as the bifunctional electrode for both anodic UOR and cathodic HER,an energy-saving electrolysis system was further explored which can greatly reduce the needed voltage of 213 mV to deliver the current density of 100 mA cm^(-2),as compared to the conventional water electrolysis system composed of *** work manifests that it is prospective to explore the hierarchically nanostructured electrodes and the innovative electrolytic technologies for high-efficiency electrocatalysis.

关键词： Hierarchical superstructures Metal–organic frameworks Layered double hydroxides Urea oxidation reaction Hydrogen evolution reaction

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The Impact of Hydrogen Energy Storage on the Electricity Harvesting

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Intelligent Automation & Soft Computing 2023年第5期36卷 1963-1978页

作者： Ghassan Mousa Ayman A.Aly imran khan DagØivind Madsen Department of Mechanical Engineering Faculty of EngineeringK.C.KARE Energy Research and Innovation CentreKing Abdulaziz UniversityJeddah21589Saudi Arabia Department of Mechanical Engineering College of EngineeringTaif UniversityP.O.Box 11099Taif21944Saudi Arabia Department of Electrical Engineering University of Engineering&Technology PeshawarPakistan University of South-Eastern Norway Bredalsveien 143511 HønefossNorway

The economics,infrastructure,transportation,and level of living of a country are all inﬂuenced by *** gap between energy usage and availabil-ity is a global ***,all countries rely on fossil fuels for energy genera-tion,and these fossil fuels are not *** hydrogen proton exchange membrane fuel cell(PEMFC)power system is both clean and efﬁ*** fuel delivery system and the PEMFC make up the majority of the PEMFC power *** lack of an efﬁcient,safe,and cost-effective hydrogen storage system is still a major barrier to its widespread *** hydrogen storage has the large capacity,safety and good *** a hydrogen source system,the hydro-gen supply characteristics affect the characteristics of the PEMFC at the *** this paper,a mathematical model of a hydrogen source reactor and PEMFC based on chemical absorption/desorption of solid hydrogen storage is established,and a simulation model of a PEMFC power system coupled with solid hydrogen storage is established using MATLAB/SIMULINK software,and the hydrogen supply of the reactor is analyzed in *** inﬂuence of prominent factors is *** research results show that the proposed method improved the system *** the same time,increasing the PEMFC temperature,increasing the area of the proton exchange membrane and the oxygen supply pressure can increase the output power of the power system.

关键词： Hydrogen energy fuel cell power system optimization electrical energy harvesting

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Evaluation of antileishmanial,antibacterial and brine shrimp cytotoxic potential of crude methanolic extract of Herb Ocimum basilicum(Lamiacea)

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Journal of Traditional Chinese Medicine 2015年第3期35卷 316-322页

作者： imran khan Kafeel Ahmad Ali Talha Khalil Jangrez khan Yusra Ali khan Muhammad Shahab Saqib Muhammad Naveed Umar Hilal Ahmad Department of Biotechnology Quaid-i-Azam University Centre of Biotechnology and Microbiology University of Peshawar Department of Biochemistry Quaid-i-Azam University Islamabad Department of Chemistry University of Malakand Institute of Biotechnology and Genetic Engineering Agriculture UniversityPeshawar

OBJECTIVE:To collect and screen for ethnopharmacological properties(antileishmanial,antibacterial and brine lethality assays) of medicinal plant Ocimum basilicum from Peshawar region(34.008 latitude and 71.57 altitudes).METHODS:In the present study a general antileishmanial activity against Leishmania tropica strain was carried *** antibacterial potential of the plant was performed against 06 gram positive and 06 gram negative *** shrimp cytotoxicity assay at different concentrations were ***:The anti-promastigotes profile of the plant showed good antileishmanial activity exhibited LC_(50) value 21.67 μg/*** result for gram positive antibacterial activity revealed that the *** leaves extract possesses significant inhibitory activity at highest two concentrations ranging from20.66 ± 0.31 to 31.86 ± 0.80 for Clostridium perfringens type C and Bacillus subtitilis,respectively,as compared to the gentamycin(27.36 ± 0.55 and21.80 ± 0.72,respectively).For gram negative bacteria good activity was observed.A highest zone of inhibition was recorded for Pseudomonas aeroginosa(28.83 ± 0.28) atthe highest concentration(10 mg/mL).The LC_(50) value obtained for brine shrimp lethality assay was 91.56 μg/***:The herb basil possesses effective cidal activities which make this plant a good candidate for the isolation of antiprotozoal and antibacterial compounds which may lead to the development of novel drug.

关键词： Ocimum basilicum Cytotoxicity tests,immunologic Anti-bacterial agents Antileishmanial activity

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Fabrication of magnetically recyclable yolk-shell Fe_(3)O_(4)@TiO_(2) nanosheet/Ag/g-C_(3)N_(4) microspheres for enhanced photocatalytic degradation of organic pollutants

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Nano Research 2021年第7期14卷 2363-2371页

作者： Yan Lv Lin Yue imran Mahmood khan You Zhou Wenbo Cao Sobia Niazi Zhouping Wang State Key Laboratory of Food Science and Technology Jiangnan UniversityWuxi 214122China School of Food Science and Technology Jiangnan UniversityWuxi 214122China International Joint Laboratory on Food Safety Jiangnan UniversityWuxi 214122China Collaborative Innovation Center of Food Safety and Quality Control of Jiangsu Province Jiangnan UniversityWuxi 214122China School of Food Science and Technology National Engineering Research Center of SeafoodDalian Polytechnic UniversityDalian 116024China

Herein,we report the fabrication of Fe_(3)O_(4)@TiO_(2) nanosheet/Ag/g-C_(3)N_(4)(Fe_(3)O_(4)@ns-TiO_(2)/Ag/g-C_(3)N_(4))composite photocatalysts with well-designed hierarchical yolk-shell *** endow the composites with fascinating features,multiple functional components are perfectly integrated into the definite *** photodegradation experiments of organic pollutants revealed a significant enhancement in photocatalytic activity of developed composites as compared to P25,which is mainly due to the synergetic interaction of the tailored three-dimensional(3D)yolk-shell porous nanostructure,extended sunlight response range,and retarded the recombination probability of photogenerated *** importantly,the hybrid samples exhibited superior magnetic properties due to the magnetic *** excellent magnetic recyclability and reusability of the photocatalysts are verified by the magnetic hysteresis loop and cyclic photocatalytic degradation experiments,which is significant for the green and sustainable applications of *** its remarkable photocatalytic performance and expectant magnetic recyclability,the composite photocatalysts are expected to be a promising candidate to dispose of future environmental issues.

关键词： TiO_(2)nanosheet Ag nanoparticles g-C_(3)N_(4) hierarchical yolk-shell structure photocatalysis magnetic separation

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Resource Allocation and Optimization in Device-to-Device Communication 5G Networks

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Computers, Materials & Continua 2021年第10期69卷 1201-1214页

作者： Fahad Ahmed Al-Zahrani imran khan Mahdi Zareei Asim Zeb Abdul Waheed Computer Engineering Department Umm Al-Qura UniversityMecca24381Saudi Arabia Department of Electrical Engineering University of Engineering and Technology PeshawarP.O.B.814Pakistan Tecnologico de Monterrey School of Engineering and SciencesZapopan45201Mexico Department of Computer Science Abbottabad University of Science and TechnologyHavelian22500Pakistan Department of Information Technology Hazara University MansehraMansehra21120Pakistan School of Electrical and Computer Engineering Seoul National UniversitySeoul08826Korea

The next-generation wireless networks are expected to provide higher capacity,system throughput with improved energy *** of the key technologies,to meet the demand for high-rate transmission,is deviceto-device(D2D)communication which allows users who are close to communicating directly instead of transiting through base stations,and D2D communication users to share the cellular user chain under the control of the cellular *** a new generation of cellular network technology,D2D communication technology has the advantages of improving spectrum resource utilization and improving system throughput and has become one of the key technologies that have been widely concerned in the ***,due to the sharing of cellular network resources,D2D communication causes severe interference to existing cellular *** of the most important factors in D2D communication is the spectrum resources utilization and energy consumption which needs considerable attention from research *** address these issues,this paper proposes an efficient algorithm based on the idea of particle swarm *** main idea is to maximize the energy efficiency based on the overall link optimization of D2D user pairs by generating an allocation matrix of spectrum and *** D2D users are enabled to reuse multiple cellular user’s resources by enhancing their total energy efficiency based on the quality of service constraints and the modification of location and speed in particle *** constraint also provides feasibility to solve the original fractional programming *** results indicate that the proposed scheme effectively improved the energy efficiency and spectrum utilization as compared with other competing alternatives.

关键词： 5G networks D2D communication resource allocation

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Energy Cost Minimization Using String Matching Algorithm in Geo-Distributed Data Centers

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Computers, Materials & Continua 2023年第6期75卷 6305-6322页

作者： Muhammad imran khan Khalil Syed Adeel Ali Shah Izaz Ahmad khan Mohammad Hijji Muhammad Shiraz Qaisar Shaheen Department of Computer Science&Information Technology University of Engineering&TechnologyPeshawar25000Pakistan Department of Computer Science Bacha Khan UniversityCharsadda24541Pakistan Computer Science Department University of TabukTabuk47512Saudi Arabia Department of Computer Science Federal Urdu University of ArtsScience and Technology Islamabad44000Pakistan Department of Computer Science and Information Technology The Islamia University of BahawalpurRahim Yar Khan CampusPunjabPakistan

Data centers are being distributed worldwide by cloud service providers(CSPs)to save energy costs through efficient workload alloca-tion *** CSPs are challenged by the significant rise in user demands due to their extensive energy consumption during workload *** research studies have examined distinct operating cost mitigation techniques for geo-distributed data centers(DCs).However,oper-ating cost savings during workload processing,which also considers string-matching techniques in geo-distributed DCs,remains *** this research,we propose a novel string matching-based geographical load balanc-ing(SMGLB)technique to mitigate the operating cost of the geo-distributed *** primary goal of this study is to use a string-matching algorithm(i.e.,Boyer Moore)to compare the contents of incoming workloads to those of documents that have already been processed in a data center.A successful match prevents the global load balancer from sending the user’s request to a data center for processing and displaying the results of the previously processed workload to the user to save *** the contrary,if no match can be discovered,the global load balancer will allocate the incoming workload to a specific DC for processing considering variable energy prices,the number of active servers,on-site green energy,and traces of incoming *** results of numerical evaluations show that the SMGLB can minimize the operating expenses of the geo-distributed data centers more than the existing workload distribution techniques.

关键词： String matching optimization geo-distributed data centers geographical load balancing green energy

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Cointegration between macroeconomic factors and the exchange rate USD/CNY

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Financial Innovation 2019年第1期5卷 76-90页

作者： Muhammad Kamran khan Jian-Zhou Teng Muhammad imran khan School of Economics Northeast Normal UniversityChangchunJilinChina

This research paper investigates the effect of macroeconomic variables on the exchange rate USD/CYN using yearly time series data for China economy from 1980 to *** bounds test approach for cointegration is applied to test the long-run relation between the dependent and the independent *** results of long-run ARDL indicate that gross domestic product growth and trade openness have a positive effect on the exchange rate USD/CNY while interest and inflation rates have a negative effect on the exchange *** on the results of this study,it is recommended that the policymakers of the Chinese government should implement vital monetary and fiscal policies to determine the less volatile and productive exchange rate for China to manage sustainable economic growth for a long time with its trading partners.

关键词： Exchange rate Macroeconomic factors ARDL

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Litter decay in rangeland sites with varying history of human disturbance: a study with Hazargangi Chiltan mountain

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Journal of Mountain Science 2020年第4期17卷 898-906页

作者： imran khan Shamim GUL Sarfraz AHMAD Gul Bano REHMAN Agha Waqar YUNUS Iram GUL imran ALI Ali AKBAR Muhammad ISLAM Department of Botany University of BalochistanQuettaBalochistan87550Pakistan Department of Natural Resource Sciences Macdonald CampusMcGill University21111 Lakeshore RoadSte-Anne-deBellevueQuebec H9X 3V9Canada Natural Resources Division Pakistan Agricultural Research CouncilIslamabad44050Pakistan Animal Sciences Institute PARC National Agricultural Research CenterPark RoadIslamabad45500Pakistan Institute of Environmental Sciences and Engineering School of Civil and Environmental EngineeringNational University of Sciences and Technology(NUST)Islamabad 24090Pakistan Department of Biochemistry University of BalochistanQuetta 87550Pakistan School of Life Sciences and Engineering Southwest University of Science and TechnologyMianyang 621010China Department of Microbiology University of BalochistanQuetta 87550Pakistan International Center for Agricultural Research in Dry Areas(ICARDA) South AsiaIslamabad 44000Pakistan

Hazarganji Chiltan National Park in Balochistan, Pakistan was established in 1980 and the protected area was further extended in 1998. Large area of this mountain is still open for unmanaged human disturbances such as collection of wood for fuel purpose and livestock grazing. Removal of vegetation of rangelands has a significant negative impact on soil organic matter(SOM). This research evaluates litter decomposition in three sites of Hazarganji Chiltan mountain with varying history of human disturbances(unprotected site, young protected site and old protected site). Twigs of Pistacia khinjuk with approximately equal weight and length were placed in litter bags of mesh size 2 mm and were buried in 0-5 cm depth in three sites in January. Half of the twigs of each site received rain simulation in April, August, October, November and January while the other half of the twigs were subjected under natural conditions for 15 months. Twigs from each plot of each treatment of each site were collected from soil after every rain simulation in the previous month of experiment and were processed for weight loss assessment. Results showed that weight loss of twigs by decomposition was significantly higher in the soil of unprotected site as compared to other two sites and there was no difference between rain simulation and control treatments except that loss of weight of twigs of unprotected site was higher under control than rain simulation condition. To confirm that SOM was the major controlling factor for the decomposition of litter decay, soils of each site were collected and burned to remove SOM;thereafter, burned soil samples were mixed with homogenous powder of oven-dried native plants, incubated for 6 months and were provided with dissolved organic matter of the soils of each site. Results showed that there was no difference in the decomposition of litter between soils under controlled laboratory condition, which confirmed that SOM was a major controlling factor for the li

关键词： Hazarganji Chiltan National Park Litter decay Grazing Litter bag Rain simulation

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When LoRa meets distributed machine learning to optimize the network connectivity for green and intelligent transportation system

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Green Energy and Intelligent Transportation 2024年第3期3卷 24-41页

作者： Malak Abid Ali khan Hongbin Ma Arshad Farhad Asad Mujeeb imran khan Mirani Muhammad Hamza National Key Lab of Autonomous Intelligent Unmanned Systems School of AutomationBeijing Institute of TechnologyBeijing 100081China Department of Computer Science Namal UniversityPakistan Department of Electrical Engineering Tsinghua UniversityBeijing 100084China Faculty of Information Technology Beijing University of TechnologyBeijing 100124China School of Mechanical Engineering Beijing Institute of TechnologyBeijing 100081China

LoRa technology contributes to green energy by enabling efficient,long-range communication for the Internet of Things(IoT).This paper addresses the challenges related to coverage range in outdoor monitoring systems utilizing LoRa,where the network performance is affected by the density of gateways(GWs)and end devices(EDs),as well as environmental *** mitigate interference,data throughput losses,and high-power consumption,the proposed spreading factor(SF)and hybrid(data rate|SF)models dynamically adjust the transmission *** orchestration of concurrent data modifications within the network server(NS)is crucial for uninterrupted communication between GWs and EDs,especially in monitoring electric vehicle(EV)stations to reduce traffic congestion and *** K-means and density-based spatial clustering of applications with noise(DBSCAN)algorithms optimizes ED allocation,averts data congestion,and improves the signal-tointerference noise ratio(SINR).These methods ensure seamless information reception by meticulously allocated EDs across various GW *** estimate the free-space losses(FSL),a log-distance path loss model(log-PL)is *** various bandwidths(BWs),bidirectional communications,and duty cycles(DCs)helps to prevent saturation,thus prolonging the operational lifespan of *** findings reveal a notable packet rejection rate(PRR)of 0%for the DBSCAN(hybrid model).In contrast,the K-means exhibits a PRR ranging from 5%(hybrid model)to 35.29%(SF model)for the ten GWs ***,the network saturation is reduced to 10.185%and 9.503%,respectively,highlighting an improvement in the average efficiency of slotted ALOHA(91.1%)and pure ALOHA(90.7%).These enhancements increase the lifespan of EDs to 15,465.27 days.

关键词： DBSCAN Green transportation Hybrid model Intelligent transportation K-means

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Non-covalent interaction of atomically dispersed dual-site catalysts featuring Co and Ni nascent pair sites for efficient electrocatalytic overall water splitting

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Journal of Materials Science & Technology 2024年第11期178卷 210-225页

作者： imran khan Yaogang Chen Zhiyang Li Wenjie Liu Salman khan Sami Ullah Linlin Liu Amir Zada Sharafat Ali Shabana Shaheen Lei Yang State Key Laboratory of Urban Water Resource and Environment Shenzhen Key Laboratory of Organic Pollution Prevention and ControlSchool of Civil and Environmental EngineeringHarbin Institute of Technology ShenzhenShenzhen 518055China School of Physics and Electronics Central South UniversityChangsha 410083China CNAS Accredited Test Center Guangdong Engineering Technology Research Center of Air PurificationHealthlead Co.Ltd.Shenzhen 518055China Key laboratory of Functional Inorganic Material Chemistry Ministry of Education of the People's Republic of ChinaHeilongjiang UniversityHarbin 150080China K.A.CARE Energy Research&Innovation Center(ERIC) King Fahd University of Petroleum&Minerals(KFUPM)Dhahran 31261Saudi Arabia Department of Chemistry Abdul Wali Khan UniversityMardanKhyber Pakhtunkhwa 23200Pakistan School of Physics University of Electronic Science and Technology of ChinaChengdu 610054China

The scarcity of highly effective and economical catalysts is a major impediment to the widespread adop-tion of electrochemical water splitting for the generation of ***_(2),a low-cost candidate,suffers from inefficient catalytic ***,a captivating strategy has emerged,which involves the en-gineering of heteroatom doping to enhance electrochemical *** investigation demonstrates a successful implementation of the strategy by combining ultrathin MoS_(2) nanosheets with Co and Ni dual single multi-atoms(DSMAs)grown directly on 2D N-doped carbon nanosheets(CoNi-MoS_(2)/NCNs)for the purpose of improving hydrogen evolution reaction(HER)and oxygen evolution reaction(OER).With the aid of a dual-atom doped bifunctional electrocatalyst,effective water splitting has been achieved across a broad pH range in *** double doping of Co and Ni strengthens their interactions,thereby altering the electromagnetic composition of the host MoS_(2) and ultimately leading to improved electrocat-alytic ***,the synergistic effect between NCNs and MoS_(2) nanosheets provided efficient electron transport channels for ions and an ample surface area with open voids for ion ***-sequently,the CoNi-MoS_(2)/NCNs catalysts demonstrated exceptional stability and activity,producing low degree overpotentials of 180.5,124.9,and 196.4 mV for HER and 200,203,and 207 mV for OER in neu-tral,alkaline,and acidic mediums,respectively,while also exhibiting outstanding overall water-splitting performance,durability,and stability when used as an electrolyzer at universal pH.

关键词： Multifunctional catalyst Water splitting Functionalized carbon nanosheets Interface engineering pH-universal electrocatalysis

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