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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

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journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua jo jonggeol Na J.Jay Liu Young-Ju kim Wangyun Won Department of Chemical and Biological Engineering Korea University Department of Chemical Engineering (Integrated process) Kyung Hee University Department of Chemical Engineering and Materials Science Ewha Womans University Department of Chemical Engineering Pukyong National University Resources Engineering Plant Research Department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

Improved continuous precipitation kinetics and tensile properties of extruded AZ80 alloy through {10-12} twin formation

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journal of Magnesium and Alloys 2023年第9期11卷 3323-3337页

作者： hyun Ji kim Sumi jo Sung Hyuk Park Department of Materials Science and Metallurgical Engineering Kyungpook National UniversityDaegu 41566the Republic of Korea

This study investigates the effect of{10-12}deformation twins on the continuous precipitation behavior of an extruded Mg-8.0Al-0.5Zn-0.2Mn(AZ80)alloy during *** extruded AZ80 alloy is compressed along the transverse direction to introduce{10-12}twins,followed by an aging treatment at 300℃.The extruded material exhibits a twin-free microstructure with low internal strain energy,whereas the pre-twinned material possesses abundant{10-12}twins and has high internal strain *** aging results reveal that the peak-aging time of the pre-twinned material(1 h)is one-eighth of that of the extruded material(8 h).Although Mg_(17)Al_(12)continuous precipitates(CPs)are observed in both the peak-aged materials,these CPs are much smaller and more densely distributed in the pre-twinned material despite the significantly shorter aging *** CPs size in the peak-aged materials increases in the following order:twinned region in the pre-twinned material(0.47μm)

关键词： AZ80 alloy {10-12}twin Aging Continuous precipitation Tensile properties

Aging Behavior of Mg-Y-Zr and Mg-Nd-Zr Cast Alloys

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journal of Materials Science & Technology 2008年第1期24卷 80-84页

作者： Yang-Do kim Nam-hyun Kang Il-Guk jo Kyung-hyun kim In-Bae kim School of Materials Science and Engineering Pusan National University 30 Jangjun-dongGeumjeong-guBusan 609-735Korea Deptartment of Materials Engineering Korea Institute of Machinery & Materials 66 Sangnam-dongChangwonGyeongsangnam-do 641-010Korea

Aging behavior of Mg-3.6Y-0.5Zr and ***-0.5Zr alloys was investigated by microhardness measurement and transmission electron *** the case of Mg-Y-Zr alloy,the presence ofβ″phase,a major strength- ener,having base centered orthorhombic structure with its lattice constants of a-（β″）=0.64 nm,b-（β″）=2.22 nm, and c-（β″）=0.52 nm was *** the case of Mg-Nd-Zr alloy aged at 250℃,the presence ofβ″andβ′phases was *** crystal structure ofβ″phase was found to be DO-（19） and its orientation relationships with Mg matrix were [0001]-（β″）//[0001]-（Mg） and [01（？）0]-（β″）//[01（？）0]-（Mg）.Theβ′phase had face centered cubic structure and its orientation relationships with Mg matrix were [011]-（β′）//[0001]-（Mg） and [（？）1（？）]β′//[（？）110]）-（Mg）. The ***-0.5Zr alloy showed higher hardness compared with Mg-3.6Y-0.5Zr alloy.

关键词： Mg-Y-Zr alloy Mg-Nd-Zr alloy Precipitation sequence

Effect of pre-deformation on precipitation behavior of AZ80 alloy:Comparison of slip-and twinning-dominant deformation

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journal of Magnesium and Alloys 2024年第9期12卷 3616-3630页

作者： hyun Ji kim Sang Cheol Jin Sumi jo Sung Hyuk Park Department of Materials Science and Metallurgical Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Graduate School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea

This study investigates the effect of the deformation mode on the precipitation behavior of an extruded Mg-8.0Al-0.5Zn-0.2Mn(AZ80)*** alloy samples are compared after the application of 3.5%tension and 3.5%compression along the extrusion direction to induce slip-dominant and twinning-dominant deformation modes,*** pre-compressed(PC)sample,which contained numerous{10-12}tension twins,has a reduced grain size and a higher internal strain than the pre-tensioned(PT)sample,which is attributed to the inherent internal strain that occurs during the formation and growth of the *** a result,the precipitation behavior of the PC sample is accelerated,leading to its short peak aging time of 32 h,which is lower than those of the PT and as-extruded samples(48 and 100 h,respectively).Furthermore,fine continuous precipitates(CPs)rapidly form within the{10-12}twins,contributing to the enhanced *** precipitates(DPs),which have a hardness comparable to the CP-containing twinned regions,in the PC sample experience less coarsening during aging than those in the PT sample due to growth inhibition by the{10-12}***,the{10-12}twins generated under the twinning-dominant deformation condition lead to enhanced precipitation behaviors,including the preferential formation and refinement of CPs and the suppressed coarsening of ***,pre-deformation that occurs{10-12}twinning exhibits more pronounced effects on precipitation acceleration and microstructural modification than slip-inducing pre-deformation.

关键词： AZ80 alloy Slip Twinning Precipitation Hardness

Promoting dynamic recrystallization and improving strength and ductility of Mg-7Bi alloy through Al addition

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journal of Magnesium and Alloys 2024年第8期12卷 3339-3356页

作者： Gun Woong An Sang-Cheol Jin hyun Ji kim Sumi jo Sung Hyuk Park Department of Materials Science and Metallurgical Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Graduate School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea

This study investigated the influence of the addition of Al to a Mg-7Bi(B7,wt%)alloy,particularly its recrystallization behavior during extrusion and its resulting mechanical *** addition of 2 wt%Al to the B7 alloy resulted in a lower grain size,a reduction in the number density of fine Mg3Bi2 particles,and a higher area fraction of relatively coarse Mg3Bi2 particles in the extrusion *** microstructural changes increased the nucleation sites for recrystallization,reduced the Zener pinning effect,and enhanced particle-stimulated nucleation,all of which promoted dynamic recrystallization behavior during *** a result,the area fraction of recrystallized grains in the extruded alloy increased from 77%to 94%.The extruded B7 alloy exhibited a strongfiber texture,whereas the extruded Mg-7Bi-2Al(BA72)alloy had a weak-texture,which was attributed to the minimal presence of unrecrystallized grains and the dispersed orientation of the recrystallized *** tensile yield strength(TYS)of the extruded BA72 alloy was higher than that of the extruded B7 alloy(170 and 124 MPa,respectively),which resulted from the enhanced grain-boundary and solid-solution strengthening *** tensile elongation(EL)of the BA72 alloy also exceeded that of the B7 alloy(20.3%and 6.1%,respectively),the result of the uniform formation of fine twins under tension in the former and the formation of a few coarse twins among the unrecrystallized grains in the ***,the addition of a small amount of Al to the B7 alloy significantly improved both the strength and ductility of the extruded alloy,resulting in a remarkable increase in the product of the TYS and EL from 756 to 3451 MPa%and expanding its potential range of applications as a lightweight extruded structural component.

关键词： Mg-7Bi alloy Al addition Extrusion Recrystallization Microstructure

High-power and long-life supercapacitive performance of hierarchical, 3-D urchin-like W18049 nanostructure electrodes

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Nano Research 2016年第3期9卷 633-643页

作者： Sangbaek Park hyun-Woo Shim Chan Woo Lee Hee jo Song Jae-Chan kim Dong-Wan kim Department of Materials Science and Engineering Seoul National University Seoul 151-744 Republic of Korea School of Civil Environmental and Architectural Engineering Korea University Seou1136-713 Republic of Korea

We report the facile, one-pot synthesis of 3-D urchin-like W18O49 nanostructures （U-WO） via a simple solvothermal approach. An excellent supercapacitive performance was achieved by the U-WO because of its large Brunauer-Emmett- Teller （BET） specific surface area （ca. 123 m2.g-1） and unique morphological and structural features. The U-WO electrodes not only exhibit a high rate-capability with a specific capacitance （Csp） of -235 F·g-1 at a current density of 20 A.g-1, but also superior long-life performance for 1,000 cycles, and even up to 7,000 cycles, showing -176 F·g-1 at a high current density of 40 A.g-1.

关键词： hierarchical structure W18O49 high-power long cycle life supercapacitor

Inhibitory Mechanisms of Water Extract of Oplopanax elatus on Lipopolysaccharide-lnduced Inflammatory Responses in RAW 264.7 Murine Macrophage Cells

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Chinese journal of Integrative Medicine 2020年第9期26卷 670-676页

作者： Ki Sun Kwon hyun Lim Yong Soo Kwon Myong jo kim Ji Hye Yoo Nam Ho Yoo hyun Pyo kim College of Pharmacy Kangwon National UniversityChuncheon(24341)Republic of Korea Department of Bio-Resource Sciences Kangwon National UniversityChuncheon(24341)Republic of Korea Bioherb Research Institute Kangwon National UniversityChuncheon(24341)Republic of Korea

Objective:To study the anti-inflammatory action and cellular mechanism of Oplopanax ***:A hot water extract of OE(WOE)was prepared and a major constituent,syringin,was successfully *** content in WOE was found to be 214.0 p.g/g dried plant(w/w).Their anti-inflammatory activities were examined using RAW 264.7 macrophages and a mouse model of croton oil-induced ear ***:In lipopolysaccharide(LPS)-treated RAW 264.7 cells,a mouse macrophage cell line,WOE was found to significantly and strongly inhibit cyclooxygenase-2(COX-2)-induced prostaglandin E2(PGE2)production[half maximal inhibitory concentration(IC50)=135.2μg/mL]and inducible nitric oxide synthase(iNOS)-induced NO production(IC50=242.9μg/mL).In the same condition,WOE was revealed to inhibit NO production by downregulating iNOS expression,mainly by interrupting mitogen activated protein kinases(MAPKs)/activator protein-1(AP-1)*** activation of all three major MAPKs,p38 MAPK,extracellular signal-regulated kinase(ERK),and c-Jun N-terminal kinase,was inhibited by WOE(50-300μg/mL).On the other hand,WOE reduced PGE2 production by inhibiting COX-2 enzyme activity,but did not affect COX-2 expression *** addition,WOE inhibited the production of proinflammatory cytokines such as interleukin-6 and tumor necrosis factor-α.In croton oil-induced ear edema in mice,oral administration of WOE(50-300 mg/kg)dose-dependently inhibited edematic ***:Water extract of OE exhibited multiple anti-inflammatory action mechanisms and may have potential for treating inflammatory disorders.

关键词： Oplopanax elatus Chinese medicine stem syringin anti-inflammation RAW 264.7

A Note on the Universal Factorization Property of Groups

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Algebra Colloquium 2021年第4期28卷 635-644页

作者： Injo Hur Jang hyun jo Department of Mathematics Education Chonnam National University Gwangju 61186Korea Department of Mathematics Sogang UniversitySeoul 04107Korea

We give criteria when a full subcategory D of the category of groups has C-universal factorization property(C-UFP)or C-strong universal factorization property(C-SUFP)for a certain category of groups *** a byproduct,we give affirmative answers to three unsettled questions in[***,***,Universal factorization property of certain polycyclic groups,*** *** 204(2006)555-567].

关键词： hereditary productive universal factorization property

Role of transcription factor acetylation n the regulation of metabolic homeostasis

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Protein & Cell 2015年第11期6卷 804-813页

作者： joo-Man Park Seong-Ho jo Mi-Young kim Tae-hyun kim Yong-Ho Ahn Department of Biochemistry and Molecular Biology Yonsei University College of Medicine 50-1 Yonsei-ro Seodaemun-gu Seoul 120-752 Republic of Korea Brain Korea 21 PLUS Project for Medical Sciences Yonsei University College of Medicine 50-1 Yonsei-ro Seodaemun-gu Seoul 120-752 Republic of Korea

Post-translational modifications （PTMs） of transcription factors play a crucial role in regulating metabolic homeostasis. These modifications include phosphory- lation, methylation, acetylation, ubiqulUnation, SUMOy- lation, and O-GIcNAcylation. Recent studies have shed light on the importance of lysine acetylation at nonhis- tone proteins including transcription factors. Acetyla- tion of transcription factors affects subcellular distribution, DNA affinity, stability, transcriptional activity, and current investigations are aiming to further expand our understanding of the role of lysine acetyla- tion of transcription factors. In this review, we summarize recent studies that provide new insights into the role of protein lysine-acetylation in the transcriptional regulation of metabolic homeostasis.

关键词： metabolic homeostasis transcriptionfactor post-translational modification type 2 diabetesmellitus