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Rapid crystallization-driven high-efficiency phase-pure deep-blue Ruddlesden–Popper perovskite light-emitting diodes

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Advanced Photonics 2023年第1期5卷 8-18页

作者： Gyumin Jang hyowon han Sunihl Ma Junwoo Lee Chan Uk Lee Wooyong Jeong Jaehyun Son Dongki Cho Ji-Hee Kim Cheolmin Park Jooho Moon Yonsei University Department of Materials Science and EngineeringSeoulRepublic of Korea Sungkyunkwan University Department of Energy ScienceSuwonRepublic of Korea Institute for Basic Science Center for Integrated Nanostructure PhysicsSuwonRepublic of Korea

Perovskite light-emitting diodes(PeLEDs)are considered as promising candidates for nextgeneration solution-processed full-color ***,the external quantum efficiencies(EQEs)and operational stabilities of deep-blue(3 is hampered completely,so that phase-pure 2D-RPP films with bandgaps suitable for deep-blue PeLEDs can be obtained *** uniquely developed rapid crystallization method also enables formation of randomly oriented 2D-RPP crystals,thereby improving the transfer and transport kinetics of the charge ***,high-performance deep-blue PeLEDs emitting at 437 nm with a peak EQE of 0.63%are successfully *** color coordinates are confirmed to be(0.165,0.044),which match well with the Rec.2020 standard blue gamut and have excellent spectral stability.

关键词： Ruddlesden–Popper perovskite rapid crystallization deep-blue light-emitting diodes phase purity randomly oriented crystals

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Zwitterion-assisted transition metal dichalcogenide nanosheets for scalable and biocompatible inkjet printing

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Nano Research 2020年第10期13卷 2726-2734页

作者： Hyeokjung Lee Min Koo Chanho Park Madhumita Patel hyowon han Tae Hyun Park Pawan Kumar Won-Gun Koh Cheolmin Park Department of Materials Science and Engineering Yonsei University Seoul 03722Republic of Korea Department of Chemical and Biomolecular Engineering Yonsei UniversitySeoul 03722Republic of Korea

Inkjet printing of two-dimensional(2D)transition metal dichalcogenide(TMD)nanosheets fabricated by liquid-phase exfoliation(LPE)allows simple,mass-producible,and low-cost photo-electronic *** LPE processes involve toxic and environmentally hazardous solvents;however,dispersants have restricted the extent of applications of 2D-TMD ***,various 2D-TMD nanosheets,including MoS2,MoSe2,WS2,and WSe2,in addition to few-layered graphene,are inkjet-printed using a LPE process based on zwitterionic dispersants in *** with cationic and anionic species are water-soluble,while alkyl chain moieties associated with two ionic species adhere universally on the surface of TMD nanosheets,resulting in high throughput liquid exfoliation of the *** zwitterion-assisted TMD nanosheets in water are successtully employed as an ink without the need for additives to adjust the viscosity and surface tension of the ink for use in an office inkjet printer;this gives rise to A4 scale,large-area inkjet-printed images on diverse substrates,such as metals,oxides,and polymer substrates patchable onto human *** with conductive graphene nanosheet inks allowed the development of mechanically flexible,biocompatible-printed arrays of photodetectors with pixelated MoSe2 channels on a paper exhibiting a photocurrent ON/OFF ratio of approximately 1038 and photocurrent switching of 500 ms.

关键词： transition metal dichalcogenide nanosheets zwitterions zwitterion-assisted liquid-phase exfoliation scalable inkjet printing biocompatible

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Dual-light emitting 3D encryption with printable fluorescent-phosphorescent metal-organic frameworks

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Light(Science & Applications) 2023年第10期12卷 2172-2186页

作者： Jin Woo Oh Seokyeong Lee hyowon han Omar Allam Ji Il Choi Hyeokjung Lee Wei Jiang Jihye Jang Gwanho Kim Seungsoo Mun Kyuho Lee Yeonji Kim Jong Woong Park Seonju Lee Seung Soon Jang Cheolmin Park Department of Materials Science and Engineering Yonsei UniversitySeoul 03722Republic of Korea The George W.Woodruff School of Mechanical Engineering Georgia Institute of Technology801 Ferst DriveAtlantaGA 30332-0405USA School of Materials Science and Engineering Georgia Institute of Technology771 Ferst DriveAtlantaGA 30332-0245USA Om Spin Convergence Research Center Korea Institute of Science and Technology(KIST)Seoul02792Republic of Korea

Optical encryption technologies based on room-temperature light-emitting materials are of considerable ***,we present three-dimensional(3D)printable dual-light-emitting materials for high-performance optical pattern *** are based on fluorescent perovskite nanocrystals(NCs)embedded in metal-organic frameworks(MOFs)designed for phosphorescent host-guest ***,perovskite-containing MOFs emit a highly efficient blue phosphorescence,and perovskite NCs embedded in the MOFs emit characteristic green or red fluorescence under ultraviolet(UV)*** dual-light-emitting MOFs with independent fluorescence and phosphorescence emissions are employed in pochoir pattern encryption,wherein actual information with transient phosphorescence is efficiently concealed behind fake information with fluorescence under UV ***,a 3D cubic skeleton is developed with the dual-light-emitting MOF powder dispersed in 3D-printable polymer filaments for 3D dual-pattern *** article outlines a universal principle for developing MOF-based room-temperature multi-light-emitting materials and a strategy for multidimensional information encryption with enhanced capacity and security.

关键词： perovskite light pattern

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