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Deep eutectic solvents for separation and purification applications in critical metal metallurgy:Recent advances and perspectives

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 1-19页

作者： Shuo Chen Shengpeng Su Yanfang huang Bingbing Liu hu Sun Shuzhen Yang Guihong Han School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China Zhongyuan Critical Metals Laboratory Henan ProvinceZhengzhou 450001China

Solvent extraction,a separation and purification technology,is crucial in critical metal *** solvents commonly used in solvent extraction exhibit disadvantages,such as high volatility,high toxicity,and flammability,causing a spectrum of hazards to human health and environmental *** solvents have been recognized as potential alternatives to these harmful organic *** the past two decades,several neoteric solvents have been proposed,including ionic liquids(ILs)and deep eutectic solvents(DESs).DESs have gradually become the focus of green solvents owing to several advantages,namely,low toxicity,degradability,and low *** this critical review,their classification,formation mechanisms,preparation methods,characterization technologies,and special physicochemical properties based on the most recent advancements in research have been systematically ***,the major separation and purification applications of DESs in critical metal metallurgy were comprehensively ***,future opportunities and challenges of DESs were explored in the current research *** conclusion,this review provides valuable insights for improving our overall understanding of DESs,and it holds important potential for expanding separation and purification applications in critical metal metallurgy.

关键词： deep eutectic solvents preparations properties separation and purification critical metal metallurgy

Luminescence property and magnetic resonance imaging of Gd_(2)O_(3):Tb^(3+) nanocrystals doped with Zn^(2+),Li^(+)

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Rare Metals 2021年第8期40卷 2049-2058页

作者： Rong Fu Yan-Yan hu hui-Na Qiao Chun-lin Yang Hao Yin Mei-Gui Ou College of Materials and Metallurgy University of GuizhouGuiyang550025China National Local Co-construction Engineering Laboratory for High Performance Metal Structure Material and Manufacture Technology Guiyang550025China College of Chemistry and Materials Engineering Guiyang UniversityGuiyang550003China Department of Neurosurgery Guizhou Provincial People’s HospitalGuiyang550002China

Gd_(2)O_(3):Tb^(3+) nanocrystal co-doped with Zn^(2+)and Li^(+) was prepared by the combination of polyol and solid-phase *** synthesized nanoparticles were characterized by X-ray diffraction(XRD),field emission scanning electron microscopy(FESEM),transmission electron microscopy(TEM),photoluminescence(PL)spectra and magnetic resonance imaging(MRI).The results revealed that both Gd_(2)O_(3):Tb^(3+)/Zn^(2+) and Gd_(2)O_(3):Tb^(3+)/Li^(+) had cubic unit structures with a spherical shape,and the fluorescence intensity of the nanoparticles reached a maximum at a doping concentration of0.050 mmol%for Zn^(2+) and 2 mol%for Li^(+),*** addition,the T_(1)/T_(2)(longitudinal/transverse relaxation time)-weighted MRI signals got enhanced due to the increased longitudinal relaxivity(r1)and transverse relaxivity(r2)after the doping by metal ***,the materials reported here can be used for fluorescence and MR bimodal imaging,as tracers and for fluorescence detections.

关键词： Gd_(2)O_(3):Tb^(3+) Zn^(2+)/Li^(+)doping Luminescent property Magnetic resonance imaging Nanomaterials

On generation source sites of internal waves in the Luzon Strait

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Acta Oceanologica Sinica 2008年第3期27卷 38-50页

作者： ZHENG Quanan SONG Y Tony lin hui hu Xiaomin MENG Junmin WANG Dan Department of Atmospheric and Oceanic Science University of Maryland College Park Maryland USA Jet Propulsion Laboratory California Institute of Technology Pasadena California USA Institute of Space and Earth Information Sciences The Chinese University of Hong Kong Hong Kong China First Institute of Oceanography. State Oceanic Administration. Oingdao 266061. China

This effort aims to determine the generation source sites in the Luzon Strait for energetic, long-crest, transbasin internal waves （IW） observed in the northern South China Sea （NSCS）. The roles of islands distributed on eastern side of the strait, Kuroshio, submarine ridges, shoaling thennocline, and strait configuration played in the IW generation are examined using the cruise data analysis, satellite data interpretation, and dynamical analysis. The islands and channels on eastern side of the strait are excluded from a list of possible IW source sites owing to their unmatched horizontal dimensions to the scale of IW crest line length, and the relative low Reynolds number. The Kuroshio has a potential to be a radiator for the long-crest IW disturbances, meanwhile, the Kurosbio west （east） wing absorbs the eastward （westward） propagating IW disturbance. Namely, the Kuroshio blockades the outside west-east propagating IW disturbances. The 3-D configuration of the Luzon Strait is characterized by a sudden, more than one order widening of the cross-section areas at the outlets on both sides, providing a favorable condition for IW type initial disturbance formation. In the Luzon Strait, the thermocline is featured by a westward shoaling all the year around, providing the dynamical conditions for the amplitude growth （declination） to the westward （eastward） propagating IW type disturbance. Thus, the west slope of western submarine ridge at the western outlet of the Luzon Strait is a high possibility source sites for energetic, long-crest, transbasin IWs in the NSCS. The interpretation results of satellite SAR images during a 13 a period from 1995 to 2007 provide the convincing evidence for the conclusions.

关键词： ocean internal waves solitary waves Luzon Strait satellite SAR image

Numerical simulation study on the hygrothermal performance of building exterior walls under dynamic wind-driven rain condition

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Building Simulation 2024年第2期17卷 207-221页

作者： Xing hu huibo Zhang hui Yu School of Design Shanghai Jiao Tong UniversityShanghai200240China

Wind-driven rain(WDR)has a significant influence on the hygrothermal performance,durability,and energy consumption of building *** calculation of WDR loads using semi-empirical models has been incorporated into the boundary conditions of coupled heat and moisture transfer ***,prior research often relied on fixed WDR absorption ratio,which fail to accurately capture the water absorption characteristics of porous building materials under rainfall ***,this study aims to investigate the coupled heat and moisture transfer of exterior walls under dynamic WDR boundary conditions,utilizing an empirically obtained WDR absorption ratio model based on field *** developed coupled heat and moisture transfer model is validated against the HAMSTAD *** findings reveal that the total WDR flux calculated with the dynamic WDR boundary is lower than that obtained with the fixed WDR boundary,with greater disparities observed in orientations experiencing higher WDR *** variations in moisture flow significantly impact the surface temperature and relative humidity of the walls,influencing the calculation of cooling and heating loads by different *** to the transient heat transfer model,the coupled heat and moisture transfer model incorporating dynamic WDR boundary exhibits maximum increases of 17.6%and 16.2%in cooling and heating loads,*** dynamic WDR boundary conditions provide more precise numerical values for surface moisture flux,offering valuable insights for the thermal design of building enclosures and load calculations for HVAC systems.

关键词： wind-driven rain building component hygrothermal model transient simulation cooling and heating loads

Atmospheric gaseous organic acids in winter in a rural site of the North China Plain

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Journal of Environmental Sciences 2022年第3期34卷 190-203页

作者： Xiaoyu hu Gan Yang Yiliang Liu Yiqun Lu Yuwei Wang hui Chen Jianmin Chen lin Wang Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP^(3)) Department of Environmental Science and EngineeringFudan UniversityShanghai 200438China IRDR International Center of Excellence on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health Fudan UniversityShanghai 200433China Collaborative Innovation Center of Climate Change Nanjing 210023China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

Organic acids are important contributors to the acidity of atmospheric precipitation,but their existence in the Chinese atmosphere is largely *** this study,twelve atmospheric gaseous organic acids,including C_(1)-C_(9) alkanoic acids,methacrylic acid,pyruvic acid,and benzoic acid,were observed in the suburb of Wangdu,Hebei Province,a typical rural site in the northern China plain from 16^(th) December,2018 to 22^(nd) January,2019,using a Vocus■ Proton-Transfer-Reaction time-of-flight mass spectrometer(Vocus PTR-ToF).The quantification of C_(2)-C_(4) alkanoic acids by the Vocus PTR-ToF was calibrated according to the titration of a NaOH solution by C_(2)-C_(4) alkanoic acids from home-made permeation sources,and the other organic acids except for formic acid were quantified based on the k_(cap)-sensitivity linearity in the Vocus PTR-ToF,whereas formic acid was not quantified because our instrument setting led to a significant underestimation in its *** average total concentration of eleven gaseous organic acids was 6.96±5.20 ppbv(parts per billion by volume).The average concentration of acetic acid was the highest(3.86±3.00 ppbv),followed by propanoic acid,butyric acid,and methacrylic *** straw burning was likely the dominant source of the observed gaseous organic acids according to the good correlations between acetonitrile and organic acids and between particulate K+and organic acids,and traffic emissions could also have *** episodes with continuously high concentrations of organic acids,short-distance transport dominated in Wangdu according to the backward trajectory ***,Shijiazhuang,and Hengshui areas were the main source areas based on potential source contribution function and concentration weighing track analysis.

关键词： Gaseous organic acids Vocus PTR-ToF North China plain

Optimization Strategies of Na_(3)V_(2)(PO_(4))_(3) Cathode Materials for Sodium‑Ion Batteries

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Nano-Micro Letters 2025年第2期17卷 204-251页

作者： Jiawen hu Xinwei Li Qianqian Liang Li Xu Changsheng Ding Yu Liu Yanfeng Gao School of Materials Science and Engineering Shanghai UniversityShanghai 200444People’s Republic of China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050People’s Republic of China

Na_(3)V_(2)(PO_(4))_(3)(NVP)has garnered great attentions as a prospective cathode material for sodium-ion batteries(SIBs)by virtue of its decent theoretical capacity,superior ion conductivity and high structural ***,the inherently poor electronic conductivity and sluggish sodium-ion diffusion kinetics of NVP material give rise to inferior rate performance and unsatisfactory energy density,which strictly confine its further application in ***,it is of significance to boost the sodium storage performance of NVP cathode *** to now,many methods have been developed to optimize the electrochemical performance of NVP cathode *** this review,the latest advances in optimization strategies for improving the electrochemical performance of NVP cathode material are well summarized and discussed,including carbon coating or modification,foreign-ion doping or substitution and nanostructure and morphology *** foreign-ion doping or substitution is highlighted,involving Na,V,and PO_(4)^(3−)sites,which include single-site doping,multiple-site doping,single-ion doping,multiple-ion doping and so ***,the challenges and prospects of high-performance NVP cathode material are also put *** is believed that this review can provide a useful reference for designing and developing high-performance NVP cathode material toward the large-scale application in SIBs.

关键词： Sodium-ion batteries Na_(3)V_(2)(PO_(4))_(3) Cathode materials Electrochemical performance Optimization strategies

Patterning mechanisms controlling digit development

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Journal of Genetics and Genomics 2008年第9期35卷 517-524页

作者： Jianxin hu lin He Bio-X Center Shanghai Jiao Tong University Shanghai 200030 China Institute for Nutritional Sciences Shanghai Institutes for Biological Sciences Chinese Academy of Sciences Shanghai 200031 China Institutes of Biomedical Sciences Fudan University Shanghai 200032 China

Vertebrate digits are essential structures for movement, feeding and communication. Specialized regions of the developing limb bud including the zone of polarizing activity （ZPA）, the apical ectodermal ridge （AER）, and the non-ridge ectoderm regulate the patterning of digits. Although a series of signaling molecules have been characterized as patterning signals from the organizing centers, the delicate cellular and molecular mechanisms that interpret how these patterning signals control the detailed digit anatomy remain unclear, Recent studies from model organisms and human hand malformations provide new insights into the mechanisms regulating this process. Here, we review the current understanding of the genetic networks governing digit morphogenesis

关键词： digit formation AER ZPA Shh gradient Fgf, patterning mechanism specification elongation segmentation

Preface: Wind turbines: aeromechanics and farm optimization

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Acta Mechanica Sinica 2020年第2期36卷 257-259页

作者： hui hu Xiaodong Wang Department of Aerospace Engineering Iowa State UniversityAmesIA50011-1096USA Department of Energy Power and Mechanical Engineering of North China Electric Power UniversityBeijing102206China

1 Preface With the oil and gas supply security and climate change emerging as high concerns,the need for renewable energy sources to alleviate dependence on hydrocarbons and reduce carbon dioxide(CO2)emissions is becoming increasingly *** energy is one of the cleanest renewable power sources in the world *** *** of Energy(DOE)initiated the Wind Vision study where the costs and benefits of continued investments on wind energy was *** study evaluated an ambitious,yet credible scenario in which wind energy will serve 20%of the nation’s total electric power demand by 2030,and 35%by *** Europe,the wind power generation accounted for 15%of all European electricity demand in the past *** power installation in China has been growing by an annual rate of^10%in recent ***,wind power has become the second largest renewable energy in China,only after hydro-power.

关键词： Wind becoming continued

Dimensions of receptor-ligand complex and the optimal radius of endocytosed virus-like particle

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Frontiers of physics 2014年第4期9卷 519-522页

作者： Yan-hui Liu Ying-Bing Chen Wei Mao lin hu lin-Hong Deng Hou-Qiang XU Key Laboratory of Animal Genetics Breeding and Reproduction in the Plateau Mountainous Region Ministry of Education College of Animal Science Guizhou University Guiyang 550025 China Soft Condensed Matter Laboratory College of Science Guizhou University Guiyang 550025 China State Key Laboratory of Theoretical Physics Institute of Theoretical Physics Chinese Academy of Sciences Beijing 100190 China Institute of Biomedical Engineering and Health Sciences Changzhou University Changzhou 213164 China Key Laboratory of Biorheological Science and Technology Ministry of Education Bioengineering College Chongqing University Chongqing 400044 China

Recent experiments have pointed out that cellular uptake is strongly dependent on the physical dimensions of endocytosed nanoparticles and tile optimal radius of endocytosed virus-like particle coated by transferrin is around 50 nm. As the same time, the dimensions of receptor-ligand complex have strong effects on the size-dependent exclusion of proteins ill cell environments. Inspired by these experimental results, a continuum elastic model is constructed to resolve the relationship between the dinlensions of receptor-ligand complex and the optimal radius of endocytosed virus-like particle. These results demonstrate that the optimal radius of endocytosed virus-like particle depends on the dimensions of reeeptor-ligand complex and the dimension of receptor-ligand complex reduces the depletion zone.

关键词： cellular uptake depletion effects dimension of receptor-ligand complex elasticitytheory