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Designing ultrastable P2/O3-type layered oxides for sodium ion batteries by regulating Na distribution and oxygen redox chemistry

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Journal of Energy Chemistry 2024年第7期94卷 466-476页

作者： Jieyou huang Weiliang Li Debin Ye Lin Xu wenwei Wu Xuehang Wu School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004GuangxiChina Guangxi Key Laboratory for High-value Utilization of Manganese Resources Guangxi Normal University for NationalitiesChongzuo 532200GuangxiChina

P2/O3-type Ni/Mn-based layered oxides are promising cathode materials for sodium-ion batteries(SIBs)owing to their high energy ***,exploring effective ways to enhance the synergy between the P2 and 03 phases remains a ***,we design a P2/O3-type Na_(0.76)Ni_(0.31)Zn_(0.07)Mn_(0.50)Ti_(0.12)0_(2)(NNZMT)with high chemical/electrochemical stability by enhancing the coupling between the two *** the first time,a unique Na*extraction is observed from a Na-rich O3 phase by a Na-poor P2 phase and systematically *** process is facilitated by Zn^(2+)/Ti^(4+)dual doping and calcination condition regulation,allowing a higher Na*content in the P2 phase with larger Na^(+)transport channels and enhancing Na transport *** of reduced Na^(+)in the O3 phase,which increases the difficulty of H^(+)/Na^(+) exchange,the hydrostability of the O3 phase in NNZMT is considerably ***,Zn^(2+)/Ti^(4+)presence in NNZMT synergistically regulates oxygen redox chemistry,which effectively suppresses O_(2)/CO_(2) gas release and electrolyte decomposition,and completely inhibits phase transitions above 4.0 *** a result,NNZMT achieves a high discharge capacity of 144.8 mA h g^(-1) with a median voltage of 3.42 V at 20 mA g^(-1) and exhibits excellent cycling performance with a capacity retention of 77.3% for 1000 cycles at 2000 mA g^(-1).This study provides an effective strategy and new insights into the design of high-performance layered-oxide cathode materials with enhanced structure/interface stability forSIBs.

关键词： Sodium-ion batteries P2/O3-type layered oxides Na distribution Oxygen redox chemistry Hydrostability

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百色市西甜瓜生产现状与发展建议

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农业工程 2024年第3期14卷 146-149页

作者：周银慧罗思良费永红农媛韦静罗顺遂黄文伟广西农业科学院百色分院百色市农业科学研究所广西百色533000

西甜瓜是人们喜爱的一种水果,近年来西甜瓜种植效益降低,栽培面积也呈下降趋势。实地调研百色市右江河谷西甜瓜产业发展现状,分析该地区西甜瓜种植栽培存在的问题,为右江河谷地区西甜瓜产业持续健康发展提出建议与对策。

关键词：西甜瓜产业发展水果产业右江河谷百色市

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Functional Optical Fiber Sensors Detecting Imperceptible Physical/Chemical Changes for Smart Batteries

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Nano-Micro Letters 2024年第8期16卷 268-308页

作者： Yiding Li Li Wang Youzhi Song wenwei Wang Cheng Lin Xiangming He Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084People’s Republic of China National Engineering Research Center of Electric Vehicles Beijing Institute of Technology(BIT)Beijing 100081People’s Republic of China Shenzhen Automotive Research Institute of BIT(Shenzhen Research Institute of National Engineering Research Center of Electric Vehicles) Shenzhen 518118People’s Republic of China

The battery technology progress has been a contradictory process in which performance improvement and hidden risks *** the battery is still a“black box”,thus requiring a deep understanding of its internal *** battery should“sense its internal physical/chemical conditions”,which puts strict requirements on embedded sensing *** paper summarizes the application of advanced optical fiber sensors in lithium-ion batteries and energy storage technologies that may be mass deployed,focuses on the insights of advanced optical fiber sensors into the processes of one-dimensional nano-micro-level battery material structural phase transition,electrolyte degradation,electrode-electrolyte interface dynamics to three-dimensional macro-safety *** paper contributes to understanding how to use optical fiber sensors to achieve“real”and“embedded”*** the inherent advantages of the advanced optical fiber sensor,it helps clarify the battery internal state and reaction mechanism,aiding in the establishment of more detailed *** advancements can promote the development of smart batteries,with significant importance lying in essentially promoting the improvement of system ***,with the help of smart batteries in the future,the importance of consistency can be weakened or even *** application of advanced optical fiber sensors helps comprehensively improve the battery quality,reliability,and life.

关键词： Smart battery Advanced embedded optical fiber sensor Battery internal physical/chemical state Quality-reliability-life characteristic

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Improving discharge voltage and ion storage dynamic in polyaniline via modulation of carrier charge density for magnesiummetal batteries

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Nano Research 2024年第7期17卷 6168-6175页

作者： Ping Luo Feiyang Chao Chunli Zuo wenwei Zhang Fangyu Xiong Zhen huang Dongyao Zhu Gongtao Yu Wenhui Zhong Xingbao Chen Han Tang Xiujuan Wei Qinyou An Hubei Provincial Key Laboratory of Green Materials for Light Industry School of Materials and Chemical EngineeringHubei University of TechnologyWuhan 430068China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China Institute for Sustainable Transformation School of Chemical Engineering and Light IndustryGuangdong University of TechnologyGuangzhou 510006China

Rechargeable magnesium-metal batteries(RMBs)have gained much attention due to their abundant resources as well as high ***,the high charge density of Mg^(2+)is one of the main reasons for the slow kinetics performance of RMBs,and modulation of the charge density is an important strategy to improve the kinetics and electrochemical performance of ***,we report on the conductive polymer polyaniline(PANI)for RMBs,which is found to have excellent kinetics and high discharge voltage when storing MgCl^(+).In the storage of MgCl^(+),PANI exhibits a high average discharge voltage platform is 2.3 V ***^(2+)/Mg,which is higher than that in storage of Mg^(2+).We demonstrated the reversible intercalation/de-intercalation of MgCl^(+)in PANI accompanying with the reversible transformation between the quinone ring(C–C,–N=)and the benzene ring(C=C,–NH–)during charging and *** functional theory calculation reveals that PANI exhibit higher voltages(2.25 V vs.1.82 V)along with lower diffusion energy barriers(1.27 eV vs.1.55 eV)for MgCl^(+)storage compared to Mg^(2+)*** work refines the storage mechanism of PANI in RMBs and provides new guidelines for the application of PANI in RMBs.

关键词： rechargeable magnesium-metal batteries cathode materials polyaniline MgCl+storage

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Silurian integrative stratigraphy,biotas,and paleogeographical evolution of the Qinghai-Tibetan Plateau and its surrounding areas

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Science China Earth Sciences 2024年第4期67卷 1005-1035页

作者： Zhongyang CHEN Qing CHEN Guangxu WANG Xiang FANG Peng TANG Guanzhou YAN wenwei YUAN Bing huang Xiaole ZHANG Kui YAN Yuandong ZHANG Yi WANG State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and PalaeontologyChinese Academy of SciencesNanjing 210008China University of Chinese Academy of Sciences Beijing 100049China

The Silurian palaeontology and stratigraphy of the Qinghai-Tibetan Plateau have been studied for more than100 *** the launch of the Second Tibetan Plateau Scientific Expedition and Research,it is necessary to update the summaries of the Silurian stratigraphy and fossil assemblages of the Qinghai-Tibetan Plateau and their correlation with its surrounding *** this study,we have selected 33 sections from the Qinghai-Tibetan Plateau and its surroundings areas,summarised the available data in terms of stratigraphic regionalisation,lithostratigraphy,chronostratigraphy,and biostratigraphy,and divided the study area into four stratigraphic provinces:the Xizang-Western Yunnan-Western Sichuan Province,the KunlunQilian Province,the South China Province,and the Tarim *** general,the Silurian strata in the Qinghai-Tibetan Plateau is more complete than those in other areas of *** studies of the vertebrate faunas,sporomorph assemblages,and brachiopod faunas of the study area indicate a closer geographical relationship between the South China,Tarim,and Indochina palaeoplates,than previously *** with the surrounding areas where Silurian strata have been extensively studied,the study of Silurian strata in the main part of the Qinghai-Tibetan Plateau is still in the preliminary *** the future,it is necessary to conduct research on the age,distribution,and resource potential of basal Silurian black shales to provide new directions for shale gas exploration and development in *** shallow marine strata of the middle to upper Silurian require further *** that the Silurian System in the Qinghai-Tibetan Plateau is more complete,it has the potential to supplement and improve the study of the carbon isotope stratigraphy of the Silurian in China.

关键词： Qinghai-Tibetan Plateau Silurian Stratigraphic regionalisation Lithostratigraphy Biostratigraphy Palaeogeographical evolution

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Long-Term Performance and Microstructural Characterization of Dam Concrete in the Three Gorges Project

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Engineering 2024年第2期33卷 237-262页

作者： Chen Lyu Cheng Yu Chao Lu Li Pan wenwei Li Jiaping Liu School of Materials Science and Engineering Southeast UniversityNanjing 211189China State Key Laboratory of High Performance Civil Engineering Materials Sobute New Materials Co.Ltd.Nanjing 211103China China Three Gorges Corporation Wuhan 430010China

This study investigates the long-term performance of laboratory dam concrete in different curing environments over ten years and the microstructure of 17-year-old laboratory concrete and actual concrete cores drilled from the Three Gorges *** mechanical properties of the laboratory dam concrete,whether cured in natural or standard environments,continued to improve over ***,the laboratory dam concrete exhibited good resistance to diffusion and a refined microstructure after 17 ***,curing and long-term exposure to the local natural environment reduced the frost *** analyses of the laboratory concrete samples demonstrated that moderate-heat cement and fine fly ash(FA)particles were almost fully hydrated to form compact micro structures consisting of large quantities of homogeneous calcium(alumino)silicate hydrate(C-(A)-S-H)gels and a few *** obvious interfacial transition zones were observed in the microstructure owing to the longterm pozzolanic *** dense and homogenous microstructure was the crucial reason for the excellent long-term performance of the dam concrete.A high FA volume also played a significant role in the microstructural densification and performance growth of dam concrete at a later *** concrete drilled from the dam surface exhibited a loose microstructure with higher microporosity,indicating that concrete directly exposed to the actual service environment suffered degradation caused by water and wind *** this study,both macro-performance and microstructural analyses revealed that the application of moderate-heat cement and FA resulted in a dense and homogenous microstructure,which ensured the excellent long-term performance of concrete from the Three Gorges Dam after 17 ***-term exposure to an actual service environment may lead to microstructural degradation of the concrete ***,the retained long-term dam concrete samples need to be further researched to

关键词： Three Gorges Dam Long-term performance Microstructural analysis Moderate-heat cement Fly ash

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Enhanced wide-angle third-harmonic generation in flat-band-engineered quasi-BIC metagratings

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Science China(Physics,Mechanics & Astronomy) 2024年第4期67卷 81-87页

作者： Yijia Zang Ruoheng Chai wenwei Liu Zhancheng Li Hua Cheng Jianguo Tian Shuqi Chen The Key Laboratory of Weak Light Nonlinear Photonics Ministry of EducationSchool of Physics and TEDA Institute of Applied PhysicsNankai UniversityTianjin 300071China School of Materials Science and Engineering Smart Sensing Interdisciplinary Science CenterNankai UniversityTianjin 300350China The Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

Nonlinear metasurfaces and photonic crystals provide a significant way to generate and manipulate nonlinear signals owing to the resonance-and symmetry-based light-matter interactions supported by the artificial ***,the nonlinear conversion efficiency is generally limited by the angular dispersion of optical resonances especially in nonparaxial ***,we propose a metagrating realizing a quasi-bound-state in the continuum in a flat band to dramatically improve the third harmonic generation(THG)efficiency.A superior operating angular range is achieved based on the interlayer and intralayer couplings,which are introduced by breaking the mirror symmetry of the *** demonstrate the relation of angular dispersion between the nonlinear and linear responses at different incident *** also elucidate the mechanism of these offaxis flat-band-based nonlinear conversions through different mode *** scheme provides a robust and analytical way for nonparaxial nonlinear generation and paves the way for further applications such as wide-angle nonlinear information transmission and enhanced nonlinear generation under tight focusing.

关键词： nonlinear metasurfaces quasi-bound-state in the continuum angular dispersion third harmonic generation efficiency

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Review of Electrical and Electronic Architectures for Autonomous Vehicles:Topologies,Networking and Simulators

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Automotive Innovation 2024年第1期7卷 82-101页

作者： wenwei Wang Kaidi Guo Wanke Cao Hailong Zhu Jinrui Nan Lei Yu National Engineering Research Center of Electric Vehicles Beijing Institute of Technology(BIT)Beijing 100081China Shenzhen Automotive Research Institute Beijing Institute of Technology(BIT)Shenzhen 518000China State Key Laboratory of Networking and Switching Technology Beijing University of Posts and TelecommunicationBeijing 100876China Purple Mountain Laboratories Nanjing 211111China Beijing Kawen New Energy Vehicle Co. LTDBeijing 102209China

With the rapid development of autonomous vehicles,more and more functions and computing requirements have led to the continuous centralization in the topology of electrical and electronic(E/E)*** certain Tier1 suppliers,such as BOSCH,have previously proposed a serial roadmap for E/E architecture development,implemented since 2015 with significant contributions to the automotive industry,lingering misconceptions and queries persist in actual engineering ***,there are concerns regarding the perspective of zone-oriented E/E architectures,characterized by zonal concentration,as successors to domain-oriented E/E architectures,known for functional *** these misconceptions and queries,this study introduces a novel parallel roadmap for E/E architecture development,concurrently evaluating domain-oriented and zone-oriented ***,the study explores hybrid E/E architectures,amalgamating features from both *** align with the evolution of E/E architectures,networking technologies must adapt *** networking mechanisms pivotal in E/E architecture design are comprehensively ***,the study delves into modeling and verification tools pertinent to E/E architecture *** conclusion,the paper outlines existing challenges and unresolved queries in this domain.

关键词： Autonomous vehicles Electrical and electronic architectures Topology Networking Domain-oriented Zone-oriented

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Morphological and Sulfur-Isotopic Characteristics of Pyrites in the Deep Sediments from Xisha Trough,South China Sea

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Journal of Ocean University of China 2024年第1期23卷 138-148页

作者： CHANG Jingyi LIU Yujia LU Hailong LU Jing’an SU Xin YE Jianliang XIE wenwei College of Engineering Peking UniversityBeijing 100871China Beijing International Center for Gas Hydrate School of Earth and Planetary SciencesPeking UniversityBeijing 100871China School of Marine Science Nanjing University of Information Science and TechnologyNanjing 210044China MLR Key Laboratory of Marine Mineral Resources Guangzhou Marine Geological SurveyMinistry of Land and ResourcesGuangzhou 510075China School of Ocean Sciences China University of GeosciencesBeijing 100083China

Pyrite is one of the common authigenic minerals in marine *** studies have shown that the morphological and isotopic characteristics of pyrite are closely related to the geochemical environment where it is *** better understand the for-mation mechanism of authigenic pyrite,we analyzed the isotopic composition,morphology,and distribution of pyrite in the sediment at 500m below the seafloor from Xisha Trough,South China *** morphologies were observed by scanning electron micros-copy and Raman spectrography.X-Ray computed tomography was applied to measure the particle size of *** size of pyrite crystals in the matrix sediment mainly ranged between 25 and 65µm(***.40µm),although crystals were larger(***.50μm)in the *** pyrites had a fine-grained truncated octahedral shape with occasionally well-developed growth steps,which implies the low growth rate and weak anaerobic oxidation of methane-sulfate reduction when pyrite was ***δ^(34)S values of pyrites ranged from+20.8‰Vienna-defined Canyon Diablo Troilite(V-CDT)to+33.2‰V-CDT and from+44.8‰V-CDT to+48.9‰,which suggest two growth *** the first stage,with the continuous low methane flux,the pyrite possibly formed in an environment with good access to *** the second stage,the pyrites mainly developed in sediment fractures and appeared in veins,probably due to the limited availability of *** less exposure of pyrite to the environment in the second stage was probably caused by sediment accumulation or *** this study,an episodic pyritization process was identified,and the paleoenvironment was reconstructed for the sediment investigated.

关键词： pyrite sulfur isotope AOM methane flux Xisha Trough South China Sea

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Ultra-robust informational metasurfaces based on spatial coherence structures engineering

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Light(Science & Applications) 2024年第7期13卷 1310-1319页

作者： Leixin Liu wenwei Liu Fei Wang Xiaofeng Peng Duk-Yong Choi Hua Cheng Yangjian Cai Shuqi Chen Shandong Provincial Engineering and Technical Center of Light Manipulations Collaborative Innovation Center of Light Manipulation and ApplicationsShandong Provincial Key Laboratory of Optics and Photonic DeviceSchool of Physics and ElectronicsShandong Normal UniversityJinan 250014China. The Key Laboratory of Weak Light Nonlinear Photonics Ministry of EducationSchool of PhysicsSchool of Materials Science and EngineeringSmart Sensing Interdisciplinary Science CenterNankai UniversityTianjin 300071China. School of Physical Science and Technology Soochow UniversitySuzhou 215006China. Laser Physics Centre Research School of PhysicsAustralian National UniversityCanberraACT 2601Australia. The Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuanShanxi 030006China

Optical information transmission is vital in modern optics and photonics due to its concurrent and multi-dimensional nature,leading to tremendous applications such as optical microscopy,holography,and optical *** optical information transmission technologies suffer from bulky optical setup and information loss/crosstalk when meeting scatterers or obstacles in the light ***,we theoretically propose and experimentally realize the simultaneous manipulation of the coherence lengths and coherence structures of the light beams with the disordered *** ultra-robust optical information transmission and self-reconstruction can be realized by the generated partially coherent beam with modulated coherence structure even 93%of light is recklessly obstructed during light transmission,which brings new light to robust optical information transmission with a single *** method provides a generic principle for the generalized coherence manipulation on the photonic platform and displays a variety of functionalities advancing capabilities in optical information transmission such as meta-holography and imaging in disordered and perturbative media.

关键词： optics coherent holography

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