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Magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell nanospheres derived from FeNi-LDH precursor anchoring on rGO nanosheets for enhanced electromagnetic wave absorption

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Journal of Materials Science & Technology 2024年第4期171卷 101-114页

作者： Kunyao Cao Yuan Fang Shuai Wang yue Zhang Jiayue wen Jun Chen Rui Zhao Weidong Xue School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 610054China

Graphene has been extensively utilized in the domain of electromagnetic wave(EMW)absorption ma-terials because of its excellent electrical ***,the inferior impedance matching per-formance and the single loss mechanism vastly restrict the ***,it’s an effective strat-egy to solve these issues by introducing magnetic ***,layer double hydroxide(LDH)is an appropriate template to obtain magnetic component *** that ferromagnetic met-als such as Fe,Co,Ni,and their corresponding metal oxides are usually treated as magnetic compo-nents which are promising candidates for EMW absorption ***,in this work,a FeNi-layered double hydroxide-reduced graphene oxide(FeNi-LDH-rGO)aerogel was synthesized through a series of processes such as electrostatic self-assembly,hydrothermal,freeze-drying,and *** magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell nanospheres were obtained from FeNi-LDH precursor,anchoring on rGO nanosheets after the annealing ***,the effects of different mass ratios of LDH to GO as well as different annealing temperatures of LDH-rGO aerogel on the EMW absorption prop-erty and impedance matching performance were *** a consequence,the fabricated ultralight 600LDH-rGO 2:1 aerogel shows a broad effective absorption bandwidth(EAB)of 7.04 GHz at a thickness of 2.3 mm with a low filling content of only 6 wt%and a low density of 4.4 mg/cm^(3).In conclusion,the synthetic LDH-rGO aerogels offer an effective strategy for preparing EMW absorption materials that own three-dimensional porous network structure and unique magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell struc-ture nanospheres.

关键词： Electrostatic self-assembly Electromagnetic wave absorption LDH-rGO aerogel Layered double hydroxide Reduced graphene oxide NiFe_(2)O_(4)@FeNi_(3)core-shell structure

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Role of Multi-scale Hierarchical Structures in Regulating Wetting State and Wetting Properties of Structured Surfaces

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Journal of Bionic Engineering 2024年第3期21卷 1347-1359页

作者： yue Jiang Xinyi Li Zhichao Ma Zhihui Zhang Cuie wen Zhonghao Jiang Nan Lin Luquan Ren Key Laboratory of Bionic Engineering of Ministry of Education College of Biological and Agricultural EngineeringJilin UniversityChangchun130022China Hubei Provincial Engineering Technology Research Center for Microgrid College of Electrical Engineering and New EnergyChina Three Gorges UniversityYichang443002China School of Mechanical and Aerospace Engineering Jilin UniversityChangchun130025China Centre for Additive Manufacturing School of EngineeringRMIT UniversityMelbourneVictoria3001Australia Key Laboratory of Automobile Materials of Ministry of Education College of Materials Science and EngineeringJilin UniversityChangchun130025China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry Jilin UniversityChangchun130012China

Amplifying the intrinsic wettability of substrate material by changing the solid/liquid contact area is considered to be the main mechanism for controlling the wettability of rough or structured *** theoretical analysis and experimental exploration,we have found that in addition to this wettability structure amplification effect,the surface structure also simultaneously controls surface wettability by regulating the wetting state via changing the threshold Young angles of the Cassie-Baxter and wenzel wetting *** wetting state regulation effect provides us with an alternative strategy to overcome the inherent limitation in surface chemistry by tailoring surface *** wetting state regulation effect created by multi-scale hierarchical structures is quite significant and plays is a crucial role in promoting the superhydrophobicity,superhydrophilicity and the transition between these two extreme wetting properties,as well as stabilizing the Cassie-Baxter superhydrophobic state on the fabricated lotus-like hierarchically structured Cu surface and the natural lotus leaf.

关键词： Hierarchical structure Wetting state regulation Wetting transition Superhydrophobicity Superhydrophilicity

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High Temperature Iron Ethylene Polymerization Catalysts Bearing N,N,N'-2-(1-(2,4-Dibenzhydryl-6-fluorophenylimino)ethyl)-6-(1-(arylphenylimino)ethyl)pyridines

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Chinese Journal of Polymer Science 2024年第2期42卷 188-201,I0007页

作者： Chantsalnyam Bariashir Qiu-yue Zhang Bayasgalan Ulambayar Gregory A.Solan Tong-Ling Liang wen-Hua Sun Institute of Chemistry and Chemical Technology Mongolian Academy of SciencesUlaanbaatar13330Mongolia Key Laboratory of Engineering Plastics and Beijing National Laboratory for Molecular Science Institute of ChemistryChinese Academy of SciencesBeijing100190China Department of Chemistry University of LeicesterUniversity RoadLeicesterLE17RHUK State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

The N,N,N'-ferrous chloride complexes,[2-{CMeN(2,4-(CHPh)_(2)-6-FC_(6)H_(2))}-6-(CMeNAr)C_(5)H_(3)N]FeCl_(2)(Ar=2,6-Me_(2)C_(6)H_(3) Fe1,2,6-Et_(2)C_(6)H_(3)Fe2,2,6-^(i)Pr_(2)C_(6)H_(3) Fe3,2,4,6-Me_(3)C_(6)H_(2) Fe4 and 2,6-Et_(2)-4-MeC_(6)H_(2) Fe5),each possessing one N-2,4-dibenzhydryl-6-fluorophenyl group,were readily synthesized from their respective unsymmetrical bis(imino)pyridines,*** identification of Fe2 highlighted the variation in the steric properties provided by the dissimilar N-aryl *** pre-treatment with either MAO or MMAO,complexes Fe1-Fe5 all displayed,at an operating temperature of 80℃,high activities for ethylene polymerization with levels falling in the order:Fe4> Fe1> Fe5> Fe2> ***,Fe4/MAO displayed the highest activity of 1.94×10^(7) g_(PE)·mol_(Fe)^(-1)·h^(-1) of the study with only a modest loss in performance at 90℃.Generally,the resulting polyethylenes were highly linear(T_(m) range:122-132℃),narrowly disperse and of low molecular weight(M_(w) range:6.73-46.04kg·mol^(-1)),with the most sterically hindered Fe3 forming the highest molecular weight polymer of the ***-group analysis by ^(1)H-and ^(13)CNMR spectroscopy revealed saturated alkyl(n-propyl and i-propyl) and unsaturated vinyl chain ends indicative of the role of both β-H elimination and chain transfer to aluminum as termination *** comparison with previou sly reported iron precatalysts with similar tridentate ligand skeletons,it is evident that the introduction of a large benzhydryl group in combination with a fluorine as the ortho-substituents of one N-aryl group has the effect of enhancing thermal stability of the iron polymerization catalyst whilst maintaining appreciable polymer molecular weight.

关键词： Iron catalyst Ethylene polymerization Linear polyethylene Fluoride effect Thermal stability

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Multi-Scale Pore Structure Heterogeneity in Tuff Reservoirs Investigated with Multi-Experimental Method and Fractal Dimensions in Chang 7 Formation,Southern Ordos Basin

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Journal of Earth Science 2024年第2期35卷 666-686页

作者： Hao Lu Qing Li Dali yue Dongdong Xia Shenghe Wu Lang wen Yu He State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing102249China College of Geosciences China University of PetroleumBeijing102249China Petroleum Exploration and Development Institute of SINOPEC Beijing100083China

The tight tuff reservoir is an unusual type of unconventional reservoir with strong ***,there is a lack of research on the microscopic pore structure that causes the heterogeneity of tuff *** the Chang 7 Formation in Ordos Basin,China as a case study,carbon-dioxide gas adsorption,nitrogen gas adsorption and high-pressure mercury injection are integrated to investigate the multi-scale pore structure characteristics of tuff ***,the fractal dimension is introduced to characterize the complexity of pore structure in tuff *** this multi-experimental method,the quantitative characterizations of the full-range pore size distribution of four tuff types were obtained and compared in the size ranges of micropores,mesopores and *** dimension curves derived from full-range pores are divided into six segments as D1,D2,D3,D4,D5 and D6 corresponding to fractal characteristics of micropores,smaller mesopores,larger mesopores,smaller macropores,medium macropores and larger macropores,*** macropore volume,average macropore radius and fractal dimension D5 significantly control petrophysical *** larger macropore volume,average macropore radius and D5 correspond to favorable pore structure and good reservoir quality,which provides new indexes for the tuff reservoir *** study enriches the understanding of the heterogeneity of pore structures and contributes to unconventional oil and gas exploration and development.

关键词： tuff reservoir pore structure carbon-dioxide gas adsorption nitrogen gas adsorption high-pressure mercury injection fractal dimension petroleum geology

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Knockdown of HE4 suppresses tumor growth and invasiveness in lung adenocarcinoma through regulation of EGFR signaling

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Oncology Research 2024年第6期32卷 1119-1128页

作者： yue ZHANG wenYU YANG XIAOWANG HAN yue QIAO HAITAO WANG TING CHEN TIANYING LI wen-BIN OU Department of Biopharmaceutics College of Life Sciences and MedicineZhejiang Provincial Key Laboratory of Silkworm Bioreactor and BiomedicineZhejiang Sci-Tech UniversityHangzhou310018China Department of Thoracic Surgery Zhejiang Provincial People’s HospitalHangzhou310014China

It has been shown that the high expression of human epididymis protein 4(HE4)in most lung cancers is related to the poor prognosis of patients,but the mechanism of pathological transformation of HE4 in lung cancer is still *** current study is expected to clarify the function and mechanism of HE4 in the occurrence and metastasis of lung adenocarcinoma(LUAD).Immunoblotting evaluated HE4 expression in lung cancer cell lines and biopsies,and through analysis of The Cancer Genome Atlas(TCGA)*** HE4 overexpression was demonstrated in LUAD,but not in lung squamous cell carcinoma(LUSC),indicating that HE4 can serve as a biomarker to distinguish between LUAD and ***4 knockdown significantly inhibited cell growth,colony formation,wound healing,and invasion,and blocked the G1-phase of the cell cycle in LUAD cell lines through inactivation of the EGFR signaling downstream including PI3K/AKT/mTOR and RAF/MAPK *** first-line EGFR inhibitor gefitinib and HE4 shRNA had no synergistic inhibitory effect on the growth of lung adenocarcinoma cells,while the third-line EGFR inhibitor osimertinib showed additive anti-proliferative ***,we provided evidence that HE4 regulated EGFR expression by transcription regulation and protein interaction in *** findings suggest that HE4 positively modulates the EGFR signaling pathway to promote growth and invasiveness in LUAD and highlight that targeting HE4 could be a novel strategy for LUAD treatment.

关键词： Lung adenocarcinoma Human epididymis protein 4 Epidermal growth factor receptor Biomarker Targeted therapies

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Age of Information for Short-Packet Covert Communication with Time Modulated Retrodirective Array

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China Communications 2024年第4期21卷 23-37页

作者： Ma yue Ma Ruiqian Lin Zhi Yang Weiwei Cai yueming Miao Chen Wu wen Key Laboratory of Near-Range RF Sensing ICs&Microsystems(NJUST) Ministry of EducationSchool of Electronic and Optical EngineeringNanjing University of Science and TechnologyNanjing 210094China College of Electronic Engineering National University of Defense TechnologyHefei 230037China College of Communications Engineering Army Engineering University of PLANanjing 210007China

In this paper,the covert age of information(CAoI),which characterizes the timeliness and covertness performance of communication,is first investigated in the short-packet covert communication with time modulated retrodirective array(TMRDA).Specifically,the TMRDA is designed to maximize the antenna gain in the target direction while the side lobe is sufficiently *** this basis,the covertness constraint and CAoI are derived in closed *** facilitate the covert transmission design,the transmit power and block-length are jointly optimized to minimize the CAoI,which demonstrates the trade-off between covertness and *** results illustrate that there exists an optimal block-length that yields the minimum CAoI,and the presented optimization results can achieve enhanced performance compared with the fixed block-length ***,we observe that smaller beam pointing error at Bob leads to improvements in CAoI.

关键词： age of information covert communication retrodirective array time modulation

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Impacts of Future Changes in Heavy Precipitation and Extreme Drought on the Economy over South China and Indochina

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Advances in Atmospheric Sciences 2024年第6期41卷 1184-1200,I0022-I0034页

作者： Bin TANG wenting HU Anmin DUAN Yimin LIU wen BAO yue XIN Xianyi YANG State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China University of Chinese Academy of Sciences Beijing 101408China State Key Laboratory of Marine Environmental Science College of Ocean and Earth SciencesXiamen UniversityXiamen 361005China Chinese Academy of Sciences the CAS Institutes of Science and DevelopmentBeijing 101408China School of Public Policy and Management University of Chinese Academy of SciencesBeijing 101408China

Heavy precipitation and extreme drought have caused severe economic losses over South China and Indochina(INCSC)in recent *** the areas with large gross domestic product(GDP)in the INCSC region are distributed along the coastline and greatly affected by global warming,understanding the possible economic impacts induced by future changes in the maximum consecutive 5-day precipitation(RX5day)and the maximum consecutive dry days(CDD)is critical for adaptation planning in this *** on the latest data released by phase 6 of the Coupled Model Intercomparison Project(CMIP6),future projections of precipitation extremes with bias correction and their impacts on GDP over the INCSC region under the fossil-fueled development Shared Socioeconomic Pathway(SSP5-8.5)are *** indicate that RX5day will intensify robustly throughout the INCSC region,while CDD will lengthen in most regions under global *** changes in climate consistently dominate the effect on GDP over the INCSC region,rather than the change of *** only considering the effect of climate change on GDP,the changes in precipitation extremes bring a larger impact on the economy in the future to the provinces of Hunan,Jiangxi,Fujian,Guangdong,and Hainan in South China,as well as the Malay Peninsula and southern Cambodia in ***,timely regional adaptation strategies are urgent for these ***,from the sub-regional average viewpoint,over two thirds of CMIP6 models agree that maintaining a lower global warming level will reduce the economic impacts from heavy precipitation over the INCSC region.

关键词： CMIP6 heavy precipitation extreme drought South China Indochina economic impact

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Effects of NLRP3 Inflammasome Mediated Pyroptosis on Cardiovascular Diseases and Intervention Mechanism of Chinese Medicine

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Chinese Journal of Integrative Medicine 2024年第5期30卷 468-479页

作者： ZHONG Yi LI Xin-yue LIANG Tian-jun DING Bao-zhu MA Ke-xin REN wen-xuan LIANG wen-jie College of Integrated Traditional Chinese and Western Medicine Hebei University of Chinese MedicineHebei Key Laboratory of Integrated Traditional Chinese and Western Medicine in Liver and Kidney DiseasesInstitute of Integrated Traditional Chinese and Western MedicineShijiazhuang 050200China Department of Cardiovascular Internal Medicine the Second Affiliated Hospital of Jiujiang UniversityJiujiangJiangxi Province 332000China Graduate School Hebei Medical UniversityShijiazhuang 050017China Rural Physician College Hebei Medical UniversityShijazhuang 050017China Medical Department the First Hospital of Hebei Medical UniversityShijiazhuang 050030China

Activation of the NOD-like receptor protein 3(NLRP3)inflammasome signaling pathway is an important mechanism underlying myocardial pyroptosis and plays an important role in inflammatory damage to myocardial tissue in patients with cardiovascular diseases(CVDs),such as diabetic cardiomyopathy,ischemia/reperfusion injury,myocardial infarction,heart failure and *** RNAs(nc RNAs)are important regulatory *** Chinese medicine(CM)compounds,including their effective components,can regulate pyroptosis and exert myocardium-protecting *** mechanisms underlying this protection include inhibition of inflammasome protein expression,Toll-like receptor 4–NF-κB signal pathway activation,oxidative stress,endoplasmic reticulum stress(ERS),and mixed lineage kinase 3 expression and the regulation of silent information regulator *** NLRP3 protein is an important regulatory target for CVD prevention and treatment with *** the effects of the interventions mediated by CM and the related mechanisms provides new ideas and perspectives for CVD prevention and treatment.

关键词： pyroptosis cardiovascular diseases Chinese medicine NOD-like receptor protein 3 mechanisms

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Dynamic synthetic analysis of circulation field of tropical cyclones affecting Shanghai

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Frontiers of Earth Science 2024年第2期18卷 347-363页

作者： wen GU Caijun yue Zhihui HAN Yanqing GAO Yuqi TANG Xiangyu AO Yao YAO Shanghai Ecological Forecasting&Remote Sensing Center Shanghai 200030China Shanghai Marine Meteorological Centre Shanghai 200030China Shanghai Typhoon Institute China Meteorological AdministrationShanghai 200030China Key Laboratory of Numerical Modeling for Tropical Cyclone(China Meteorological Administration) Shanghai 200030China

Eleven tropical cyclones(TCs)affected Shanghai and crossed the same latitude as Shanghai from 2007 to *** to similar tracks from best-track data,TCs that cause significant precipitation in Shanghai can be divided into three types:landfall TCs,nearshore northward TCs,and western *** on ERA5 reanalysis data,the dynamic synthesis method was used to synthesize TC circulation situations to compare thermal,dynamic,water vapor,and stability conditions within TC circulations during the period when they affected *** conclusions are as follows.1)When the three TC types are at the same latitude as Shanghai,they are all in the divergent field in the upper *** the landfall type,the subtropical high at 500 hPa is stronger and farther north than usual,and there is a high-pressure dam on the north side of the TCs.2)The warm advection of the three TC types at 925 hPa is located in the northern quadrant of the *** dynamic and water vapor conditions are good in the north-western quadrant of landfall and western TCs,and more favorable in the eastern quadrant of nearshore northward TCs.3)The favorable effects of all three types on precipitation in Shanghai come from the boundary *** vapor,upward motion,and instability conditions of landfall TCs are superior to the other two TC *** best water vapor,dynamic,and convective instability conditions are at the northern boundary in Shanghai during landfall TCs,and the main sources of water vapor in Shanghai come from the eastern and northern *** nearshore northward TCs,the main contribution to precipitation is from the eastern boundary,while better dynamic and water vapor conditions come from the western and northern boundaries during western *** above findings provide scientific and technical support for operational forecasting precipitation from TCs affecting mega-cities.

关键词： tropical cyclones dynamic synthetic analysis ERA5 reanalysis Shanghai similar track

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Solidification behaviour and hot cracking susceptibility of a novel Ni-based superalloy

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Journal of Iron and Steel Research International 2024年第4期31卷 956-966页

作者： yue Chen Shao-min Lv Xing-fei Xie Xiao-can wen Jng-long Qu Jin-hui Du High-Temperature Materials Institute China Iron and Steel Research Institute Group Co.Ltd.Beijing 100081China Beijing GAONA Materials and Technology Co. Ltd.Beijing 100081China Sichuan CISRI-GAONA Forging Co. Ltd.Deyang 610000SichuanChina

A novel Ni-based superalloy GH4151,with a γ′ volume fraction of about 55%and a service temperature capability up to 8oo oC,was *** to the different cooling conditions of various regions during the solidification of ingots,significant cooling rate variations may lead to the occurrence of hot *** scanning laser microscope was utilised to investigate the solidification process and phase precipitation behaviour of the GH4151 under wide range cooling *** characteristics of L→γ transformation were analysed,and the growth rates of at each stage were *** segregation behaviour was predicted using the Scheil equation,and the predicted results match well with the experimental *** sensitivity coefficient for hot cracking was modified,and cracking sensitivity coefficient values for the alloy under different cooling rates were computed,revealing that the alloy is most susceptible to hot cracking at 10℃/min cooling ***,controlling the cooling rate can reduce the possibility of hot cracking in ingot.

关键词： Ni-based superalloy Solidification behaviour In-situ observation Clyne and Davies's criterion:Hot cracking susceptibility

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