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Global air-sea CO_(2) exchange fl ux since 1980s: results from CMIP6 Earth System Models

Journal of Oceanology and Limnology 2022年第4期40卷 1417-1436页

作者： Baoxiao QU Jinming SONG Xuegang LI huamao yuan Kun ZHANG Suqing XU Key Laboratory of Marine Ecology and Environmental Sciences Institute of OceanologyChinese Academy of SciencesQingdao 266071China Marine Ecology and Environmental Sciences Laboratory Pilot National Laboratory for Marine Science and Technology(Qingdao)Qingdao 266237China University of Chinese Academy of Sciences Beijing 100049China Center for Ocean Mega-Science Chinese Academy of SciencesQingdao 266071China Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of SciencesQingdao 266071China Key Laboratory of Global Change and Marine-Atmospheric Chemistry Third Institute of OceanographyMinistry of Natural ResourcesXiamen 361005China

The ocean could profoundly modulate the ever-increasing atmospheric CO_(2) by air-sea CO_(2) exchange process,which is also able to cause signifi cant changes of physical and biogeochemical properties in *** this study,we assessed the long-term average and spatial-temporal variability of global air-sea CO_(2) exchange fl ux(F CO_(2))since 1980s basing on the results of 18 Coupled Model Intercomparison Project Phase 6(CMIP6)Earth System Models(ESMs).Our fi ndings indicate that the CMIP6 ESMs simulated global CO_(2) sink in recent three decades ranges from 1.80 to 2.24 Pg C/a,which is coincidence with the results of cotemporaneous ***’s more,the CMIP6 ESMs consistently show that the global oceanic CO_(2) sink has gradually intensifi ed since 1980s as well as the *** study confi rms the simulated F CO_(2) could reach agreements with the observations in the aspect of primary climatological characteristics,however,the simulation skills of CIMP6 ESMs in diverse open-sea biomes are *** of the 18 CMIP6 ESMs could reproduce the observed F CO_(2) increasement in the central-eastern tropical Pacifi c and the midlatitude Southern *** ciencies of some CMIP6 ESMs in reproducing the atmospheric pressure systems of the Southern Hemisphere and the El Niño-Southern Oscillation(ENSO)mode of the tropical Pacifi c are probably the major causes.

关键词： air-sea CO_(2)fl ux Coupled Model Intercomparison Project Phase 6(CMIP6) Earth System Model(ESM) long-term average spatial-temporal variability

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Prokaryotic diversity and community composition in the surface sediments of the Changjiang River Estuary in summer

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Acta Oceanologica Sinica 2023年第9期42卷 113-124页

作者： Changfeng Qu Xixi Wang Liping Zhang huamao yuan Xuegang Li Ning Li Fushan Chen Jinlai Miao Key Laboratory of Marine Eco-Environmental Science and Technology First Institute of OceanographyMinistry of Natural ResourcesQingdao 266061China CAS Key Laboratory of Marine Ecology and Environmental Sciences Institute of OceanologyChinese Academy of SciencesQingdao 266071China College of Chemistry and Molecular Engineering Qingdao University of Science and TechnologyQingdao 266042China Marine Natural Products R&D Laboratory Qingdao Key LaboratoryQingdao 266061China

Microorganisms are fundamental for the functioning of marine ecosystems and are involved in the decomposition of organic matter, transformation of nutrients and circulation of biologically-important chemicals. Based on the complexity of the natural geographic characteristics of the Changjiang River Estuary, the geographic distribution of sedimentary microorganisms and the causes of this distribution are largely unexplored. In this work, the surface sediment samples from the adjacent sea area of the Changjiang River Estuary were collected. Their prokaryotic diversity was examined by high-throughput sequencing technology, and the environmental factors of the bacterial community were investigated. The results indicated that the distribution of prokaryotic communities in the sediments of the study areas showed obvious spatial heterogeneity. The sampling sequences divided the sample regions into three distinct clusters. Each geographic region had a unique community structure, although Proteobacteria, Bacteroidota, Desulfobacterota, Acidobacteriota, and Actinobacteriota all existed in these three branches. Canonical correspondence analysis demonstrated that prokaryotic diversity and community distribution were significantly correlated with the geographic location of sediment, seawater depth, and in particular, nutrient content(e.g., total phosphorus, total organic carbon and dissolved oxygen). Moreover, it was found for the first time that the metal ions obviously affected the composition and distribution of the prokaryotic community in this area. In general, this work provides new insights into the structural characteristics and driving factors of prokaryotic communities under the background of the ever-changing Changjiang River Estuary.

关键词： prokaryotic diversity 16S rRNA gene geophysicochemical factors high-throughput sequencing(HTS) Changjiang River Estuary

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水环境中新污染物的分离富集与测定——以磺胺类合成药物为例

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海洋科学 2024年第2期48卷 88-101页

作者：戴佳佳宋金明李学刚马骏袁华茂段丽琴温丽联中国科学院海洋研究所中国科学院海洋生态与环境科学重点实验室山东青岛266071 青岛海洋科学与技术试点国家实验室海洋生态与环境科学功能实验室山东青岛266237 中国科学院大学北京100049 中国科学院海洋大科学研究中心山东青岛266071

作为新污染物的磺胺类(Sulfonamides,SAs)是应用最早的一类人工合成抗菌药物,被广泛应用于人类、农业、畜牧业和水产养殖。进入体内的磺胺类合成药物随代谢排入水环境中,对水生生态系统和人类健康构成潜在威胁。环境中磺胺类合成药物的... 详细信息

作为新污染物的磺胺类(Sulfonamides,SAs)是应用最早的一类人工合成抗菌药物,被广泛应用于人类、农业、畜牧业和水产养殖。进入体内的磺胺类合成药物随代谢排入水环境中,对水生生态系统和人类健康构成潜在威胁。环境中磺胺类合成药物的准确分析测定是探析其环境生物地球化学特性的基础,近年来,随着科学技术的进步,已构建了适于水环境中痕量磺胺类合成药物的快速灵敏测定方法,特别是样品的前处理与分离富集技术有了跨越式的发展。总结归纳了近年来水环境中磺胺类合成药物的样品前处理技术以及分析方法的研究进展,分析了不同环境样品前处理技术和分析方法的优缺点,在此基础上,前瞻分析了水环境磺胺类合成药物分析测定的发展思路。具有回收率高、选择性强、重现性好、成本低、环境友好及可自动化等优势的固相萃取(Solid phase extraction,SPE)作为液相萃取(Liquid-liquid extraction,LLE)的替代方法,现已被广泛应用于水环境中痕量磺胺类合成药物的分离和富集,随着新型吸附剂材料的发展,SPE的灵敏度和选择性得到了明显提升。液相色谱(Liquid chromatography,LC)与串联质谱(Tandem mass spectrometry,MS/MS)联用技术是目前磺胺类合成药物的主要定量分析方法,具有检测限低、灵敏度高、多种目标物的同时检测及重现性好等优点。未来应从重点关注磺胺类代谢产物及降解产物在水环境中残留的角度,开发更为操作简单、快速且灵敏的分析测定方法,以便更有效地监管水环境中人工合成药物的生态环境效应。

关键词：磺胺类合成药物(SAs) 样品前处理固相萃取水环境液质质谱测定(LC-MS/MS)

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Compositional characteristics of sediment from Jiaozhou Bay in North China and the implication to the provenance

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Journal of Oceanology and Limnology 2023年第5期41卷 1729-1741页

作者： Ziwei SUN Jin LIU Yue ZHANG Jinming SONG yuanyuan XIAO huamao yuan Ning LI Xuegang LI College of Chemistry and Molecular Engineering College of Marine Science and Biological EngineeringQingdao University of Science and TechnologyQingdao 266042China Public Technology Service Center Institute of OceanologyChinese Academy of SciencesQingdao 266071China Key Laboratory of Marine Ecology&Environmental Sciences Institute of OceanologyChinese Academy of SciencesQingdao 266071China Center for Ocean Mega-Science Chinese Academy of SciencesQingdao 266071China Qingdao National Laboratory for Marine Science and Technology Qingdao 266061China Key Laboratory of Marine Geology and Environment Institute of OceanologyChinese Academy of SciencesQingdao 266071China

Rare earth elements(REEs)can be used to trace source materials and identify their provenances,because of significant conservation and immobility during chemical alteration processes after erosion of materials from the *** study focused on the temporal variation of REEs for columnar sediments from the mouth of Jiaozhou Bay in North China to understand the potential controls for the geochemical variations of *** extraction experiments,we identified that the residual fraction is the main host for REEs compared with other fractions(i.e.,exchangeable and carbonate fraction,easily reducible oxides fraction,reducible oxides fraction,magnetite fraction).REE ratios(e.g.,La_(N)/Sm_(N)and La_(N)/Yb_(N);N:normalized by chondrite)lack correlations with grain size or the chemical index of alteration(CIA),which is correlated with major *** these indicate that these REE variations reflect the varying contribution of source materials from different provenances instead of grain size or chemical weathering *** ratios(e.g.,La_(N)/Sm_(N)and La_(N)/Yb_(N))remain relatively constant until the depth of roughly 40 cm(equivalent to the year 1995),and show obvious changes beyond this *** REE characteristics of Jiaozhou Bay with those of neighboring rivers and bedrocks,the relative contributions of Dagu River-Jiaolai River,and Licun River may have been increased during the sedimentary processes,which could be caused by the construction of reservoir and related change of aquaculture(e.g.,rapid accumulation of organic materials).

关键词： Jiaozhou Bay sediments rare earth elements(REEs) sequential extraction provenance

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我国近海生态环境灾害发生的生源要素驱动机制及健康调控

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应用生态学报 2024年第2期35卷 564-576页

作者：邢建伟宋金明袁华茂李学刚段丽琴曲宝晓王启栋马骏王越奇戴佳佳中国科学院海洋研究所中国科学院海洋生态与环境科学重点实验室山东青岛266071 中国科学院大学海洋学院山东青岛266400 中国科学院海洋大科学研究中心山东青岛266400

近几十年来,我国近海生态环境在气候变化和高强度人类活动等多重压力下发生重大变化,以赤潮和绿潮为代表的有害藻华发生次数和规模呈快速增长态势,同时海水低氧和酸化等环境问题也日渐突出,迫切需要探明海洋生态环境灾害的发生机制和防... 详细信息

近几十年来,我国近海生态环境在气候变化和高强度人类活动等多重压力下发生重大变化,以赤潮和绿潮为代表的有害藻华发生次数和规模呈快速增长态势,同时海水低氧和酸化等环境问题也日渐突出,迫切需要探明海洋生态环境灾害的发生机制和防治措施。本文首次阐明“海洋生态环境灾害”概念的内涵,并从营养物质外源输入、海洋有机质矿化分解与营养盐再生、近海水体营养盐结构异常等方面系统阐释了我国近海生态环境灾害发生的生源要素驱动机制,指出日益增强的人类活动引发的陆源营养物质输入剧增以及生源要素入海后的复杂生物地球化学循环过程共同导致近海生态环境灾害的频发。在此基础上,结合本领域最新研究进展,提出了基于海水生源要素管理的近海生态环境健康调控思路。即基于陆海一体化战略,通过技术手段,从陆源减排、海岸带缓冲和近海治理链条式降低陆源污染物特别是无机氮的排放强度,并通过人为调控技术促进近海海水营养盐结构的正常化,从而达到降低和控制近海生态环境灾害发生的目的,改善和提升近海生态环境质量。

关键词：海洋生态环境灾害营养盐调控陆海统筹生态环境健康中国近海

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Organic carbon source and burial during the past one hundred years in Jiaozhou Bay,North China

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Journal of Environmental Sciences 2008年第5期20卷 551-557页

作者： LI Xuegang yuan huamao LI Ning SONG Jinming Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China.

Organic carbon （OC）, total nitrogen （TN）, and ^210Pb in core sediment were measured to quantify the burial of organic carbon and the relative importance of allochthonous and autochthonous contributions during the past one hundred years in Jiaozhou Bay, North China. The core sediment was dated using ^210Pb chronology, which is the most promising method for estimation of sedimentation rate on a time scale of 100-150 years. The variation of the burial flux of organic carbon in the past one hundred years can be divided into the following three stages：（1） relatively steady before 1980s; （2） increasing rapidly from the 1980s to a peak in the 1990s, and （3） decreasing from the 1990s to the present. The change is consistent with the amount of solid waste and sewage emptied into the bay. The OC：TN ratio was used to evaluate the source of organic carbon in the Jiaozhou Bay sediment. In the inner bay and bay mouth, the organic carbon was the main contributor from terrestrial sources, whereas only about half of organic carbon was contributed from terrestrial source in the outer bay. In the inner bay, the terrestrial source of organic carbon showed a steady change with an increase in the range of 69%-77% before 1990 to 93% in 2000, and then decreased from 2000 because of the decrease in the terrestrial input. In the bay mouth, the percentage of organic carbon from land reached the highest value with 94% in 1994. In the outer bay, the sediment source maintained steady for the past one hundred years.

关键词： organic carbon source burial Jiaozhou Bay

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One century record of contamination by polycyclic aromatic hydrocarbons and polychlorinated biphenyls in core sediments from the southern Yellow Sea

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Journal of Environmental Sciences 2009年第8期21卷 1080-1088页

作者： ZHANG Peng SONG Jinming FANG Jie LIU Zhigang LI Xuegang yuan huamao Key Laboratory Marine Ecology and Environmental Sciences Institute of Oceanology Chinese Academy of Scienees Qingdao 266071 China The Graduate University of Chinese Academy of Sciences Beijing 100039 China Zhejiang Zhoushan Marine Ecological Environmental Monitoring Station Zhoushan 316004 China

Sixteen polycyclic aromatic hydrocarbons （PAHs） and 28 polychlorinated biphenyls （PCBs） were measured at a 2-cm interval in a core sample from the middle of the southern Yellow Sea for elucidating their historical variations in inflow and sources. The chronology was obtained using the ^210Pb method. PAHs concentrations decreased generally with depth and two climax values occurred in 14-16 cm and 20-22 cm layers, demonstrating that the production and usage of PAHs might reach peaks in the periods of 1956-1962 and 1938-1944. The booming economy and the navy battles of the Second World War might explain why the higher levels were detected in the two layers. The result of principal component analysis （PCA） revealed that PAHs were primarily owing to the combustion product. Down-cored variation of PCB concentrations was complex. Higher concentrations besides the two peaks being the same as PAHs were detected from 4 to 8 cm, depositing from 1980 to 1992, which probably resulted from the disposal of the out-dated PCB-containing equipment. The average Cl percentage of PCBs detected was similar to that of the mixture of Aroclor 1254 and 1242, suggesting they might origin from the dielectrical and heat-transfer fluid. The total organic carbon （TOC） content played a prevalent role in the adsorption of high molecular weight PAHs （≥ring）, while no obvious relationship among total PCBs, the concentration of congeners, and TOC was found.

关键词： PAHs PCBs the southern Yellow Sea contamination history

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Dissolved barium as a tracer of Kuroshio incursion in the Kuroshio region east of Taiwan Island and the adjacent East China Sea

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Science China Earth Sciences 2017年第7期60卷 1356-1367页

作者： LIU Wei SONG JinMing yuan huamao LI Ning LI XueGang DUAN LiQin Chinese Academy of Sciences Key Laboratory of Marine Ecology and Environmental Sciences Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China University of Chinese Academy of Sciences Beijing 100049 China Shandong Analysis and Test Center Jinan 250014 China Laboratory for Marine Ecology and Environmental Sciences Qingdao National Laboratory for Marine science and Technology Qingdao 266237 China

From May to June 2014, the geochemical characteristics of dissolved barium(Ba) in sea water and its influx from the Kuroshio into the East China Sea(ECS) were studied by investigation of the Kuroshio mainstream east of Taiwan Island and the adjacent ECS. This allowed for the scope and extent of the Kuroshio incursion to be quantitatively described for the first time by using Ba as a tracer. The concentration of Ba in the Kuroshio mainstream increased gradually downward from the surface in the range 4.91–19.2 μg L.1. In the surface layer of the ECS, the Ba concentration was highest in coastal water and gradually decreased seaward, while it was higher in coastal and offshore water but lowest in middle shelf for bottom layer. The influx of Ba from Kuroshio into the ECS during May to October was calculated to be 2.19×108 kg by a water exchange model, in which the subsurface layer had the largest portion. The distribution of Ba indicated that Kuroshio upwelled in the sea area northeast of Taiwan Island. The north-flowing water in the Taiwan Strait restrained the incursion of Kuroshio surface water onto the ECS shelf, while Kuroshio subsurface water gradually affected the bottom of the ECS from outside. The results of end member calculation, using Ba as a parameter, showed that the Kuroshio surface water had little impact on the ECS, while the Kuroshio subsurface water formed an intrusion current by climbing northwest along the bottom of the middle shelf from the sea area northeast of Taiwan Island into the Qiantang Estuary, of which the volume of Kuroshio water was nearly 65%. Kuroshio water was the predominant part of the water on the outer shelf bottom and its proportion in areas deeper than the 100 m isobath could reach more than 95%. In the DH9 section(north of Taiwan Island), Kuroshio subsurface water intruded westward along the bottom from the shelf edge and then rose upward(in lower proportion). Kuroshio water accounted for 95% of the ocean volume could reach as f

关键词： Dissolved barium Tracer Geochemical characteristics Kuroshio incursion The ECS shelf

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Carbon sinks/sources in the Yellow and East China Seas Air-sea interface exchange, dissolution in seawater, and burial in sediments

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Science China Earth Sciences 2018年第11期61卷 1583-1593页

作者： Jinming SONG Baoxiao QU Xuegang LI huamao yuan Ning LI Liqin DUAN Key Laboratory of Marine Ecology and Environmental Sciences Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China Function Laboratory of Marine Ecology and Environmental Sciences Qingdao National Laboratory for Marine Science and Technology Qingdao 266237 China University of Chinese Academy of Sciences Beijing 100049 China Center for Ocean Mega-Science Chinese Academy of Sciences Qingdao 266071 China

The sinks/sources of carbon in the Yellow Sea(YS) and East China Sea(ECS), which are important continental shelf seas in China, could exert a great influence on coastal ecosystem dynamics and the regional climate change process. The CO_2 exchange process across the seawater-air interface, dissolved and particulate carbon in seawater, and carbon burial in sediments were studied to understand the sinks/sources of carbon in the continental shelf seas of China. The YS and the ECS generally have different patterns of seasonal air-sea CO_2 exchange. In the YS, regions west of 124°E can absorb CO_2 from the atmosphere during spring and winter, and release CO_2 to the atmosphere during summer and autumn. The entire YS is considered as a CO_2 source throughout the year with respect to the atmosphere, but there are still uncertainties regarding the exact air-sea CO_2 exchange flux. Surface temperature and phytoplankton production were the key controlling factors of the air-sea CO_2 exchange flux in the offshore region and nearshore region of the YS, respectively. The ECS can absorb CO_2 during spring, summer, and winter and release CO_2 to the atmosphere during autumn. The annual average exchange rate in the ECS was-4.2±3.2 mmol m^(-2) d^(-1) and it served as an obvious sink for atmospheric CO_2 with an air-sea exchange flux of 13.7×10~6 t. The controlling factors of the air-sea CO_2 exchange in the ECS varied significantly seasonally. Storage of dissolved inorganic carbon(DIC) and dissolved organic carbon(DOC) in the YS and the ECS were 425×10~6 t and 1364×10~6 t, and 28.2×10~6 t and 54.1×10~6 t,respectively. Long-term observation showed that the DOC content in the YS had a decreasing trend, indicating that the "practical carbon sink" in the YS was decreasing. The total amount of particulate organic carbon(POC) stored in the YS and ECS was10.6×10~6 t, which was comparable to the air-sea CO_2 flux in these two continental shelf seas. The amounts of carbon sequestered by phyto

关键词： Sink/source of carbon Air-sea CO2 exchange Dissolved inorganic carbon Dissolved organic carbon Particulateorganic carbon Sediment Yellow Sea East China Sea

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The bacterial diversity and community composition altered in the oxygen minimum zone of the Tropical Western Pacific Ocean

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Journal of Oceanology and Limnology 2021年第5期39卷 1690-1704页

作者： Qiqi SUN Jinming SONG Xuegang LI huamao yuan Qidong WANG Shandong Peanut Research Institute Qingdao 266100China Key Laboratory of Marine Ecology and Environmental Sciences Institute ofOceanologyChinese Academy of SciencesQingdao 266071China Laboratory for Marine Ecology and Environmental Science Pilot NationalLaboratory for Marine Science and Technology(Qingdao)Qingdao 266237China University of Chinese Academy of Sciences Beijing 100049China Center for Ocean Mega-Science Chinese Academy of SciencesQingdao266071China

The oxygen minimum zones(OMZs)are globally expanding,yet the variation pattern of microbial communities related to dissolved oxygen levels remain *** variability of bacterial diversity and community composition(repre sented by 16 S rRNA)of six stations was investigated within the water column in the seamount area of Tropical Western Pacific Ocean(TWPO)in May *** seawater has dissolved oxygen(DO)concentration of 3.01-6.68 mg/L and the core of the oxygen minimum zones was located between the depths of 650 m and 1750 *** bacterial alpha-diversity showed unimodal pattern with the decreasing DO with depths and peaked in the upper oxycline(UO)of *** bacterial community structure of the mixed layer(ML)and the bottom layer clustered and separated from each other,while those of UO and the OMZ core(OM)clustered and ***,bacterial community composition transitioned from being Alphaproteobacteria and Gammaproteobacteria-dominant in ML to being Gammaproteobacteria and Nitrososphaeria/Deltaproteobacteria-dominant in UO and OM,and then changed to being Clostridia and unidentified Actinobacteria-dominant in the bottom ***,both bacterial alpha-diversity and the abundant classes fitted varying sectioned functions with *** DO solely explained 40.37%of the variation of bacterial community composition among layers(P<0.001).The predicted function profiling showed that the water column was predominant by chemoheterotrophy,cyanobacteria,and photoautotrophy in ML,by chemoheterotrophy and nitrate/sulfide cycling in UO and OM,and by chemoheterotrophy and ferme ntation in the bottom *** findings revealed the DO-associated variation in bacterial diversity and community composition,and help to clarify the potential responses of microbes and their involved biogeochemical processes to the expansion and intensification of OMZs.

关键词： bacterial diversity community composition oxygen minimum zones(OMZs) dissolved oxygen Tropical Western Pacific Ocean(TWPO)

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