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Collaboratively enhancing electrochemical properties of liNi_(0.83)Co_(0.11)Mn_(0.06)O_(2) through doping and coating of quadrivalent elements

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Rare Metals 2023年第12期42卷 4103-4114页

作者： Zhao-Zhe Yu Gui-Quan Zhao Fang-li Ji Hao Tong Qi-lin Tong hua-cheng li Yan cheng Guangxi Key Laboratory of Manufacturing Systems and Advanced Manufacturing Technology Guilin University of Electronic TechnologyGuilin 541004China Engineering Research Center of Electronic Information Materials and Devices Ministry of EducationGuilin University of Electronic TechnologyGuilin 541004China Guangxi CNGR New Energy Science&Technology Co. Ltd.Qinzhou 535000China

Ni-rich layered oxides(Ni>80%)with high energy density have become a mainstream cathode material for li-ion ***,irreversible phase transitions and interface instability are deep-seated challenges in commercializing Ni-rich *** study used a collaborative modification strategy involving doping and coating with quadrivalent elements to construct Ni-rich *** particular,introducing tetravalent Zr makes the valence change of Ni(2+to 4+)more accessible to complete spontaneously during the charging and discharging processes,which significantly suppresses the cationic mixing and irreversible phase transition(H2?H3).Combining the strategy of constructing CeO_(2) coatings on the surface and interfacial spinel-like phases improves the li+diffusion kinetics and interfacial ***,part of the strongly oxidizing four-valence Ce^(4+)diffuses to the surface layer,further increasing the average valence state of ***,liNi_(0.83)Co_(0.11)Mn_(0.06)O_(2)(NCM)-Zr@Ce achieves 78.5%outstanding retention at1.0C after 200 cycles within 3.0-4.3 V compared to unmodified NCM with 41.4%*** improved cyclic stability can be attributed to the collaborative modification strategy of the quadrivalent elements,which provides an effective synergistic modification strategy for developing high-performance li-ion battery cathode materials.

关键词： Collaborative modification strategy Quadrivalent elements Phase transitions Structural degradation Ni-rich layered oxides

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Effect of Mn and Mo on microstructure and mechanical properties of Al-Si-Cu-Mg-0.6Fe alloy

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China Foundry 2023年第6期20卷 511-518页

作者： Hao He Jing Zou Hai-tao Zhang Da-chuan Hu Zhi-jun Feng Yu-fei li Ze-hua li hua-cheng li National Key Laboratory of Advanced Casting Technologies Shenyang 110022China Key Laboratory of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang 110819China

Effect of different Mn and Mo contents on microstructure and mechanical properties of Al-Si-Cu-Mg-0.6Fe alloy was *** indicate that the increase of Mo and decrease of Mn lead to a decrease in the size of theα-Al_(15)(FeMnMo)_(3)Si_(2) phase formed during ***α-Al_(15)(FeMnMo)_(3)Si_(2) phase reaches a minimum value of about 16.3μm at 0.2wt.%Mo and 0.1wt.%Mn *** solution treatment,theα-Al(FeMnMo)Si dispersed phase is *** only Mn is added,theα-Al(FeMnMo)Si dispersed phase mainly distributes near the grain boundaries,while when only Mo is added,it primarily distributes in the central region of the *** both Mn and Mo are added,the dispersed phase has a larger and denser dispersed region and is uniformly distributed near the Al matrix and grain ***,the best overall mechanical properties of the alloy are obtained with the combined addition of 0.1wt.%Mn and 0.2wt.%Mo,due to the smaller size ofα-Al_(15)(FeMnMo)_(3)Si_(2) phase and the larger area fraction and higher density of theα-Al(FeMnMo)Si dispersed *** yield strength,ultimate tensile strength,and elongation are respectively improved 67.7 MPa,48.5 MPa and 5.3%,respectively,compared to that of the alloy with only 0.3wt.%Mn.

关键词： Al-Si-Cu-Mg-0.6Fe alloy Mn and Mo microstructure mechanical properties solution treatment

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Lunar cratering asymmetries with high lunar orbital obliquity and inclination of the Moon

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Research in Astronomy and Astrophysics 2021年第6期21卷 281-293页

作者： hua-cheng li Nan Zhang Zong-Yu Yue Yi-Zhuo Zhang Key Laboratory of Orogenic Belts and Crustal Evolution School of Earth and Space SciencesPeking UniversityBeijing 100871China Earth Dynamics Research Group School of Earth and Planetary SciencesCurtin University6102 WAAustralia State Key Laboratory of Remote Sensing Science Aerospace Information Research InstituteChinese Academy of SciencesBeijing 100101China

Accurate estimation of cratering asymmetry on the Moon is crucial for understanding Moon evolution *** studies of cratering asymmetry have omitted the contributions of high lunar obliquity and ***,we include lunar obliquity and inclination as new controlling variables to derive the cratering rate spatial variation as a function of longitude and *** examining the influence of lunar obliquity and inclination on the asteroids population encountered by the Moon,we then have derived general formulas of the cratering rate spatial variation based on the crater scaling *** formulas with addition of lunar obliquity and inclination can reproduce the lunar cratering rate asymmetry at the current Earth-Moon distance and predict the apex/ant-apex ratio and the pole/equator ratio of this lunar cratering rate to be 1.36 and 0.87,*** apex/ant-apex ratio is decreasing as the obliquity and inclination *** with the evolution of lunar obliquity and inclination,our model shows that the apex/ant-apex ratio does not monotonically decrease with Earth-Moon distance and hence the influences of obliquity and inclination are not negligible on evolution of apex/ant-apex *** model is generalizable to other planets and moons,especially for different spin-orbit resonances.

关键词： Moon meteorites meteors meteoroids planets and satellites:surfaces

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Choline dehydrogenase interacts with SQSTM1 to activate mitophagy and promote coelomocyte survival in Apostichopus japonicus following Vibrio splendidus infection

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动物学研究(英文) 2023年第5期44卷 905-918页

作者： lian-lian Sun Ying-Fen Dai Mei-Xiang You cheng-hua li State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Ningbo UniversityNingboZhejiang 315211China Laboratory for Marine Fisheries Science and Food Production Processes Qingdao National Laboratory for Marine Science and TechnologyQingdaoShandong 266071China

Previous studies have shown that Vibrio splendidus infection causes mitochondrial damage in Apostichopus japonicus coelomocytes,leading to the production of excessive reactive oxygen species(ROS)and irreversible apoptotic cell *** evidence suggests that mitochondrial autophagy(mitophagy)is the most effective method for eliminating damaged mitochondria and ROS,with choline dehydrogenase(CHDH)identified as a novel mitophagy receptor that can recognize non-ubiquitin damage signals and microtubule-associated protein 1 light chain 3(LC3)in ***,the functional role of CHDH in invertebrates is largely *** this study,we observed a significant increase in the mRNA and protein expression levels of *** CHDH(AjCHDH)in response to *** infection and lipopolysaccharide(LPS)challenge,consistent with changes in mitophagy under the same ***,AjCHDH was localized to the mitochondria rather than the cytosol following *** ***,AjCHDH knockdown using si RNA transfection significantly reduced mitophagy levels,as observed through transmission electron microscopy and confocal *** investigation into the molecular mechanisms underlying CHDH-regulated mitophagy showed that AjCHDH lacked an LC3-interacting region(liR)for direct binding to LC3 but possessed a FB1 structural domain that binds to *** interaction between AjCHDH and SQSTM1 was further confirmed by immunoprecipitation ***,laser confocal microscopy indicated that SQSTM1 and LC3 were recruited by AjCHDH in coelomocytes and HEK293T *** contrast,AjCHDH interference hindered SQSTM1 and LC3 recruitment to the mitochondria,a critical step in damaged mitochondrial ***,AjCHDH interference led to a significant increase in both mitochondrial and intracellular ROS,followed by increased apoptosis and decreased coelomocyte ***,these findings indicate that AjCHDH-mediated mitophagy plays a

关键词： Choline dehydrogenase Mitophagy SQSTM1 Microtubule-associated protein 1 light chain 3 Apostichopus japonicus

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ROS-mediated BNIP3-dependent mitophagy promotes coelomocyte survival in Apostichopus japonicus in response to Vibrio splendidus infection

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Zoological Research 2022年第2期43卷 285-300页

作者： lian-lian Sun Yi-Na Shao Mei-Xiang You cheng-hua li State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Ningbo UniversityNingboZhejiang 315211China Laboratory for Marine Fisheries Science and Food Production Processes Qingdao National Laboratory for Marine Science and TechnologyQingdaoShandong 266071China State-Province Joint Laboratory of Marine Biotechnology and Engineering Ningbo UniversityNingboZhejiang 315211China

Organisms produce high levels of reactive oxygen species(ROS)to kill pathogens or act as signaling molecules to induce immune responses;however,excessive ROS can result in cell *** maintain ROS balance and cell survival,mitophagy selectively eliminates damaged mitochondria via mitophagy receptors in *** marine invertebrates,however,mitophagy and its functions remain largely *** the current study,Vibrio splendidus infection damaged mitochondrial morphology in coelomocytes and reduced mitochondrial membrane potential(ΔΨm)and mitophagosome *** colocalization of mitochondria and lysosomes further confirmed that lipopolysaccharide(LPS)treatment increased mitophagy *** explore the regulatory mechanism of mitophagy,we cloned Bcl2/adenovirus E1 B 19 kDa protein-interacting protein 3(BNIP3),a common mitophagy receptor,from sea cucumber Apostichopus japonicus(Aj BNIP3)and confirmed that Aj BNIP3 was significantly induced and accumulated in mitochondria after *** infection and LPS *** the mitochondrial membrane,Aj BNIP3 interacts with microtubule-associated protein 1 light chain 3(LC3)on phagophore membranes to mediate *** Aj BNIP3 interference,mitophagy flux decreased ***,Aj BNIP3-mediated mitophagy was activated by ROS following the addition of exogenous hydrogen peroxide(H2 O2),ROS scavengers,and ROS ***,inhibition of BNIP3-mediated mitophagy by Aj BNIP3 small interfering RNA(si RNA)or high concentrations of lactate increased apoptosis and decreased coelomocyte *** findings highlight the essential role of Aj BNIP3 in damaged mitochondrial degradation during *** mitophagy activity is required for coelomocyte survival in *** against *** infection.

关键词： Apostichopus japonicus Mitophagy Bcl2/adenovirus E1B 19 kDa protein-interacting protein 3 Reactive oxygen species Microtubule-associated protein 1 light chain 3

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Microstructure and property of laser additive manufactured alloy Ti-6Al-2V-1.5Mo-0.5Zr-0.3Si after aged at different temperatures

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Rare Metals 2024年第5期43卷 2275-2281页

作者： Guo-Chao li Xu cheng hua-Ming Wang National Engineering Laboratory of Additive Manufacturing for Large Metallic Components and Engineering Research Center of Ministry of Education on Laser Direct Manufacturing for Large Metallic Components School of Materials Science and EngineeringBeihang UniversityBeijing 100191China

The solid solution and aging treatment for conventional manufacturing processes might not be suitable for laser additive manufactured titanium alloys due to the different lamellar *** this study,the influence of aging temperatures(600,700 and 800°C)on microstructure and mechanical properties of titanium alloy Ti-6Al-2V-1.5Mo-0.5Zr-0.3Si was *** results indicate that after solid solution treatment at 970°C followed by water quenching,the alloy mainly consists of coarsening lamellar a phase in martensite α' *** at 600°C will not change the size of primary lamellar α phase but lead to huge amount of secondary a phases(α_(s))generating with very fine *** increasing the aging temperature,the number of α_(s) decreases but with coarsened *** aged at 800°C,the width of the asphase reaches 350 nm,almost 7 times wider than that aged at 600°*** changing size of α_(s) obviously influences the property of the *** fine α_(s) leads to high strength and microhardness but low plasticity,and specimen aged at 700°C with suitable assize has the best comprehensive properties.

关键词： α+βtitanium alloy Laser additive manufacturing Solid solution and aging treatment Microstructure Room temperature tensile property

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Improving anammox activity and reactor start-up speed by using CO_(2)/NaHCO_(3) buffer

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Journal of Environmental Sciences 2024年第5期139卷 60-71页

作者： Shaoan cheng huahua li Xinyuan He hua Chen Longxin li State Key Laboratory of Clean Energy Utilization College of Energy EngineeringZhejiang UniversityHangzhou 310027China

Anammox bacteria grow slowly and can be affected by large pH *** suitable buffers could make the start-up of anammox reactors easy and *** this study,the effects of three kinds of buffers on the nitrogen removal and growth characteristics of anammox sludge were *** with CO_(2)/NaHCO_(3)buffer solution(CCBS)performed the best in nitrogen removal,while 4-(2-hydroxyerhyl)piperazine-1-ethanesulfonic acid(HEPES)and phosphate buffer solution(PBS)inhibited the anammox *** with 50 mmol/L CCBS could start up in 20 days,showing the specific anammox activity and anammox activity of 1.01±0.10 gN/(gVSS·day)and 0.83±0.06 kgN/(m^(3)·day),*** Kuenenia was the dominant anammox bacteria,with a relative abundance of 71.8%.Notably,anammox reactors could also start quickly by using 50 mmol/L CCBS under nonstrict anaerobic *** findings are meaningful for the quick start-up of engineered anammox reactors and prompt enrichment of anammox bacteria.

关键词： Anammox bacteria Buffer solution CO_(2)/NaHCO_(3) Physiological characteristics Microbial community shift

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Two new phenolic glycosides from the aerial parts of Androsace umbellata

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Chinese Chemical Letters 2009年第7期20卷 836-838页

作者： Zhi Qi Yin cheng hua li Ying Wang Wen Cai Ye Jian Zhang Department of Phytochemistry China Pharmaceutical University Nanfing 210009 China Institute of life and Health Engineering Jinan University Guangzhou 510632 China Institute of Traditional Chinese Medicine and Natural Products Jinan University Guangzhou 510632 China Plant Resources and Chemistry of Traditional Chinese Medicine Jiangsu Provincial Academy of-Traditional Chinese Medicine Nanjing 210028 China

Two new phenolic glycosides, 2-hydroxy-4-O-β-D-glucopyranosylphenylacetic acid methyl acetate （1） and 2-hydroxy-4-O-β-D- glucopyranosylphenylacetic acid （2） were isolated from the aerial parts ofAndrosace umbellata. Their structures were elucidated by spectral techniques. C 2009 Wen Cai Ye. Published by Elsevier B.V. on behalf of Chinese Chemical Society. All rights reserved.

关键词： Androsace umbellata Phenolic glycosides Phenylacetic acid

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Dissipationless layertronics in axion insulator MnBi2Te4

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National Science Review 2024年第6期11卷 189-196页

作者： Shuai li Ming Gong Shuguang cheng hua Jiang X.C.Xie School of Physical Science and Technology Soochow University Institute for Advanced Study Soochow University International Center for Quantum Materials School of Physics Peking University Department of Physics Northwest University Interdisciplinary Center for Theoretical Physics and Information Sciences Fudan University Hefei National Laboratory

Surface electrons in axion insulators are endowed with a topological layer degree of freedom followed by exotic transport phenomena, e.g., the layer Hall effect. Here, we propose that such a layer degree of freedom can be manipulated in a dissipationless way based on the antiferromagnetic MnBi2Te4with tailored domain structure. This makes MnBi2Te4a versatile platform to exploit the ‘layertronics’ to encode, process and store information. Importantly, the layer filter, layer valve and layer reverser devices can be achieved using the layer-locked chiral domain wall modes. The dissipationless nature of the domain wall modes makes the performance of the layertronic devices superior to those in spintronics and valleytronics. Specifically, the layer reverser, a layer version of the Datta–Das transistor, also fills up the blank in designing the valley reverser in valleytronics. Our work sheds light on constructing new generation electronic devices with high performance and low-energy consumption in the framework of layertronics.

关键词： axion insulator MnBi2Te4 layertronics antiferromagnetic domain wall dissipationless transport

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Identification of global alternative splicing and sex-specific splicing via comparative transcriptome analysis of gonads of Chinese tongue sole(Cynoglossus semilaevis)

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Zoological Research 2022年第3期43卷 319-330页

作者： Yi-Fang Lu Qian liu Kai-Qiang liu Hong-Yan Wang cheng-hua li Qian Wang Chang-Wei Shao School of Marine Sciences Ningbo UniversityNingboZhejiang 315211China Key Lab of Sustainable Development of Marine Fisheries Ministry of AgricultureYellow Sea Fisheries Research InstituteChinese Academy of Fishery SciencesQingdaoShandong 266071China Laboratory for Marine Fisheries Science and Food Production Processes Pilot National Laboratory for Marine Science and TechnologyQingdaoShandong 266000China College of Fisheries and life Science Shanghai Ocean UniversityShanghai 201306China

Chinese tongue sole(Cynoglossus semilaevis)is an economically important marine fish species with a ZZ/ZW sex determination mechanism,which can be influenced by *** splicing(AS)is an important mechanism regulating the expression of genes related to sex determination and gonadal differentiation,but has rarely been reported in *** this study,to explore the molecular regulatory mechanisms of sex determination and gonadal differentiation,we combined isoform and RNA sequencing(Iso-Seq and RNA-Seq)to perform transcriptome profiling of male and female gonads in *** total,81883 and 32341 full-length transcripts were obtained in males and females,respectively.A total of 8279 AS genes were identified,including 2639 genes showing differential AS(DAS)between males and *** intersecting DAS genes and differentially expressed genes(DEGs)were enriched in the meiotic cell cycle pathway,and genes related to gonadal differentiation,such as esrrb and wt1a,were found to have sex-specific ***,this study revealed AS events in the gonadal transcriptomes of male and female ***,described the characteristics of active transcription in the testes,and identified candidate genes for studying the regulatory mechanisms of AS during gonadal differentiation.

关键词： Gonadal differentiation Alternative splicing Sex-specific splicing Cynoglossus semilaevis Iso-Seq RNA-Seq

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