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Investigating the impact of dynamic structural changes of Au/rutile catalysts on the catalytic activity of CO oxidation

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Carbon Energy 2024年第4期6卷 222-232页

作者： Xiaochun hu Qianwenhao Fan Mingwu Tan yuqing Luo Xianyue Wu Manoel y.Manuputty Jie Ding Tej s.Choksi Markus Kraft Rong Xu Zhiqiang sun Wen Liu school of Energy.s.ience and Engineering Central South UniversityChangshaChina school of Chemistry Chemical Engineering and BiotechnologyNanyang Technological UniversitySingaporeSingapore Cambridge Centre for Advanced Research and Education SingaporeSingapore Institute of sustainability for Chemicals Energy and EnvironmentJurong IslandSingapore College of Chemistry and Chemical Engineering Central South UniversityChangshaChina Department of Chemical Engineering and Biotechnology University of CambridgeCambridgeUK

The surface properties of oxidic supports and their interaction with the supported metals play critical roles in governing the catalytic activities of oxide‐supported metal *** metals are supported on reducible oxides,dynamic surface reconstruction phenomena,including strong metal–support interaction(sMsI)and oxygen vacancy formation,complicate the determination of the structural–functional relationship at the active ***,we performed a systematic investigation of the dynamic behavior of Au nanocatalysts supported on flame‐synthesized TiO_(2),which takes predominantly a rutile phase,using CO oxidation above room temperature as a probe *** analysis conclusively elucidated a negative correlation between the catalytic activity of Au/TiO_(2) and the oxygen vacancy at the Au/TiO_(2) *** the reversible formation and retracting of sMsI overlayers have been ubiquitously observed on Au/TiO_(2) samples,the catalytic consequence of sMsI remains *** functional theory.s.ggests that the electron transfer from TiO_(2) to Au is correlated to the presence of the interfacial oxygen vacancies,retarding the catalytic activation of CO oxidation.

关键词： CO oxidation electronic metal-support interactions flame‐synthesis metal-support interactions oxygen vacancy strong metal-support interaction

Coal/Gangue Volume Estimation with Convolutional Neural Network and separation Based on Predicted Volume and Weight

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Computers, Materials & Continua 2024年第4期79卷 279-306页

作者： Zenglun Guan Murad s.Alfarzaeai Eryi hu Taqiaden Alshmeri Wang Peng school of Mechatronic Engineering China University of Mining and TechnologyXuzhou221116China China National Coal Group Corp. Beijing100029China Information Institute Ministry of Emergency Management of the ChinaBeijing100029China school of Mechanical Engineering Sana’a UniversitySana’a31220Yemen

In the coal mining industry,the gangue separation phase imposes a key challenge due to the high visual similaritybetween coal and ***,separation methods have become more intelligent and efficient,using newtechnologies and applying different features for *** such method exploits the difference in substancedensity,leading to excellent coal/gangue ***,this study uses density differences to distinguishcoal from gangue by performing volume prediction on the *** training samples maintain a record of3-side images as input,volume,and weight as the ground truth for the *** prediction process relieson a Convolutional neural network(CGVP-CNN)model that receives an input of a 3-side image and then extractsthe needed features to estimate an approximation for the *** classification was comparatively performedvia ten different classifiers,namely,K-Nearest Neighbors(KNN),Linear support Vector Machines(Linear sVM),Radial Basis Function(RBF)sVM,Gaussian Process,Decision Tree,Random Forest,Multi-Layer Perceptron(MLP),Adaptive Boosting(AdaBosst),Naive Bay.s.and Quadratic Discriminant Analysis(QDA).After severalexperiments on testing and training data,results yield a classification accuracy of 100%,92%,95%,96%,100%,100%,100%,96%,81%,and 92%,*** test reveals the best timing with KNN,which maintained anaccuracy level of 100%.Assessing themodel generalization capability to newdata is essential to ensure the efficiencyof the model,so by applying a cross-validation experiment,the model generalization was *** useddataset was isolated based on the volume values to ensure the model generalization not only on new images of thesame volume but with a volume outside the trained ***,the predicted volume values were passed to theclassifiers group,where classification reported accuracy was found to be(100%,100%,100%,98%,88%,87%,100%,87%,97%,100%),*** obtaining a classification with hi

关键词： Coal coal gangue convolutional neural network CNN object classification volume estimation separation system

Distributed Fault-Tolerant Control of Uncertain Multi-Agent systems with Connectivity Maintenance

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Journal of systems science & Complexity 2024年第1期37卷 40-62页

作者： XING Xueyan hu Guoqiang Continental-NTU Corporate Lab Nanyang Technological UniversitySingapore 639798Singapore Continental-NTU Corporate Lab and the school of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore 639798Singapore

In this paper,a distributed cooperative control protocol is presented to deal with actuator failures of multi-agent systems in the presence of connectivity *** the developed strategy,each agent can track the reference trajectory of the leader in the presence of actuator failures,disturbances and *** connectivity of the multi-agent system can always be ensured during the control *** achieve the aforementioned control objectives,a potential function is introduced to the distributed adaptive fault-tolerant control algorithm to preserve the initial connected network among the *** uncertainty of the multi-agent system,which is allowed to be described by discontinuous functions,is approximated and compensated using the fuzzy logic *** asymptotic stability of the closed-loop system is demonstrated through the use of Cellina’s approximate selection theorem of nonsmooth *** to the developed adaptive laws,the upper bound of the disturbance is allowed to be uncertain,which facilitates the implementation of the control ***,simulation results are provided to verify the effectiveness of the proposed control scheme.

关键词： Actuator failure connectivity maintenance coordination control uncertainties

Antibodies elicited by Newcastle disease virus-vectored H7N9 avian influenza vaccine are functional in activating the complement system

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Journal of Integrative Agriculture 2024年第6期23卷 2052-2064页

作者： Zenglei hu ya huang Jiao hu Xiaoquan Wang shunlin hu Xiufan Liu Joint International Research Laboratory of Agriculture and Agri-Product safety of the Ministry of Education of China Yangzhou UniversityYangzhou 225009China Animal Infectious Disease Laboratory School of Veterinary MedicineYangzhou UniversityYangzhou 225009China Jiangsu Co-innovation Center for Prevention and Control of Important Animal Infectious Diseases and Zoonoses Yangzhou UniversityYangzhou 225009China

H7N9 subtype avian influenza virus poses a great challenge for poultry *** disease virus(NDV)-vectored H7N9 avian influenza vaccines(NDV_(vec)H7N9)are effective in disease control because they are protective and allow mass *** note,these vaccines elicit undetectable H7N9-specific hemagglutination-inhibition(HI)but high IgG antibodies in ***,the molecular basis and protective mechanism underlying this particular antibody immunity remain ***,immunization with an NDV_(vec)H7N9 induced low anti-H7N9 HI and virus neutralization titers but high levels of hemagglutinin(HA)-binding IgG antibodies in *** residues(s150,G151 and s152)in HA of H7N9 virus were identified as the dominant epitopes recognized by the NDV_(vec)H7N9 immune *** transferred NDV_(vec)H7N9 immune serum conferred complete protection against H7N9 virus infection in *** NDV_(vec)H7N9 immune serum can mediate a potent lysis of HA-expressing and H7N9 virus-infected cells and significantly.s.ppress H7N9 virus *** activities of the serum were significantly impaired after heat-inactivation or treatment with complement inhibitor,suggesting the engagement of the complement ***,mutations in the 150-sGs-152 sites in HA resulted in significant reductions in cell lysis and virus neutralization mediated by the NDV_(vec)H7N9 immune serum,indicating the requirement of antibody-antigen binding for complement ***,antibodies induced by the NDV_(vec)H7N9 can activate antibody-dependent complement-mediated lysis of H7N9 virus-infected cells and complement-mediated neutralization of H7N9 *** findings unveiled a novel role of the complement in protection conferred by the NDV_(vec)H7N9,highlighting a potential benefit of engaging the complement system in H7N9 vaccine design.

关键词： H7N9 subtype avian influenza virus NDV vector vaccine antibody immunity complement protection

A functional gel polymer electrolyte based on PVDF-HFP/gelatin toward dendrite-free lithium metal batteries

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Nano Research 2024年第4期17卷 2790-2799页

作者： Xiaoyi hu Kangli Liu shijie Zhang Guosheng shao s.Ravi P.silva Peng Zhang state Center for International Cooperation on Designer Low-carbon and Environmental Materials(CDLCEM) School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Zhengzhou Materials Genome Institute(ZMGI) ZhongyuanzhiguXingyang 450100China Nanoelectronics Center Advanced Technology InstituteUniversity of SurreyGuildfordGU27XHUK

The leakage of liquid electrolyte and the formation of lithium dendrites pose challenges to safety and stability of lithium metal batteries(LMBs).The appearance of gel polymer electrolyte(GPE)has obviously improved the safety of traditional ***,the limited inhibition of GPE on lithium dendrites is detrimental to the safety of ***,a kind of poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP)/gelatin(GN)GPE with high ionic conductivity,high-temperature resistance,and flame-retardancy,was prepared by electrospinning and soaking *** the electrospinning network of PVDF-HFP,its affinity to liquid electrolytes,makes this GPE more beneficial to ions transport and the formation of ***,the GN with sol–gel properties,enhances the mechanical property(13.5 MPa)of HFP-GN ***,X-ray photoelectron spectroscopy(XPs)and density functional theory(DFT)suggest that the attraction of polar groups of GN to Li+can regulate the distribution of Li+and protect Li ***,the application of HFP-GN GPEs to LMBs with cathodes of LiFePO_(4) and LiCoO_(2) deliver excellent electrochemical performances:after 300 cycles,the LiFePO_(4)/HFP-GN GPE/Li battery keeps a low capacity decay rate of 0.09%at 5 C;after 400 cycles at 2 C,the LiCoO_(2)/HFP-GN GPE/Li cell retains a high capacity retention of 74%.This GPE is demonstrated for the application prospect of safe LMBs.

关键词： poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP) gelatin polar groups lithium metal battery lithium dendrite

Quantitative estimation of global mean precipitation throughout the Phanerozoic era

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science China Earth sciences 2024年第5期67卷 1616-1624页

作者： Xiujuan BAO yongyun hu Laboratory for Climate and Ocean-Atmospheric studies Department of Atmospheric and Oceanic SciencesSchool of PhysicsPeking UniversityBeijing 100871China

Quantitatively estimating the global mean precipitation(GMP)throughout Earth's history is crucial for enhancing our understanding of long-term climate evolution and the hydrological ***,currently there is no established methodology for estimating global mean ***,we present the first study that estimates GMP in the Phanerozoic *** relationship between GMP and global mean surface temperature(GMsT)is investigated by analyzing data from 23 models in the Coupled Model Intercomparison Project phase 6(CMIP6).The result reveals consistent and significant impact of temperature on precipitation,with a sensitivity range of 2–3%K^(-1).Additionally,we propose a method for accessing latitudinal variations in precipitation caused by land area distributions and paleo-Koppen climatic *** climatic belts are determined based on geological indicators such as coals,evaporites,and glacial *** GMP is thus quantitatively estimated by combining variations in GMsT,land area distributions,and paleo-koppen climatic belts,spanning from 540 Ma to the present *** quantitative GMP curve demonstrates fluctuations in GMP about 500 mm yr^(-1),with values ranging from 948 to1442 mm yr-1over the Phanerozoic *** curve aligns closely with findings derived from numerical *** presented paleoprecipitation variations facilitate a more comprehensive understanding of the interconnected geological and paleoclimatic developments.

关键词： Paleoprecipitation Paleoclimate K?ppen climatic belts Global mean precipitation Hydrological cycle

Design,preparation,and characterization of a novel ZnO/CuO/Al energetic diode with dual functionality:Logic and destruction

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Defence Technology（防务技术） 2024年第4期34卷 57-68页

作者： Jialu yang Jiaheng hu yinghua ye Jianbing Xu yan hu Ruiqi shen school of Chemistry and Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094China Micro-Nano Energetic Devices Key Laboratory of MIIT Nanjing 210094China Institute of space Propulsion Nanjing University of Science and TechnologyNanjing 210094China

self-destructing chips have promising applications for securing *** paper proposes a new concept of energetic diodes for the first time,which can be used for self-destructive chips.A simple two-step electrochemical deposition method is used to prepare ZnO/CuO/Al energetic diode,in which N-type ZnO and P-type CuO are constricted to a PN *** paper comprehensively discusses the material properties,morphology.s.miconductor characteristics,and exploding performances of the energetic *** results show that the energetic diode has typical rectification with a turn-on voltage of about 1.78 V and a reverse leakage current of about 3×10^(-4)*** a constant voltage of 70 V loads to the energetic diode in the forward direction for about 0.14 s or 55 V loads in the reverse direction for about 0.17 s,the loaded power can excite the energetic diode exploding and the current rises to about100 *** to the unique performance of the energetic diode,it has a double function of rectification and *** energetic diode can be used as a logic element in the normal chip to complete the regular operation,and it can release energy to destroy the chip accurately.

关键词： Energetic diode ZnO—CuO—Al thermite ZnO/CuO PN junction Electrical explosion performance self-destructing chips

studies on the temporal,structural,and interacting features of the clubroot resistance gene Rcr1 using CRIsPR/Cas9-based systems

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Horticultural Plant Journal 2024年第4期10卷 1035-1048页

作者： Hao hu Fengqun yu Agriculture and Agri-Food Canada Saskatoon Research and Development Centre107 Science PlaceSaskatoonSKS7N OX2Canada

Clubroot disease is a severe threat to Brassica crops globally,particularly in western *** resistance,achieved through pyramiding clubroot resistance(CR)genes with different modes of action,is the most important strategy for managing the ***,studies on the CR gene functions are quite *** this study,we have conducted investigations into the temporal,structural,and interacting features of a newly cloned CR gene,Rcr1,using CRIsPR/Cas9 *** temporal functionality,we developed a novel CRIsPR/Cas9-based binary vector,pHHIGR-Hsp18.2,to deliver Rcr1 into a susceptible canola line(DH12075)and observed that early expression of Rcr1 is critical for conferring *** structural functionality.s.veral independent mutations in specific domains of Rcr1 resulted in loss-offunction,highlighting their importance for CR *** the study of the interacting features of Rcr1,a cysteine protease gene and its homologous allele in canola were successfully disrupted via CRIsPR/Cas9 as an interacting component with Rcr1 protein,resulting in the conversion from clubroot resistant to susceptible in plants carrying intact *** results indicated an indispensable role of these two cysteine proteases in Rcr1-mediated resistance *** study,the first of its kind,provides valuable insights into the functionality of ***,the new vector p HHIGR-Hsp18.2 demonstrated an inducible feature on the removal of add-on traits,which should be useful for functional genomics and other similar research in brassica crops.

关键词： Clubroot resistance Brassica crops Canola Rcr1 CRIsPR/Cas9 system Gene knock-out Timing control Non-synonymous mutation Protein-protein interaction

Intraseasonal variability of the Kuroshio observed via mooring at 18°N

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Journal of Oceanology and Limnology 2024年第2期42卷 468-483页

作者： Xin yUAN Qingye WANG Jie MA shijian hu Dunxin hu Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of SciencesQingdao 266071China University of Chinese Academy of sciences Beijing 100049China Laoshan Laboratory Qingdao 266237China Center for Ocean Mega-science Chinese Academy of SciencesQingdao 266071China

Insufficient observations near the origin of the Kuroshio have led to incomplete understanding of the intraseasonal variability(IsV)of the *** measurements of the Kuroshio velocity were performed with an array of three profiler moorings(122.7°E,123°E,and 123.3°E)along 18°N from January 2018 to February *** IsV of the Kuroshio at 18°N was investigated based on a combination of mooring observations and global high-resolution Hybrid Coordinate Ocean Model reanalysis *** estimated time-averaged transport in the upper 350 m across the observation transect was 6.5±2.6 sv(1.0 sv=10^(6)m^(3)/s).Two significant IsV peaks at 50-60 and~100 d were recognized in the power spectra of the meridional velocity and *** analysis indicated that the IsV at 50-60 d was caused by westward-propagating eddies at average propagation speed of~13 cm/s and wavelength of~635 *** IsV peak at~100 d was mainly caused by northward-propagating eddies generated in the North Equatorial Current *** investigation indicated that the IsV of the Kuroshio at 18°N is dominated by meridional transport,rather than by the zonal migration of the Kuroshio main *** findings provide a better understanding of the IsV of the Kuroshio east of Luzon Island.

关键词： intraseasonal variability(IsV) Kuroshio mooring observation eddy