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Chemico-biological conversion of carbon dioxide

Journal of Energy Chemistry 2024年第2期89卷 371-387,I0009页

作者： Liangwei hu Junzhu Yang Qi Xia Jin Zhang Hongxin Zhao Yuan lu Zhejiang Province Key Laboratory of Plant Secondary Metabolism and Regulation College of Life Sciences and MedicineZhejiang Sci-Tech UniversityHangzhou 310018ZhejiangChina Key Laboratory of Industrial Biocatalysis Ministry of EducationTsinghua UniversityBeijing 100084China Department of Chemical Engineering Tsinghua UniversityBeijing 100084China College of Biological and Chemical Engineering Jiaxing UniversityJiaxing 314000ZhejiangChina

The unabated carbon dioxide(CO_(2))emission into the atmosphere has exacerbated global climate change,resulting in extreme weather events,biodiversity loss,and an intensified greenhouse *** address these challenges and work toward carbon(C)neutrality and reduced CO_(2)emissions,the capture and utilization of CO_(2)have become imperative in both scientific research and *** cutting-edge approach to achieving efficient catalytic performance involves integrating green bioconversion and chemical *** innovative strategy offers several advantages,including environmental friendliness,high efficiency,and *** study provides a comprehensive review of existing technical routes for carbon sequestration(CS)and introduces two novel CS pathways:the electrochemicalbiological hybrid and artificial photosynthesis *** also thoroughly examines the synthesis of valuable Cnproducts from the two CS systems employing different catalysts and *** both systems heavily rely on electron transfer,direct and mediated electron transfer has been discussed and summarized in ***,this study explores the conditions suitable for different catalysts and assesses the strengths and weaknesses of *** also explored the biocompatibility of the electrode materials and developed novel *** materials were specifically engineered to combine with enzymes or microbial cells to solve the biocompatibility problem,while improving the electron transfer efficiency of ***,this review summarizes the relevant systems developed in recent years for manufacturing different products,along with their respective production efficiencies,providing a solid database for development in this *** novel chemical-biological combination proposed herein holds great promise for the future conversion of CO_(2)into advanced organic ***,it offers exciting prospects for utilizing CO_(2)in synthesizing

关键词： Carbon dioxide Bioelectric synthesis Artificial photosynthesis Synthetic product

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Exploring the ultrahigh rolling contact fatigue life of M50 bearing steel by adjusting the cryogenic sequence

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Journal of Materials Science & Technology 2024年第2期169卷 243-250页

作者： Xin Cai Xiaoqiang hu Xingyu lu Hongwei Liu Yanfei Cao Dianzhong Li Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China

The influence of different cryogenic sequences on the rolling contact fatigue(RCF)life of M50-bearing steel has been *** results show that direct cryogenic treatment after quenching can effectively improve RCF *** L_(10)life is strikingly 5 times longer than that with cryogenic treatment after *** is caused by the distinct lattice construction of martensite and the transformation of retained *** secondary nanocarbides and fine twins are formed via cryogenic treatment before tem-pering compared with cryogenic treatment after *** improvement in the RCF life of the steel is attributed to the joint effects of the secondary nanocarbides and twin boundaries with a width of 5-13 nm,which delays significantly crack initiation and *** study highlights a common method to improve the service life of high-carbon and high-alloy steels by adjusting the cryogenic se-quence.

关键词： M50 steel Cryogenic treatment Rolling contact fatigue life Carbide Twin

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Type Synthesis of Self-Alignment Parallel Ankle Rehabilitation Robot with Suitable Passive Degrees of Freedom

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 160-175页

作者： Ya Liu Wenjuan lu Dabao Fan Weijian Tan Bo hu Daxing Zeng School of Mechanical Engineering Yanshan UniversityQinhuangdao 066004China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China Dongguan Engineering Technology Research Center for Parallel Robot Dongguan 523808China The DGUT Innovation Center of Robotics and Intelligent Equipment Dongguan 523808China

The current parallel ankle rehabilitation robot(ARR)suffers from the problem of difficult real-time alignment of the human-robot joint center of rotation,which may lead to secondary injuries to the *** study investigates type synthesis of a parallel self-alignment ankle rehabilitation robot(PSAARR)based on the kinematic characteristics of ankle joint rotation center drift from the perspective of introducing"suitable passive degrees of freedom(DOF)"with a suitable number and ***,the self-alignment principle of parallel ARR was proposed by deriving conditions for transforming a human-robot closed chain(HRCC)formed by an ARR and human body into a kinematic suitable constrained system and introducing conditions of"decoupled"and"less limb".Second,the relationship between the self-alignment principle and actuation wrenches(twists)of PSAARR was analyzed with the velocity Jacobian matrix as a"bridge".Subsequently,the type synthesis conditions of PSAARR were ***,a PSAARR synthesis method was proposed based on the screw theory and type of PSAARR synthesis ***,an HRCC kinematic model was established to verify the self-alignment capability of the *** this study,93 types of PSAARR limb structures were synthesized and the self-alignment capability of a human-robot joint axis was verified through kinematic analysis,which provides a theoretical basis for the design of such an ARR.

关键词： Ankle rehabilitation robot Self-alignment Parallel mechanism Type synthesis Screw theory

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Effect of Post-weld Heat Treatment on the Microstructure and Mechanical Properties of 2.25Cr-1Mo-0.25V Ultra-Thick Steel Plate

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Acta Metallurgica Sinica(English Letters) 2024年第6期37卷 1104-1114页

作者： Yanyang Wu Zongye Ding Wenquan lu Jingchao Hou Qiaodan hu Jianguo Li Shanghai Key Laboratory of Materials Laser Processing and Modification School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai200240China State Key Laboratory of Advanced Special Steel Shanghai UniversityShanghai200444China School of Mechatronic Engineering and Automation Foshan UniversityFoshan528225GuangdongChina WuYang Iron and Steel Wugang450000HenanChina

Ensuring the homogeneous and excellent mechanical properties of 2.25Cr-1Mo-0.25V ultra-thick steel plate is the key to the production of hydrogenation reactor ***,it is required to understand the heterogeneity of microstructures and properties of ultra-thick plate after heat *** this work,the effect of post-weld heat treatment(PWHT)on the strength,plasticity,toughness and microstructures of the 193-mm-thick steel plate was investigated,and the formation mechanism of heterogeneity was *** PWHT decreased the room-and high-temperature yield strength(YS)and ultimate tensile strength(UTS)of the steel plate after normalizing and tempering(NT),while the room-and high-temperature YS and UTS decreased from the surface to the center of 193-mm-thick steel *** was attributed to the enhanced decomposition of martensite-austenite(M-A)constituents and coarsening of grains and precipitated carbides.

关键词： Cr-Mo steel Ultra-thick steel plate Microstructure Mechanical properties Heterogeneity

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Slippery hydrogel with desiccation-tolerant‘skin’for high-precision additive manufacturing

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International Journal of Extreme Manufacturing 2024年第2期6卷 486-500页

作者： Desheng Liu Pan Jiang Yue hu Yaozhong lu Yixian Wang Jiayu Wu Danli hu Tao Wu Xiaolong Wang State Key Laboratory of Solid lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000People’s Republic of China CAS Key Laboratory of Chemistry of Northwestern Plant Resources Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000People’s Republic of China Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai Yantai Zhongke Research Institute of Advanced Materials and Green Chemical EngineeringYantai 264006People’s Republic of China Key Laboratory of Materials-Oriented Chemical Engineering of Xinjiang Uygur Autonomous Region School of Chemistry and Chemical EngineeringShihezi UniversityShihezi 832003People’s Republic of China

Hydrogels inevitably undergo dehydration,structural collapse,and shrinkage deformation due to the uninterrupted evaporation in the atmosphere,thereby losing their flexibility,slipperiness,and manufacturing ***,we propose a novel bioinspired strategy to construct a spontaneously formed‘skin’on the slippery hydrogels by incorporating biological stress metabolites trehalose into the hydrogel network,which can generate robust hydrogen bonding interactions to restrain water *** contents of trehalose in hydrogel matrix can also regulate the desiccation-tolerance,mechanical properties,and lubricating performance of slippery hydrogels in a wide *** vat photopolymerization three-dimensional printing and trehalose-modified slippery hydrogels enables to achieve the structural hydrogels with high resolution,shape fidelity,and sophisticated architectures,instead of structural collapse and shrinkage deformation caused by *** thus,this proposed functional hydrogel adapts to manufacture large-scale hydrogels with sophisticated architectures in a long-term *** a proof-of-concept demonstration,a high-precision and sophisticated slippery hydrogel vascular phantom was easily fabricated to imitate guidewire ***,the proposed protocol is universally applicable to diverse types of hydrogel *** strategy opens up a versatile methodology to fabricate dry-resistant slippery hydrogel for functional structures and devices,expanding their high-precision processing and broad applications in the atmosphere.

关键词： slippery hydrogel trehalose desiccation tolerance vat photopolymerization 3D printing hydrogen bonding

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白酒酿造中不同原料和曲种对风味物质影响的研究进展

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酿酒科技 2024年第2期 76-83页

作者：钱春勤刘婷婷杨佳佳路虎潘成康贵州习酒股份有限公司贵州习水564600

白酒,是微生物利用粮食经过一系列复杂变化造就的一件“完美艺术品”,是世界上最具特色和知名度的蒸馏酒类之一。在白酒的酿造过程,原料和曲种直接影响着白酒风味物质的呈现及品质。本文综述了白酒酿造过程中原料与曲种的选择对于白酒... 详细信息

白酒,是微生物利用粮食经过一系列复杂变化造就的一件“完美艺术品”,是世界上最具特色和知名度的蒸馏酒类之一。在白酒的酿造过程,原料和曲种直接影响着白酒风味物质的呈现及品质。本文综述了白酒酿造过程中原料与曲种的选择对于白酒风味物质的影响,以期为白酒企业在筛选使用原料与曲种上提供参考。

关键词：白酒酿造原料曲种

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Bioinspired Hemostatic Strategy via Pulse Ejections for Severe Bleeding Wounds

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Research 2024年第1期2023卷 281-299页

作者： Bitao lu Enling hu Weiwei Ding Wenyi Wang Ruiqi Xie Kun Yu Fei lu Guangqian Lan Fangyin Dai State Key Laboratory of Silkworm Genome Biology College of SericultureTextile and Biomass SciencesSouthwest UniversityChongqing 400715China Chongqing Engineering Research Center of Biomaterial Fiber and Modern Textile Chongqing 400715China Division of Trauma and Surgical Intensive Care Unit Research Institute of General SurgeryJinling HospitalMedical School of Nanjing UniversityNanjing210002 Jiangsu ProvinceChina Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHong KongChina

Efficient hemostasis during emergency trauma with massive bleeding remains a critical challenge in prehospital ***,multiple hemostatic strategies are critical for treating large bleeding *** this study,inspired by bombardier beetles to eject toxic spray for defense,a shape-memory aerogel with an aligned microchannel structure was proposed,employing thrombin-carrying microparticles loaded as a built-in engine to generate pulse ejections for enhanced drug *** aerogels,after contact with blood,can rapidly expand inside the wound,offering robust physical barrier blocking,sealing the bleeding wound,and generating a spontaneous local chemical reaction causing an explosivelike generation of CO_(2) microbubbles,which provide propulsion thrust to accelerate burst ejection from arrays of microchannels for deeper and faster drug *** ejection behavior,drug release kinetics,and permeation capacity were evaluated using a theoretical model and experimentally *** novel aerogel showed remarkable hemostatic performance in severely bleeding wounds in a swine model and demonstrated good degradability and biocompatibility,displaying great potential for clinical application in humans.

关键词： wound sealing offering

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Cold Model of Coal Gas Component Concentration Distribution in Blast Furnace Raceway

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Journal of Iron and Steel Research International 2009年第6期16卷 1-6页

作者： ZHANG Sheng-fu WEN Liang-ying BAI Chen-guang QIU Gui-bao hu Mei-long lu Xue-wei College of Materials Science and Engineering Chongqing University Chongqing 400030 China

Primary distribution of coal gas in blast furnace raceway has an important effect on blast furnace ironmaking process. The coal gas component concentration distribution was studied experimentally using a three-dimensional cold model. The results showed that CH4 concentration diminishes along with the height increasing on vertical section of raceway, and the concentration is the highest in the bottom of raceway. CH4 concentration increases gradually *** raceway depth with the lowest concentration value in front of the tuyere. The distribution of CH4 concentration has different characteristics in different raceway zones.

关键词： blast furnace raceway coal gas component concentration distribution

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Trust Degree of Web Services and Its Evaluation with Neural Network

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Wuhan University Journal of Natural Sciences 2006年第5期11卷 1302-1305页

作者： huANG Baohua hu Heping lu Zhengding YAO Hanbing LI Ruixuan College of Computer Science and Technology HuazhongUniversity of Science and Technology Wuhan 430074Hubei China

The concept and definition of trust degree of Web service is given. Evaluating trust degree of Web services with the method of neural network from the aspect of trust history sequence is proposed. The principle of the method, applicable neural network structure, neural network construc ting, input standardization, training sample constructing, and the procedure of evaluating trust degree of Web services with trained neural network are described. Experiments show that it is feasible and effective to evaluate trust degree of Web Service with neural network.

关键词： Web services trust degree neural network

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New strategies for asymmetric photocatalysis: asymmetric organocatalytic/photoredox relay catalysis for efficient synthesis of polycyclic compounds containing vicinal amino alcohols

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Science China Chemistry 2024年第3期67卷 945-952页

作者： Jia-lu Zhang Wen-Bo He Xiu-Qin hu Peng-Fei Xu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000China State Key Laboratory of Veterinary Etiological Biology College of Veterinary MedicineLanzhou UniversityLanzhou Veterinary Research InstituteChinese Academy of Agricultural SciencesLanzhou 730000China MOE Frontiers Science Center for Rare Isotopes Lanzhou UniversityLanzhou 730000China

An asymmetric catalytic strategy in photocatalysis utilizing a chirality-induced approach through an organocatalytic/photoredox relay catalysis strategy is successfully achieved for the rapid construction of polycyclic compounds containing vicinal amino alcohols in a one-pot protocol. This methodology facilitates the efficient synthesis of diverse substituted polycyclic tetrahydroquinoline and benzofuran-derived vicinal amino alcohols, each containing five consecutive chiral centers, with high yields,excellent diastereoselectivities and enantioselectivities(up to 95% yield, >20:1 dr and 98% ee), under mild reaction conditions driven by sequential bifunctional squaramide organocatalyst-catalyzed [4+2] annulation and photocatalyst-catalyzed ketyl radical addition cyclization reaction process. Furthermore, investigations into the stereoselectivity mechanism and high-resolution mass spectrometry(HRMS) experiments on free radical trapping have provided evidence for elucidating the detailed mechanism of chirality-induced processes and chiral intermediate conversions in this procedure.

关键词： enantioselective photocatalysis asymmetric organocatalytic/photocatalysis relay catalysis five consecutive chiral centers chirality-induced strategy chirality vicinal amino alcohols

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