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Experimental study of enhanced oil recovery by CO_(2) huff-n-puff in shales and tight sandstones with fractures

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Petroleum Science 2021年第3期18卷 852-869页

作者： Chao-Fan Zhu Wei Guo You-Ping Wang Ya-Jun Li hou-jian gong Long Xu Ming-Zhe Dong College of Construction Engineering Jilin UniversityChangchun 130026JilinChina School of Petroleum Engineering China University of Petroleum(East China)Qingdao 266580China Petroleum Exploration and Production Research Institute SinopecBeijing 100083China Department of Chemical and Petroleum Engineering University of CalgaryCalgaryAB T2N 1N4Canada

The fractures and kerogen,which generally exist in the shale,are signifcant to the CO_(2) huf-n-puf in the shale *** is important to study the efects of fractures and kerogen on oil recovery during CO_(2) huf-n-puf operations in the fracture-matrix *** this study,a modifed CO_(2) huf-n-puf experiment method is developed to estimate the recovery factors and the CO_(2) injectivity in the fractured organic-rich shales and tight *** efects of rock properties,injection pressure,and injection time on the recovery factors and CO_(2) usage efciency in shales and sandstones are discussed,*** results show that although the CO_(2) injectivity in the shale is higher than that in the sandstone with the same porosity;besides,the recovery factors of two shale samples are much lower than that of two sandstone *** demonstrates that compared with the tight sandstone,more cycles are needed for the shale to reach a higher recovery ***,there are optimal injection pressures(close to the minimum miscible pressure)and CO_(2) injection volumes for CO_(2) huf-npuf in the *** the optimal CO_(2) injection volume in the shale is higher than that in the sandstone,more injection time is needed to enhance the oil recovery in the *** is a reference sense for CO_(2) huf-n-puf in the fractured shale oil reservoir for enhanced oil recovery(EOR)purposes.

关键词： Shale Tight sandstone CO_(2)huf-n-puf Fracture Injectivity of CO_(2)

Defective Nickel-Iron Layered Double Hydroxide for Enhanced Photocatalytic NO Oxidation with Significant Alleviation of NO2 Production

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Engineering 2024年第5期36卷 276-284页

作者： Xiaoyu Li Xiaoshu Lv jian Pan Peng Chen Huihui Peng Yan jiang Haifeng gong Guangming jiang Li’an hou Engineering Research Center for Waste Oil Recovery Technology and Equipment Ministry of EducationChongqing Technology and Business UniversityChongqing 400067China State Key Laboratory of Water Environment Simulation School of EnvironmentBeijing Normal UniversityBeijing 100875China Environmental Technology Innovation Center of jiande Hangzhou Bertzer Catalyst Co.Ltd.Hangzhou 310058China Chongqing Key Laboratory of Green Synthesis and Application College of ChemistryChongqing Normal UniversityChongqing 401331China

Photocatalysis offers a sustainable means for the oxidative removal of low concentrations of NOx(NO,NO2,N2O,N2O5,etc.)from the *** double hydroxides(LDHs)are promising candidate photocatalysts owing to their unique layered and tunable chemical structures and abundant surface hydroxide(OH)moieties,which are hydroxyl radical(OH)***,the practical applications of LDHs are limited by their poor charge-separation ability and insufficient active ***,we developed a facile N_(2)H_(4)-driven etching approach to introduce dual Ni^(2+)and OHvacancies(Niv and OHv,respectively)into NiFe-LDH nanosheets(hereafter referred to as NiFe-LDH-et)to facilitate improved charge-carrier separation and active Lewis acidic site(Fe^(3+)and Ni^(2+)exposed at OHv)*** contrast to inert pristine LDH,NiFe-LDH-et actively removed NO under visible-light ***,Ni_(76)Fe_(24)-LDH-et etched with 1.50 mmol·L^(-1)N_(2)H_(4)solution removed 32.8%of the NO in continuously flowing air(NO feed concentration:500 parts per billion(ppb))under visible-light illumination,thereby outperforming most reported *** and theoretical data revealed that the dual vacancies promoted the production of reactive oxygen species(O_(2)·^(-)andOH)and the adsorption of NO on the *** situ spectroscopy demonstrated that NO was preferentially adsorbed at Lewis acidic sites,particularly exposed Fe^(3+)sites,converted into NO+,and subsequently oxidized to NO3without the notable formation of the more toxic intermediate NO2,thereby alleviating risks associated with its production and emission.

关键词： Vacancie Layered double hydroxide NO+ Photocatalysis NO removal

Research on the Asymmetric Effect of Fixed-Asset Investment on China's Primary Energy Production in the Context of Energy Transformation

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Journal of Systems Science & Complexity 2024年第3期37卷 1163-1183页

作者： CHAI jian HE Peng ZHANG Xiaokong hou Yamin School of Economics and Management Xidian UniversityXi'an 710126China

Under China’s“Dual Carbon”target(DCT),“clean replacement”on the energy supply side and“electric energy replacement”on the energy consumption side are the ways to achieve energy ***,energy projects have a long construction period,complex technology categories,and investment risks that greatly affect the development of energy *** judging the effect of investment changes on primary energy production is of great practical significance to the realization of the *** on this,NARDL and TVP-SV-VAR models are innovatively used to reveal the nonlinear effect of fixed-asset investment on China’s primary energy *** results show that the marginal effect of investment growth on coal production is about 1.44 times that of investment ***,the marginal effect of oil and gas investment growth is about 1.21times that of investment *** to the influence of resource constraints,China’s traditional fossil energy still has varying degrees of path dependence on the investment-driven development *** non-fossil energy,investment in hydropower and nuclear power has an inverse correlation with the change in *** marginal efficiency and diseconomies of scale have hindered the development of the hydropower and nuclear power *** addition,the asymmetric effect is not yet significant for the short development time and technical constraints of wind and solar *** the impulse response results,the impact curves of investment in wind and solar power are generally positive,and investment has different degrees of time-delay and time-varying effects on various energy production,which verifies the heterogeneity of investment adjustment mechanisms in different energy industries.

关键词： "Dual Carbon"target fixed-asset investment primary energy NARDL nonlinearity

Provably secure attribute-based authenticated encryption with keyword search from ideal lattices

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Science China(Information Sciences) 2024年第1期67卷 308-309页

作者： Lisha YAO Lin hou jian WENG Feixiang ZHAO College of Cyber Security Jinan University

A public-key authenticated encryption with keyword search(PAEKS)[1, 2] system overcomes the problem of an inside adversary forging searchable ciphertexts and guessing the keyword information from the given token. This system allows the sender to encrypt and authenticate a ***, traditional PAEKS schemes require the sender to specify the intended receiver in advance, losing much flexibility.

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Eco-evolutionary evidence for the global diversity pattern of Cycas(Cycadaceae)

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Journal of Integrative Plant Biology 2024年第6期66卷 1170-1191页

作者： jian Liu Anders JLindstrom Yiqing gong Shanshan Dong Yusheng(Chris)Liu Shouzhou Zhang Xun gong CAS Key Laboratory for Plant Diversity and Biogeography of East Asia Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China Department of Economic Plants and Biotechnology Yunnan Key Laboratory for Wild Plant ResourcesKunming Institute of BotanyChinese Academy of SciencesKunming 650201China University of Chinese Academy of Sciences Beijing 100049China Global Biodiversity Conservancy 144/124 Moo3Soi Bua ThongBangsalaeSattahipChonburi 20250Thailand Key Laboratory of Southern Subtropical Plant Diversity Fairy Lake Botanical GardenShenzhen&Chinese Academy of SciencesShenzhen 518004China Department of Earth and Environmental Sciences Indiana University-IndianapolisIndianapolisIN 46202USA

The evolution of the latitudinal diversity gradient(LDG),characterized by a peak in diversity toward the tropics,has captured significant attention in evolutionary biology and ***,the inverse LDG(i-LDG)mechanism,wherein species richness increases toward the poles,remains inadequately *** are among one of the oldest lineages of extant seed plants and have undergone extensive diversification in the ***,the extant cycad abundance exhibits an i-LDG pattern,and the underlying causes for this phenomenon remain largely ***,using 1,843 nuclear genes from a nearly complete sampling,we conducted comprehensive phylogenomic analyses to establish a robust species-level phylogeny for Cycas,the largest genus within *** then reconstructed the spatial-temporal dynamics and integrated global environmental data to evaluate the roles of species ages,diversification rates,contemporary environment,and conservatism to ancestral niches in shaping the i-LDG *** found Cycas experienced decreased diversification rates,coupled with the cooling temperature since its origin in the Eocene from continental *** regions have distinctively contributed to the formation of i-LDG for Cycas,with the northern hemisphere acting as evolutionary museums and the southern hemisphere serving as ***,water-related climate variables,specifically precipitation seasonality and potential evapotranspiration,were identified as paramount factors constraining Cycas species richness in the rainforest biome near the ***,the adherence to ancestral monsoonal climates emerges as a critical factor in sustaining the diversity *** study underscores the imperative of integrating both evolutionary and ecological approaches to comprehensively unravel the mechanisms underpinning global biodiversity patterns.

关键词： cycads latitudinal diversity gradient niche conservatism spatiotemporal diversification species richness

An efficient schedulability analysis based on worst-case interference time for real-time systems

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Science China(Information Sciences) 2024年第09期67卷 88-104页

作者： Hongbiao LIU Mengfei YANG Lei QIAO Xi CHEN jian gong School of Computer Science and Technology Xidian University China Academy of Space Technology Beijing Institute of Control Engineering

Real-time systems are widely implemented in the Internet of Things(IoT) and safety-critical systems, both of which have generated enormous social value. Aiming at the classic schedulability analysis problem in real-time systems, we proposed an exact Boolean analysis based on interference(EBAI) for schedulability analysis in real-time systems. EBAI is based on worst-case interference time(WCIT), which considers both the release jitter and blocking time of the task. We improved the efficiency of the three existing tests and provided a comprehensive summary of related research results in the field. Abundant experiments were conducted to compare EBAI with other related results. Our evaluation showed that in certain cases, the runtime gain achieved using our analysis method may exceed 73% compared to the stateof-the-art schedulability test. Furthermore, the benefits obtained from our tests grew with the number of tasks, reaching a level suitable for practical application. EBAI is oriented to the five-tuple real-time task model with stronger expression ability and possesses a low runtime overhead. These characteristics make it applicable in various real-time systems such as spacecraft, autonomous vehicles, industrial robots, and traffic command systems.

关键词： five-tuple real-time task model real-time system spacecraft Internet of Things exact schedulability analysis worst-case interference time

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Embedded Majorana islands

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Science China(Physics,Mechanics & Astronomy) 2024年第9期67卷 154-164页

作者： Jin-Xing hou Alex Weststrom Rui Wang Wen-Li Yang jian Li Institute of Modern Physics Northwest UniversityXi’an 710127China Department of Physics School of ScienceWestlake UniversityHangzhou 310030China Shaanxi Key Laboratory for Theoretical Physics Frontiers Xi’an 710127China Institute of Natural Sciences Westlake Institute for Advanced StudyHangzhou 310024China National Laboratory of Solid State Microstructures and Department of Physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center for Advanced Microstructures Nanjing 210093China Peng Huanwu Center for Fundamental Theory Xi’an 710127China

Mesoscopic superconducting islands hosting Majorana zero modes(MZMs),or Majorana islands in short,offer a prototype of topological *** this work we investigate theoretically the model of a generic Majorana island tunneling-coupled to a singlepiece metallic substrate,hence an embedded Majorana *** show the crucial consequences of an interplay between the topological ground states nonlocally addressed by the MZMs and the metallic bath with coherent electron propagation:on the one hand,the topological degeneracy on the Majorana island can be preserved,by virtue of the particle-hole symmetry,despite the apparent bath-induced coupling between MZMs;on the other hand,the electronic interference in the metallic bath may lead to profound alterations to the renormalization group behavior of the hybrid system towards low energy/temperature compared with conventional Kondo *** work serves to establish the model of embedded Majorana islands as an experimentally relevant and theoretically intriguing problem particularly in the direction of topological quantum computation.

关键词： topological quantum computation Majorana zero modes topological qubit mesoscopic superconductor topological Kondo effect

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Stable hydrogen-bonded organic frameworks and their photo-and electro-responses

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Nano Research 2024年第8期17卷 7675-7699页

作者： Ying hou Xin-Song Huang Sheng-Hao gong Chen Liu Yangyang Liu Tian-Fu Liu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China University of Chinese Academy of Sciences Beijing 100049China Department of Chemistry and Biochemistry California State UniversityLos AngelesCalifornia 90032USA College of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350007China

Hydrogen-bonded organic frameworks(HOFs)are a recent class of porous materials that have garnered considerable research interest owing to their distinctive *** can be constructed through judicious selection of H-bonding motifs,which are further enforced by other weak intermolecular interactions such asπ–πstacking,van der Waals forces,and framework *** advantage of these interactions,we can expand the functional field of HOFs by introducing active ***,researchers have made substantial advancements in using HOFs for chemical sensing,catalysis,proton conduction,biological applications,and *** low bonding energy of H-bonds allows for precise control over the concentration of ligands in solvents,forming diverse HOF *** varied structures offer significant advantages for producing HOFs with photo-responsive and electro-responsive ***,the presence of H-bonds in HOFs results in their inherent lower stability compared to metal-organic frameworks(MOFs)and covalent-organic frameworks(COFs)formed via coordination and covalent bonds,*** a result,the pursuit of stable and innovative HOF materials with novel functional sites remains an ongoing *** review provides an overview of recent research progress in the development of new strategies for stable HOF synthesis and applications of HOFs with stimuli-responsive *** first classified all synthetic methods reported to date and discussed the stable HOFs synthesized,as well as their unique properties and *** addition,we summarized the applications of HOFs utilizing their synergistic responses to external stimuli,including photo,electrical,pressure,and chemical *** systematically reviewed stable HOF synthesis and applications,which may lead to a deeper understanding of the structure–activity relationship for these materials and guide future HOF design.

关键词： stable hydrogen-bonded organic frameworks(HOFs) photo-response electro-response photoelectric synergistic response

∼2.5 nm pores in carbon-based cathode promise better zinc-iodine batteries

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Chinese Chemical Letters 2024年第5期35卷 471-476页

作者： Yajun hou Chuanzheng Zhu Qiang Wang Xiaomeng Zhao Kun Luo Zongshuai gong Zhihao Yuan School of Materials Science and Engineering Tianjin Key Laboratory of Photoelectric Materials&DevicesTianjin University of TechnologyTianjin 300384China

The relationship mechanism between the material pore structures and cathodic iodine chemistry plays a vital role in efficient Zn-I_(2) batteries,but is unclear,retarding further *** work innovatively indicates a great contribution of∼2.5nm pore structure of nanocarbons to efficient iodine adsorption,rapid I^(−)↔I_(2) conversion,and polyiodide inhibition,via scrupulously designing catalysts with controllable pore sizes *** I_(2)-loading within the designed nitrogen-doped nanocarbons can reach up to as high as 60.8 wt%.The batteries based on the cathode deliver impressive performances with a large capacity of 178.8 mAh/g and long-term cycling stability more than 4000 h at 5.0 ***,these is no polyiodide such as I_(3)−and I_(5)−detected during the charge-discharge processes from comprehensive electrochemical cyclic voltammetry,X-ray photoelectron spectroscopy,and Raman *** work provides a novel knowledge-guided concept for rational pore design,promising better Zn-I_(2) batteries,which is also hoped to benefit other advanced energy technologies,such as Li-S,Li-ion,and Al-I_(2) batteries.

关键词： Zinc-iodine batteries Structure-performance relationship Iodine conversion chemistry Cathode materials Porous carbon