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Powering the future: A comprehensive review on calcium-ion batteries

Journal of Energy Chemistry 2024年第3期90卷 77-97,I0004页

作者： Ameneh Taghavi-Kahagh hos.ein roghani-mamaqani Mehdi Salami-Kalajahi Faculty of Polymer Engineering Sahand University of TechnologyP.0.Box 51335-1996Tabriz Iran Institute of Polymeric Materials Sahand University of TechnologyP.0.Box 51335-1996Tabriz Iran

Due to concerns regarding the future availability,cost,and safety of lithium in Li-ion batteries(LIBs),researchers are exploring alternative chemistries such as Na-ion,Li-S,Li-air,and multivalent ion *** ion technologies,which utilize divalent or trivalent ions,like Mg^(2+),Ca^(2+),and Al^(3+),show promise in achieving greater energy densities than LIBs due to their ability to deposit uniformly on anodes and intercalate into *** magnesium-ion batteries(MIBs) have been the primary area of research for multivalent ion batteries,the cost-effectiveness and abundance of calcium have sparked a growing interest in calcium-ion batteries(CIBs) in recent *** to LIBs,CIBs have the potential to provide longer cycle life,enhanced safety,and increased energy ***,the development of CIBs comes with several challenges,such as finding suitable electrode and electrolyte materials that ensure the stability and safety of the *** primary hurdle in CIBs lies in the plating/stripping *** is a significant hindrance preventing the occurrence of plating/stripping in CIBs,which lies in the formation of a passive layer resulting from the decomposition of the *** objective of this article is to examine the advancements made in ***,it aims to comprehensively assess the mechanisms and materials employed in various battery components,as well as the obstacles encountered in *** includes recent advancements in electrode materials,electrolytes,cell configurations,and the challenges and opportunities for enhancing the performance and commercial viability of CIBs.

关键词： Ca-ion batteries Cathode Anode Electrolyte

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A COMPREHENSIVE MONTE CARLO SIMULATION OF STYRENE ATOM TRANSFER RADICAL POLYMERIZATION

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Chinese Journal of Polymer Science 2010年第4期28卷 483-497页

作者： Mohammad Najafi hos.ein roghani-mamaqani Mehdi Salami-Kalajahi Vahid Haddadi-Asl International Affairs Research Institute of Petroleum Industry(RIPI)***TehranIran Polymer Engineering Department Amirkabir University of TechnologyP.O.Box 15875-4413TehranIran

An optimized and high-performance Monte Carlo simulation is developed to take thorough account of four different cases of termination in styrene ATRP. According to the simulation results, the bimolecular termination rate constant sharply drops throughout the polymerization when either chain-length dependency of termination rate constant, gel effect, or both together is applied to the simulation. In addition, as expected, the initiator is quickly decomposed at the early stages of the polymerization. The concentration of the catalyst in lower oxidation state decreases at first and then plateaus at higher conversion; furthermore, the steady concentration of Ml^nY/L in the polymerization is the highest when the chain-lengthdependent diffusion-controlled termination rate constant is employed in the simulation. The rates of deactivation and chain end degradation reactions are also smaller in this case. Therefore, the fraction of dormant chains is higher throughout the reaction and consequently the portion of dead polymers decreases. Besides, molecular weight increases linearly with conversion; however, when neither gel effect nor chain-length dependency of termination rate constant is considered, the molecular weight deviates from linearity at the end of the reaction. The peak of chain length distribution shifts toward higher molecular weight too during the reaction. Finally, the molecular weight distribution broadens at higher conversion; however, the chain length distribution of polymers produced under conditions of applying chain-length-dependent diffusion-controlled termination rate constant is narrower.

关键词： Styrene ATRP Monte Carlo simulation Chain length distribution Gel effect Chain-length-dependent termination.

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