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A novel electro-Fenton hybrid system for enhancing the interception of volatile organic compounds in membrane distillation desalination

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Journal of Environmental Sciences 2024年第4期138卷 189-199页

作者： hongxin liu Kuiling Li Kunpeng Wang Zhiyong Wang Zimou liu Sichao Zhu Dan Qu Yu Zhang Jun Wang State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China State Key Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua UniversityBeijing 100084China School of Chemical and Environmental Engineering Beijing CampusChina University of Mining and TechnologyBeijing 100083China Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Membrane distillation(MD)is a promising alternative desalination technology,but the hydrophobic membrane cannot intercept volatile organic compounds(VOCs),resulting in aggravation in the quality of permeate.In term of this,electro-Fenton(EF)was coupled with sweeping gas membrane distillation(SGMD)in a more efficient way to construct an advanced oxidation barrier at the gas-liquid interface,so that the VOCs could be trapped in this layer to guarantee the water quality of the distillate.During the so-called EF-MD process,an interfacial interception barrier containing hydroxyl radical formed on the hydrophobic membrane surface.It contributed to the high phenol rejection of 90.2% with the permeate phenol concentration lower than 1.50 mg/L.Effective interceptions can be achieved in a wide temperature range,even though the permeate flux of phenol was also intensified.The EF-MD system was robust to high salinity and could electrochemically regenerate ferrous ions,which endowed the long-term stability of the system.This novel EF-MD configuration proposed a valuable strategy to intercept VOCs in MD and will broaden the application of MD in hypersaline wastewater treatment.

关键词： Membrane distillation VOC interception Interfacial oxidation Electro-Fenton Hypersaline wastewater

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Strategies and prospects for melatonin to alleviate abiotic stress in horticultural plants

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Horticultural Plant Journal 2024年第3期10卷 601-614页

作者： Xiaoyun Wang Meng Cao hongxin Li Ying liu Shuangxi Fan Na Zhang Yangdong Guo College of Horticulture China Agricultural UniversityBeijing100193China College of Plant Science and Technology Beijing University of AgricultureBeijing102206China Beijing Bei Nong Enterprise Management Co. Ltd.Beijing102206China Sanya Institute of China Agricultural University SanyaHainan572000China

Melatonin is a conserved pleiotropic molecule in animals and plants.Melatonin is involved in many development processes and stress responses;thus,exploring its function in plants,particularly in horticultural plants,has become a rapidly developing field.Many studies have revealed that phytomelatonin acts as a plant biostimulant and increase its tolerance to various abiotic stressors,including extreme temperature,drought,osmotic disturbance,heavy metals,and ultraviolet(UV).Melatonin appears to have roles in the scavenging of reactive oxygen species(ROS)and other free radicals,affecting the primary and secondary metabolism of plants,regulating the transcripts of stress-related enzymes and transcription factors,and crosstalk with other hormones under different environmental conditions.This pleiotropy makes phytomelatonin an attractive regulator to improve resistance to abiotic stress in plants.The recent discovery of the potential phytomelatonin receptor CAND2/PMTR1 and the proposition of putative models related to the phytomelatonin signaling pathways makes phytomelatonin a new plant hormone.Based on relevant studies from our laboratory,this review summarizes the phytomelatonin biosynthetic and metabolic pathways in plants and the latest research progress on phytomelatonin in abiotic stress of horticultural plants.This study will provide a reference for elucidating the regulatory mechanism of phytomelatonin affecting the resistance to abiotic stress in plants.

关键词： Abiotic stress Biostimulant Horticultural plants Phytomelatonin

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A brief review on the recent development of phonon engineering and manipulation at nanoscales

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International Journal of Extreme Manufacturing 2024年第1期6卷 177-206页

作者： Siqi Xie hongxin Zhu Xing Zhang Haidong Wang Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Department of Engineering MechanicsTsinghua UniversityBeijing 100084People’s Republic of China

Phonons are the quantum mechanical descriptions of vibrational modes that manifest themselves in many physical properties of condensed matter systems. As the size of electronic devices continues to decrease below mean free paths of acoustic phonons, the engineering of phonon spectra at the nanoscale becomes an important topic. Phonon manipulation allows for active control and management of heat fow, enabling functions such as regulated heat transport. At the same time, phonon transmission, as a novel signal transmission method, holds great potential to revolutionize modern industry like microelectronics technology, and boasts wide-ranging applications. Unlike fermions such as electrons, polarity regulation is difficult to act on phonons as bosons, making the development of effective phonon modulation methods a daunting task.This work reviews the development of phonon engineering and strategies of phonon manipulation at different scales, reports the latest research progress of nanophononic devices such as thermal rectifiers, thermal transistors, thermal memories, and thermoelectric devices,and analyzes the phonon transport mechanisms involved. Lastly, we survey feasible perspectives and research directions of phonon engineering. Thermoelectric analogies, external field regulation, and acousto-optic co-optimization are expected to become future research hotspots.

关键词： phonon engineering phononic device nanoscale

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Origin of the Yueguang gold deposit in Xinhua, Hunan Province, South China: insights from fl uid inclusion and hydrogen–oxygen stable isotope analysis

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Acta Geochimica 2024年第2期43卷 235-254页

作者： hongxin Fan Qiang Wang Yulong Yang Yao Tang Hao Zou College of Earth Sciences Chengdu University of TechnologyChengdu 610059China College of Earth Sciences Jilin UniversityJilin 130061China

The Yueguang gold deposit is located in Fengjia,Xinhua County,Hunan Province,South China.It represents a recently discovered small-scale gold deposit situated in the southwestern region of the Jiangnan Orogenic Belt,west of the Baimashan granitic batholith.In order to discern the characteristics of the ore-formingﬂuids,the underlying mineralization processes,and establish a foundation for the origin of the Yueguang gold depositﬂuid inclusion micro-thermometry,as well as quartz hydrogen and oxygen isotope analysis,have been carried out on samples obtained from various stages of mineralization.The hydrothermal miner-alization stages within the Yueguang gold deposit can be categorized into three stages:(i)the barren,pre-ore quartz-pyrite stage(Stage Ⅰ),the quartz-pyrite-gold stage(Stage Ⅱ),and the post-ore quartz-carbonate stage(Stage Ⅲ),with the second stage being the main mineralization stage.Theﬂuid inclusions identiﬁed in samples from the main min-eralization stage can predominantly be described with the NaCl–H_(2)O and CO_(2)–NaCl–H_(2)O systems.These inclusions display homogenization temperatures ranging from 158.8 to 334.9℃,and theﬂuid salinity ranges from 0.3%to 4.0%(wt.%NaCl equiv.).Laser Raman spectroscopy analysis of individual inclusions further reveals the presence of gas-phases such as CO_(2),CH_(4),and N_(2).Isotopic analysis indicatesδ^(18)Oﬂuid values ranging from 3.95 to 6.7‰ and δDH_(2)O values ranging from-71.9 to-55.7‰.These results indi-cate that the ore-formingﬂuid of the Yueguang gold deposit belongs to metamorphic hydrothermalﬂuids of middle-low temperature and low salinity.In the process of ore formation,gold is transported in the form of Au(HS)2-complexes,with gold deposition being driven byﬂuid immiscibility.Therefore,the Yueguang gold deposit is categorized as an orogenic gold deposit dominated by metamorphic hydrother-malﬂuid.It may become a new target for gold exploration in the Baimashan region,central Hunan Province.

关键词： Hunan province Yueguang gold deposit Fluid inclusions Hydrogen–oxygen isotopes Laser Raman Fluid immiscibility Orogenic gold deposit

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Chemico-biological conversion of carbon dioxide

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Journal of Energy Chemistry 2024年第2期89卷 371-387,I0009页

作者： Liangwei Hu Junzhu Yang Qi Xia Jin Zhang hongxin Zhao Yuan Lu Zhejiang Province Key Laboratory of Plant Secondary Metabolism and Regulation College of Life Sciences and MedicineZhejiang Sci-Tech UniversityHangzhou 310018ZhejiangChina Key Laboratory of Industrial Biocatalysis Ministry of EducationTsinghua UniversityBeijing 100084China Department of Chemical Engineering Tsinghua UniversityBeijing 100084China College of Biological and Chemical Engineering Jiaxing UniversityJiaxing 314000ZhejiangChina

The unabated carbon dioxide(CO_(2))emission into the atmosphere has exacerbated global climate change,resulting in extreme weather events,biodiversity loss,and an intensified greenhouse effect.To address these challenges and work toward carbon(C)neutrality and reduced CO_(2)emissions,the capture and utilization of CO_(2)have become imperative in both scientific research and industry.One cutting-edge approach to achieving efficient catalytic performance involves integrating green bioconversion and chemical conversion.This innovative strategy offers several advantages,including environmental friendliness,high efficiency,and multi-selectivity.This study provides a comprehensive review of existing technical routes for carbon sequestration(CS)and introduces two novel CS pathways:the electrochemicalbiological hybrid and artificial photosynthesis systems.It also thoroughly examines the synthesis of valuable Cnproducts from the two CS systems employing different catalysts and biocatalysts.As both systems heavily rely on electron transfer,direct and mediated electron transfer has been discussed and summarized in detail.Additionally,this study explores the conditions suitable for different catalysts and assesses the strengths and weaknesses of biocatalysts.We also explored the biocompatibility of the electrode materials and developed novel materials.These materials were specifically engineered to combine with enzymes or microbial cells to solve the biocompatibility problem,while improving the electron transfer efficiency of both.Furthermore,this review summarizes the relevant systems developed in recent years for manufacturing different products,along with their respective production efficiencies,providing a solid database for development in this direction.The novel chemical-biological combination proposed herein holds great promise for the future conversion of CO_(2)into advanced organic compounds.Additionally,it offers exciting prospects for utilizing CO_(2)in synthesizing a wide range of industrial products.Ultimately,t

关键词： Carbon dioxide Bioelectric synthesis Artificial photosynthesis Synthetic product

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Magnetic resonance imaging techniques for lithium-ion batteries:Principles and applications

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Magnetic Resonance Letters 2024年第2期4卷 22-39页

作者： hongxin Lin Yanting Jin Mingming Tao Yingao Zhou Peizhao Shan Danhui Zhao Yong Yang State Key Laboratory for Physical Chemistry of Solid Surfaces Collaborative Innovation Center of Chemistry for Energy Materials and Department of ChemistryCollege of Chemistry and Chemical EngineeringTan Kah Kee Innovation Laboratory(IKKEM)Xiamen UniversityXiamen361005China School of Energy Xiamen UniversityXiamen361005China

Operando monitoring of internal and local electrochemical processes within lithium-ion batteries(LIBs)is crucial,necessitating a range of non-invasive,real-time imaging characterization techniques including nuclear magnetic resonance(NMR)techniques.This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging(MRI)techniques in LIBs.It initially introduces the principles and hardware of MRI,followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes,electrodes and commercial batteries.This encompasses the determination of electrolytes'transport properties,acquisition of ion distribution profile,and diagnosis of battery defects.By focusing on experimental parameters and optimization strategies,our goal is to explore MRI methods suitable to a variety of research subjects,aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs.

关键词： Lithium-ion batteries Magnetic resonance imaging(MRI) Electrolytes Electrodes Commercial batteries

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Evaluation of the nonmarket value of livestock and poultry feces returning to farmland utilization using CVM in Heilongjiang,China

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International Journal of Agricultural and Biological Engineering 2023年第2期16卷 48-56页

作者： Jiajie Shang Yongtao Xie Lifeng Guo Jinxia Fan hongxin liu College of Engineering Northeast Agricultural UniversityHarbin 150036China Key Laboratory of Swine Facilities Engineering Ministry of Agriculture and Rural AffairsHarbin 150036China College of Mechanical and Electrical Engineering Suqian UniversitySuqian 223800JiangsuChina

Aiming at a series of hot issues and topics,such as resource waste,environmental pollution,and Mollisol protection,related to the arbitrary discharge of livestock and poultry feces,livestock and poultry feces are taken as the research object,a questionnaire survey was conducted to investigate residents’cognition and willingness to pay(WTP)for the nonmarket value of livestock and poultry feces returning to farmland in Heilongjiang Province,China.The contingent valuation method(CVM)was used for the correlation analysis of WTP and socioeconomic characteristics,and correlation analysis of payment mode and socioeconomic characteristics.Meanwhile,the factors influencing WTP and payment mode were analyzed.The results show that the majority of the respondents are aware of the harmfulness of the arbitrary discharge of livestock and poultry feces and the importance of its nonmarket regeneration value.Approximately 90.09% of respondents were willing to pay for the return of livestock and poultry feces to fields.In 2020,the total value of WTP of livestock and poultry feces returning to farmland in Heilongjiang Province was 4.65 billion CNY,equivalent to 1.32% of the total agricultural production of Heilongjiang Province in the same year.And the nonmarket value of livestock and poultry feces is estimated to be 1456.69 CNY/t.The annual average WTP of rural and urban households is 286.42 CNY and 422.90 CNY per household,accounting for 0.46% and 0.52% of the average annual income of households,respectively.Therefore,the return of livestock and poultry feces to farmland utilization has a high nonmarket value.The analysis shows that the average annual household income is a significant factor in WTP,and the registered permanent residence type and the average annual household income are significant factors in payment mode.The research results should provide a scientific and theoretical basis for the government’s policy and decision-making on the return of livestock and poultry feces to farmland.

关键词： nonmarket value livestock and poultry feces farmland utilization CVM WTP

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Anomalous valley Hall effect in two-dimensional valleytronic materials

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Chinese Physics B 2024年第4期33卷 2-14页

作者：陈洪欣原晓波任俊峰 School of Physics and Electronics Shandong Normal UniversityJinan 250358China Shandong Provincial Engineering and Technical Center of Light Manipulations&Institute of Materials and Clean Energy Shandong Normal UniversityJinan 250358China

The anomalous valley Hall effect(AVHE)can be used to explore and utilize valley degrees of freedom in materials,which has potential applications in fields such as information storage,quantum computing and optoelectronics.AVHE exists in two-dimensional(2D)materials possessing valley polarization(VP),and such 2D materials usually belong to the hexagonal honeycomb lattice.Therefore,it is necessary to achieve valleytronic materials with VP that are more readily to be synthesized and applicated experimentally.In this topical review,we introduce recent developments on realizing VP as well as AVHE through different methods,i.e.,doping transition metal atoms,building ferrovalley heterostructures and searching for ferrovalley materials.Moreover,2D ferrovalley systems under external modulation are also discussed.2D valleytronic materials with AVHE demonstrate excellent performance and potential applications,which offer the possibility of realizing novel low-energy-consuming devices,facilitating further development of device technology,realizing miniaturization and enhancing functionality of them.

关键词： anomalous valley Hall effect valley polarization valleytronics two-dimensional materials

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Oscillation of Dzyaloshinskii–Moriya interaction driven by weak electric fields

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Chinese Physics B 2024年第2期33卷 487-491页

作者：陈润泽曹安妮王馨苒柳洋杨洪新赵巍胜 Fert Beijing Institute MIIT Key Laboratory of SpintronicsSchool of Integrated Circuit Science and EngineeringBeihang UniversityBeijing 100191China Hefei Innovation Research Institute Beihang UniversityHefei 230013China Beihang-Goertek Joint Microelectronics Institute Qingdao Research InstituteBeihang UniversityQingdao 266000China National Laboratory of Solid State Microstructures School of PhysicsCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China Beijing Microelectronics Technology Institute Beijing 100076China

Dzyaloshinskii–Moriya interaction(DMI) is under extensive investigation considering its crucial status in chiral magnetic orders, such as Néel-type domain wall(DW) and skyrmions. It has been reported that the interfacial DMI originating from Rashba spin–orbit coupling(SOC) can be linearly tuned with strong external electric fields. In this work, we experimentally demonstrate that the strength of DMI exhibits rapid fluctuations, ranging from 10% to 30% of its original value, as a function of applied electric fields in Pt/Co/MgO heterostructures within the small field regime(< 10-2V/nm). Brillouin light scattering(BLS) experiments have been performed to measure DMI, and first-principles calculations show agreement with this observation, which can be explained by the variation in orbital hybridization at the Co/MgO interface in response to the weak electric fields. Our results on voltage control of DMI(VCDMI) suggest that research related to the voltage control of magnetic anisotropy for spin–orbit torque or the motion control of skyrmions might also have to consider the role of the external electric field on DMI as small voltages are generally used for the magnetoresistance detection.

关键词： Dzyaloshinskii-Moriya interaction weak electric field control effect Rashba spin-orbit coupling interfacial orbital hybridization

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Goat casein hydrolysates alleviated insomnia in mice via modulating the level of neurotransmitters and the composition of gut microbiota

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Food Science and Human Wellness 2024年

作者： Ling Mo Huijuan Jing Xiaojing Du Chaochao Zhao Yintao Lin Jie Li hongxin Wang State Key Laboratory of Food Science and Technology Jiangnan University Sweet Inn (Guangzhou) Technology Development Co. Ltd School of Public Health Guilin Medical University School of Food Science and Technology Jiangnan University

Insomnia is associated with neurotransmitters and intestinal dysbiosis. Though studies have demonstrated the ameliorative effects of milk hydrolysates on insomnia， the underlying mechanisms require further exploration. In this study， we investigated how papain hydrolysates of goat casein (CPH) and whey protein (WPH) affected mice’s sleeplessness. Here， we show that CPH effectively improved the total sleep time in 12 h and restoring neurotransmitters (5-hydroxytryptamine (5-HT)， γ-aminobutyric acid (GABA)， dopamine (DA)， and norepinephrine (NE)) in mice. Further gut microbiota analysis revealed a significant increase in the relative abundance of Helicobacter and Escherichia-Shigella and a decrease in the relative abundance of Lactobacillus in the insomnia model mice (Model). Compared to the Model group， both CPH and WPH significantly increased the relative abundance of Akkermansia and Lactobacillus while lowering the relative abundance of Helicobacter and Escherichia-Shigella. Notably， while diazepam (DZP) increased mouse sleep duration， it also increased the relative abundance of Colidextribacter， Parasutterella， Muribaculaceae， and Prevotella. Additionally， the gene expression and protein expression of GABAAreceptor， cAMP-response element binding protein (CREB)， and brain-derived neurotrophic factor (BDNF) were upregulated in the hypothalamus. We also discovered a link between intestinal gut microbiota and neurotransmitters. Overall， our results suggest that goat milk hydrolysates， especially CPH， can effectively improve insomnia， providing a theoretical basis for further experimentation and individualized designs.

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