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Construction of a Cu@hollow TS-1.nanoreactor based on a hierarchical full-spectrum solar light utilization strategy for photothermal synergistic artificial photosynthesis

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Carbon Energy 2024年第2期6卷 25-36页

作者： Sixian Zhu Qiao Zhao hongxia Guo Li Liu Xiao Wang Xiwei Qi Xianguang Meng Wenquan Cui Hebei Key Laboratory for Environment Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshanChina School of Materials Science and Engineering National Institute for Advanced MaterialsTKL of Metal and Molecule-Based Material ChemistryNankai UniversityTianjinChina Hebei Iron and Steel Laboratory TangshanChina

The artificial photosynthesis technology has been recognized as a promising solution for CO_(2) *** catalysis has been proposed as a novel strategy to promote the efficiency of artificial photosynthesis by coupling both photochemistry and ***,strategies for maximizing the use of solar spectra with different frequencies in photothermal catalysis are urgently ***,a hierarchical full-spectrum solar light utilization strategy is *** on this strategy,a Cu@hollow titanium silicalite-1.zeolite(TS-1.nanoreactor with spatially separated photo/thermal catalytic sites is designed to realize high-efficiency photothermal catalytic artificial *** space-time yield of alcohol products over the optimal catalyst reached 64.4μmol g−1.h−1.with the selectivity of CH3CH2OH of 69.5%.This rationally designed hierarchical utilization strategy for solar light can be summarized as follows:(1.high-energy ultraviolet light is utilized to drive the initial and difficult CO_(2) activation step on the TS-1.shell;(2)visible light can induce the localized surface plasmon resonance effect on plasmonic Cu to generate hot electrons for H2O dissociation and subsequent reaction steps;and(3)low-energy near-infrared light is converted into heat by the simulated greenhouse effect by cavities to accelerate the carrier *** work provides some scientific and experimental bases for research on novel,highly efficient photothermal catalysts for artificial photosynthesis.

关键词： artificial photosynthesis full spectrum nanoreactors photothermal catalysis

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The exploration and practice of low-altitude airspace flight service and traffic management in China

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Green Energy and Intelligent Transportation 2024年第2期3卷 1-8页

作者： Xiangmin Guan hongxia Shi Dongsong Xu Binhua Zhang Jian Wei Jun Chen CAAC Key Laboratory of General Aviation Operation Department of General AviationCivil Aviation Management Institute of ChinaBeijing 100102China Research Institute of Civil Aviation Regulations and Standardization China Academy of Civil Aviation Science and TechnologyBeijing 100028China Department of Technology Platform Phoenix Wings Technology(Shen zhen)Co.LtdShenZhen 518054China Shenzhen Highgreat Innovation Technology Development Co. Ltd dShenzhen 518000China School of Engineering and Materials Science Queen Mary University of LondonLondonE14NSUK

Due to the inherent nature of being highly digitalized,networked and intelligent,Unmanned Aerial System(UAS)operations pose a huge challenge to traditional aviation regulation and technical *** to keep safe,efficient and integrated operation for different Airspace users has become a pressing issue faced by civil aviation around the *** paper focuses on the main operational scenarios and characteristics of unmanned aviation development in *** operational characteristics and associated challenges due to diverse low-altitude users are analyzed,including operation concepts,UAS traffic management,technological test and verification,and *** light on the practices in Europe and the United States,this paper summarizes China's practices and progress in low-altitude operations management,and analyzes future technological development needs and trends,as well as feasible implementation pathways and measures based on actual needs.

关键词： UAS Low-altitude airspace UAS traffic management Exploration and practice

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Frost Resistance of Pervious Concrete Mixed with Waste Glass Powder

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1325-1336页

作者： AN Baofeng LI Qiong QIAO hongxia SU Rui WANG Xi WANG Chaoqun JIAO Daowei School of Civil Engineering Lanzhou University of TechnologyLanzhou 730050China Gansu Advanced Civil Engineering Materials Engineering Research Center Lanzhou 730050China China Construction First Group The Fifth Construction Co.Ltd Beijing 100000China

The contents of waste glass powder(WGP)(0%,1.%,1.%,20%,25%)and water-binder ratio(W/C)(0.24,0.26,0.28)were used as influencing factors,and the quality loss rate(Δm)and compressive strength loss rate(Δfc)were used as characterization *** Ca/Si ratio and main element contents of C-S-H gels with different WGP content were investigated by energy dispersive spectrometry(EDS).The pore structure evolution characteristics of WGP composite cementing materials were investigated by low field nuclear magnetic resonance(NMR).UsingΔfc as the index of frost resistance degradation and Weibull function,the frost resistance degradation of glass doped pervious concrete(WGP-PC)was *** results show that,with WGP,for the same number of cycles,Δm andΔfc decrease and increase with the increase of *** the same WGP content,Δm andΔfc decrease first and then increase with the increase of W/*** 1.0 freeze-thaw cycles,the samples with WGP content of 20%and W/C of 0.26 have the best *** tests show that with the increase of WGP content,the Ca/Si ratio of C-S-H gel decreases at first and then increases with the increase of WGP *** extreme value of Ca/Si is 2.36 when WGP is added by 20%.The pore volume of hardened paste with 20%WGP content decreased by 1..6%compared with that of cement system without *** overall compactness of the specimen was *** the basis of the test data,a life prediction model was established according to Weibull *** experiment showed thatΔfc could be used as a durability degradation index,and the slope of the reliability curve became gentle after WGP was added,which reduced the damage degradation rate of PC.W/C was ***'s about 5000 hours.

关键词： pervious concrete glass powder frost resistance energy dispersive analysis test low field nuclear magnetic resonance instrument life prediction

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Autophagy-targeting modulation to promote peripheral nerve regeneration

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Neural Regeneration Research 2025年第7期20卷 1864-1882页

作者： Yan Chen hongxia Deng Nannan Zhang Department of Obstetrics and Gynecology West China Second HospitalSichuan UniversityChengduSichuan ProvinceChina Key Laboratory of Birth Defects and Women and Children’s Diseases Ministry of EducationSichuan UniversityChengduSichuan ProvinceChina Laboratory of Reproductive Endocrinology and Reproductive Regulation Sichuan UniversityChengduSichuan ProvinceChina National Center for Birth Defect Monitoring West China Second University HospitalSichuan UniversityChengduSichuan ProvinceChina

Nerve regeneration following traumatic peripheral nerve injuries and neuropathies is a complex process modulated by diverse factors and intricate molecular *** studies have focused on factors that stimulate axonal outgrowth and myelin ***,recent studies have highlighted the pivotal role of autophagy in peripheral nerve regeneration,particularly in the context of traumatic ***,autophagy-targeting modulation has emerged as a promising therapeutic approach to enhancing peripheral nerve *** current understanding suggests that activating autophagy facilitates the rapid clearance of damaged axons and myelin sheaths,thereby enhancing neuronal survival and mitigating injury-induced oxidative stress and *** actions collectively contribute to creating a favorable microenvironment for structural and functional nerve regeneration.A range of autophagyinducing drugs and interventions have demonstrated beneficial effects in alleviating peripheral neuropathy and promoting nerve regeneration in preclinical models of traumatic peripheral nerve *** review delves into the regulation of autophagy in cell types involved in peripheral nerve regeneration,summarizing the potential drugs and interventions that can be harnessed to promote this *** hope that our review will offer novel insights and perspectives on the exploitation of autophagy pathways in the treatment of peripheral nerve injuries and neuropathies.

关键词： autophagy autophagy related genes Charcot–Marie–Tooth diseases diabetic peripheral neuropathy metformin myelination peripheral nerve injury Schwann cells sciatic nerve Wallerian degeneration

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Toward understanding the cross-linking from molecular chains to aggregates by engineering terminals of supramolecular hyperbranched polysiloxane

Aggregate

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Aggregate 2024年第1期5卷 228-235页

作者： Yuanbo Zhang Junshan Yuan Jingzhi Hu Zhixuan Tian Weixu Feng hongxia Yan Shaanxi Key Laboratory of Macromolecular Science and Technology Xi’an Key Laboratory of Hybrid Lumines-cent Materials and Photonic DeviceSchool of Chemistry and Chemical engineeringNorthwestern Polytechnical UniversityXi’anChina

Crosslinking thermosets with hyperbranched polymers confers them superior comprehensive ***,it still remains a further understanding of polymer crosslinking from the molecular chains to the role of *** this study,three hyperbranched polysiloxane structures(HBPSi-R)are synthesized as model macromolecules,each featuring distinct terminal groups(R denotes amino,epoxy,and vinyl groups)while similar molecular backbone(Si-O-C).These structures were subsequently copolymerized with epoxy monomers to construct interpenetrating HBPSi-R/epoxy/anhydride co-polymer *** spatial molecular configuration and flexible Si-O-C branches of HBPSi-R endow them with remarkable reinforcement and toughening ***,an optimum impact strength of 28.9 kJ mol^(−1. is achieved with a mere 3%loading of HBPSi-V,nearly three times that of the native epoxy(1..9 kJ mol^(−1.).By contrasting the terminal effects,the aggregation states and crosslinking modes were proposed,thus clarifying the supramolecular-dominant aggregation mechanism and covalent-dominant dispersion mechanism,which influences the resulting material *** work underscores the significance of aggregate science in comprehending polymer crosslinking and provides theoretical insights for tailoring material properties at a refined molecular level in the field of polymer science.

关键词： aggregates crosslinking hyperbranched polymers

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Effects of Using Municipal Solid Waste Incineration Tailings as Lightweight Aggregate on the Mechanical Properties of Specified Density Concrete

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1229-1245页

作者： SHANG Minggang FENG Qiong ZHANG Yunsheng HE Zhongmao QIAO hongxia XUE Cuizhen WANG Jinpen HAN Yuehui School of Civil Engineering Lanzhou University of TechnologyLanzhou 730050China Gansu Advanced Civil Engineering Materials Engineering Research Center Lanzhou 730050China College of Science&Technology Ningbo UniversityNingbo 315211China

Municipal solid waste incineration tailings were used as lightweight aggregate(MSWIT-LA)in the preparation of specified density concrete to study the effects on compressive strength,axial compressive strength,flexural strength,microhardness,total number of pores,pore area,and pore *** results showed that the internal curing and morphological effects induced by an appropriate quantity of MSWIT-LA improved the compressive response of specified density concrete specimens,whereas an excessive quantity of MSWIT-LA significantly reduced their mechanical *** analysis of pore structure indicated that the addition of MSWIT-LA increased the total quantity of pores and promoted cement hydration,resulting in a denser microstructure than that of ordinary *** results of a principal component analysis showed that the mechanical response of specified density concrete prepared with 25%MSWIT-LA was superior to that of an equivalent ordinary *** was therefore concluded that MSWIT-LA can be feasibly applied to achieve excellent specified density concrete properties while utilising municipal solid waste incineration tailings to protect the environment and alleviate shortages of sand and gravel resources.

关键词： municipal solid waste incineration tailings X-ray computed tomography lightweight aggregate microhardness principal component analysis

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A lateral-immobilization zebrafish microfluidic chip-based system for in vivo real-time evaluation of antithrombotic agents

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Chinese Chemical Letters 2024年第3期35卷 312-315页

作者： Lijuan He hongxia Du Yi Yang Zhihua Guan Jinjin Li Honglin Li Xudong Lin Lili Zhu Shanghai Key Laboratory of New Drug Design School of PharmacyEast China University of Science&TechnologyShanghai 200237China Guangdong Provincial Key Laboratory of Sensor Technology and Biomedical Instrument School of Biomedical EngineeringShenzhen Campus of Sun Yat-sen UniversityShenzhen 518000China Innovation Center for AI and Drug Discovery East China Normal UniversityShanghai 200062China

Thrombosis remains a major global health concern mainly characterized by high rates of morbidity and *** models serve as an indispensable tool to understand the underlying pathogenesis of thrombosis and assess the efficacy of novel antithrombotic ***,zebrafish has emerged as a valuable model organism for thrombosis ***,the traditional method of studying zebrafish thrombosis requires a laborious and time-consuming procedure,including anesthesia and manual immobilization of *** this study,based on hydrodynamic force,a lateral-immobilization zebrafish microfluidic chip(LIZMC)was designed to evaluate the cardiovascular system of multiple larvae within a single microscope field of ***,coupling with microscope imaging,real-time monitoring of the peripheral blood circulation in the tail of phenylhydrazine(PHZ)-induced zebrafish thrombosis was ***,the reliability of LIZMC for in vivo evaluation of antithrombotic agents in zebrafish was verified using ***,this novel LIZMC-based system can be used for in vivo zebrafish thrombosis studies and rapid screening of antithrombotic agents.

关键词： Microfluidic chip Zebrafish Thrombosis In vivo evaluation Real-time monitor

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Volumetric and viscometric properties of aqueous 1.2-dimethylethylenediamine solution for carbon capture application

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Petroleum 2024年第2期10卷 326-337页

作者： Hossein Haghani Teerawat Sema Pipat Na Ranong Thanthip Kiattinirachara Benjapon Chalermsinsuwan hongxia Gao Zhiwu Liang Paitoon Tontiwachwuthikul Department of Chemical Technology Faculty of ScienceChulalongkorn UniversityBangkok10330Thailand Center of Excellence on Petrochemical and Materials Technology Chulalongkorn UniversityBangkok10330Thailand Department of Chemical Engineering Faculty of EngineeringMahidol UniversityNakhon Pathom73170Thailand Joint International Center for CO_(2)Capture and Storage(iCCS) Provincial Hunan Key Laboratory for Cost-effective Utilization of Fossil Fuel Aimed at Reducing CO_(2)EmissionsCollege of Chemistry and Chemical EngineeringHunan UniversityChangsha410082PR China Clean Energy Technologies Research Institute(CETRi) Faculty of Engineering and Applied ScienceUniversity of ReginaSKS4S0A2Canada

The present work investigates the volumetric and viscometric properties of an aqueous solution of 1.2-dimethylethylenediamine(DEEDA)over an entire concentration range and an absorber operating temperature range of 31..1.K-333.1.K at atmospheric *** investigated volumetric properties included the density,excess molar volume,partial molar volume,and the investigated viscometric properties included the viscosity,viscosity deviation,free energy for activation of viscous flow,excess free energy for activation of viscous flow,and excess entropy for activation of viscous *** results indicated that there are strong intermolecular interactions and suitable molecular packing in the binary DEEDA-water ***,the mixture was found to deviate from a real mixture according to the calculated excess *** DEEDA solvent's preliminary volumetric and viscometric properties revealed convincing potential as a novel amine for carbon ***,the Redlich-Kister-based correlations showed favorable correlative performance for excess molar volume,viscosity deviation,and excess entropy for activation of viscous flow.

关键词： Density Viscosity Excess property Amine Carbon capture

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Enhancing electromagnetic wave absorption with core‐shell structured SiO_(2)@MXene@MoS_(2)nanospheres

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Carbon Energy 2024年第8期6卷 90-104页

作者： Xuewen Jiang Qian Wang Limeng Song hongxia Lu Hongliang Xu Gang Shao Hailong Wang Rui Zhang Changan Wang Bingbing Fan School of Material Science and Engineering Zhengzhou UniversityZhengzhouHenanChina Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhouHenanChina School of Materials Science and Engineering Tsinghua UniversityBeijingChina

Material composition and structural design are important factors influencing the electromagnetic wave(EMW)absorption performance of *** alleviate the impedance mismatch attributed to the high dielectric constant of Ti_(3)C_(2)T_(x)MXene,we have successfully synthesized core‐shell structured SiO_(2)@MXene@MoS_(2)*** architecture,comprising SiO_(2)as the core,MXene as the intermediate layer,and MoS_(2)as the outer shell,is achieved through an electrostatic self‐assembly method combined with a hydrothermal *** complex core‐shell structure not only provides a variety of loss mechanisms that effectively dissipate electromagnetic energy but also prevents self‐aggregation of MXene and MoS_(2)***,the synergistic combination of SiO_(2)and MoS_(2)with highly conductive MXene enables the suitable dielectric constant of the composites,ensuring optimal impedance ***,the core‐shell structured SiO_(2)@MXene@MoS_(2)nanospheres exhibit excellent EMW absorption performance,featuring a remarkable minimum reflection loss(RL_(min))of−52.1. dB(2.4 mm).It is noteworthy that these nanospheres achieve an ultra‐wide effective absorption bandwidth(EAB)of 6.72 *** work provides a novel approach for designing and synthesizing high‐performance EMW absorbers characterized by“wide bandwidth and strong reflection loss.”

关键词： core‐shell structure electromagnetic wave absorption multiloss mechanism SiO_(2)@MXene@MoS_(2)

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Woven fabric triboelectric nanogenerators for human-computer interaction and physical health monitoring

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Nano Research 2024年第6期17卷 5540-5548页

作者： Yu Miao Mengjuan Zhou Jia Yi Yanyan Wang Guangjin Tian hongxia Zhang Wenlong Huang Wenhao Wang Ronghui Wu Liyun Ma College of Textile and Clothing Xinjiang UniversityUrumqi 830046China College of Textiles Donghua UniversityShanghai 201620China College of Physics Xiamen UniversityXiamen 201620China Department of Bioengineering Imperial College LondonLondon SW72AZUK

Triboelectric nanogenerator(TENG)converts mechanical energy into valuable electrical energy,offering a solution for future energy *** an indispensable part of TENG,textile TENG(T-TENG)has incredible advantages in harvesting biomechanical energy and physiological signal ***,the application of T-TENG is restricted,partly because the fabric structure parameter and structure on T-TENG performance have not been fully *** study comprehensively investigates the effect of weaving structure on fabric TENGs(F-TENGs)for direct-weaving yarn TENGs and post-coating fabric *** direct-weaving F-TENGs,a single-yarn TENG(Y-TENG)with a core-sheath structure is fabricated using conductive yarn as the core layer yarn and polytetrafluoroethylene(PTFE)filaments as the sheath *** fabrics with five different sets of parameters were designed and *** post-coating F-TENGs,fabrics with weaving structures of plain,twill,satin,and reinforced twill were fabricated and coated with conductive silver ***,the twill F-TENGs have the best electrical outputs,followed by the satin F-TENGs and plain weave ***,the increase of the Y-TENG gap spacing was demonstrated to improve the electrical output ***,T-TENGs are demonstrated for human-computer interaction and self-powered real-time *** systematic work provides guidance for the future T-TENG’s design.

关键词： single-yarn triboelectric nanogenerators woven fabric triboelectric nanogenerators fabric weaving structures and parameters human-computer interaction physical health monitoring

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