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Unveiling the geometric site dependent activity of spinel Co_(3)O_(4)for electrocatalytic chlorine evolution reaction

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Journal of Energy Chemistry 2024年第5期92卷 95-103页

作者： Linke Cai Yao Liu Jingfang Zhang Qiqi Jia Jiacheng Guan hongwei sun Yu Yu Yi Huang Key Laboratory of Pesticide&Chemical Biology of Ministry of Education Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction of Ministry of EducationCollege of ChemistryCentral China Normal UniversityWuhan 430079HubeiChina Key Laboratory of Green Chemical Engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationHubei Key Laboratory of Novel Reactor and Green Chemical TechnologySchool of Chemical Engineering&PharmacyWuhan Institute of TechnologyWuhan 430205HubeiChina College of Materials Science and Engineering Fuzhou UniversityFuzhou 350108FujianChina School of Chemistry and Chemical Engineering Anhui UniversityHefei 230601AnhuiChina

Spinel cobalt oxide(Co_(3)O_(4)),consisting of tetrahedral Co^(2+)(CoTd)and octahedral Co^(3+)(CoOh),is considered as promising earth-abundant electrocatalyst for chlorine evolution reaction(CER).Identifying the catalytic contribution of geometric Co site in the electrocatalytic CER plays a pivotal role to precisely modulate electronic configuration of active Co sites to boost CER.Herein,combining density functional theory calculations and experiment results assisted with operando analysis,we found that the Co_(Oh) site acts as the main active site for CER in spinel Co_(3)O_(4),which shows better Cl^(-)adsorption and more moderate intermediate adsorption toward CER than CoTd site,and does not undergo redox transition under CER condition at applied potentials.Guided by above findings,the oxygen vacancies were further introduced into the Co_(3)O_(4) to precisely manipulate the electronic configuration of Co_(Oh) to boost Cl^(-)adsorption and optimize the reaction path of CER and thus to enhance the intrinsic CER activity significantly.Our work figures out the importance of geometric configuration dependent CER activity,shedding light on the rational design of advanced electrocatalysts from geometric configuration optimization at the atomic level.

关键词： Chlorine evolution reaction Geometry effects Active chlorine Electronic configuration optimization Spinel oxides

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Symmetry dependent activation and reactivity of peroxysulfates on FeS_(2)(001)surface

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Science Bulletin 2024年第2期69卷 154-158页

作者： Cancan Ling Meiqi Li Hao Li Xiufan Liu Guangming Zhan hongwei sun Chuan Liang Yaling Li Bing Zhou Jincai Zhao Lizhi Zhang School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of Pesticide&Chemical Biology of Ministry of Education Institute of Environmental&Applied ChemistryCentral China Normal UniversityWuhan 430079China

Heterogeneous peroxysulfates-based advanced oxidation processes(AOPs)have garnered significant attention for purifying organic wastewater since they offer many advantages like low cost,safe storage,facile activation and reactive species participation[1].Nonradical and radical pathways have been proposed to be involved in peroxysulfates activation.

关键词： activation radical reactivity

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Identification of fractional order Hammerstein models based on mixed signals

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Journal of Control and Decision 2024年第1期11卷 132-138页

作者： Mengqi sun hongwei Wang Qian Zhang School of Control Science and Engineering Dalian University of TechnologyDalianPeople’s Republic of China School of Electrical Engineering Xinjiang UniversityUrumqiPeople’s Republic of China

An algorithm based on mixed signals is proposed,to solve the issues of low accuracy of identification algorithm,immeasurable intermediate variables of fractional order Hammerstein model,and how to determine the magnitude of fractional order.In this paper,a special mixed input signal is designed to separate the nonlinear and linear parts of the fractional order Hammerstein model so that each part can be identified independently.The nonlinear part is fitted by the neural fuzzy network model,which avoids the limitation of polynomial fitting and broadens the application range of nonlinear models.In addition,the multi-innovation Levenberg-Marquardt(MILM)algorithm and auxiliary recursive least square algorithm are innovatively integrated into the parameter identification algorithm of the fractional order Hammerstein model to obtain more accurate identification results.A simulation example is given to verify the accuracy and effectiveness of the proposed method.

关键词： Mixed signal fractional order Hammerstein model neural fuzzy network model multi-innovation Levenberg-Marquardt algorithm

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Comprehensive Exergoeconomic Analysis and Optimization of a Novel Zero-Carbon-Emission Multi-Generation System based on Carbon Dioxide Cycle

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Journal of Thermal Science 2024年第3期33卷 1065-1081页

作者： sun Yan LI hongwei WANG Di DU Changhe School of Energy and Power Engineering Northeast Electric Power UniversityJilin132012China School of Automation Engineering Northeast Electric Power UniversityJilin132012China Xi’an Institute of Electromechanical Information Technology Xi’an710065China

This paper aims to conduct a comprehensive exergoeconomic analysis of a novel zero-carbon-emission multi-generation system and propose a fast optimization method combined with machine learning.The detailed exergoeconomic analysis of a novel combined power,freshwater and cooling multi-generation system is performed in this study.The exergoeconomic analysis model is established by exergy flow theory.A comprehensive exergy,exergoeconomic and environmental analysis is carried out.Five critical decision variables are researched to bring out effects on the multi-generation system exergoeconomic performance.A novel fast optimization method combining genetic algorithm and Bagging neural network is proposed.The advanced nature comparison is made between the proposed system and four similar cases.Results display that increasing the turbine inlet temperature can improve exergy efficiency and decrease the total product unit cost.The multi-generation system exergy destruction directly determines exergy efficiency and total exergy destruction cost rate.The total product unit cost in the cost optimal design case is reduced by 7.7%and 25%,respectively,compared with exergy efficiency optimal design case and basic design case.Compared with four similar cases,the proposed multi-generation system has great advantages in thermodynamic performance and exergoeconomic performance.This paper can provide research methods and ideas for performance analysis and fast optimization of multi-generation system.

关键词： waste heat recovery exergoeconomic analysis supercritical carbon dioxide optimization machine learning

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Application of system identification in a practical active noise control system

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Control Theory and Technology 2024年第2期22卷 282-291页

作者： Yu Yuan Zhaoyang sun hongwei Zhang School of Mechanical Engineering Xihua UniversityChengdu610039SichuanChina School of Electrical Engineering Southwest Jiaotong UniversityChengdu611756SichuanChina School of Mechanical Engineering and Automation Harbin Institute of TechnologyShenzhen518055GuangdongChina

Noise pollution has become increasingly severe around the world due to fast urbanization. How to soundproof windows from outside noise is of significant interest for both academia and industry. This paper reports an experimental implementation of normalized minmax active noise control (ANC) algorithm on an open window system, where identifying the model of acoustic sound paths plays a central role. By doing this, traffic noise is attenuated by the ANC system, leading to a relatively quiet indoor environment, while the natural lighting and ventilation functions of a window are remained. Our experiments show that an average of 19 dB(A) noise reduction is achieved.

关键词： Active noise control Multi-input-multi-output system Normalized minimax algorithm System identification

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Computing-aware network (CAN): a systematic design of computing and network convergence

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Frontiers of Information Technology & Electronic Engineering 2024年第5期25卷 633-644页

作者： Xiaoyun WANG Xiaodong DUAN Kehan YAO Tao sun Peng LIU hongwei YANG Zhiqiang LI China Mobile Communications Corporation Beijing 100032China China Mobile Research Institute Beijing 100053China

The coverage of network resources is increasingly extensive,and computing resources have likewise gradually become fundamental infrastructures,providing ubiquitous computing services.However,in wide area networks(WANs),the underlying network and computing resources are not closely investigated or co-designed,and there are still problems reflected in slow computing service scheduling,inflexible data distribution,and inefficient data transmission.

关键词： computing network service

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Sugarcane leaves-derived polyphenols alleviate metabolic syndrome and modulate gut microbiota of ob/ob mice

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Food Science and Human Wellness 2024年第2期13卷 633-648页

作者： Li sun Tao Wang Baosong Chen Cui Guo Shanshan Qiao Jinghan Lin Huan Liao Huanqin Dai Bin Wang Jingzu sun hongwei Liu State Key Laboratory of Mycology Institute of MicrobiologyChinese Academy of SciencesBeijing 100101China Savaid Medicine School University of Chinese Academy of SciencesBeijing 100101China Guangxi Academy of Sciences Nanning 530007China

Sugarcane leaves-derived polyphenols(SLP)have been demonstrated to have diverse health-promoting benefits,but the mechanism of action has not been fully elucidated.This study aimed to investigate the anti-metabolic disease effects of SLP and the underlying mechanisms in mice.In the current study,we prepared the SLP mainly consisting of three flavonoid glycosides,three phenol derivatives,and two lignans including one new compound,and further demonstrated that SLP reduced body weight gain and fat accumulation,improved glucose and lipid metabolism disorders,ameliorated hepatic steatosis,and regulated short-chain fatty acids(SCFAs)production and secondary bile acids metabolism in ob/ob mice.Notably,SLP largely altered the gut microbiota composition,especially enriching the commensal bacteria Akkermansia muciniphila and Bacteroides acidifaciens.Oral gavage with the above two strains ameliorated metabolic syndrome(MetS),regulated secondary bile acid metabolism,and increased the production of SCFAs in high-fat diet(HFD)-induced obese mice.These results demonstrated that SLP could be used as a prebiotic to attenuate MetS via regulating gut microbiota composition and further activating the secondary bile acids-mediated gut-adipose axis.

关键词： Sugarcane leaves-derived polyphenols Metabolic syndrome Bacteroides acidifaciens Akkermansia muciniphila Secondary bile acids metabolism

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Pythagorean Theorem & Curvature with Lower or Upper Bound

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Chinese Annals of Mathematics,Series B 2022年第1期43卷 95-114页

作者： Xiaole SU hongwei sun Yusheng WANG School of Mathematical Sciences(and Lab.math.Com.Sys.) Beijing Normal UniversityBeijing100875China School of Mathematics Science Capital Normal UniversityBeijing100037China

In this paper,the authors give a comparison version of Pythagorean theo-rem to judge the lower or upper bound of the curvature of Alexandrov spaces(including Riemannian manifolds).

关键词： Pythagorean theorem Alexandrov space Toponogov's theorem

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Reduced-order modeling and vibration transfer analysis of a fluid-delivering branch pipeline that consider fluid–solid interactions

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Frontiers of Mechanical Engineering 2024年第2期19卷 75-97页

作者： Wenhao JI hongwei MA Wei sun Yinhang CAO School of Mechanical Engineering and Automation Northeastern UniversityShenyang 110819China Key Laboratory of Vibration and Control of Aero-Propulsion Systems(Ministry of Education) Northeastern UniversityShenyang 110819China College of Power and Energy Engineering Harbin Engineering UniversityHarbin 150001China

The efficient dynamic modeling and vibration transfer analysis of a fluid-delivering branch pipeline(FDBP)are essential for analyzing vibration coupling effects and implementing vibration reduction optimization.Therefore,this study proposes a reduced-order dynamic modeling method suitable for FDBPs and then analyzes the vibration transfer characteristics.For the modeling method,the finite element method and absorbing transfer matrix method(ATMM)are integrated,considering the fluid–structure coupling effect and fluid disturbances.The dual-domain dynamic substructure method is developed to perform the reduced-order modeling of FDBP,and ATMM is adopted to reduce the matrix order when solving fluid disturbances.Furthermore,the modeling method is validated by experiments on an H-shaped branch pipeline.Finally,transient and steady-state vibration transfer analyses of FDBP are performed,and the effects of branch locations on natural characteristics and vibration transfer behavior are analyzed.Results show that transient vibration transfer represents the transfer and conversion of the kinematic,strain,and damping energies,while steady-state vibration transfer characteristics are related to the vibration mode.In addition,multiple-order mode exchanges are triggered when branch locations vary in frequency-shift regions,and the mode-exchange regions are also the transformation ones for vibration transfer patterns.

关键词： fluid-delivering branch pipeline vibration transfer analysis reduced-order modeling fluid-solid interactions finite element method absorbing transfer matrix method

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Residual fluoride self-activated effect enabling upgraded utilization of recycled graphite anode

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Journal of Energy Chemistry 2024年第6期93卷 24-31,I0002页

作者： Shuzhe Yang Qingqing Gao Yukun Li hongwei Cai Xiaodan Li Gaoxing sun Shuxin Zhuang Yujin Tong Hao Luo Mi Lu School of Materials Science and Engineering Xiamen University of TechnologyXiamen 361024FujianChina Faculty of Physics University of Duisburg-EssenDuisburg D-47057Germany

Recycling graphite anode from spent lithium-ion batteries(SLIBs)is regarded as a crucial approach to promoting sustainable energy storage industry.However,the recycled graphite(RG)generally presents degraded structure and performance.Herein,the residual fluoride self-activated effect is proposed for the upgraded utilization of RG.Simple and low-energy water immersion treatment not only widens the interlayer spacing,but also retains appropriate fluoride on the surface of RG.Theoretical analysis and experiments demonstrate that the residual fluoride can optimize Li~+migration and deposition kinetics,resulting in better Li~+intercalation/deintercalation in the interlayer and more stable Li metal plating/stripping on the surface of RG,As a result,the designed LFP||RG full cells achieve ultrahigh reversibility(~100%Coulombic efficiency),high capacity retention(67%after 200 cycles,0.85 N/P ratio),and commendable adaptability(stable cycling without short-circuiting,0.15 N/P ratio).The energy density is improved from 334 Wh kg^(-1)of 1.1 N/P ratio to 367 Wh kg^(-1)of 0.85 N/P ratio(total mass based on cathode and anode).The exploration of RG by residual fluoride self-activated effect achieves upgraded utilization beyond fresh commercial graphite and highlights a new strategy for efficient reuse of SLIBs.

关键词： Spent lithium-ion batteries Recycled graphite anode Fluoride Self-activated effect Upgraded utilization

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