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Perception of fundamental science to boost lithium metal anodes toward practical application

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Green Energy & Environment 2024年第3期9卷 454-472页

作者： Jinkun Wang Li Wang hong xu Li Sheng Xiangming He Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing100084China

As a key material for lithium metal batteries(LMBs),lithium metal is one of the most promising anode materials to break the bottleneck of battery energy density and a commonly used active material for reference *** lithium anodes are regarded as the holy grail of lithium batteries,decades of exploration have not led to the successful commercialization of LMBs,due mainly to the challenges related to the inherent properties of lithium *** pave the way for further investigation,herein,a comprehensive review focusing on the fundamental science of lithium are ***,the natures of lithium atoms and their isotopes,lithium clusters and lithium crystals are revisited,especially their structural and energetic ***,the electrochemical properties of lithium metal are *** important concepts and scientific questions,including the electronic structure of lithium,influence of high pressure and low temperature on the properties of lithium,factors influencing lithium deposition,generation of lithium dendrites,and electrode potential of lithium in different electrolytes,are explained and analyzed in *** to improve the performance of lithium anodes and thoughtfulness about the electrode potential in lithium battery research are proposed.

关键词： Lithium Cluster Crystal Physicochemical property Fundamental science

A seismic elastic moduli module for the measurements of low-frequency wave dispersion and attenuation of fluid-saturated rocks under different pressures

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Petroleum Science 2024年第1期21卷 162-181页

作者： Yan-Xiao He Shang-xu Wang gen-Yang Tang Chao Sun hong-Bing Li San-Yi Yuan Xian Wei Li-Deng Gan Xiao-Feng Dai Qiang Ge Peng-Peng Wei Hui-Qing Zhang National Key Laboratory of Petroleum Resources and Engineering CNPC Key Lab of Geophysical ExplorationCollege of GeophysicsChina University of Petroleum(Beijing)Beijing102249China School of Resources and Geosciences China University of Mining and TechnologyXuzhou221116JiangsuChina Research Institute of Petroleum Exploration and Development CNPCBeijing100083China Beijing Vocational College of Labour and Social Security Beijing100029China PetroChina Dagang Oilfield Exploration and Development Research Institute CNPCTianjin300280China

Knowledge about the seismic elastic modulus dispersion,and associated attenuation,in fluid-saturated rocks is essential for better interpretation of seismic observations taken as part of hydrocarbon identification and time-lapse seismic surveillance of both conventional and unconventional reservoir and overburden performances.A Seismic Elastic Moduli Module has been developed,based on the forced-oscillations method,to experimentally investigate the frequency dependence of Young's modulus and Poisson's ratio,as well as the inferred attenuation,of cylindrical samples under different confining pressure *** with three standard samples showed that the measured elastic moduli were consistent with the published data,indicating that the new apparatus can operate reliably over a wide frequency range of f∈[1-2000,10^(6)]*** Young's modulus and Poisson's ratio of the shale and the tight sandstone samples were measured under axial stress oscillations to assess the frequency-and pressure-dependent *** dry condition,both samples appear to be nearly frequency independent,with weak pressure dependence for the shale and significant pressure dependence for the *** particular,it was found that the tight sandstone with complex pore microstructure exhibited apparent dispersion and attenuation under brine or glycerin saturation conditions,the levels of which were strongly influenced by the increased effective *** addition,the measured Young's moduli results were compared with the theoretical predictions from a scaled poroelastic model with a reasonably good agreement,revealing that the combined fluid flow mechanisms at both mesoscopic and microscopic scales possibly responsible for the measured dispersion.

关键词： Low-frequency measurements Dispersion and attenuation Rock physics Fluid flow

治疗性ERCP术后十二指肠乳头出血与原发疾病的关系

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世界华人消化杂志 2017年第8期25卷 755-759页

作者：徐洪根马进温岭市第一人民医院肝胆外科浙江省温岭市317500

目的探讨内镜下逆行胰胆管造影(endoscopic retrograde cholangiopancreatography,ERCP)术后十二指肠乳头出血与原发疾病的关系.方法回顾性分析温岭市第一人民医院收治的661例行治疗性ERCP术患者的临床资料.根据是否发生ERCP术后十二指... 详细信息

目的探讨内镜下逆行胰胆管造影(endoscopic retrograde cholangiopancreatography,ERCP)术后十二指肠乳头出血与原发疾病的关系.方法回顾性分析温岭市第一人民医院收治的661例行治疗性ERCP术患者的临床资料.根据是否发生ERCP术后十二指肠乳头出血,分为出血组和未出血组,评价原发疾病类型与出血风险的关系.结果共纳入患者661例,其中40例发生出血,其总体发生率为6.1%.出血组患者合并高血压病发生率明显高于未出血组,差异有统计学意义(P0.05).结论壶腹部嵌顿结石及恶性胆胰疾病ERCP术后十二指肠乳头出血的风险更大,重在预防出血,内镜止血安全有效.

关键词：内镜逆行胰胆管造影治疗并发症十二指肠乳头出血内镜止血

Percutaneous transhepatic cholangioscopy-assisted biliary polypectomy for local palliative treatment of intraductal papillary neoplasm of the bile duct

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World Journal of Gastrointestinal Oncology 2024年第5期16卷 1821-1832页

作者： xu Ren Yong-Ping Qu Chun-Lan Zhu Xiao-hong xu hong Jiang Yi-Xia Lu hong-Peng xue Digestive Disease Hospital of Heilongjiang Provincial Hospital Heilongjiang Provincial Clinical Medical Research Center for Minimally Invasive Diagnosis and Treatment of Pancreaticobiliary DiseasesHarbin 150001Heilongjiang ProvinceChina Digestive Endoscopy Center of Heilongjiang Provincial Hospital Heilongjiang Provincial Clinical Medical Research Center for Minimally Invasive Diagnosis and Treatment of Pancreaticobiliary DiseasesHarbin 150001Heilongjiang ProvinceChina Second Department of Gastroenterology Digestive Disease Hospital of Heilongjiang Provincial Hospitaland Heilongjiang Provincial Clinical Medical Research Center for Minimally Invasive Diagnosis and Treatment of Pancreaticobiliary DiseasesHarbin 150001Heilongjiang ProvinceChina Department of Pathology Heilongjiang Provincial HospitalHarbin 150001Heilongjiang ProvinceChina

BACKGROUND Intraductal papillary neoplasm of the bile duct(IPNB)is a premalignant biliarytype epithelial neoplasm with intraductal papillary or villous *** reported local palliative therapeutic modalities,including endoscopic nasobiliary drainage,stenting and biliary curettage,endoscopic biliary polypectomy,percutaneous biliary drainage,laser ablation,argon plasma coagulation,photodynamic therapy,and radiofrequency ablation to relieve mechanical obstruction are limited with weaknesses and *** have applied percutaneous transhepatic cholangioscopy(PTCS)-assisted biliary polypectomy(PTCS-BP)technique for the management of IPNB including mucin-hypersecreting cast-like and polypoid type tumors since *** To assess the technical feasibility,efficacy,and safety of PTCS-BP for local palliative treatment of *** Patients with mucin-hypersecreting cast-like or polypoid type IPNB and receiving PTCS-BP between September 2010 and December 2019 were ***-BP was performed by using a half-moon type snare with a soft stainless-steel wire,and the tumor was snared and resected with *** primary outcome was its feasibility,indicated by technical *** secondary outcomes were efficacy,including therapeutic success,curative resection,and clinical success,and *** Five patients(four with mucin-hypersecreting cast-like type and one with polypoid type IPNB)were ***-and high-grade intraepithelial neoplasia(HGIN)and recurrent IPNB with invasive carcinoma were observed in one,two,and two patients,*** cholangitis and/or obstructive jaundice were presented in all four patients with mucin-hypersecreting cast-like type *** five patients achieved technical success of *** patients(three with mucin-hypersecreting cast-like type and one with polypoid type IPNB)obtained therapeutic success;one with mucin-hypersecreting cast-like type tumors in the intrahepatic small bile duct and HGIN h

关键词： Intraductal papillary neoplasm of the bile duct Percutaneous transhepatic cholangioscopy Biliary polypectomy Feasibility Efficacy

Influence of meteorological factors on open biomass burning at a background site in Northeast China

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Journal of Environmental Sciences 2024年第4期138卷 1-9页

作者： Yulong Wang Linlin Liang Wanyun xu Chang Liu hongbing Cheng Yusi Liu gen Zhang Xiaobin xu Dajiang Yu Peng Wang Qingli Song Jiumeng Liu Yuan Cheng State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China State Key Laboratory of Severe Weather&Key Laboratory for Atmospheric Chemistry Chinese Academy of Meteorological SciencesBeijing 100081China Longfengshan Regional Background Station China Meteorological AdministrationHeilongjiang 150200China Heilongjiang Climate Center Heilongjiang 150030China

Biomass burning(BB)is a very important emission source that significantly adversely impacts regional air *** produces a large number of primary organic aerosol(POA)and black carbon(BC).Besides,BB also provides many precursors for secondary organic aerosol(SOA)*** this work,the ratio of levoglucosan(LG)to organic carbon(OC)and the fire hotspots map was used to identify the open biomass burning(OBB)events,which occurred in two representative episodes,October 13 to November 30,2020,and April1 to April 30,*** ratio of organic aerosol(OA)to reconstructed PM_(2.5)concentration(PM_(2.5)^(*))increased with the increase of LG/*** LG/OC ratio is higher than 0.03,the highest OA/PM_(2.5)^(*)ratio can reach 80%,which means the contribution of OBB to OA is *** to the ratio of LG to K^(+),LG to mannosan(MN)and the regional characteristics of Longfengshan,it can be determined that the crop residuals are the main *** occurrence of OBB coincides with farmers’preferred choices,i.e.,burning biomass in“bright weather”.The“bright weather”refers to the meteorological conditions with high temperature,low humidity,and without *** factors indirectly affect regional biomass combustion pollution by influencing farmers’active choices.

关键词： Air pollution Biomass burning Meteorological factors Organic trace Agricultural fires

Resolving the geometric structure of trastuzumab by mobility capillary electrophoresis and native mass spectrometry

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Chinese Chemical Letters 2024年第3期35卷 221-225页

作者： Wenjing Zhang Jie hong Lei Yang Zuqiang xu Yu Xiang Wei xu School of Life Science Beijing Institute of TechnologyBeijing 100081China

Available online Immunoglobulins G(IgGs)are Y-shaped globular proteins,however,their high flexibility and heterogeneity pose great challenges to their structure and conformation *** structure of IgG closely correlates to its biofunctions,such as the antibody escape of human immunodeficiency virus(HIV)could attribute to the distance mismatch between the ends of two Fab arms(antigen-binding sites)and envelope glycoprotein spikes on virion ***,we report the first use of mobility capillary electrophoresis(MCE)and native mass spectrometry(nMS)to resolve the internal geometric structure and conformation of an IgG(trastuzumab)in solution *** proteolysis,the ellipsoid dimensions of IgG and its subunits were measured by MCE-nMS *** was then reconstructed,in which the sizes and relative positions of these three subunits in three-dimensional space were *** was found that the two Fab arms have an angle of~102.1°and a distance of~11.0 nm between the two antigen-binding sites under native condition,and the Fc arm was tilted~16.0°towards one of the Fab *** was not on the plane of Fab-Fab,but has an angle of no larger than 103.1°.Under acidic environment(pH 3.0),each subunit of the IgG would unfold into larger dimensions,and the angles between these subunits also *** great potential for tumor imaging and therapy,the structure of F(ab')_(2)fragments was also measured and validated by molecular dynamic *** was found that the electrostatic force among these three subunits and steric hindrance stemming from Fc help maintaining the angle between two Fab arms.

关键词： Native mass spectrometry Mobility capillary electrophoresis Trastuzumab Protein structure Geometric structure

Enhancing Log Anomaly Detection with Semantic Embedding and Integrated Neural Network Innovations

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Computers, Materials & Continua 2024年第9期80卷 3991-4015页

作者： Zhanyang xu Zhe Wang Jian xu hongyan Shi hong Zhao School of Computer and Software Nanjing University of Information Science and TechnologyNanjing210044China

System logs,serving as a pivotal data source for performance monitoring and anomaly detection,play an indispensable role in assuring service stability and *** this,the majority of existing log-based anomaly detection methodologies predominantly depend on the sequence or quantity attributes of logs,utilizing solely a single Recurrent Neural Network(RNN)and its variant sequence models for *** approaches have not thoroughly exploited the semantic information embedded in logs,exhibit limited adaptability to novel logs,and a single model struggles to fully unearth the potential features within the log *** these challenges,this article proposes a hybrid architecture based on amultiscale convolutional neural network,efficient channel attention and mogrifier gated recurrent unit networks(LogCEM),which amalgamates multiple neural network *** on the superior performance of robustly optimized BERT approach(RoBERTa)in the realm of natural language processing,we employ RoBERTa to extract the original word vectors from each word in the log *** conjunction with the enhanced Smooth Inverse Frequency(SIF)algorithm,we generate more precise log sentence vectors,thereby achieving an in-depth representation of log ***,these log vector sequences are fed into a hybrid neural network,which fuses 1D Multi-Scale Convolutional Neural Network(MSCNN),Efficient Channel Attention Mechanism(ECA),and Mogrifier Gated Recurrent Unit(GRU).This amalgamation enables themodel to concurrently capture the local and global dependencies of the log sequence and autonomously learn the significance of different log sequences,thereby markedly enhancing the efficacy of log anomaly *** validate the effectiveness of the LogCEM model,we conducted evaluations on two authoritative open-source *** experimental results demonstrate that LogCEM not only exhibits excellent accuracy and robustness,but also outperfo

关键词： Deep learning log analysis anomaly detection natural language processing

0^(--) hidden-heavy tetraquark states via QCD sum rules

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Chinese Physics C 2024年第9期48卷 50-59页

作者： Bing-Dong Wan hong-Tai xu Department of Physics Liaoning Normal UniversityDalian 116029China Center for Theoretical and Experimental High Energy Physics Liaoning Normal UniversityDalian 116029China

In this study,we evaluated the mass spectra of the prospective 0^(--) hidden-charm and hidden-bottom tetraquark states in molecular configuration via QCD sum *** our calculation,the nonperturbative condensate contributions are considered up to dimension eight in operator product *** is found that there could exist 4possible 0^(--) hidden-charm tetraquark states with masses(4.68±0.07),(4.22±0.09),(4.53±0.09),and(4.26±0.13) *** corresponding hidden-bottom partners are found lying at(11.04±0.10),(10.71±0.12),(11.09±0.10),and(11.82±0.14) GeV,*** possible tetraquark decay modes were analyzed,which are expected to be measured in BESⅢ,BELLEⅡ,and LHCb experiments.

关键词： exotic hadronic states QCD sum rules tetraquarks

Ten key issues for ecological restoration of territorial space

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National Science Review 2024年第7期11卷 75-79页

作者： Jian Peng Dongmei xu Zihan xu Hui Tang hong Jiang Jianquan Dong Yanxu Liu Technology Innovation Center for Integrated Ecosystem Restoration and Sustainable Utilization Ministry of Natural Resources College of Urban and Environmental Sciences Peking University School of Soil and Water Conservation Beijing Forestry University Key Laboratory for Environmental and Urban Sciences School of Urban Planning and DesignShenzhen Graduate School Peking University School of Landscape Architecture Beijing Forestry University State Key Laboratory of Earth Surface Processes and Resource Ecology Faculty of Geographical Science Beijing Normal University

Ecological restoration is an effective measure to protect biodiversity, sustain ecosystem services and enhance socialecological resilience. It is defined as the process of assisting the recovery of an ecosystem that h... 详细信息

关键词： PRIORITY AREAS