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Plasmonic tandem heterojunctions enable high-efficiency charge transfer for broad spectrum photocatalytic hydrogen production

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Journal of Energy Chemistry 2025年第1期100卷 710-720页

作者： Wenxuan Chen Xiu-Qing Qiao Guo Hui Bojing sun Dongfang Hou Meidi Wang Xueqian Wu Tao Wu Dong-Sheng Li College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials China Three Gorges University Hubei Three Gorges Laboratory College of Chemistry and Materials Science and Guangdong Provincial Key Laboratory of Supramolecular Coordination Chemistry Jinan University

Rational engineering of semiconductor photocatalysts for efficient hydrogen production is of great significance but still challenging,primarily due to the limitations in charge transfer ***,a fascinating plasmonic tandem heterojunction with the hc-CdS/Mo2C@C heterostructure is aimfully prepared for effectively promoting the charge separation kinetics of the CdS photocatalyst via the synergistic strategy of phase junction,Schottky junction,and photothermal *** difference in atomic configuration between cubic-CdS （c-CdS） and hexagonal-CdS （h-CdS） leads to effective charge separation through a typical Ⅱ charge transfer mechanism,and plasmonic Schottky junction further extracts the electrons in the hc-CdS phase junction to realize gradient charge ***,the photothermal effect of Mo2C@C helps to expand the light absorption,accelerate charge transfer kinetics,and reduce the hydrogen evolution energy *** carbon layer provides a fast channel for charge transfer and protects the photocatalyst from *** a result,the optimized hc-CMC photocatalyst exhibits a significantly high photocatalytic H2production activity of 28.63 mmol/g/h and apparent quantum efficiency of 61.8%,surpassing most of the reported *** study provides a feasible strategy to enhance the charge transfer kinetics and photocatalytic activity of CdS by constructing plasmonic tandem heterogeneous junctions.

关键词： Heterojunctions LSPR Photocatalyst Phase junction Schottky junction Photothermal effect

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Lattice Boltzmann Model for Compressible Fluid on a Square Lattice

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Chinese Physics Letters 2000年第10期17卷 743-745页

作者： sun cheng-Hai State Key Laboratory of Tribology Department of Engineering MechanicsTsinghua UniversityBeijing 100084

A two-level four-direction lattice Boltzmann model is formulated on a square lattice to simulate compressible flows with a high Mach number. The particle velocities are adaptive to the mean velocity and internal energy. Therefore, the mean flow can have a high Mach number. Due to the simple form of the equilibrium distribution, the 4th order velocity tensors are not involved in the calculations. Unlike the standard lattice Boltzmann model, o special treatment is need for the homogeneity of 4th order velocity tensors on square lattices. The Navier-Stokes equations were derived by the Chapman-Enskog method from the BGK Boltzmann equation. The model can be easily extended to three-dimensional cubic lattices. Two-dimensional shock-wave propagation was simulated.

关键词： equation. energy. lattice

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Metal nanoparticles decorated CoFe-(oxy)hydroxysulfides nanosheets fabricated by a general strategy for electrocatalytic water splitting

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Journal of Energy Chemistry 2025年第1期100卷 26-38页

作者： Xiaodong Yang Haochen Shen Xiaoming Xiao Zhichao Li Qi Zhou Wei Yang Bin Jiang Yongli sun Luhong Zhang Zhenhua Yan School of Chemical Engineering and Technology Tianjin University Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University

This study presents a novel method to fabricate metal-decorated,sulfur-doped layered double hydroxides （M/SLDH） through spontaneous redox and sulfurization *** developed Ag/SLDH and Pt/SLDH catalysts with abundant heterogeneous interfaces and hierarchical nanostructures demonstrated outstanding oxygen evolution reaction （OER） and hydrogen evolution reaction （HER） performance,achieving low overpotentials of 212 and 35 mV at 10 mA cm-2in 1 M KOH,*** both anode and cathode in water splitting,they required only 1.47 V to reach 10 mA cm-2and exhibited high structural robustness,maintaining stability at 1000 mA cm-2for 300 ***-situ Raman analysis revealed that the synergistic effects of metal nanoparticles and S doping significantly promote the transformation into the S-Co1-xFexOOH layer,which serves as the active phase for water ***,ultraviolet photoelectron spectroscopy （UPS） and density functional theory （DFT） analyses indicated that incorporating metal nanoparticles and S doping increase electron density near the Fermi level and reduce reaction energy barriers,thus enhancing intrinsic OER and HER *** study provides a scalable strategy for synthesizing high-performance electrocatalysts for water splitting,with promising potential for broader applications.

关键词： LDH Spontaneous reaction Metal nanoparticles Water splitting

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Thermal Lattice Boltzmann Model for Compressible Fluid

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Chinese Physics Letters 2000年第3期17卷 209-211页

作者： sun cheng-Hai State Key Laboratory of Tribology Department of Engineering MechanicsTsinghua UniversityBeijing 100084

Wfe formulate a new thennal lattice Boltzmann model to simulate compressible flows with a high Mach *** main difference from the standard lattice Boltzmanii models is that the p&rticlc velocities are no longer a constantj varying with the mean velocity and internal *** proper heat conduction term in the energy equation is recovered by modiHcation of the fluctuating kinetic energy transported by *** simulation of Couette How is in good agreement with the analytical solutions.

关键词： particles. energy. lattice

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Quantifying the Temporal and Spatial Spread of COVID-19:Empirical Evidence from Shanghai

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Journal of Systems Science and Information 2024年第3期12卷 309-322页

作者： Haowen BAO Zishu cheng Yuying sun Yongmiao hong Shouyang WANG Academy of Mathematics and Systems Science Chinese Academy of SciencesBeijing 100190China School of Economics and Management and MOE Social Science Laboratory of Digital Economic Forecasts and Policy SimulationUniversity of Chinese Academy of SciencesBeijing 100190China School of Entrepreneurship and Management ShanghaiTech UniversityShanghai 201210China

The worldwide spread of COVID-19 has caused a grave threat to human life, health, and socio-economic development. It is of great significance to study the transmission mechanism of COVID-19 and evaluate the effect of epidemic prevention policies. This paper employs a spatial dynamic panel data(SDPD) model to analyze the temporal and spatial spread of COVID-19, incorporating the time-varying features of epidemic transmission and the impact of geographic *** studies on the COVID-19 outbreak in Shanghai during early 2022 show that the intra-regional transmission of COVID-19 dominated the cross-regional one. Additionally, strict policies are found to effectively reduce the transmission risk of COVID-19 and curb the spillover effect of the epidemic in Shanghai on other regions. Based on these results, we provide three policy suggestions. Furthermore,this research methodology can be extended to investigate other infectious diseases, thereby providing a scientific framework and theoretical basis for evaluating the spread risk of pandemics and formulating appropriate strategies.

关键词： COVID-19 spatial econometrics epidemic prevention policy dynamic

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A Central Limit Theorem for Branching Brownian Motion with Random Immigration

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Acta Mathematica Sinica,English Series 2014年第1期30卷 69-78页

作者： hong Yan sun School of Mathematical Sciences Beijing Normal University

We establish a central limit theorem for a branching Brownian motion with random immigration under the annealed law,where the immigration is determined by another branching Brownian *** limit is a Gaussian random measure and the normalization is t3/4for d=3 and t1/2for d≥4,where in the critical dimension d=4 both the immigration and the branching Brownian motion itself make contributions to the covariance of the limit.

关键词： Branching Brownian motion random immigration central limit theorem occupation time

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Destroying a Peldan Electrostatic Solution Black Hole

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Chinese Physics Letters 2017年第4期34卷 9-12页

作者： Hao Tang Yu Song Rui-hong Yue cheng-Yi sun Institute of Modern Physics and Shaanxi Key Laboratory for Theoretical Physics Frontiers Northwest University Xi＇an 710069 College of Physical and Technology Yangzhou University Yangzhou 225009

By throwing a particle with electric charge and angular momentum into the black holes, much evidence shows that the naked singularity of some （3＋1）-dimensional black holes might be seen, which is not allowed in the weak cosmic censorship conjecture. In this study, we consider a （2＋1）-dimensional Peldan black hole and find that it could be destroyed under certain conditions in both extreme and near-extreme cases.

关键词： Destroying a Peldan Electrostatic Solution Black Hole

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ITERATIVE METHODS FOR THE FORWARD-BACKWARD HEAT EQUATION

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Journal of Computational Mathematics 2005年第4期23卷 419-424页

作者： Xiao-liang cheng Jie sun Department of Mathematics Zhejiang University Hangzhou 310028 China Department of Mathematics Zhejiang University of Finance and Economics Hangzhou 310012 China

In this paper we propose the finite difference method for the forward-backward heat equation. We use a coarse-mesh second-order central difference scheme at the middle line mesh points and derive the error estimate. Then we discuss the iterative method based on the domain decomposition for our scheme and derive the bounds for the rates of convergence. Finally we present some numerical experiments to support our analysis.

关键词： Forward-backward heat equation Finite difference method Iterative method Coarse mesh

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MnO_(2)/carbon nanocomposite based on silkworm excrement for high-performance supercapacitors

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International Journal of Minerals,Metallurgy and Materials 2021年第10期28卷 1735-1744页

作者： Pian Zhang Yun-hao Wu Hao-ran sun Jia-qi Zhao Zhi-ming cheng Xiao-hong Kang Department of Chemistry School of ScienceBeijing Jiaotong UniversityBeijing 100044China

MnO_(2)/biomass carbon nanocomposite was synthesized by a facile hydrothermal *** excrement acted as a carbon precursor,which was activated by ZnCl_(2) and FeCl_(3) combining chemical agents under Ar *** and flower-like MnO_(2) nanowires were in-situ anchored on the surface of the biomass *** biomass carbon not only offered high conductivity and good structural stability but also relieved the large volume expansion during the charge/discharge *** obtained MnO_(2)/biomass carbon nanocomposite electrode exhibited a high specific capacitance(238 F·g^(-1) at 0.5 A·g^(-1))and a superior cycling stability with only 7% degradation after 2000 *** observed good electrochemical performance is accredited to the materials’high specific surface area,multilevel hierarchical structure,and good *** study proposes a promising method that utilizes biological waste and broadens MnO_(2)-based electrode material application for next-generation energy storage and conversion devices.

关键词： manganese dioxide specific capacitance cyclic stability biomass carbon silkworm excrement

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Intramolecular Hydrogen Bond Improved Durability and Kinetics for Zinc‑Organic Batteries

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Nano-Micro Letters 2024年第3期16卷 138-148页

作者： Tianjiang sun Jun Pan Weijia Zhang Xiaodi Jiang Min cheng Zhengtai Zha hong Jin Fan Zhanliang Tao Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Renewable Energy Conversion and Storage CenterCollege of ChemistryNankai UniversityHaihe Laboratory of Sustainable Chemical TransformationsTianjin 300071People’s Republic of China School of Physical and Mathematical Sciences Nanyang Technological UniversitySingapore 637371Singapore Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology School of Physics Science and EngineeringTongji UniversityShanghai 200092People’s Republic of China

Organic compounds have the advantages of green sustainability and high designability,but their high solubility leads to poor durability of zinc-organic ***,a high-performance quinone-based polymer(H-PNADBQ)material is designed by introducing an intramolecular hydrogen bonding(HB)*** intramolecular HB(C=O⋯N-H)is formed in the reaction of 1,4-benzoquinone and 1,5-naphthalene diamine,which efficiently reduces the H-PNADBQ solubility and enhances its charge transfer in *** situ ultraviolet-visible analysis further reveals the insolubility of H-PNADBQ during the electrochemical cycles,enabling high durability at different current ***,the H-PNADBQ electrode with high loading(10 mg cm^(-2))performs a long cycling life at 125 mA g^(-1)(>290 cycles).The H-PNADBQ also shows high rate capability(137.1 mAh g^(−1)at 25 A g^(−1))due to significantly improved kinetics inducted by intramolecular *** work provides an efficient approach toward insoluble organic electrode materials.

关键词： Zn-organic batteries H-PNADBQ polymer Intramolecular hydrogen bond Reduced solubility Improvedπ-conjugated level

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