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Efficient Pt/KFI zeolite catalysts for the selective catalytic reduction of NOxby hydrogen

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Journal of Environmental Sciences 2024年第4期138卷 102-111页

作者： Ligang Zhang Yulong Shan Zidi yan Zhongqi Liu Yunbo Yu hong He School of Rare Earths University of Science and Technology of ChinaHefei 230026China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou 341119China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Aiming at purification of NO_(x)from hydrogen internal combustion engines(HICEs),the hydrogen selective catalytic reduction(H_(2)-SCR)reaction was investigated over a series of Pt/KFI zeolite catalysts.H_(2)can readily reduce NO_(x)to N_(2)and N_(2)O while O_(2)inhibited the deNO_(x)efficiency by consuming the reductant H_(2).The Pt/KFI zeolite catalysts with Pt loading below 0.1wt.% are optimized H_(2)-SCR catalysts due to its suitable operation temperature window since high Pt loading favors the H_(2)-O_(2)reaction which lead to the insufficient of *** to metal Pt^(0)species,Pt^(δ+)species showed lower activation energy of H_(2)-SCR reaction and thought to be as reasonable active ***,Eley-Rideal(E-R)reaction mechanism was proposed as evidenced by the reaction orders in kinetic ***,the optimized reactor was designed with hybrid Pt/KFI catalysts with various Pt loading which achieve a high NO_(x)conversion in a wide temperature range.

关键词： Pt/KFI zeolite Pt loading H_(2)-SCR Reaction conditions Kinetics studies

The Effect of Blending Ratio on the Structure and Properties of the PPR/PS In situ Fiber Reinforced System Prepared by Multi-Flow Vibration Injection Molding

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Chinese Journal of Polymer Science 2024年第6期42卷 851-863页

作者： yan-Jiang Li Meng-Long Hu Jun-wen Zhang Qiang Fu Jie Zhang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu610065China

To enhance the mechanical properties of polypropylene random copolymer(PPR),polystyrene(PS)with four different contents were added to the PPR matrix through melt ***,using the Multi-Flow Vibration Injection Molding(MFVIM)technology,PPR/PS in situ microfiber composites(MFC)with different blending ratios were *** results indicated that blending ratio had a great impact on the phase morphology and crystal structure of MFVIM samples,which was different from those of conventional injection molding(CIM)*** ultrafine fibers could be formed under the shear field and could absorb the PPR molecular chains to form hybrid shish-kebab ***,the PPR matrix could also form shish-kebab structures under the effect of strong *** the PS content reached 20%,under the combined action of PS in situ microfibers and highly oriented crystal structure,the tensile strength and Young’s modulus of the sample were obviously improved and the impact strength remained at a relatively high *** a strong and tough balanced PPR based material was *** results provide valuable insights for expanding the industrial and daily-life applications of PPR and show promising development prospects.

关键词： PPR MFVIM In situ microfibers Shearfield Hybrid shish-kebab structures

Adhesion strength of tetrahydrofuran hydrates is dictated by substrate stiffness

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Petroleum Science 2024年第1期21卷 667-673页

作者： yan-wen Lin Tong Li Yi Zhang Wei-Wei yan Xiao-Ming Chen Zhi-Sen Zhang Jian-yang Wu Department of Physics Research Institute for Biomimetics and Soft MatterJiujiang Research Institute and Fujian Provincial Key Laboratory for Soft Functional Materials ResearchXiamen UniversityXiamen361005FujianChina Key Laboratory of Marine Materials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo315201ZhejiangChina Key Laboratory of Icing and Anti/De-icing China Aerodynamics Research and Development CenterMianyang621000SichuanChina Micro-and Nano-technology Research Center State Key Laboratory for Manufacturing Systems EngineeringXi’an Jiaotong UniversityXi’an710049ShaanxiChina Electronic Materials Research Lab Key Laboratory of the Ministry of EducationXi’an Jiaotong UniversityXi’an710049ShaanxiChina NTNU Nanomechanical Lab Norwegian University of Science and Technology(NTNU)Trondheim7491Norway

Understanding the hydrate adhesion is important to tackling hydrate accretion in ***,the relationship between the Tetrahydrofuran(THF)hydrate adhesion strength(AS)and surface stiffness on elastic coatings is systemically examined by experimental shear force measurements and theoretical *** mechanical factor-elastic modulus of the coatings greatly dictates the hydrate AS,which is explained by the adhesion mechanics theory,beyond the usual factors such as wettability and structural ***,the hydrate AS increases with reducing the thickness of the elastic coatings,resulted from the decrease of the apparent surface elastic *** effect of critical thickness for the elastic materials with variable elastic modulus on the hydrate AS is also *** study provides deep perspectives on the regulation of the hydrate AS by the elastic modulus of elastic materials,which is of significance to design anti-hydrate surfaces for mitigation of hydrate accretion in petro-pipelines.

关键词： Hydrate Adhesion strength Elastic modulus Coatings

PDOL-Based Solid Electrolyte Toward Practical Application:Opportunities and Challenges

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Nano-Micro Letters 2024年第7期16卷 109-141页

作者： Hua yang Maoxiang Jing Li Wang hong Xu Xiaohong yan Xiangming He Institute for Advanced Materials School of Materials Science and EngineeringJiangsu UniversityZhenjiang 212013People’s Republic of China Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084People’s Republic of China

Polymer solid-state lithium batteries(SSLB)are regarded as a promising energy storage technology to meet growing demand due to their high energy density and *** conductivity,interface stability and battery assembly process are still the main challenges to hurdle the commercialization of *** the main component of SSLB,poly(1,3-dioxolane)(PDOL)-based solid polymer electrolytes polymerized in-situ are becoming a promising candidate solid elec-trolyte,for their high ion conductivity at room temperature,good battery elec-trochemical performances,and simple assembly *** review analyzes opportunities and challenges of PDOL electrolytes toward practical application for polymer *** focuses include exploring the polymerization mechanism of DOL,the performance of PDOL composite electrolytes,and the application of ***,we provide a perspective on future research directions that need to be emphasized for commercialization of PDOL-based electrolytes in *** exploration of these schemes facilitates a comprehensive and profound understanding of PDOL-based polymer electrolyte and provides new research ideas to boost them toward practical application in solid-state batteries.

关键词： Poly(1,3-dioxolane) Solid electrolyte Polymerization mechanism Composite electrolyte Practical application

Clinicopathological features and treatment of extremity bone metastasis in patients with endometrial carcinoma： a case report and review

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Chinese Medical Journal 2011年第4期124卷 622-626页

作者： JIANG Guo-qing GAO Yu-nong GAO Min ZHENG hong yan Xin WANG wen AN Na CAO Kun Department of Gynecologic Oncology Peking University School of Oncology Beijing Cancer Hospital & Institute Beijing 100142 China

Unlike other non-gynecologic solid tumors, such as breast cancer, lung cancer, metastasis to bone from endometrial carcinoma is rare, metastasis to extremity is extremely rare. We report a 51-year-old multiparous woman with FIGO Stage IVb Grade 2 endometrial adenocarcinoma which metastasized to left lower extremity bone. She received an amputation of left lower extremity below the knees, and a total abdominal hysterectomy and bilateral salpingo-oophorectomy, and followed by systemic chemotherapy, radiation therapy to the pelvis and progestational agent. She had a complete response to above treatments, and disease-free survival for 10 months. After recurrence, she received chemotherapy, radiotherapy and progestational agent once again. She had lived 56 months and is still alive by the time of report. Metastasis of endometrial carcinoma to extremity bone can rarely occur and should be considered when the patient with endometrial carcinoma complained of unexplained pain and swelling associated with extremity bone.

关键词： endometrial carcinoma lower-extremity bone metastasis therapy clinicopathological

Enhancement of comprehensive properties of Nb-Si based in-situ composites by Ho rare earth doping

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Rare Metals 2024年第9期43卷 4508-4520页

作者： Wei Wei Qi Wang Rui-Run Chen Chao-wen Zheng yan-Qing Su National Key Laboratory for Precision Hot Processing of Metals School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150001China

This study examines the microstructure,mechanical properties(with a focus on room-temperature toughness),and oxidation resistance of Ho-doped NbDSi based in-situ *** base alloy consists of the coarse primary Nb_(5)Si_(3)phase and the Nb_(5)Si_(3)+Nbss(Nb solid solution)eutectic *** doping influences the solidification *** the Ho doping is higher than0.2 at%,the alloys transform into eutectic *** can be solid-solved in trace amounts in the Nbss ***,most of Ho forms a stable Ho oxide phase,which alleviates oxygen contamination problem to some ***,the interface separation between Ho oxide and other phases reduces the plastic deformation ***,with 0.4 at%Ho doping,the K_(Q)value is18.03 MPa·m^(1/2),which is 31.1%higher than that of the base *** strength of the Ho-doped alloys does not deteriorate with an increase in ***,the large network-like Ho_(2)O_(3)in the 0.8Ho alloy causes a decrease in toughness and *** addition,the Ho oxide phase effectively blocks the inward oxygen *** 0.8 at%Ho doping,the oxidation mass gain per unit area is 10.16 mg·cm^(2),which is 39.7%lower than that of the base alloy.

关键词： Nb-Si based composites Rare earth elements Ho Microstructure Properties

市场环境下发电机组竞争能力的关联规则挖掘方法

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电网技术 2006年第13期30卷 61-65页

作者：颜宏文长沙理工大学计算机与通信工程学院湖南省长沙市410076

针对常规的模糊综合评判中各因素的模糊化区间以及各因素之间的关联性对选择权重的影响,提出了应用关联规则的数据挖掘算法修正权重的新方法。首先对电力市场中发电商的竞争数据库进行挖掘并寻找发电商竞争能力评估体系中各因素之间的... 详细信息

针对常规的模糊综合评判中各因素的模糊化区间以及各因素之间的关联性对选择权重的影响,提出了应用关联规则的数据挖掘算法修正权重的新方法。首先对电力市场中发电商的竞争数据库进行挖掘并寻找发电商竞争能力评估体系中各因素之间的关联关系;然后根据关联关系的强弱分析了各因素权重设置的合理性并重新修正了权重因子;最后建立了合理的模糊综合评判模型并将其应用于电力市场中发电商竞争能力的评判决策。数字仿真结果表明了该方法的有效性。

关键词：关联规则挖掘 Apriori算法电力市场模糊综合评判机组竞争能力

Megafossils of Betulaceae from the Oligocene of Qaidam Basin and their paleoenvironmental and phytogeographic implications

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Plant Diversity 2024年第1期46卷 101-115页

作者： Tao yang Jia-Hao Cai yan-Zhi Dai hong-Yu Chen Lei Han Li Zhang Wei-Yu Liang Xu-Jun Li wen-Jia Li Jing-Yu Wu San-Ping Xie De-Fei yan School of Earth Sciences and Key Laboratory of Mineral Resources in Western China(Gansu Province) Lanzhou UniversityLanzhou 730000China Key Laboratory of Vertebrate Evolution and Human Origins of Chinese Academy of Sciences Institute of Vertebrate Paleontology and PaleoanthropologyChinese Academy of SciencesBeijing 100044China State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and Palaeontology and Center for Excellence in Life and PaleoenvironmentChinese Academy of SciencesNanjing 210008China Center for Research and Education on Biological Evolution and Environments School of Earth Sciences and EngineeringNanjing UniversityNanjing 210023China

Understanding the paleoenvironment and phytogeographical history of the Tibetan Plateau,China relies on discovering new plant *** Qaidam Basin has long been regarded as an ideal‘field laboratory’to investigate the paleoclimate and paleobiological evolution of the northern Tibetan ***,fossil angiosperms from the Qaidam Basin are rare,and our knowledge of its paleovegetation is ***,we report fossil leaves and fruits of Betulaceae found from the Oligocene Shangganchaigou Formation of northwestern Qaidam Basin(Huatugou area).Comparative morphological analysis led us to assign the fruits to the Betula subgenus Betula and the leaves to Carpinus *** findings,together with other reported fossil plants from the same locality,reveal a close floristic linkage between the Qaidam Basin and Europe during the *** northern pathway of this floristic exchange may have crossed through the Qaidam Basin during the late *** floristic linkage may have been facilitated by the continuous narrowing of the Turgai Strait and stronger westerlies,which transported moisture and provided favorable climatic ***,fossil plants collected from the Qaidam Basin suggest that during the Oligocene this region had warm and humid deciduous broad-leaf forest,which differs from the region’s modern vegetation and indicates that the Qaidam Basin may have been a suitable region for these plants to flourish and spread during the Oligocene.

关键词： Paleoenvironment Biogeography Betulaceous fossil Qaidam basin Tibetan Plateau Oligocene

Magnetic Fields Reduce Apoptosis by Suppressing Phase Separation of Tau-441

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Research 2024年第1期2023卷 181-197页

作者： wen-Juan Lin wen-Pu Shi Wan-Yi Ge Liang-Liang Chen Wei-hong Guo Peng Shang Da-Chuan Yin Key Laboratory for Space Bioscience and Biotechnology School of Life SciencesNorthwestern Polytechnical University127 Youyixi RoadXi'an 710072ShaanxiPR China

The biological effects of magnetic fields(MFs)have been a controversial ***,in recent years,there has been increasing evidence that MFs do affect biological ***,the physical mechanism remains ***,we show that MFs(16 T)reduce apoptosis in cell lines by inhibiting liquid–liquid phase separation(LLPS)of Tau-441,suggesting that the MF effect on LLPS may be one of the mechanisms for understanding the“mysterious”magnetobiological *** LLPS of Tau-441 occurred in the cytoplasm after induction with *** phase-separated droplets of Tau-441 recruited hexokinase(HK),resulting in a decrease in the amount of free HK in the *** cells,HK and Bax compete to bind to the voltage-dependent anion channel(VDAC I)on the mitochondrial membrane.A decrease in the number of free HK molecules increased the chance of Bax binding to VDAC I,leading to increased Bax-mediated *** the presence of a static MF,LLPS was marked inhibited and HK recruitment was reduced,resulting in an increased probability of HK binding to VDAC I and a decreased probability of Bax binding to VDAC I,thus reducing Bax-mediated *** findings revealed a new physical mechanism for understanding magnetobiological effects from the perspective of *** addition,these results show the potential applications of physical environments,such as MFs in this study,in the treatment of LLPS-related diseases.

关键词： inhibited Apoptosis finding