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STABILITY OF POLY(N,N'-METHYLENEBISACRYLAMIDE-co-4-VINYLPYRIDINE)MICROGEL DISPERSION AND ADJUSTMENT OF THE HYDROPHOBICITY IN THE MICROGELS

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Chinese Journal of Polymer Science 2005年第6期23卷 635-642页

作者： Qing-de Chen Xing-hai Shen and hong-cheng gao Department of Applied Chemistry,College of Chemistry and Molecular Engineering,Peking University,Beijing 100871,China Peking Univ Dept Appl Chem Coll Chem & Mol Engn Beijing 100871 Peoples R China

In the UV-Vis spectra of pure light-scattering systems, there is an exponential relationship between absorbance and wavelength （A = Kλ^-n）. Here, the exponent n is named as flocculation-coagulation parameter. In the present paper, the effects of different additives on the stability of poly（N,N＇-methylenebisacrylamide-co-4-vinylpyridine）（poly（Bis-co-4-VP）） microgel dispersion were studied in detail via this parameter. The results showed that the stability of the dispersion mainly comes from the ionization of pyridine groups, making the microgel positively charged on its surface. This was confirmed by the measurement of Zeta potential and the result of conductometric titration. The result of fluorescence analysis indicated that the hydrophobicity in the microgels is enhanced with the increase in total 4-VP unit content.

关键词： Microgel dispersion(s) 4-Vinylpyridine Flocculation-coagulation parameter Zeta potential

EFFECTS OF L-PHENYLALANINE ON THE RADIATION SYNTHESIS OF POLY(N,N'-METHYLENEBISACRYLAMIDE-co-4-VINYLPYRIDINE)(MICRO)GELS

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Chinese Journal of Polymer Science 2005年第6期23卷 643-650页

The effects of L-phenylalanine （L-Phe） on the synthesis ofpoly（N,N＇-methylenebisacrylamide-co-4-vinylpyridine）（poly（Bis-co-4-VP））（micro）gels by γ-ray irradiation were studied. The addition of L-Phe could not only decrease the gelation dose （Dg） of the synthesis obviously, but also transform the morphology of copolymer from microgel to gel. In addition, the swelling ability of the （micro）gels was also affected in the presence of L-Phe. The decrease of Dg was ascribed to the effect of pH, while the transformation of the morphology was ascribed to the effect of L-Phe on the stability of the poly（Bis-co-4-VP） microgel. Such an effect was confirmed further as compared with the effects of L-alanine, L-glutamic acid, L-arginine, sulfuric acid and aqueous ammonia.

关键词： L-Phenylalanine γ-Ray irradiation Gelation dose Morphology transformation (Micro)gel

Engineering Strategies for Suppressing the Shuttle Effect in Lithium–Sulfur Batteries

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Nano-Micro Letters 2024年第1期16卷 187-221页

作者： Jiayi Li Li gao Fengying Pan cheng Gong Limeng Sun hong gao Jinqiang Zhang Yufei Zhao Guoxiu Wang Hao Liu Joint International Laboratory On Environmental and Energy Frontier Materials School of Environmental and Chemical EngineeringShanghai UniversityShanghaiPeople’s Republic of China Centre for Clean Energy Technology University of Technology SydneyBroadwaySydneyNSW 2007Australia

Lithium–sulfur(Li–S)batteries are supposed to be one of the most potential next-generation batteries owing to their high theoretical capacity and low ***,the shuttle effect of firm multi-step two-electron reaction between sulfur and lithium in liquid electrolyte makes the capacity much smaller than the theoretical *** methods were proposed for inhibiting the shuttle effect of polysulfide,improving corresponding redox kinetics and enhancing the integral performance of Li–S ***,we will comprehensively and systematically summarize the strategies for inhibiting the shuttle effect from all components of Li–S ***,the electrochemical principles/mechanism and origin of the shuttle effect are described in ***,the efficient strategies,including boosting the sulfur conversion rate of sulfur,confining sulfur or lithium polysulfides(LPS)within cathode host,confining LPS in the shield layer,and preventing LPS from contacting the anode,will be discussed to suppress the shuttle ***,recent advances in inhibition of shuttle effect in cathode,electrolyte,separator,and anode with the aforementioned strategies have been summarized to direct the further design of efficient materials for Li–S ***,we present prospects for inhibition of the LPS shuttle and potential development directions in Li–S batteries.

关键词： Shuttle effect Designed strategies Li-S battery Lithium polysulfides

Equalizer Zero-Determinant Strategy in Discounted Repeated Stackelberg Asymmetric Game

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Journal of Systems Science & Complexity 2024年第1期37卷 184-203页

作者： cheng Zhaoyang CHEN Guanpu hong Yiguang Key Laboratory of Systems and Control Academy of Mathematics and Systems ScienceChinese Academy of SciencesBeijing 100190China School of Mathematical Sciences University of Chinese Academy of SciencesBeijing 100049China School of Electrical Engineering and Computer Science KTH Royal Institute of Technology10044 StockholmSweden. Department of Control Science and Engineering Tongji UniversityShanghai 201804China Shanghai Research Institute for Intelligent Autonomous Systems Tongji UniversityShanghai 210201China

This paper focuses on the performance of equalizer zero-determinant(ZD)strategies in discounted repeated Stackelberg asymmetric *** the leader-follower adversarial scenario,the strong Stackelberg equilibrium(SSE)deriving from the opponents’best response(BR),is technically the optimal strategy for the ***,computing an SSE strategy may be difficult since it needs to solve a mixed-integer program and has exponential complexity in the number of *** this end,the authors propose an equalizer ZD strategy,which can unilaterally restrict the opponent’s expected *** authors first study the existence of an equalizer ZD strategy with one-to-one situations,and analyze an upper bound of its performance with the baseline SSE *** the authors turn to multi-player models,where there exists one player adopting an equalizer ZD *** authors give bounds of the weighted sum of opponents’s utilities,and compare it with the SSE ***,the authors give simulations on unmanned aerial vehicles(UAVs)and the moving target defense(MTD)to verify the effectiveness of the proposed approach.

关键词： Discounted repeated Stackelberg asymmetric game equalizer zero-determinant strategy strong Stackelberg equilibrium strategy

Nutrient transport following water transfer through the world's largest water diversion channel

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Journal of Environmental Sciences 2024年第1期135卷 703-714页

作者： Yuanhui cheng hong Zhang Wei Yin State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085 China Changjiang Water Resources Protection Institute Wuhan 430051China University of Chinese Academy of Sciences Beijing 100049China

Nutrient levels in the artificial channel constructed for the Middle Route Project are significant indicators of water quality safety and aquatic ecological integrity for this large,interbasin ***,the distribution and transport of nutrients along the channel were poorly *** on a time-series dataset as well as mass balance and material flow analysis methods,the water and nutrient transport fluxes in the Middle Route of the South-to-North Water Diversion Project were identified in this *** results indicate that the nutrient concentrations varied considerably with time,but there was no significant difference among the 30 stations of the main *** temperature difference was the major factor in the large fluctuations of water quality indicators over *** nutrient loadings varied with the water volume outputs from the main channel to the waterreceiving *** deposition was an important source of nutrients in the main channel,accounting for 9.13%,20.6%,and 0.635%of the nitrogen,phosphorus,and sulfur input from the Danjiangkou Reservoir,*** 2021,a net accumulation of 988 tons of N,29 tons of P,and 2,540 tons of S,respectively,were present in the main *** increase of these external and internal nutrient loadings would cause water quality fluctuation and deterioration in some local sections of the main *** study quantified the spatial and temporal patterns of nutrient transport in the Middle Route and revealed the ecological effects on the aquatic environment,assisting authorities on the project to develop effective water conservation strategies.

关键词： Nutrient transport Spatiotemporal patterns The Middle Route The South-to-North Diversion Project Hydro-ecological effects Water-receiving cities

Traumatic Diaphragmatic Hernia Associated with Pelvic Ring Fracture

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Chinese Medical Journal 2015年第9期128卷 1272-1274页

作者： Yin Zhang Tao cheng hong gao Xian-Long Zhang Department of Orthopedic Shanghai Jiao Tong University Affliated Sixth People@s Hospital Shanghai 200233 China

Traumatic diaphragmatic hernia （TDH） is an uncommon injury and a marker of severe *** injury is rarely associated with pelvic ring fracture,although TDH is one of the most dangerous comorbidities of such *** this condition is easily misdiagnosed in emergency cases,we reported two cases and analyzed the clinical symptoms,diagnosis,treatment,and outcome of this *** on these results,we recommended an appropriate method for diagnosis and treatment and proposed a contraindication in treating TDH associated with pelvic fracture.

关键词： Emergency Injury Control Pelvic Ring Fracture Pelvic Straps Traumatic Diaphragmatic

On the global smooth solutions of 3D incompressible Hall-MHD equations

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Applied Mathematics(A Journal of Chinese Universities) 2024年第2期39卷 319-327页

作者： YUE gao-cheng SUN Wen-da School of Mathematics Nanjing University of Aeronautics and AstronauticsNanjing 211106China

The present paper is devoted to the well-posedness issue for the 3D incompressible Hall-MHD system obtained from kinetic models. Our analysis strongly relies on the use of the Fourier analysis. We establish the global existence of smooth solutions for a class of large initial data, this result implies the initial velocity and magnetic field can be arbitrarily large.

关键词： 3D Hall-MHD well-posedness Fourier analysis

Performance of double-arch tunnels under internal BLEVE

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Underground Space 2024年第6期19卷 6-25页

作者： Ruishan cheng Wensu Chen hong Hao Center for Infrastructural Monitoring and Protection School of Civil and Mechanical EngineeringCurtin UniversityPerth 6000Australia Earthquake Engineering Research&Test Center Guangzhou UniversityGuangzhou 510000China

Double-arch tunnels,as one of the popular forms of tunnels,might be exposed to boiling liquid expanding vapour explosions(BLEVEs)associated with transported liquified petroleum gas(LPG),which could cause damage to the tunnel and even catastrophic collapse of the tunnel in extreme ***,very limited study has investigated the performance of double-arch tunnels when exposed to internal BLEVEs and in most analyses of tunnel responses to accidental *** TNT-equivalence method was used to approximate the explosion load,which may lead to inaccurate tunnel response *** study numerically investigates the response of typical double-arch tunnels to an internal BLEVE resulting from the instantaneous rupture of a 20 m^(3) LPG *** of various factors,including in-situ stresses,BLEVE locations,and lining configurations on tunnel responses are *** results show that the double-arch tunnels at their early-operation ages are more vulnerable to severe damage when exposed to the BLEVE due to the low action of in-situ stress of rock mass on the response of early-age *** is also found that directing the LPG tank to different driving lanes inside tunnels can affect the BLEVE-induced tunnel response more significantly than varying the configurations of tunnel ***,installing section-steel arches in the mid-wall can effectively improve the blast resistance of the double-arch tunnels against the internal *** addition,the prediction models based on multi-variate nonlinear regressions and machine learning methods are developed to predict the BLEVE-induced damage levels of the double-arch tunnels without and with section-steel arches.

关键词： Double-arch tunnel BLEVE Lining configuration Section-steel arch Damage prediction

Towards a blood ecosystem approach to dissect systemic diseases

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Science China(Life Sciences) 2024年第7期67卷 1528-1531页

作者： hong Wang Tao cheng State Key Laboratory of Experimental Hematology Haihe Laboratory of Cell EcosystemNational Clinical Research Center for Blood DiseasesInstitute of Hematology&Blood Diseases HospitalChinese Academy of Medical Sciences&Peking Union Medical CollegeTianjin 300020China Tianjin Institutes of Health Science Tianjin 301600China

Systemic diseases,in contrast to localized ailments,exert widespread effects and can impact the entire *** of systemic diseases encompass autoimmune disorders,infectious diseases,metabolic disorders,and chronic conditions like *** diseases often entail intricate interactions among diverse organs,tissues,and physiological systems,influenced by a myriad of factors.

关键词： diseases organs autoimmune