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Critical Operation Strategies Toward High-Performance Lithium Metal Batteries

Renewables 2023年第2期1卷 114-141页

作者： Lanting Qian Tyler Or Yun Zheng Matthew Li Dana Karim Andy Cui Moin Ahmed heywoong park Zhen Zhang Yaping Deng Aiping Yu Zhongwei Chen Khalil Amine Department of Chemical Engineering Waterloo Institute for NanotechnologyUniversity of WaterlooWaterlooOntario N2L 3G1 Chemical Sciences and Engineering Division Argonne National LaboratoryLemontIllinois 60439 Hinsdale Central High School HindsaleIllinois 50521 Henry Gunn High School Palo AltoCalifornia 94306

Commercial lithium(Li)-ion batteries(LIBs)are approaching their theoretical limits in energy *** a result,Li metal batteries(LMBs)with either liquid or solid-state electrolytes have been proposed as a next-generation alternative,although they currently pose major safety and stability *** resolve these issues,most research has focused on the development and production of novelmaterials and *** promising performance benchmarks have been achieved,these strategiesmay generate issues for large-scale production,due to the added costs associated with using novel materials and developing the required cell fabrication process and *** external conditions,such as selecting specific cell cycling protocols,testing the cell or synthesizing materials at specific temperatures,testing or fabricating the cell under specific mechanical pressures,etc.,are often overlooked as a means of directly improving battery performance without requiring complex material *** this review,we will discuss how these external parameters can address the key failure mechanisms and challenges in LMBs that use either liquid or solid *** and differences in mechanisms(Li+transport,Li dendrite propagation,thermal effects,etc.)observed in liquid and solid-state configurations will also be ***,we propose the outstanding scientific and economic gaps in LMBs,thereby providing future directions to explore.

关键词： energy storage lithium metal batteries solidstate batteries temperature protocols pressure

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