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Journal of Environmental Sciences 2024年第2期136卷 390-399页

作者： Aihua Cheng Yi he Xiaohe liu Chi he Department of Environmental Engineering College of Geology and EnvironmentXi’an University of Science and TechnologyXi’an 710054China State Key Laboratory of Multiphase Flow in power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs pollution Control Material and Technology University of Chinese Academy of SciencesBeijing 101408China

Achieving an efficient and stable heterogeneous Fenton reaction over a wide pH range is of great significance for wastewater ***,a pollen-derived biochar catalyst with a unique honeycomb-like structure,coupled with the dispersion of magnetic Fe_(3)O_(4)/FeS(Fe/S)nanoparticles,was synthesized by simple impregnation precursor,followed by *** prepared Fe/S-biochar catalyst demonstrated outstanding phenol degradation efficiency across a wide pH range,with 98%of which eliminated even under neutral conditions(pH 7.0).The high catalytic activity was due to the multilevel porous structure of pollenderived biochar provided enough active sites and allowed for better electron transfer,then increases oxidation ability to promote the ***,the acid microenvironment formed by SO_(4)^(2-)group from Fe/S composite extended the pH range for Fenton reaction,and S^(2-)facilitated the conversion of≡Fe^(3+)to≡Fe^(2+),resulting in remarkable degradation ***,biochar can effectively promote cycling stability by limiting Fe *** work may provide a general strategy for designing 3D framework biochar-based Fe/S catalysts with excellent performance for heterogeneous Fenton reactions.

关键词： Biomass Biochar Fenton reaction Fe_(3)O_(4)/FeS(Fe/S) phenol degradation

Study on a semi-resolved CFD-DEM method for rod-like particles in a gas-solid fluidized bed

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particuology 2024年第4期87卷 20-36页

作者： Lip.ng he Zhengxian liu Yongzhi Zhao Department of Mechanics School of Mechanical EngineeringTianjin UniversityTianjin300350China Insttute of process quipment College of Energy EngineeringZhejiang UniversityHangzhou30027China

Based on a semi-resolved CFD-DEM coupling method,this study proposed a method that uses the minimum distance between the fluid grid and the particle boundary as a reference value to determine the degree of influence of the target fluid grid on the particle's drag force.A fluidized bed of rod-like particles was chosen as a typical case to investigate the effect of different fluid grid scales on various fluidized bed characteristic *** calculation performance of the semi-resolved and unre-solved CFD-DEM coupling algorithm on key fluidized bed characteristic parameters such as average pressure drop,particle frequency distribution with bed height,and particle orientation distribution were *** was found that the semi-resolved CFD-DEM coupling algorithm gradually obtained results with higher consistency with decreasing fluid grid scale for key parameters such as particle frequency distribution with bed height,particle orientation distribution,and time-history mixing index,exhibiting a phenomenon similar to grid independence in fluid *** comparing with experimental results,it was verified that the semi-resolved CFD-DEM coupling algorithm can be applied to simulate multi-granular gas-solid systems with fluid grid scales equivalent to particle *** algorithm solves the limitation of fluid grid scale in the unresolved CFD-DEM coupling framework and improves the grid adaptability of the CFD-DEM coupling simulation algorithm.

关键词： CFD-DEM Semi-resolved method Fluid-solid flow Non-spherical particle Fluidized bed

Toxicity mechanisms of photodegraded polyvinyl chloride nanoplastics on pea seedlings

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Frontiers of Environmental Science & Engineering 2024年第4期18卷 111-124页

作者： Hao Wu Beibei he Bocheng Chen An liu College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China

Nanoplasctics(Nps),which are very small in particle size,exert toxic effect to ***,compared to original Nps,photodegraded Nps would pose higher *** is because their relatively higher specific surface areas and the presence of additives which can more easily *** original Nps and aged Nps affect plant growth has not been widely *** work chose polyvinyl chloride Nps(pVC-Nps)that were subjected to up to 1000 h UV light radiation to explore the impact of pVC-Nps on the growth of pea seedlings(pisum Sativum L.).The results indicated the existence of pVC-Nps with longer UV light radiation time and higher concentrations had more negative influences on pea seedlings’growth such as germination rate(decreased by 10.6%–22.5%),stem length(decreased by 2.8%–8.1%),dry weight(decreased by 6.3%–7.1%)and fresh weight(decreased by 6.7%–14.8%).It was also noted that photodegraded pVC-Nps resulted in damage to leaf stomata and roots,hindering photosynthesis and absorption of nutrients and hence the decrease in chlorophyll and soluble sugar *** to transcriptomic investigation results,the presence of aged pVC-Nps primarily influenced protein processing in endoplasmic reticulum(upregulated metabolic pathway)and phenylpropanoid biosynthesis(downregulated metabolic pathway)of pea *** results provide an in-depth understanding of how Nps influence the growth of plants.

关键词： Nanoplasctics polyvinyl chloride Toxicity mechanisms plant growth

Effects of vibration conditions,spatial confinement and friction on mixing and segregation characteristics of mixed pebble beds for CFETR WCCB blanket

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particuology 2024年第2期85卷 268-279页

作者： Yong liu Chongyang he Cong Wang Lei Chen Songlin liu Institute of plasma physics Hefei Institutes of Physical ScienceChinese Academy of SciencesHefei230031China University of Science and Technology of China Hefei230027China Chengdu University Chengdu610106China Zhejiang Lab Hangzhou310000China

This paper presents the study of the dynamic characteristics of confined mixed pebble beds with different friction under different vibration conditions using the discrete element ***λsegre-gation index is used to quantify the degree of particle mixing or *** percolation,convection and diffusion mechanisms are responsible for the segregation patterns of the mixed *** results show the degree of segregation can be suppressed by decreasing the vibration acceleration or free space height below a *** simulation reveals the threshold of vibration acceleration or free space height both are related to the bed height increment which determines the strength of the percolation *** addition,the strength of percolation and convection becomes weaker by decreasing the friction of particles and walls,which makes the pebbled bed remains in a mixed state under *** findings are significant to clarify the main factors behind the three segregation mechanisms and hence provide solutions to retaining the mixed state of the Li2TiO3&Be12Ti mixed pebble bed.

关键词： Vibration Segregation Binary pebble bed Discrete element method

Identification of the optimal dop.ng position of hetero-atoms in chalcogen-doped Fe-N-C catalysts for oxygen reduction reaction

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particuology 2024年第6期89卷 99-108页

作者： Weihao liu Huanhuan he Qingtao liu Xin Wan Jianglan Shui School of Materials Science and Engineering Beihang UniversityBeijing100191China School of Space and Environment Beihang UniversityBeijing102206China Tianmushan Laboratory Hangzhou310023China

The excellent oxygen reduction reaction(ORR)activity of Fe–N–C catalysts in acidic media makes them potential for low-cost proton exchange membrane fuel *** recent years,it has been shown that heteroatoms(B,O,S,p,Cl,F,etc.)can be used as electron-withdrawing groups to modulate the planar structure and electron distribution of the Fe–Nx active sites to achieve simultaneous improvement of catalytic activity and ***,the optimal location of the heteroatoms remains ***,taking chalcogen heteroatoms(S and Se)as an example,we control the dop.ng positions and investigate their effect on the ORR performance of the Fe–N–C *** first coordination shell of the iron single atom is identified as the optimal dop.ng *** optimized catalysts Fe–N_(3)Se_(1)/NC and Fe–N_(3)Se_(1)/NC demonstrate improved activity and stability in both half cells and fuel *** work provides insights into the enhancement mechanism of heteroatom dop.ng in single-atom catalysts.

关键词： Oxygen reduction reaction Fe-N-C catalysts hetero-atom dop.ng Dop.ng position Enhancement mechanism

GraphSTGAN:Situation understanding network of slow-fast high maneuvering targets for maritime monitor services of IoT data

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Digital Communications and Networks 2024年第3期10卷 620-630页

作者： Guanlin Wu Haip.ng Wang Yu liu You he Shenzhen International Graduate School Tsinghua UniversityShenzhen518071China Institute of Space Science and Applied Technology Harbin Institute of TechnologyShenzhen518055China Department of Electronic Engineering Tsinghua UniversityBeijing100084China

With the rapid growth of the maritime Internet of Things(IoT)devices for Maritime Monitor Services(MMS),maritime traffic controllers could not handle a massive amount of data in *** unmanned MMS,one of the key technologies is situation ***,the presence of slow-fast high maneuvering targets and track breakages due to radar blind zones make modeling the dynamics of marine multi-agents difficult,and pose significant challenges to maritime situation *** order to comprehend the situation accurately and thus offer unmanned MMS,it is crucial to model the complex dynamics of multi-agents using IoT big ***,previous methods typically rely on complex assumptions,are plagued by unstructured data,and disregard the interactions between multiple agents and the spatial-temporal correlations.A deep learning model,Graph Spatial-Temporal Generative Adversarial Network(GraphSTGAN),is proposed in this paper,which uses graph neural network to model unstructured data and uses STGAN to learn the spatial-temporal dependencies and *** experiments show the effectiveness and robustness of the proposed method.

关键词： Internet of things Multi-agents Graph neural network Maritime monitoring services

Interaction of yttrium barrier and calcium-rich phase on production and properties of WC precursor powders and alloys

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Journal of Rare Earths 2024年第1期42卷 228-236,I0008页

作者： Wen he Dunqiang Tan Zhiqiang Yi Zhiqiang liu School of Materials Science and Engineering Nanchang UniversityNanchang330031China Instrumental Analysis Center of Nanchang Hangkong University Nanchang330063China

In order to reduce or eliminate the adverse effects of calcium impurity,the interaction of Ca and rare earth Y co-dop.ng on the preparation of WC-Co cemented carbides was investigated.X-ray diffraction,scanning electron microscopy and transmission electron microscopy were employed to analyze the phase compositions,particle sizes and morphologies of them,*** results show that the second type of"yttrium barrier effect"is observed and the adverse influence of Ca-rich phase on tungsten powder can be eliminated by *** flexural strength and fracture toughness of YG6-0.01%Ca+0.09%Y alloy are 2199.5 Mpa and 11.49 Mpa·m^(1/2),showing improvement of 6.5% and 2.7% compared to YG6 alloy,*** evolutions of Ca-rich phase and Y-rich phase at the every alloy preparation stage of WO_(3),W,WC and cemented carbides are ***,the strengthening mechanism of WC-Co cemented carbide with co-addition of Ca and Y is proposed.

关键词： Yttrium barrier effect Ca-rich phase WC-Co cemented Carbide Microstructures Mechanisms Rare earths

Review on synergistic damage effect of irradiation and corrosion on reactor structural alloys

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Nuclear Science and Techniques 2024年第3期35卷 109-141页

作者： Hui liu Guan-Hong Lei he-Fei Huang Shanghai Institute of Applied physics Chinese Academy of SciencesShanghai 201800China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China

The synergistic damage effect of irradiation and corrosion of reactor structural materials has been a prominent research *** paper provides a comprehensive review of the synergistic effects on the third-and fourth-generation fission nuclear energy structural materials used in pressurized water reactors and molten salt *** competitive mechanisms of multiple influencing factors,such as the irradiation dose,corrosion type,and environmental temperature,are summarized in this *** approaches are proposed to alleviate the synergistic damage caused by irradiation and corrosion,thereby promoting in-depth research in the future and solving this key challenge for the structural materials used in reactors.

关键词： Irradiation and corrosion Synergistic effect Austenitic stainless steels Nickel-based alloys Reactors

p2p Energy Trading Considering prosumer preference and System Risk

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CSEE Journal of power and Energy Systems 2024年第3期10卷 1179-1194页

作者： Xinyu he p.ng Dong Mingbo liu Xuewei Huang Wenli Deng Ruijin he School of Electric power Engineering South China University of TechnologyGuangzhou 510640China IEEE

As an important means of mobilizing demand-side resources,peer-to-peer(p2p)energy trading has drawn more and more attention from *** paper constructs a p2p energy trading framework considering prosumers’trading partner preferences(Tpps)and system *** first,we build the p2p trading models of prosumers equipped with different distributed energy resources(DERs),and Tpp ***,to solve the established energy trading problem,a fully distributed double-consensus alternating direction method of multipliers(DC-ADMM)is proposed,which can achieve transaction consensus when considering market players’***,a risk-based security constrained economic dispatch(RBSCED)model based on AC power flow is established for the first time,by which a distribution system operator(DSO)checks system security and obtains risk-based locational marginal prices(RLMps).Moreover,double-regulated price signals related to RLMps which contain grid utilization prices(GUps)and DSO’s retail prices realize management of players’*** the end,the proposed method is applied to an IEEE33 bus distribution *** show the proposed method effectively reduces system risk and ensures secure operation of system without direct management.

关键词： Double-consensus ADMM grid utilization price price signal risk-based locational marginal price trading partner preference

Effect of surfactant frequently used in soil flushing on oxygen mass transfer in micro-nano-bubble aeration system

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Chinese Journal of Chemical Engineering 2024年第3期67卷 174-181页

作者： Mei Bai Zhibin liu Zhu liu Chenfei he Zhanhuang Fan Miaoxin Yuan Jiangsu Key Laboratory of Urban Underground Engineering and Environmental Safety Southeast UniversityNanjing 211189China CECEp DADI(Hangzhou)Environmental Remediation Co. Ltd.Hangzhou 310020China

In-site soil flushing and aeration are the typical synergetic remediation technology for contaminated *** surfactant present in flushing solutions is bound to affect the aeration *** purpose of this study is to evaluate the effect of surfactant frequently used in soil flushing on the oxygen mass transfer in micro-nano-bubble(MNB)aeration ***,bio-surfactants and chemical surfactants were used to investigate their effects on Sauter mean diameter of bubble(dBS),gas holdup(ε),volumetric mass-transfer coefficient(kLa)and liquid-side mass-transfer coefficient(kL)in the MNB aeration ***,based upon the experimental results,the Sardeing's and Frossling's models were modified to describe the effect of surfactant on kL in the MNB *** results showed that,for the twenty aqueous surfactant solutions,with the increase in surfactant concentration,the value of dBS,kLa and kL decreased,while the value ofεand gas-liquid interfacial area(a)*** phenomena were mainly attributed to the synergistic effects of immobile bubble surface and the suppression of coalescence in the surfactant *** addition,with the presence of electric charge,MNBs in anionic surfactant solutions were smaller and higher in number than in non-ionic surfactant ***,the accumulation of surfactant on the gas-liquid interface was more conspicuous for small MNB,so the reduction of kL in anionic surfactant solutions was larger than that in non-ionic surfactant ***,the modified Frossling's model predicted the effect of surfactant on kL in MNB aeration system with reasonable accuracy.

关键词： Soil flushing Micro-nano-bubble aeration Bio-surfactant Mass transfer coefficient