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Microwave-accelerated direct regeneration of LiCoO_(2)cathodes for Li-ion batteries

Science China Chemistry 2024年第7期67卷 2181-2189页

作者： Xueshan Hu Yun-Chao Yin Chao Li Lihui Zhou Lin Yang Yitian Feng Daxian Zuo Chenhui Ning Das Soham Sheng Dai Longbin Qiu Lin Zeng haw jiunn woo Jiayu Wan Future Battery Research Center Global Institute of Future TechnologyShanghai Jiao Tong UniversityShanghai 200240China Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhen 518055China Centre for Ionics University of Malaya Department of PhysicsFaculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China Department of Natural and Applied Sciences Duke Kunshan UniversityKunshan 215316China

Recycling spent lithium-ion batteries is integral to today's low-carbon environmental protection *** concept of direct regeneration,acknowledged for its environmental sustainability,economic viability,and consistent performance of recycled materials,is gaining *** study presents an efficient and nondestructive approach by utilizing an ultrafast microwave technology to directly regenerate spent lithium cobaltate(LCO)cathode *** contrast to conventional furnacebased processes,this method significantly reduces the regeneration *** subjecting the spent LCO mixed with lithium sources to three microwave heating cycles(at approximately 1,350 K),LCO regeneration is achieved,yielding a specific capacity of 140.8 mAh g^(-1)(0.2 C)with a robust cycle *** further environmental and economic benefits,the ultrafast microwave technology holds scientific promise for directly regenerating cathode materials,while establishing competitiveness for industrial applications.

关键词： battery recycling spent lithium cobaltate microwave directly regeneration cathode materials

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Performance of pulsed plasma thruster at low discharge energy

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Plasma Science and Technology 2024年第4期26卷 122-132页

作者：李鸿俊林泽豪胡浩俊吴文东陈爱虹杜德扬 Department of Physics Faculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Faculty of Engineering The University of Nottingham Malaysia CampusSemenyih 43500Malaysia Faculty of Engineering Multimedia UniversityCyberjaya 63100Malaysia

As the size of satellites scales down, low-power and compact propulsion systems such as the pulsed plasma thruster(PPT) are needed for stabilizing these miniature satellites in orbit. Most PPT systems are operated at 2 J or more of discharge energy. In this work, the performance of a PPT with a side-fed, tongue-flared electrode configuration operated within a lower discharge energy range of 0.5-2.5 J has been investigated. Ablation and charring of the polytetrafluoroethylene propellant surface were analyzed through field-effect scanning electron microscopy imaging and energy-dispersive X-ray spectroscopy. When the discharge energy fell below 2 J, inconsistencies occurred in the specific impulse and the thrust efficiency due to the measurement of the low mass bit. At energy ≥2 J, the performance parameters are compared with other PPT systems of similar configuration and discussed in depth.

关键词： pulsed plasma thruster low discharge energy performance parameters

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A low power 50Hz argon plasma for surface modification of polytetrafluoroethylene

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Plasma Science and Technology 2022年第11期24卷 1-13页

作者： Yen Theng LAU Wee Siong CHIU Hong Chun LEE haw jiunn woo Oi Hoong CHIN Teck Yong TOU Department of Physics Faculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Faculty of Engineering Multimedia UniversityPersiaran CyberjayaCyberjaya 63100Malaysia

The characteristics of a low power 50 Hz argon plasma for surface treatment of polytetrafluoroethylene(PTFE)film is presented in this *** current–voltage behavior of the discharge and time-varying intensity of the discharge showed that a DC glow discharge was generated in reversed polarity at every *** discharge power between 0.5 and 1 W,the measured electron temperature and density were 2–3 eV and∼10^(8) cm^(−3),*** optical emission spectrum of the argon plasma showed presence of some‘impurity species’such as OH,N_(2) and H,which presumably originated from the residual air in the discharge *** exposure of PTFE films to the argon glow plasma at pressure 120 Pa and discharge power 0.5 to 1 W,the water contact angle reduced by 4%to 20%from the original 114°at pristine condition,which confirms improvement of its surface *** increase in wettability was attributed to incorporation of oxygen-containing functional groups on the treated surface and concomitant reduction in fluorine as revealed by the XPS analysis and increase in surface roughness analyzed from the atomic force *** upon storage in ambient air showed retention of the induced increase in surface wettability.

关键词： 50 Hz glow discharge plasma surface treatment PTFE hydrophobic recovery ageing effect

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Alkali and alkaline ions co-substitution of P2 sodium layered oxides for sodium ion batteries

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Chinese Journal of Structural Chemistry 2023年第5期42卷 13-21页

作者： Yuncai Chen Maolin Yang Liangtao Yang Ziwei Chen Huiyun Li haw jiunn woo Shang-Sen Chi Yinguo Xiao Jun Wang Chaoyang Wang Yonghong Deng Key University Laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of Guangdong Department of Materials Science&EngineeringSchool of Innovation and EntrepreneurshipSouthern University of Science and TechnologyShenzhen518055China Centre for Ionics University Malaya Department of PhysicsFaculty of ScienceUniversity of MalayaKuala Lumpur50603Malaysia School of Advanced Materials Peking UniversityShenzhen Graduate SchoolShenzhen518055China Shenzhen Institutes of Advanced Technology Chinese Academy of SciencesShenzhen518055China Research Institute of Materials Science South China University of TechnologyGuangzhou510640China

Alkali and alkaline ion substitutions enhance the electrochemical properties of P2 sodium layered oxide,while the effect on electrochemical property enhancement of alkali and alkaline ions co-substitution is still *** this work,the structural and electrochemical properties of the Li alkali and Mg alkaline ions co-substituted P2 layered oxide Na_(0.67)(Li_(0.5)Mg_(0.5))_(0.1)(Ni_(0.33)Mn_(0.67))_(0.9)O_(2)are investigated in *** to the pristine and single-ion substituted materials,the co-substituted material shows an enhanced cycling performance with a reversible ca-pacity of 127 mAh/g and a capacity retention of 75%over 100 cycles at *** intermittent titration technique(GITT)and cyclic voltammetry(CV)results show that the Li and Mg synergistically improve the ion ***,the structure stability is also improved by the Li and Mg co-substitution that is clarified by operando X-ray diffraction(XRD)*** results explain the origin of the enhanced electrochemical properties of the Li/Mg co-substituted P2 layered oxides for sodium ion batteries.

关键词： Sodium ions batteries Sodium layered oxides Alkali and alkaline elements co-substitution Neutron diffraction Structural evolution

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Evaluations of Novel Waveform Coding Signals Based on Finite Projective Plane

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Journal of Electronic Science and Technology 2016年第1期14卷 54-59页

作者： Chien-Hsing Liao Tai-Kuo woo Chi-Chung Chen Ing-jiunn Su the Program of Information Technology Fooyin University the Department of Information Management National Defense University the Department of Electrical and Electronic Engineering National Defense University

The most popular and representative classic waveform codes are referred to as orthogonal,bi-orthogonal,simplex,and etc,but the choice of waveform codes is essentially identical in error performance and cross correlation *** bi-orthogonal coding requires half the bandwidth of the others,such coding scheme is attractive only when large bandwidth is *** this paper,a novel finite projective plane（FPP） based waveform coding scheme is proposed,which is with similar error performance and cross ***,the bandwidth requirement will grow in a quadratic way,but not in an exponential way with the values of message bit numbers（k）.The proposed scheme takes obvious advantages over the bi-orthogonal scheme when k ≥ 6.

关键词： Finite projective plane orthogonal coding simplex coding waveform coding

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Hierarchically designed MoWSe_(2)/WO_(3)/C anode for fast and efficient Na+storage

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Journal of Energy Chemistry 2023年第5期80卷 291-301,I0008页

作者： Jian Wang Yachuan Shao Fei Yuan Huilan Sun Di Zhang Zhaojin Li S.Ramesh H.J.woo Bo Wang Centre for Ionics University of Malay1 Department of PhysicsFaculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Hebei Key Laboratory of Flexible Functional Materials School of Materials Science and EngineeringHebei University of Science and TechnologyShjiazhuang 0500000HebeiChina

Exploring anode materials with high energy and power density is one of the critical milestones in developing sodium-ion batteries/capacitors(SIBs/SICs).Here,the Mo and W-based bimetallic organic framework(Mo-W-MOF)with core-shell structure is first formed by a facile strategy,followed by a selenization and carbonization strategy to finally prepare multileveled Mo WSe_(2)/WO_(3)/C anode materials with core-shell petal like curled nanosheet *** the petal(MoSe_(2))-core(WO_(3))structure,the formation of WSe_(2)flakes by partial selenization on the surface of WO_(3)serves as a heterogeneous connection between MoSe_(2)and WO_(3).The enlarged layer distance(0.677 nm)between MoSe_(2)and WSe_(2)can facilitate the rapid transfer of Na+and *** density functional theory(DFT)calculations verify that the Mo WSe_(2)/WO_(3)/C heterostructure performs excellent metallic ***-situ X-ray diffraction(XRD),X-ray photoelectron spectroscopy(XPS),and transmission electron microscopy(TEM)confirm the activation process from the initial insertion reaction to the later conversion ***,when employed as the anode of SIBs,a remarkable capacity of 384.3 mA h g-1after 950 cycles at 10 A g^(-1)is ***,the SICs assembled with commercial activated carbon(AC)as the cathode exhibits a remarkable energy density of 81.86 W h kg^(-1)(at 190 W kg^(-1))and 72.83 W h kg^(-1)(at 3800 W kg^(-1)).The unique structural design and the reaction investigation of the electrode process can provide a reference for the development of transition metal chalcogenides anodes.

关键词： Multileveled MoWSe2/WO_(3)/C Structure change Heterostructure Metallic properties Enlarged lattice distance The activation process

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