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Science China(Information Sciences) 2024年

作者： haoran wu Kaiming NIE Jiangtao XU Qinglong LIN Yingying JIAO 1.School of Microelectronics, Tianjin University 2.Tianjin Key Laboratory of Imaging and Sensing Microelectronic Technology

In recent years, Flash LiDAR sensors based on direct timeof-flight(DToF) have been playing an increasingly important role in various 3D imaging fields. In order to perform a histogram on the chip to reduce the data rate, it is inevitable to use a large-size histogramming time-to-digital converter(hT DC) in a Flash LiDAR sensor. However, a large-size hT DC limits the spatial resolution of the sensor.

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Gut microbiota-dependent phenylacetylglutamine in cardiovascular disease:current knowledge and new insights

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Frontiers of Medicine 2024年第1期18卷 31-45页

作者： Yaonan Song haoran Wei Zhitong Zhou Huiqing Wang Weijian Hang Junfang wu Dao Wen Wang Division of Cardiology Department of Internal MedicineTongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan430030China Hubei Key Laboratory of Genetics and Molecular Mechanisms of Cardiological Disorders Wuhan430030China

Phenylacetylglutamine(PAGln)is an amino acid derivate that comes from the amino acid phenylalanine.There are increasing studies showing that the level of PAGln is associated with the risk of different cardiovascular diseases.In this review,we discussed the metabolic pathway of PAGln production and the quantitative measurement methods of PAGln.We summarized the epidemiological evidence to show the role of PAGln in diagnostic and prognostic value in several cardiovascular diseases,such as heart failure,coronary heart disease/atherosclerosis,and cardiac arrhythmia.The underlying mechanism of PAGln is now considered to be related to the thrombotic potential of platelets via adrenergic receptors.Besides,other possible mechanisms such as inflammatory response and oxidative stress could also be induced by PAGln.Moreover,since PAGln is produced across different organs including the intestine,liver,and kidney,the cross-talk among multiple organs focused on the function of this uremic toxic metabolite.Finally,the prognostic value of PAGln compared to the classical biomarker was discussed and we also highlighted important gaps in knowledge and areas requiring future investigation of PAGln in cardiovascular diseases.

关键词： PAGln cardiovascular disease gut microbiota uremic metabolite biomarker

Development of sustainable and efficient recycling technology for spent Li-ion batteries: Traditional and transformation go hand in hand

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Green Energy & Environment 2024年第5期9卷 802-830页

作者： Zejian Liu Gongqi Liu Leilei Cheng Jing Gu haoran Yuan Yong Chen Yufeng wu Guangzhou Institute of Energy Conversion Chinese Academy of Sciences(CAS)Guangzhou510640China School of Engineering Science University of Science and Technology of ChinaHefei230026China Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development Guangzhou510640China Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing100124China

Clean and efﬁcient recycling of spent lithium-ion batteries(LIBs)has become an urgent need to promote sustainable and rapid development of human society.Therefore,we provide a critical and comprehensive overview of the various technologies for recycling spent LIBs,starting with lithium-ion power batteries.Recent research on raw material collection,metallurgical recovery,separation and puriﬁcation is highlighted,particularly in terms of all aspects of economic efﬁciency,energy consumption,technology transformation and policy management.Mechanisms and pathways for transformative full-component recovery of spent LIBs are explored,revealing a clean and efﬁcient closed-loop recovery mechanism.Optimization methods are proposed for future recycling technologies,with a focus on how future research directions can be industrialized.Ultimately,based on life-cycle assessment,the challenges of future recycling are revealed from the LIBs supply chain and stability of the supply chain of the new energy battery industry to provide an outlook on clean and efﬁcient short process recycling technologies.This work is designed to support the sustainable development of the new energy power industry,to help meet the needs of global decarbonization strategies and to respond to the major needs of industrialized recycling.

关键词： Spent LIBs Transformative recycling LCA analysis Policy guidance High value utilization

A bifunctional wood membrane modified by MoS_(2)/covalent organic framework heterojunctions for effective solar-driven water evaporation and contaminant degradation

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Science China Chemistry 2024年第6期67卷 2111-2120页

作者： Ziwei Cui Jianfei wu haoran Li Yaning Xu Tiantian wu Lixing Kang Qing Huang Yahui Cai Jianzhang Li Dan Tian Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing210037China Key Laboratory of Multifunctional Nanomaterials and Smart Systems Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou215123China State Key Laboratory of Efficient Production of Forest Resources Beijing Forestry UniversityBeijing100083China

Interfacial solar evaporation technology is considered one of the most promising strategies for alleviating the scarcity of freshwater resources.However,solar-driven evaporation technology cannot eliminate the pollutants in the residual wastewater.To solve this problem,we have prepared a two-in-one solar-driven evaporation/photocatalysis system by decorating MoS_(2)/covalent organic framework(COF)heterojunctions on wood(MoS_(2)/COF-wood).Thanks to the unique porous structure of wood,it provides a strong guarantee for water transport and vapor release during the evaporation process.The introduction of MoS_(2) and COFs can promote the breaking of hydrogen bonds between water molecules,which leads to a significant decrease in the enthalpy of evaporation,achieving a water evaporation rate as high as 2.17 kg m^(-2)h^(-1)under 1 sun irradiation.Meanwhile,the resulting MoS_(2)/COF-wood exhibits good salt resistance and reusability.In addition,the heterojunctions formed between COFs and MoS_(2) can effectively inhibit charge carrier complexation and improve the photocatalytic degradation ability of pollutants(over 99%).This study highlights the construction strategy of bifunctional wood-based materials for freshwater production and wastewater remediation.

关键词： covalent organic framework MoS_(2) wood photocatalysis solar-driven evaporation

Detachment Behavior of Gecko Toe in Functional Strategies for Bionic Toe

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Journal of Bionic Engineering 2024年第2期21卷 707-717页

作者： Qingfei Han Wei Wang Huan Shen Xincheng Feng haoran Zhang Qian Li Yi Sun Huapeng wu Aihong Ji Lab of Locomotion Bioinspiration and Intelligent Robots College of Mechanical and Electrical EngineeringNanjing University of Aeronautics and AstronauticsNanjing210016China Laboratory of Intelligent Machines School of Energy SystemsLappeenranta-Lahti University of Technology53850LappeenrantaFinland State Key Laboratory of Mechanics and Control for Aerospace Structures Nanjing University of Aeronautics and AstronauticsNanjing210016China

Geckos can efficiently navigate complex terrains due to their multi-level adhesive system that is present on their toes.The setae are responsible for the gecko’s extraordinary adhesion and have garnered wide attention from the scientific community.The majority of the reported works in the literature that have dealt with the peeling models mainly focus on the gecko hierarchical adhesive system,with limited attention given to investigating the influence of gecko toe structure on the detachment.Along these lines,to gain a deeper understanding of the rapid and effortless detachment abilities of gecko toes,the peeling behavior of gecko toes on vertical surfaces was primarily investigated in this work.More specifically,the detachment time of a single toe on a smooth acrylic plate was measured to be 0.41±0.21 s.Moreover,it was observed that the toe assumed a"U"-shaped structure upon complete detachment.Additionally,Finite Element Analysis(FEA)models for three different types of gecko toes were developed to simulate both the displacement-peel and the moment-peel modes.Increasing the segmentation of the adhesive layer led to a gradual decrease in the resultant force,as well as the normal and tangential components.Lastly,a gecko-inspired toe model was constructed and powered by Shape Memory Alloy(SMA).A systematic comparison between the vertical drag separation and the outward flip separation was also conducted.From our analysis,it was clearly demonstrated that outward peel separation significantly necessitated the reduction of the peeling force,thus confirming the advantageous nature of the outward motion in gecko toe detachment.Our data not only contribute to a deeper understanding of the gecko detachment behavior but also offer valuable insights for the advancement of the wall-climbing robot feet.

关键词： Gecko toes Detachment behavior Finite element analysis Gecko-inspired toe

Artificial rabbit optimization algorithm based on chaotic mapping and Levy flight improvement

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The Journal of China Universities of Posts and Telecommunications 2024年

作者： wu Jin Su Zhengdong Gao Yaqiong Feng haoran School of Electronic Engineering Xi’an University of Posts and Telecommunications

An artificial rabbit optimization algorithm based on chaotic mapping and Levy flight improvement is proposed， which has the advantages of good initial population quality and fast convergence compared with the traditional artificial rabbit optimization algorithm， called CLARO. CLARO is improved by applying three methods. Chaotic mapping is introduced， which can optimize the quality of the initial population of the algorithm. Add Levy flight in the exploration phase， which can avoid the algorithm from falling into a local optimum. The threshold of the energy factor is optimized， which can better balance exploration and exploitation. The efficiency of CLARO is tested on a set of 23 benchmark function sets by comparing it with artificial rabbit optimization (ARO) and different meta-heuristics algorithms. At last， the comparison experiments conclude that all three improvement strategies enhance the performance of ARO to some extent， with Levy flight providing the most significant improvement in ARO performance. The experimental results show that CLARO has better results and faster convergence compared to other algorithms， while successfully addressing the drawbacks of ARO and being able to face more challenging problems.

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Local-to-Global Causal Reasoning for Cross-Document Relation Extraction

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IEEE/CAA Journal of Automatica Sinica 2023年第7期10卷 1608-1621页

作者： haoran wu Xiuyi Chen Zefa Hu Jing Shi Shuang Xu Bo Xu Institute of Automation Chinese Academy of SciencesBeijing 100190China. School of Artificial Intelligence University of Chinese Academy of SciencesBeijing 100190China

Cross-document relation extraction(RE),as an extension of information extraction,requires integrating information from multiple documents retrieved from open domains with a large number of irrelevant or confusing noisy texts.Previous studies focus on the attention mechanism to construct the connection between different text features through semantic similarity.However,similarity-based methods cannot distinguish valid information from highly similar retrieved documents well.How to design an effective algorithm to implement aggregated reasoning in confusing information with similar features still remains an open issue.To address this problem,we design a novel local-toglobal causal reasoning(LGCR)network for cross-document RE,which enables efficient distinguishing,filtering and global reasoning on complex information from a causal perspective.Specifically,we propose a local causal estimation algorithm to estimate the causal effect,which is the first trial to use the causal reasoning independent of feature similarity to distinguish between confusing and valid information in cross-document RE.Furthermore,based on the causal effect,we propose a causality guided global reasoning algorithm to filter the confusing information and achieve global reasoning.Experimental results under the closed and the open settings of the large-scale dataset Cod RED demonstrate our LGCR network significantly outperforms the state-ofthe-art methods and validate the effectiveness of causal reasoning in confusing information processing.

关键词： Causal reasoning cross document graph reasoning relation extraction(RE)

One-pot synthesis of bimetallic CeCu-SAPO-34 for high-efficiency selective catalytic reduction of nitrogen oxides with NH_(3) at low temperature

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Chinese Journal of Chemical Engineering 2023年第4期56卷 193-202页

作者： Shuang Qiu Yonghou Xiao haoran wu Shengnan Lu Qidong Zhao Gaohong He Panjin Institute of Industrial Technology Liaoning Key Laboratory of Chemical Additive Synthesis and SeparationDalian University of TechnologyPanjin 124221China State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyPanjin 124221China School of Petrochemical Engineering Shenyang University of TechnologyLiaoyang 111003China

NH_(3) selective catalytic reduction(SCR) has been widely recognized as a promising technique for reducing nitrogen oxides from diesel vehicle exhausts. High-efficiency SCR catalysts that could perform at low temperatures are essential to denitration. In this work, a series of bimetallic CeCu-SAPO-34 molecular sieves were synthesized by one-step hydrothermal method. The Ce Cu-SAPO-34 maintained good crystallinity and a regular hexahedron appearance of Cu-SAPO-34 after introducing Ce species, while exhibiting a higher specific surface area and pore volume. The as-prepared CeCu-SAPO-34 with 0.02%(mass) Ce constituent exhibited the best catalytic activity below 300℃ and a maximum NO_(x) conversion of 99% was attained;the NO_(x) removal rates of more than 68% and 94% were achieved at 150℃ and 200℃, respectively. And the introduction of cerium species in Cu-SAPO-34 improves the low-temperature hydrothermal stability of the catalyst towards NH_(3)-SCR reaction. Additionally, the introduced Ce species could enhance the formation of abundant weak Br?nsted acid centers and promote the synergistic effect between CuO grains and isolated Cu^(2+) to enhance the redox cycle, which benefit the NH_(3)-SCR reaction.This work provides a facile synthesis method of high-efficiency SCR denitration catalysts towards diesel vehicles exhaust treatment under low temperature.

关键词： CeCu-SAPO-34 Selective catalytic reduction(SCR) Low temperature DeNO_(x) One-pot synthesis

High nitrogen fertilizer input enhanced the microbial network complexity in the paddy soil

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Soil Ecology Letters 2024年第2期6卷 97-109页

作者： Yanan Chen Yan Li Tianyi Qiu haoran He Ji Liu Chengjiao Duan Yongxing Cui Min Huang Chunyan wu Linchuan Fang The Research Center of Soil and Water Conservation and Ecological Environment Chinese Academy of Sciences and Ministry of EducationYangling712100China State Key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau Institute of Soil and Water Conservation CAS and MWRYangling712100China University of Chinese Academy of Sciences Beijing100049China Institute of Environment Resource and Soil Fertilizer Zhejiang Academy of Agricultural SciencesHangzhou310021China College of Natural Resources and Environment Northwest A&F UniversityYangling712100China Hubei Province Key Laboratory for Geographical Process Analysis and Simulation Central China Normal UniversityWuhan430079China Department of Ecohydrology Leibniz Institute of Freshwater Ecology and Inland FisheriesBerlin12587Germany Sino-French Institute for Earth System Science College of Urban and Environmental SciencesPeking UniversityBeijing100871China College of Resources and Environmental Engineering Wuhan University of TechnologyWuhan430070China CAS Center for Excellence in Quaternary Science and Global Change Xi’an710061China

N fertilizer altered bacterial community compositions by changing soil nutrients.•Bacterial ammonia oxidation became predominated with the increasing N rate.•Excessive N input caused the information of a more complex microbial network.•Intensified microbial competition by excessive N was due to negative link increase.Nitrogen(N)fertilization drives the structure and function of soil microbial communities,which are crucial for regulating soil biogeochemical cycling and maintaining ecosystem stability.Despite the N fertilizer effects on soil microbial composition and diversity have been widely investigated,it is generally overlooked that ecosystem processes are carried out via complex associations among microbiome members.Here,we examined the effects of five N fertilization levels(0,135,180,225,and 360 kg N ha−1)on microbial co-occurrence networks and key functional taxa such as ammonia-oxidizers in paddy soils.The results showed that N addition altered microbial community composition,which were positively related to soil total N and available phosphorus(P)contents.The abundance of ammonia-oxidizing archaea(AOA)significantly decreased after N addition,whereas ammonia-oxidizing bacteria(AOB)increased in N360 treatment.Compared with low-N group(N0 and N135),the high-N group(N225 and N360)shaped more complex microbial webs and thus improved the stability of the microbial community.Partial least squares path modeling further revealed that N fertilizer had a higher effect on microbial network complexity in the high-N group(0.83)than the low-N group(0.49).Although there were more positive links across all microbial networks,the proportion of negative links significantly increased in the high-N network,suggesting that excess N addition aggravated the competition among microbial species.Disentangling these interactions between microbial communities and N fertilization advances our understanding of biogeochemical processes in paddy soils and their effects on nutrient supply to rice production.Our findings highlighted that h

关键词： nitrogen fertilizer paddy soil co-occurrence network microbial interaction

Unlocking the potential of thin-film composite reverse osmosis membrane performance:Insights from mass transfer modeling

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Chinese Chemical Letters 2024年第5期35卷 66-76页

作者： Kexin Yuan Yulei Liu haoran Feng Yi Liu Jun Cheng Beiyang Luo Qinglian wu Xinyu Zhang Ying Wang Xian Bao Wanqian Guo Jun Ma State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China College of Architecture and Environment Sichuan UniversityChengdu 610065China School of Municipal and Environmental Engineering Shandong Jianzhu UniversityJi’nan 250101China College of Water Conservancy and Hydropower Engineering Sichuan Agricultural UniversityYaan 625014China

Thin-film composite(TFC)reverse osmosis(RO)membranes have attracted considerable attention in water treatment and desalination processes due to their specific separation advantages.Nevertheless,the trade-off effect between water flux and salt rejection poses huge challenges to further improvement in TFC RO membrane performance.Numerous research works have been dedicated to optimizing membrane fabrication and modification for addressing this issue.In the meantime,several reviews summarized these approaches.However,the existing reviews seldom analyzed these methods from a theoretical perspective and thus failed to offer effective optimization directions for the RO process from the root cause.In this review,we first propose a mass transfer model to facilitate a better understanding of the entire process of how water and solute permeate through RO membranes in detail,namely the migration process outside the membrane,the dissolution process on the membrane surface,and the diffusion process within the membrane.Thereafter,the water and salt mass transfer behaviors obtained from model deduction are comprehensively analyzed to provide potential guidelines for alleviating the trade-off effect between water flux and salt rejection in the RO process.Finally,inspired by the theoretical analysis and the accurate identification of existing bottlenecks,several promising strategies for both regulating RO membranes and optimizing operational conditions are proposed to further exploit the potential of RO membrane performance.This review is expected to guide the development of high-performance RO membranes from a mass transfer theory standpoint.

关键词： Reverse osmosis Mass transfer model Trade-off effect Membrane performance Optimization strategies