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Residents’perceptions of ecosystem services in an urbanizing basin:A case study in the Guanting Reservoir basin,China

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Geography and Sustainability 2024年第3期5卷 430-444页

作者： Yansong Bai Qingxu Huang Luis Inostroza haoran Xu Dan Yin Ziwen Liu Ling Zhang Fangjin Xu State Key Laboratory of Earth Surface Processes and Resource Ecology(ESPRE) Beijing Normal UniversityBeijing 100875China School of Natural Resources Faculty of Geographical ScienceBeijing Normal UniversityBeijing 100875China Faculty of Regional Development and International Studies Mendel University in BrnoBrno 61300Czechia Universidad Autonoma de Chile Santiago 7500912Chile Nanjing Zhongchuang Bookstore Co. Ltd.Nanjing 210018China

Understanding stakeholders’differences in perceptions of ecosystem services(ES)is crucial for guiding ecolog-ical conservation and ***,the variations of ES perception amongst different types of residents in urbanizing areas along an urban-rural gradient are still poorly *** a questionnaire-based survey,redundancy analysis,and statistical tests,we delineated the urban-rural gradient according to local res-idents’socio-economic characteristics,and investigated the differences in local residents’perceptions of ES and potential factors affecting them in the Guanting Reservoir basin,a rapidly urbanizing basin in *** results showed that residents living in urban-rural transitional areas attached great importance to provisioning services of providing food and domestic water,regulating services of carbon sequestration and air purification,and cul-tural services of providing education and training,which were 0.7%-1..1.,0.7%-9.1.and 2.5%-21.2%higher than that of residents in other areas,*** and occupation were major factors affecting residents’*** terms of land-use types that deliver ES,the difference in perceptions of ES delivered by grassland was the greatest amongst *** results support recommendations for policymakers to take into account the stakeholders’diverse perceptions,thus promoting residents’sense of gain on ES.

关键词： Ecosystem services Stakeholder Urban-rural gradient Urbanization Urban sustainability

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Recent advances in functional utilisation of environmentally friendly and recyclable high-performance green biocomposites: A review

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Chinese Chemical Letters 2024年第4期35卷 73-85页

作者： Guiyang Zheng Xuelian Kang haoran Ye Wei Fan Christian Sonne Su Shiung Lam Rock Keey Liew Changlei Xia Yang Shi Shengbo Ge Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037China School of Textile Science and Engineering&Key Laboratory of Functional Textile Material and Product of Ministry of Education Xi'an Polytechnic UniversityXi'an 710048China Department of Bioscience Arctic Research Centre(ARC)Aarhus UniversityFrederiksborgvej 399PO Box 358DK-4000 RoskildeDenmark Sustainability Cluster School of EngineeringUniversity of Petroleum&Energy StudiesDehradunUttarakhand 248007India Higher Institution Centre of Excellence(HICoE) Institute of Tropical Aquaculture and Fisheries(AKUATROP)Universiti Malaysia Terengganu21030 Kuala NerusTerengganuMalaysia Center for Transdisciplinary Research Saveetha Institute of Medical and Technical SciencesSaveetha UniversityChennai 600072India NV Western PLT Georgetown 10400PenangMalaysia Aerospace Kaitian Environmental Technology Co. Ltd.Changsha 410000China Hunan Hongsen Novel Material Technology Co. Ltd.Yiyang 413407China

Humans have relied on biomass for survival and development since the Stone Age. All aspects of human needs for materials are covered by tools, fuel, and buildings. Nowadays, metals and petroleum-based materials are widely used in highly developed industries. Unfortunately, environmental contamination and the loss of natural resources have led to the reemergence of biomass resources as efficient and sustainable energy sources. Notably, simple and direct applications can no longer meet the demand for functionalization, high performance of materials and construction materials. Therefore, it is imperative to modify biomass and combine its utilisation to produce functionalization and high performance materials. For example, construction materials with superior mechanical properties and water resistance can be produced by reinforcing fibres to facilitate crosslinking. Water-oil separation or adsorption effects of hydrogels and aerogels are determined by the porosity and lightness of biomass, biocomposite conductor is prepared by chimaeric conductive material. Here, we review the approaches that have been taken to devise an environmentally friendly yet fully recyclable and sustainable functionalised biocomposites from biomass and its potential directions for future research.

关键词： Biocomposite Renewable Sustainability Advanced functional material Pollution mitigation

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Approaching Ultimate Synthesis Reaction Rate of Ni-Rich Layered Cathodes for Lithium-Ion Batteries

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Nano-Micro Letters 2024年第10期16卷 392-402页

作者： Zhedong Liu Jingchao Zhang Jiawei Luo Zhaoxin Guo haoran Jiang Zekun Li Yuhang Liu Zijing Song Rui Liu Wei-Di Liu Wenbin Hu Yanan Chen School of Materials Science and Engineering Tianjin UniversityTianjin 300072People's Republic of China School of Materials Science and Engineering Shandong University of Science and TechnologyQingdao 266590People's Republic of China Australian Institute of Bioengineering and Nanotechnology The University of QueenslandSt LuciaQLD 4072Australia

Nickel-rich layered oxide LiNi_(x)Co_(y)MnzO_(2)(NCM,x+y+z=1.is the most promising cathode material for high-energy lithium-ion ***,conventional synthesis methods are limited by the slow heating rate,sluggish reaction dynamics,high energy consumption,and long reaction *** overcome these chal-lenges,we first employed a high-temperature shock(HTS)strategy for fast synthesis of the NCM,and the approaching ultimate reaction rate of solid phase transition is deeply investigated for the first *** the HTS process,ultrafast average reaction rate of phase transition from Ni_(0.6)Co_(0.2)Mn_(0.2)(OH)_(2) to Li-containing oxides is 66.7(%s^(-1.),that is,taking only 1.5 *** ultrahigh heating rate leads to fast reaction kinetics,which induces the rapid phase transition of NCM *** HTS-synthesized nickel-rich layered oxides perform good cycling performances(94%for NCM523,94%for NCM622,and 80%for NCM81. after 200 cycles at 4.3 V).These findings might also assist to pave the way for preparing effectively Ni-rich layered oxides for lithium-ion batteries.

关键词： Nickel-rich layered oxides High-temperature shock Solid reaction kinetics Phase transition Reaction rate

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Asymmetric NiH-Catalyzed Regioselective Hydroalkynylation of Unactivated Alkenes

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CCS Chemistry 2024年第8期6卷 1929-1940页

作者： Mengyuan Liu haoran Shi Xiao Meng Rui He Jie Huang Jiaxin Wang Jun Lv Chao Wang Tianjin Key Laboratory of Structure and Performance for Functional Molecules College of ChemistryTianjin Normal UniversityTianjin 300387

Herein,we disclose a ligand-controlled,directing group-assisted strategy to facilitate NiH-catalyzed hydroalkynylation of allyl amides at remoteα-position adjacent to nitrogen and initial olefinic site in a predictable and switchable *** regiodivergent hydroalkynylation and asymmetric hydroalkynylation with a wide alkyne scope were achieved,producingα-and(enantioenriched)β-branched alkynyl-functionalized amine derivatives from the same raw *** formation of a carbonyl-ligated 5-or 6-membered nickelacycle intermediate via Ni migration or nonmigration was believed to be the key step in controlling the *** asymmetric protocol could be applied to synthesizing other value-added chiral aliphatic amines.

关键词： asymmetric catalysis hydroalkynylation regiodivergent chain-walking nickel catalysis

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Tailoring Iron-Ion Release of Cellulose-Based Aerogel-Coated Iron Foam for Long-Term High-Power Microbial Fuel Cells

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Transactions of Tianjin University 2024年第5期30卷 436-447页

作者： Zhengyang Ni Huitao Yu haoran Wang Mengmeng Qin Feng Li Hao Song Xiangyu Chen Yiyu Feng Wei Feng School of Material Science and Engineering Tianjin UniversityTianjin 300350China School of Chemical Engineering and Technology Tianjin UniversityTianjin 300350China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 100083China

The presence of iron(Fe) has been found to favor power generation in microbial fuel cells(MFCs). To achieve long-term power production in MFCs, it is crucial to effectively tailor the release of Fe ions over extended operating periods. In this study, we developed a composite anode(A/IF) by coating iron foam with cellulose-based aerogel. The concentration of Fe ions in the anode solution of A/IF anode reaches 0.280 μg/mL(Fe^(2+) vs. Fe^(3+) = 61.:39%) after 720 h of aseptic primary cell operation. This value was significantly higher than that(0.1.8 μg/mL, Fe^(2+) vs. Fe^(3+) = 92%:8%) on uncoated iron foam(IF), indicating a continuous release of Fe ions over long-term operation. Notably, the resulting MFCs hybrid cell exhibited a 23% reduction in Fe ion concentration(compared to a 47% reduction for the IF anode) during the sixth testing cycle(600-720 h). It achieved a high-power density of 301.± 55 mW/m^(2) at 720 h, which was 2.62 times higher than that of the IF anode during the same period. Furthermore, a sedimentary microbial fuel cell(SMFCs) was constructed in a marine environment, and the A/IF anode demonstrated a power density of 1.3 ± 3 mW/m^(2) at 3240 h, representing a 75% improvement over the IF anode. These findings elucidate the significant enhancement in long-term power production performance of MFCs achieved through effective tailoring of Fe ions release during operation.

关键词： Microbial fuel cells Coating Fe ions Tailor release Long-term

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Three-dimensional porous In_(2)O_(3) arrays for self-powered transparent solar-blind photodetectors with high responsivity and excellent spectral selectivity

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Nano Research 2024年第5期17卷 4471-4477页

作者： Nana Zhang Xinyu Gao haoran Guan Simin Sun Jiaming Liu Zhitao Shao Qiyue Gao Yuan Zhang Ruyu Sun Guang Yang Feng Gao Wei Feng College of Chemistry Chemical Engineering and Resource UtilizationNortheast Forestry UniversityHarbin 150040China Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Physics and Electronic EngineeringHarbin Normal UniversityHarbin 150025China

Transparent solar-blind ultraviolet photodetectors(SBUV PDs)have extensive applications in versatile scenarios,such as optical ***,it is still challenging to simultaneously achieve high responsivity,high transparency,and satisfying self-powered ***,we demonstrated high-performance,transparent,and self-powered photoelectrochemical-type(PEC)SBUV PDs based on vertically grown ultrathin In_(2)O_(3) nanosheet arrays(NAs)with a three-dimensional(3D)porous *** 3D porous structure simultaneously improves the transmittance in the visible light region,accelerates interfacial reaction kinetics,and promotes photogenerated carrier *** performance of In_(2)O_(3) NAs photoanodes exceeds most reported self-powered PEC SBUV PDs,exhibiting a high transmittance of approximately 80%in the visible light region,a high responsivity of 86.1. mA/W for 254 nm light irradiation,a fast response speed of 1./1. ms,and good multicycle *** In_(2)O_(3) NAs also show excellent spectral selectivity with an ultrahigh solar-blind rejection ratio of 1.1..30,attributed to the quantum confinement effect induced by the ultrathin feature(2-3 nm).Furthermore,In_(2)O_(3) NAs photoanodes show good capability in underwater optical *** work demonstrated that a 3D porous structure is a powerful strategy to synchronously achieve high responsivity and transparency and provides a new perspective for designing high-performance,transparent,and self-powered PEC SBUV PDs.

关键词： In_(2)O_(3) three-dimensional porous transparent photoelectrochemical solar-blind photodetectors

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An Aerial–Wall Robotic Insect That Can Land, Climb, and Take Off from Vertical Surfaces

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Research 2024年第1期2023卷 149-163页

作者： Qian Li Haoze Li Huan Shen Yangguang Yu haoran He Xincheng Feng Yi Sun Zhiyuan Mao Guangming Chen Zongjun Tian Lida Shen Xiangming Zheng Aihong Ji College of Mechanical and Electrical Engineering Nanjing University of Aeronautics and AstronauticsNanjingChina College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsNanjingChina State Key Laboratory of Mechanics and Control for Aerospace Structures Nanjing University of Aeronautics and AstronauticsNanjingChina

Insects that can perform flapping-wing flight,climb on a wall,and switch smoothly between the 2 locomotion regimes provide us with excellent biomimetic ***,very few biomimetic robots can perform complex locomotion tasks that combine the 2 abilities of climbing and ***,we describe an aerial–wall amphibious robot that is self-contained for flying and climbing,and that can seamlessly move between the air and *** adopts a flapping/rotor hybrid power layout,which realizes not only efficient and controllable flight in the air but also attachment to,and climbing on,the vertical wall through a synergistic combination of the aerodynamic negative pressure adsorption of the rotor power and a climbing mechanism with bionic adhesion *** the basis of the attachment mechanism of insect foot pads,the prepared biomimetic adhesive materials of the robot can be applied to various types of wall surfaces to achieve stable *** longitudinal axis layout design of the rotor dynamics and control strategy realize a unique cross-domain movement during the flying–climbing transition,which has important implications in understanding the takeoff and landing of ***,it enables the robot to cross the air–wall boundary in 0.4 s(landing),and cross the wall–air boundary in 0.7 s(taking off).The aerial–wall amphibious robot expands the working space of traditional flying and climbing robots,which can pave the way for future robots that can perform autonomous visual monitoring,human search and rescue,and tracking tasks in complex air–wall environments.

关键词： robot smoothly Vertical

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The transition from 2G to 3G-feedstocks enabled efﬁcient production of fuelsand chemicals

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Green Energy & Environment 2024年第11期9卷 1759-1770页

作者： Kai Wang Changsheng Su haoran Bi Changwei Zhang Di Cai Yanhui Liu Meng Wang Biqiang Chen Jens Nielsen Zihe Liu Tianwei Tan College of Life Science and Technology Beijing University of Chemical TechnologyBeijing Advanced Innovation Center for Soft Matter Science and EngineeringNo.15 North 3rd Ring Rd EastBeijing100029China National Energy R&D Center for Biorefnery Beijing Key Lab of BioprocessBeijing University of Chemical TechnologyNo.15 North 3rd Ring Rd EastBeijing100029China Department of Life Sciences Chalmers University of TechnologyGothenburgSE41296Sweden

For decades micoorganisms have been engineered for the utilization of lignocellulose-based second-generation (2G) feedstocks, but with theconcerns of increased levels of atmospheric CO_(2) causing global warming there is an emergent need to transition from the utilization of 2Gfeedstocks to third-generation (3G) feedstocks such as CO_(2) and its derivatives. Here, we established a yeast platform that is capable ofsimultaneously converting 2G and 3G feedstocks into bulk and value-added chemicals. We demonstrated that by adopting 3G substrates such asCO_(2) and formate, the conversion of 2G feedstocks could be substantially improved. Speciﬁcally, formate could provide reducing power andenergy for xylose conversion into valuable chemicals. Simultaneously, it can form a concentrated CO_(2) pool inside the cell, providing thermodynamically and kinetically favoured amounts of precursors for CO_(2) ﬁxation pathways, e.g., the Calvin–Benson–Bassham (CBB) ***, we demonstrated that formate could directly be utilized as a carbon source by yeast to synthesize endogenous amino acids. Theengineered strain achieved a one-carbon (C1. assimilation efﬁciency of 9.2%, which was the highest efﬁciency observed in the co-utilization of2G and 3G feedstocks. We applied this strategy for productions of both bulk and value-added chemicals, including ethanol, free fatty acids(FFAs), and longifolene, resulting in yield enhancements of 1..4%, 49.0%, and ~1.0%, respectively. The strategy demonstrated here for coutilization of 2G and 3G feedstocks sheds lights on both basic and applied research for the up-coming establishment of 3G bioreﬁneries.

关键词： transition utilized Benson

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Identification of Highly Repetitive Enhancers with Long-range Regulation Potential in Barley via STARR-seq

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Genomics, Proteomics & Bioinformatics 2024年第2期22卷 107-120页

作者： Wanlin Zhou haoran Shi Zhiqiang Wang Yuxin Huang Lin Ni Xudong Chen Yan Liu Haojie Li Caixia Li Yaxi Liu State Key Laboratory of Crop Gene Exploration and Utilization in Southwest China Sichuan Agricultural UniversityChengdu 611130China Triticeae Research Institute Sichuan Agricultural UniversityChengdu 611130China Chengdu Academy of Agricultural and Forestry Sciences Chengdu 611130China

Enhancers are DNA sequences that can strengthen transcription ***,the global identification of plant enhancers is complicated due to uncertainty in the distance and orientation of enhancers,especially in species with large *** this study,we performed self-transcribing active regulatory region sequencing(STARR-seq)for the first time to identify enhancers across the barley genome.A total of 7323 enhancers were successfully identified,and among 45 randomly selected enhancers,over 75%were effective as validated by a dual-luciferase reporter assay system in the lower epidermis of tobacco ***,up to 53.5%of the barley enhancers were repetitive sequences,especially transposable elements(TEs),thus reinforcing the vital role of repetitive enhancers in gene *** the common active mark H3K4me3 and repressive mark H3K27me3 were abundant among the barley STARR-seq *** addition,the functional range of barley STARR-seq enhancers seemed much broader than that of rice or maize and extended to±1.0 kb of the gene body,and this finding was consistent with the high expression levels of genes in the *** study specifically depicts the unique features of barley enhancers and provides available barley enhancers for further utilization.

关键词： Barley Enhancer Transposable element Gene expression Repetitive sequence

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Unlocking the potential of thin-film composite reverse osmosis membrane performance:Insights from mass transfer modeling

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Chinese Chemical Letters 2024年第5期35卷 66-76页

作者： Kexin Yuan Yulei Liu haoran Feng Yi Liu Jun Cheng Beiyang Luo Qinglian Wu Xinyu Zhang Ying Wang Xian Bao Wanqian Guo Jun Ma State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China College of Architecture and Environment Sichuan UniversityChengdu 610065China School of Municipal and Environmental Engineering Shandong Jianzhu UniversityJi’nan 250101China College of Water Conservancy and Hydropower Engineering Sichuan Agricultural UniversityYaan 625014China

Thin-film composite(TFC)reverse osmosis(RO)membranes have attracted considerable attention in water treatment and desalination processes due to their specific separation ***,the trade-off effect between water flux and salt rejection poses huge challenges to further improvement in TFC RO membrane *** research works have been dedicated to optimizing membrane fabrication and modification for addressing this *** the meantime,several reviews summarized these ***,the existing reviews seldom analyzed these methods from a theoretical perspective and thus failed to offer effective optimization directions for the RO process from the root *** this review,we first propose a mass transfer model to facilitate a better understanding of the entire process of how water and solute permeate through RO membranes in detail,namely the migration process outside the membrane,the dissolution process on the membrane surface,and the diffusion process within the ***,the water and salt mass transfer behaviors obtained from model deduction are comprehensively analyzed to provide potential guidelines for alleviating the trade-off effect between water flux and salt rejection in the RO ***,inspired by the theoretical analysis and the accurate identification of existing bottlenecks,several promising strategies for both regulating RO membranes and optimizing operational conditions are proposed to further exploit the potential of RO membrane *** review is expected to guide the development of high-performance RO membranes from a mass transfer theory standpoint.

关键词： Reverse osmosis Mass transfer model Trade-off effect Membrane performance Optimization strategies

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