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Low-temperature chlorination roasting technology for the simultaneous recovery of valuable metals from spent LiCoO_(2)cathode material

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 80-91页

作者： Junjie Shi Changle Hou Jingjing Dong Dong chen Jianzhong Li Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819China School of Metallurgy Northeastern UniversityShenyang 110819China

With the continuous increase in the disposal volume of spent lithium-ion batteries(LIBs),properly recycling spent LIBs has become essential for the advancement of the circular *** study presents a systematic analysis of the chlorination roasting kinetics and proposes a new two-step chlorination roasting process that integrates thermodynamics for the recycling of LIB cathode *** activation energy for the chloride reaction was 88.41 kJ/mol according to thermogravimetric analysis–derivative thermogravimetry data obtained by using model-free,model-fitting,and Z(α)function(αis conversion rate).Results indicated that the reaction was dominated by the first-order(F1)model when the conversion rate was less than or equal to 0.5 and shifted to the second-order(F2)model when the conversion rate exceeded *** conditions were determined by thoroughly investigating the effects of roasting temperature,roasting time,and the mass ratio of nH_(4)Cl to LiCoO_(2).Under the optimal conditions,namely 400℃,20 min,and nH_(4)Cl/LiCoO_(2)mass ratio of 3:1,the leaching efficiency of Li and Co reached 99.43% and 99.05%,*** of the roasted products revealed that valuable metals in LiCoO_(2)transformed into CoCl_(2) and ***,the reaction mechanism was elucidated,providing insights for the establishment of a novel low-temperature chlorination roasting technology based on a crystal structure *** technology can guide the development of LIB recycling processes with low energy consumption,low secondary pollution,high recovery efficiency,and high added value.

关键词： spent lithium-ion battery thermodynamics chlorination roasting kinetics circular economy

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Bioinspired Passive Tactile Sensors Enabled by Reversible Polarization of Conjugated Polymers

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nano-Micro Letters 2025年第1期17卷 361-377页

作者： Feng He Sitong chen Ruili Zhou Hanyu Diao Yangyang Han Xiaodong Wu School of Mechanical Engineering Sichuan UniversityChengdu 610065People’s Republic of China School of Software Engineering Chongqing University of Posts and TelecommunicationsChongqing 400065People’s Republic of China State Key Laboratory of Polymer Materials Engineering Sichuan UniversityChengdu 610065People’s Republic of China

Tactile perception plays a vital role for the human body and is also highly desired for smart prosthesis and advanced *** to active sensing devices,passive piezoelectric and triboelectric tactile sensors consume less power,but lack the capability to resolve static ***,we address this issue by utilizing the unique polarization chemistry of conjugated polymers for the first time and propose a new type of bioinspired,passive,and bio-friendly tactile sensors for resolving both static and dynamic ***,to emulate the polarization process of natural sensory cells,conjugated polymers(including poly(3,4-ethylenedioxythiophen e):poly(styrenesulfonate),polyaniline,or polypyrrole)are controllably polarized into two opposite states to create artificial potential *** controllable and reversible polarization process of the conjugated polymers is fully in situ ***,a micro-structured ionic electrolyte is employed to imitate the natural ion channels and to encode external touch stimulations into the variation in potential difference *** with the currently existing tactile sensing devices,the developed tactile sensors feature distinct characteristics including fully organic composition,high sensitivity(up to 773 mV n^(−1)),ultralow power consumption(nW),as well as superior *** demonstrations,both single point tactile perception(surface texture perception and material property perception)and two-dimensional tactile recognitions(shape or profile perception)with high accuracy are successfully realized using self-defined machine learning *** tactile sensing concept innovation based on the polarization chemistry of conjugated polymers opens up a new path to create robotic tactile sensors and prosthetic electronic skins.

关键词： Passive tactile sensors Reversible polarization of conjugated polymers Tactile perception Machine learning algorithm Object recognition

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Salsolinol as an RnA m~6A methylation inducer mediates dopaminergic neuronal death by regulating YAP1 and autophagy

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neural Regeneration Research 2025年第3期20卷 887-899页

作者： Jianan Wang Yuanyuan Ran Zihan Li Tianyuan Zhao Fangfang Zhang Juan Wang Zongjian Liu Xuechai chen Beijing International Science and Technology Cooperation Base for Antiviral Drugs College of Chemistry and LifeBeijing University of TechnologyBeijingChina Department of Rehabilitation Beijing Rehabilitation HospitalCapital Medical UniversityBeijingChina

Salsolinol(1-methyl-6,7-dihydroxy-1,2,3,4-tetrahydroisoquinoline,Sal)is a catechol isoquinoline that causes neurotoxicity and shares structural similarity with 1-methyl-4-phenyl-1,2,3,6-tetrahydropyridine,an environmental toxin that causes Parkinson's ***,the mechanism by which Sal mediates dopaminergic neuronal death remains *** this study,we found that Sal significantly enhanced the global level of n~6-methyladenosine(m~6A)RnA methylation in PC12 cells,mainly by inducing the downregulation of the expression of m~6A demethylases fat mass and obesity-associated protein(FTO)and alk B homolog 5(ALKBH5).RnA sequencing analysis showed that Sal downregulated the Hippo signaling *** m~6A reader YTH domain-containing family protein 2(YTHDF2)promoted the degradation of m~6A-containing Yes-associated protein 1(YAP1)mRnA,which is a downstream key effector in the Hippo signaling ***,downregulation of YAP1 promoted autophagy,indicating that the mutual regulation between YAP1 and autophagy can lead to *** findings reveal the role of Sal on m~6A RnA methylation and suggest that Sal may act as an RnA methylation inducer mediating dopaminergic neuronal death through YAP1 and *** results provide greater insights into the neurotoxic effects of catechol isoquinolines compared with other studies and may be a reference for assessing the involvement of RnA methylation in the pathogenesis of Parkinson's disease.

关键词： ALKBH5 autophagy FTO Hippo pathway m~6A Parkinson's disease RnA methylation salsolinol YAP1 YTHDF2

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Computed tomography enterography-based radiomics for assessing mucosal healing in patients with small bowel Crohn's disease

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World Journal of Gastroenterology 2025年第3期31卷 62-72页

作者： Hao Ding Yuan-Yuan Fang Wen-Jie Fan chen-Yu Zhang Shao-Fei Wang Jing Hu Wei Han Qiao Mei Department of Gastroenterology The First Affiliated Hospital of Anhui Medical UniversityHefei 230022Anhui ProvinceChina Department of Radiation Oncology The First Affiliated Hospital of Anhui Medical UniversityHefei 230022Anhui ProvinceChina Department of Gastroenterology Suzhou First People's HospitalSuzhou 234099Anhui ProvinceChina

BACKGROUnD Mucosal healing(MH)is the major therapeutic target for Crohn's disease(CD).As the most commonly involved intestinal segment,small bowel(SB)assessment is crucial for CD ***,it poses a significant challenge due to its limited accessibility through conventional endoscopic *** To establish a noninvasive radiomic model based on computed tomography enterography(CTE)for MH assessment in SBCD *** Seventy-three patients diagnosed with SBCD were included and divided into a training cohort(n=55)and a test cohort(n=18).Radiomic features were obtained from CTE images to establish a radiomic *** demographics were analysed to establish a clinical model.A radiomic-clinical nomogram was constructed by combining significant clinical and radiomic *** diagnostic efficacy and clinical benefit were evaluated via receiver operating characteristic(ROC)curve analysis and decision curve analysis(DCA),*** Of the 73 patients enrolled,25 patients achieved *** radiomic-clinical nomogram had an area under the ROC curve of 0.961(95%confidence interval:0.886-1.000)in the training cohort and 0.958(0.877-1.000)in the test cohort and provided superior clinical benefit to either the clinical or radiomic models alone,as demonstrated by *** These results indicate that the CTE-based radiomic-clinical nomogram is a promising imaging biomarker for MH and serves as a potential noninvasive alternative to enteroscopy for MH assessment in SBCD patients.

关键词： Crohn’s disease Computed tomography enterography Mucosal healing nomogram Radiomics

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On MAXWELL EQUATIOnS WITH THE TRAnSPAREnT BOUnDARY COnDITIOn

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Journal of Computational Mathematics 2008年第3期26卷 284-296页

作者： Zhiming chen Jean-Claude nédélec LSEC ICMSEC Academy of Mathematics and Systems Science Chinese Academy of Sciences Beijing 100080 China Centre de Mathématiques Appliquées Ecole Polytechnique 91228 Palaiseau Cedex France

In this paper we show the well-posedness and stability of the Maxwell scattering problem with the transparent boundary condition. The proof depends on the well-posedness of the time-harmonic Maxwell scattering problem... 详细信息

关键词： Electromagnetic scattering Well-posedness Stability

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Comparison between phylogeny of introns and exons in primates

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Chinese Science Bulletin 1999年第21期44卷 1940-1946页

作者： Wang, n chen, RS Chinese Acad Sci Prot Engn Lab Inst Biophys Beijing 100101 Peoples R China

Introns and exons of 7 genes ( epsilon globin, gamma-1 globin, gamma-2 globin, delta globin, beta globin, Immunoglobulin and prepro-insulin) in primates have been separated out and used to infer phylogeny respectively. For each gene, results based on these two parts have been compared and showed that: ( i ) the topology of introns is almost

关键词： phylogeny inference intron substitution rate molecular evolution.

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Surface plasma treatment effects on the molecular structure at polyimide/air and buried polyimide/epoxy interfaces

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Chinese Chemical Letters 2015年第4期26卷 449-454页

作者： John n.Myers Zhan chen Department of Chemistry University of Michigan

Polyimides are widely used as chip passivation layers and organic substrates in microelectronic packaging. Plasma treatment has been used to enhance the interfacial properties of polyimides, but its molecular mechanism is not clear. In this research, the effects of polyimide surface plasma treatment on the molecular structures at corresponding polyimide/air and buried polyimideJepoxy interfaces were investigated in situ using sum frequency generation （SFG） vibrational spectroscopy. SFG results show that the polyimide backbone molecular structure was different at polyimide/air and polyimideJepoxy interfaces before and after plasma treatment. The different molecular structures at each interface indicate that structural reordering of the polyimide backbone occurred as a result of plasma treatment and contact with the epoxy adhesive. Furthermore, quantitative orientation analysis indicated that plasma treatment of polyimide surfaces altered the twist angle of the polyimide backbone at corresponding buried polyimide/epoxy interfaces. These SFG results indicate that plasma treatment of polymer surfaces can alter the molecular structure at corresponding polymer/air and buried polymer interfaces.

关键词： Molecular structureVibrational spectroscopySum frequency generation spectroscopy

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Multi-Model Communication and Data Assimilation for Mitigating Model Error and Improving Forecasts

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Chinese Annals of Mathematics,Series B 2019年第5期40卷 689-720页

作者： Yian chen Samuel n.STECHMAnn Department of Mathematics University of Wisconsin-MadisonMadisonWI 53706USA Department of Statistics University of ChicagoChicagoIL 60637USA Department of Mathematics and Department of Atmospheric and Oceanic Sciences University of Wisconsin-MadisonMadisonWI 53706USA

Models for weather and climate prediction are complex, and each model typically has at least a small number of phenomena that are poorly represented, such as perhaps the Madden-Julian Oscillation(MJO for short) or El nino-Southern Oscillation(EnSO for short) or sea ice. Furthermore, it is often a very challenging task to modify and improve a complex model without creating new deficiencies. On the other hand, it is sometimes possible to design a low-dimensional model for a particular phenomenon, such as the MJO or EnSO, with significant skill, although the model may not represent the dynamics of the full weather-climate system. Here a strategy is proposed to mitigate these model errors by taking advantage of each model’s strengths. The strategy involves inter-model data assimilation, during a forecast simulation, whereby models can exchange information in order to obtain more faithful representations of the full weather-climate system. As an initial investigation, the method is examined here using a simplified scenario of linear models, involving a system of stochastic partial differential equations(SPDEs for short)as an imperfect tropical climate model and stochastic differential equations(SDEs for short) as a low-dimensional model for the MJO. It is shown that the MJO prediction skill of the imperfect climate model can be enhanced to equal the predictive skill of the lowdimensional model. Such an approach could provide a route to improving global model forecasts in a minimally invasive way, with modifications to the prediction system but without modifying the complex global physical model itself.

关键词： MJO Multi-Model communication Data assimilation Kalman filter algorithm

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Atomic-scale roles of Zn element in age-hardened AlMgSiZn alloys

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Journal of Materials Science & Technology 2021年第11期70卷 105-112页

作者： n.n.Jiao Y.X.Lai S.L.chen P.Gao J.H.chen Center for High-Resolution Electron Microscopy College of Materials Science&EngineeringHunan UniversityChangsha410082China Electron Microscopy Laboratory and International Center for Quantum Materials School of PhysicsPeking UniversityBeijing100871China

Adding alloying elements to improve the performances or the manufacturing processes of Al-Mg-Si alloys has long been a serious issue in developing advanced automotive aluminum *** Zn element,among those promising ones,has demonstrated positive alloying effects on Al-Mg-Si ***,the atomic-scale roles of Zn in an age-hardened Al-Mg-Si-Zn alloy have not been adequately *** atomic-resolution electron microscopy,here we report the precise locations of Zn elements in all hardening precipitates involved and their alloying mechanism at the atomic scale when alloying the *** results show that Zn atoms enter all the major hardening phases to occupy specific featured atomic sites of the original elements,*** Si1 and Mg2 sites in theβ’-2 phase,and modify their crystal structures,interfacial structures and morphologies in characteristic *** is revealed that for theβ’-phase,Zn atoms occupy unique atomic sites,whereas for other phases,they demonstrate similar behaviors as other additive alloying elements such as Ag and Cu do.

关键词： Al-Mg-Si alloy Zn addition Precipitate Electron microscopy

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A novel adaptive harmonic balance method with an asymptotic harmonic selection

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Applied Mathematics and Mechanics(English Edition) 2023年第11期44卷 1887-1910页

作者： Rongzhou LIn Lei HOU Yi chen Yuhong JIn n.A.SAEED Yushu chen School of Astronautics Harbin Institute of TechnologyHarbin 150001China Department of Physics and Engineering Mathematics Faculty of Electronic EngineeringMenoufia UniversityMenouf 32952Egypt Department of Automation Biomechanicsand MechatronicsFaculty of Mechanical EngineeringLodz University of TechnologyLodz 90924Poland Mathematics Department Faculty of ScienceGalala UniversityGalala 43511Egypt

The harmonic balance method(HBM)is one of the most widely used methods in solving nonlinear vibration problems,and its accuracy and computational efficiency largely depend on the number of the harmonics *** adaptive harmonic balance(AHB)method is an improved HBM *** paper presents a modified AHB method with the asymptotic harmonic selection(AHS)*** new harmonic selection procedure selects harmonics from the frequency spectra of nonlinear terms instead of estimating the contribution of each harmonic to the whole nonlinear response,by which the additional calculation is avoided.A modified continuation method is proposed to deal with the variable size of nonlinear algebraic equations at different values of path parameters,and then all solution branches of the amplitude-frequency response are *** experiments are carried out to verify the performance of the AHB-AHS *** typical nonlinear dynamic equations with different types of nonlinearities and excitations are chosen as the illustrative *** with the classical HBM and Runge-Kutta methods,the proposed AHB-AHS method is of higher accuracy and better *** AHB-AHS method proposed in this paper has the potential to investigate the nonlinear vibrations of complex high-dimensional nonlinear systems.

关键词： harmonic balance method(HBM) adaptive harmonic balance(AHB)method harmonic selection nonlinear vibration multi-frequency excitation

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