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Low cost and low density chloride solid electrolyte for all solid state cathode with high active material ratio

Nano Research 2024年第10期17卷 8826-8833页

作者： hao-yuan tan Mei-Yu Zhou Zhongyuan Huang Jin-Da Luo Jing-Tian Yang Jian-Ping Wang Ye-Chao Wu Xiao-Bin Cheng Zi-Wei Wang Xu-Dong hao Linjun Wang Ke Gong Yi-Chen Yin Yinguo Xiao Hong-Bin Yao Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China Department of Applied Chemistry University of Science and Technology of ChinaHefei 230026China School of Advanced Materials Peking University Shenzhen Graduate SchoolShenzhen 518055China

Chloride solid electrolytes(SEs)have attracted widespread attention due to their high room-temperature ionic conductivity and excellent cathode ***,the conventionally selected central metal elements(e.g.,In,Y and Ta)are usually rare and heavy,inevitably causing the high cost and high density of the obtained chloride ***,by choosing abundant and light Mg and Al as central metal elements,we develop a cheap and low density Li_(1.2)Mg_(0.95)Al_(0.3)Cl_(4)SE for high active material ratio in all solid state *** replacement of Mg^(2+)by Al^(3+)in the framework yields vacancies and lowers the non-lithium metal ions occupancy at Mg/Li co-occupied 16d site,effectively relieving the blocking effects by Mg^(2+)in the pristine spinel Li_(2-2x)Mg_(1+x)Cl_(4).Thus,a significantly improved room-temperature conductivity of 3.08×10^(-4)S·cm^(-1)is achieved,two orders of magnitude higher than that of Li_(1.2)Mg_(1.4)Cl_(4).More attractively,its low density of only 1.98 g·cm-3 enables low SE mass ratio in cathodes(only 16 wt.%)with still effective electrolyte/cathode contact and lithium-ion conduction *** charged to potential of 4.30 V,the asfabricated Li_(1.2)Mg_(0.95)Al_(0.3)Cl_(4)-based solid lithium battery with uncoated NCM523 cathode can be cycled for over 100 cycles with a capacity retention of 86.68%at room temperature.

关键词： chloride solid electrolytes low cost low density Li+conductivities

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Learnware:small models do big

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Science China(Information Sciences) 2024年第1期67卷 39-50页

作者： Zhi-Hua ZHOU Zhi-hao tan National Key Laboratory for Novel Software Technology Nanjing University

There are complaints about current machine learning techniques such as the requirement of a huge amount of training data and proficient training skills,the difficulty of continual learning,the risk of catastrophic forgetting,and the leaking of data privacy/*** research efforts have been focusing on one of those concerned issues separately,paying less attention to the fact that most issues are entangled in *** prevailing big model paradigm,which has achieved impressive results in natural language processing and computer vision applications,has not yet addressed those issues,whereas becoming a serious source of carbon *** article offers an overview of the learnware paradigm,which attempts to enable users not to need to build machine learning models from scratch,with the hope of reusing small models to do things even beyond their original purposes,where the key ingredient is the specification which enables a trained model to be adequately identified to reuse according to the requirement of future users who know nothing about the model in advance.

关键词： artificial intelligence machine learning learnware

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Dynamic mechanical characteristics of deep Jinping marble in complex stress environments

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第2期16卷 630-644页

作者： Chendi Lou Heping Xie Ru Zhang Hai Ren hao Luo Kun Xiao yuan Peng Qiang tan Li Ren Institute for Disaster Management and Reconstruction Sichuan UniversityChengdu610207China College of Water Resource&Hydropower Sichuan UniversityChengdu610065China MOE Key Laboratory of Deep Earth Science&Engineering Sichuan UniversityChengdu610065China Yalong River Hydropower Development Company Ltd.Chengdu610051China (Chongqing)International Engineering Technology Company Ltd.Chongqing401121China

To reveal the dynamic mechanical characteristics of deep rocks,a series of impact tests under triaxial static stress states corresponding to depths of 300-2400 m were *** results showed that both the strain rates and the stress environments in depth significantly affect the mechanical characteristics of *** sensitivity of strain rate to the dynamic strength and deformation modulus shows a negative correlation with depth,indicating that producing penetrative cracks in deep environments is more difficult when damage *** dynamic strength shows a tendency to decrease and then increase slightly,but decreases sharply *** demonstrates a similar trend as that of strength,whereas reflectivity indicates the opposite ***,two critical depths with high dynamically induced hazard possibilities based on the China Jinping Underground Laboratory(CJPL)were proposed for deep *** first critical depth is 600-900 m,beyond which the sensitivity of rock dynamic characteristics to the strain rate and restraint of circumferential stress decrease,causing instability of surrounding rocks under axial stress *** second one lies at 1500-1800 m,where the wave impedance and dynamic strength of deep surrounding rocks drop sharply,and the dissipation energy presents a negative *** suggests that the dynamic instability of deep surrounding rocks can be divided into dynamic load dominant and dynamic load induced types,depending on the second critical depth.

关键词： Rock mechanics Split-Hopkinson pressure bar Coupled static‒dynamic loading Different depths Holmquist-Johnson-Cook(HJC)model

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Highly coupled off-resonance lattice design in diffraction-limited light sources

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NUCLEAR SCIENCE AND TECHNIQUES 2024年第9期35卷 1-11页

作者： Gong, Yi-hao Tian, Shun-Qiang Liu, Xin-Zhong Xuan, Shou-Zhi tan, Li-yuan Mao, Ling-Long Chinese Acad Sci Shanghai Shanghai Adv Res Inst Shanghai Synchrotron Radiat Facil Shanghai 201204 Peoples R China Chinese Acad Sci Shanghai Shanghai Inst Appl Phys Shanghai 201800 Peoples R China Univ Chinese Acad Sci Beijing 100049 Peoples R China

The round-beam operation presents many benefits for scientific experiments regarding synchrotron radiation and the weakening influences of intra-beam scattering in diffraction-limited synchrotron light sources. A round-beam generation method based on the global setting of skew quadrupoles and the application of a non-dominated sorting genetic algorithm was proposed in this study. Two schemes, including large-emittance coupling introduced via betatron coupling and vertical dispersion, were explored in a candidate lattice for an upgrade-proposal of the Shanghai synchrotron radiation facility. Emittance variations with lattice imperfections and their influence on the beam dynamics of beam optic distortions were investigated. The results demonstrated that a precise coupling control ranging from 10 to 100% was achieved under low optical distortion, whereas full-coupling generation and its robustness were achieved by our proposed method by adjusting the skew quadrupole components located in the dispersion-free sections. The Touschek lifetime increased by a factor of 2-2.5.

关键词： Diffraction-limited storage ring (DLSR) Shanghai synchrotron radiation facility upgrade (SSRF-U) Round beam Off-resonance coupling EMITtanCE OPTICS

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Recent advancements in thermal conductivity of magnesium alloys

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Journal of Magnesium and Alloys 2024年第5期12卷 1687-1708页

作者： hao Lv Jun tan Qian yuan Fanglei Wang Yunxuan Zhou Quan Dong Aitao tang Jürgen Eckert Bin Jiang Fusheng Pan National Engineering Research Center for Magnesium Alloys College of Materials Science and EngineeringChongqing UniversityChongqing 400044China National Key Laboratory of Advanced Casting Technologies Chongqing UniversityChongqing 400044China Department of Materials Science Chair of Materials PhysicsMontanuniversität LeobenJahnstraße 12Leoben A-8700Austria Erich Schmid Institute of Materials Science Austrian Academy of SciencesJahnstraße 12Leoben A-8700Austria

As highly integrated circuits continue to advance,accompanied by a growing demand for energy efficiency and weight reduction,materials are confronted with mounting challenges pertaining to thermal conductivity and lightweight *** virtue of numerous intrinsic mechanisms,as a result,the thermal conductivity and mechanical properties of the Mg alloys are often inversely related,which becomes a bottleneck limiting the application of Mg *** on several effective modification methods to improve the thermal conductivity of Mg alloys,this paper describes the law of how they affect the mechanical properties,and clearly indicates that peak aging treatment is one of the best ways to simultaneously enhance an alloy's thermal conductivity and mechanical *** the most frequently used Mg alloy,cast alloys exhibit substantial potential for achieving high thermal ***,recent reports indicate that hot deformation can significantly improve the mechanical properties while maintaining,and potentially slightly enhancing,the alloy's thermal *** presents a meaningful way to develop Mg alloys for applications in the field of small-volume heat dissipation components that require high *** comprehensive review begins by outlining standard testing and prediction methods,followed by the theoretical models used to predict thermal conductivity,and then explores the primary influencing factors affecting thermal *** review summarizes the current development status of Mg alloys,focusing on the quest for alloys that offer both high thermal conductivity and high *** concludes by providing insights into forthcoming prospects and challenges within this field.

关键词： Mg alloy Thermal conductivity Mechanical properties Solute atom Second phase

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Numerical investigation of the photo-thermal characteristics of a direct absorption solar collector using Monte Carlo and finite volume methods

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Science China(Technological Sciences) 2024年第8期67卷 2436-2448页

作者： ZHU YanLong LI SuNing FAN JianHua KONG WeiQiang yuan yuan tan HePing School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China Department of Civil Engineering and Mechanical Engineering Technical University of DenmarkKoppels AlléBuilding 4042800 Kgs.LyngbyDenmark School of Vehicle and Energy Yanshan UniversityQinhuangdao 066004China

In this study, a novel model of photothermal conversion in a direct absorption solar collector based on the Monte Carlo and finite volume methods was built and validated and the temperatures of the novel and traditional solar collectors were compared. The sensitivity of the parameters to the radiative heat loss was investigated. Finally, the radiative heat transfer characteristics were discussed using the radiative exchange factor. The results of this study validated the advantages of the novel solar collector at both the surface and fluid temperatures. Under the conditions used in this study, the maximum temperature difference of the novel solar collector was 30 K, compared with 193 K for the traditional solar collector. Furthermore, the collector was divided into several units along the flow direction. The radiative exchange factor indicated that with an increase in the attenuation coefficient, the percentage of radiation intensity in the total solar radiation absorbed by the corresponding unit ***, it decreased with an increase in the incident angle and scattering albedo. These results provide a reference for addressing the low efficiency and thermal damage caused by traditional solar collectors at high temperatures.

关键词： direct absorption solar collector radiative heat transfer Monte Carlo

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FL-EASGD:Federated Learning Privacy Security Method Based on Homomorphic Encryption

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Computers, Materials & Continua 2024年第5期79卷 2361-2373页

作者： hao Sun Xiubo Chen Kaiguo yuan Information Security Center State Key Laboratory ofNetworking and Switching TechnologyBeijing University of Posts and TelecommunicationsBeijing100876China

Federated learning ensures data privacy and security by sharing models among multiple computing nodes instead of plaintext ***,there is still a potential risk of privacy leakage,for example,attackers can obtain the original data through model inference ***,safeguarding the privacy of model parameters becomes *** proposed solution involves incorporating homomorphic encryption algorithms into the federated learning ***,the existing federated learning privacy protection scheme based on homomorphic encryption will greatly reduce the efficiency and robustness when there are performance differences between parties or abnormal *** solve the above problems,this paper proposes a privacy protection scheme named Federated Learning-Elastic Averaging Stochastic Gradient Descent(FL-EASGD)based on a fully homomorphic encryption ***,this paper introduces the homomorphic encryption algorithm into the FL-EASGD scheme to preventmodel plaintext leakage and realize privacy security in the process ofmodel ***,this paper designs a robust model aggregation algorithm by adding time variables and constraint coefficients,which ensures the accuracy of model prediction while solving performance differences such as computation speed and node anomalies such as downtime of each *** addition,the scheme in this paper preserves the independent exploration of the local model by the nodes of each party,making the model more applicable to the local data ***,experimental analysis shows that when there are abnormalities in the participants,the efficiency and accuracy of the whole protocol are not significantly affected.

关键词： Federated learning homomorphic encryption privacy security stochastic gradient descent

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Surface roughness classification using light scattering matrix and deep learning

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Science China(Technological Sciences) 2024年第2期67卷 520-535页

作者： SUN hao tan Wei RUAN YiXiao BAI Long XU JianFeng State Key Laboratory of Intelligent Manufacturing Equipment and Technology School of Mechanical Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Wuhan Digital Design and Manufacturing Innovation Center Co. LtdWuhan 430074China

High-quality optical components have been widely used in various applications;thus,extremely high beam quality is ***,surface roughness is a key indicator of the surface *** this study,the angular distribution of light scattering field intensity was obtained for surfaces having different roughness profiles based on the finite difference time domain(FDTD)method,and the results were compared with those obtained using the generalized Harvey-Shack(GHS)*** was shown that the FDTD approach can be used for an accurate simulation of the scattered field of a rough surface,and the superposition of results obtained from many surfaces that have the same roughness level was in good agreement with the result given by the analytic GHS model.A light scattering matrix(LSM)method was proposed based on the FDTD simulation results that could obtain rich surface roughness *** classification effect of LSM was compared with that of the single-incidence scattering distribution(SISD)based on a ResNet-50 deep learning *** classification accuracy of the model trained with the LSM dataset was obtained as 95.74%,which was 23.40%higher than that trained using the SISD ***,the effects of different noise types and filtering methods on the classification performance were analyzed,and the LSM was also shown to improve the robustness and generalizability of the trained surface roughness ***,the proposed LSM method has important implications for improving the data acquisition scheme of current light scattering measurement systems,and it also has the potential to be used for detection and characterization of surface defects of optical components.

关键词： surface roughness FDTD simulation GHS theory deep learning light scattering matrix

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Structural engineering of hard carbon through spark plasma sintering for enhanced sodium-ion storage

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Rare Metals 2024年第9期43卷 4274-4285页

作者： hao-Ming Xiao Heng Zheng Ping yuan Jun-Hui Luo Lin-Lin Shen Jie-Feng tan Xian-You Luo De Li Yong Chen Guangdong Key Laboratory for Hydrogen Energy Technologies School of Materials Science and Hydrogen EnergyFoshan University State Key Laboratory of Marine Resource Utilization in South China Sea Hainan Provincial Key Laboratory of Research on Utilization of Si-Zr-Ti ResourcesHainan University

Hard carbon （HC） has emerged as one of the superior anode materials for sodium-ion batteries （SIBs）,with its electrochemical performance significantly influenced by the presence of oxygen functional groups and its closed pore ***,current research on the structural adjustment of these oxygen functional groups and the closed pore architecture within HC remains ***,energy-efficient and contamination-free spark plasma sintering technology was employed to tune the structure of coconut-shell HC,resulting in significant adjustments to the content of carboxyl （decreasing from 5.71 at%to 2.12 at%） and hydroxyl groups （decreasing from 7.73 at % to 6.26 at%）.Crucially,these modifications reduced the irreversible reaction of oxygen functional groups with Na+.Simultaneously,a substantial number of closed pores with an average diameter of 1.22 nm were generated within the HC,offering an ideal environment for efficient Na+*** structural changes resulted in a remarkable improvement in the electrochemical performance of the modified *** reversible specific capacity of the modified HC surged from 73.89 mAh·g-1to an impressive 251.97 m Ah·g-1at a current density of 50 mA·*** at 400 mA·g-1,the reversible specific capacity increased significantly from 14.55 to 85.44 mAh·***,this study provides a novel perspective for designing tailored HC materials with the potential to develop high-performance SIBs.

关键词： Closed pores Hard carbon Oxygen functional groups Sodium-ion batteries Spark plasma sintering

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Analytical solution for the effective elastic properties of rocks with the tilted penny-shaped cracks in the transversely isotropic background

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Petroleum Science 2024年第1期21卷 221-243页

作者： Zheng-Qian Ma Xing-Yao Yin Zhao-Yun Zong yuan-yuan tan Ya-Ming Yang National Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)Qingdao266580ShandongChina School of Geosciences China University of Petroleum(East China)Qingdao 266580ShandongChina Pilot National Laboratory for Marine Science and Technology(Qingdao) Qingdao266200ShandongChina

Seismic prediction of cracks is of great significance in many disciplines,for which the rock physics model is ***,up to now,multitudinous analytical models focus primarily on the cracked rock with the isotropic background,while the explicit model for the cracked rock with the anisotropic background is rarely investigated in spite of such case being often encountered in the ***,we first studied dependences of the crack opening displacement tensors on the crack dip angle in the coordinate systems formed by symmetry planes of the crack and the background anisotropy,respectively,by forty groups of numerical *** on the conclusion from the experiments,the analytical solution was derived for the effective elastic properties of the rock with the inclined penny-shaped cracks in the transversely isotropic ***,we comprehensively analyzed,according to the developed model,effects of the crack dip angle,background anisotropy,filling fluid and crack density on the effective elastic properties of the cracked *** analysis results indicate that the dip angle and background anisotropy can significantly either enhance or weaken the anisotropy degrees of the P-and SH-wave velocities,whereas they have relatively small effects on the SV-wave velocity ***,the filling fluid can increase the stiffness coefficients related to the compressional modulus by reducing crack compliance parameters,while its effects on shear coefficients depend on the crack dip *** increasing crack density reduces velocities of the dry rock,and decreasing rates of the velocities are affected by the crack dip *** comparing with exact numerical results and experimental data,it was demonstrated that the proposed model can achieve high-precision estimations of stiffness ***,the assumption of the weakly anisotropic background results in the consistency between the proposed model and Hudson's published theory for the or

关键词： Effective elastic property Tilted crack Transverse isotropy Analytical solution Crack opening displacement

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