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Noncovalent cross-linked engineering hydrogel with low hysteresis and high sensitivity for flexible self-powered electronics

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Journal of Energy Chemistry 2024年第7期94卷 136-147页

作者： Hang Yuan Shaowei Han Jia Wei Songwei Li Peipei yang hao-yang mi Chuntai Liu Changyu Shen National Engineering Research Center for Advanced Polymer Processing Technology Key Laboratory of Materials Processing and Mold(Ministry of Education)Zhengzhou UniversityZhengzhou450002HenanChina Yunnan TobaccoQuality Inspection&Supervision Station Kunming 650106YunnanChina

In this study,the hydrogel network was reinforced by covalent-like hydrogen bonding,and the strong binding ability of boron-nitrogen coordination served as the main driving *** them,acrylamide(AM)and 3-acrylamidophenylboronic acid(AAPBA)were the main body,and the numerous hydroxyl groups in the trehalose(Treh)molecule and other polymer groups formed strong hydrogen bonding interactions to improve the mechanical properties of the PAM/PAAPBA/Treh(PAAT)hydrogel and ensured the simplicity of the synthesis *** hydrogel possessed high strain at break(1239%),stress(64.7 kPa),low hysteresis(100%to 500%strain,corresponding to dissipation energy from 1.37 to 7.80 kJ/m^(3)),and outstanding cycling stability(retained more than 90%of maximum stress after 200 ten-sile cycles).By integrating carbon nanotubes(CNTs)into PAAT hydrogel(PAATC),the PAATC hydrogel with excellent strain response performance was successfully *** PAATC conductive hydro-gel exhibited high sensitivity(gauge factor(GF)=10.58 and sensitivity(S)=0.304 kPa^(-1)),wide strain response range(0.5%-1000%),fast response time(450 ms),and short recovery time(350 ms),excellent fatigue resistance,and strain response ***,the PAATC-based triboelectric nanogener-ator(TENG)displayed outstanding energy harvesting performance,which shows its potential for appli-cation in self-powered electronic devices.

关键词： Low hysteresis Covalent-like hydrogen bonding Boron-nitrogen coordination Hydrogel sensor Triboelectric nanogenerator

Improved oxygen electrocatalysis at Fe N4 and Co N4 sites via construction of axial coordination

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Chinese Chemical Letters 2025年第2期36卷 482-487页

作者： Ze Zhang Lei yang Jin-Ru Liu hao Hu Jian-Li mi Chao Su Bei-Bei Xiao Zhi-min Ao School of Energy and Power Engineering Jiangsu University of Science and Technology Institute for Computation in Molecular and Materials Science School of Chemistry and Chemical Engineering Nanjing University of Science and Technology Institute for Advanced Materials School of Materials Science and Engineering Jiangsu University Advanced Interdisciplinary Institute of Environment and Ecology Beijing Normal University

The quest for efficient and durable catalysts using abundant resources has garnered significant interest in the field of bifunctional oxygen *** this contribution,we have designed a FeN4or CoN4embedded graphene-based bilayer as active layer and TMC3or TMN3doped graphene as supporting layer,named as FeN4/TMC3or FeN4/TMN3and CoN4/TMC3or CoN4/TMN3,wherein TM strands for transition *** on density functional theory calculations,our results demonstrate that the interaction formed between dual metal atoms in the bilayer interspace leads to the coordination environment altered from flat four-coordination to spatial five-coordination,further stabilizing the bilayer structure and impairing its affinity toward the O-containing *** to thermodynamic analysis,the bilayers of CoN4/CoN3,FeN4/FeC3,FeN4/CoC3,FeN4/NiC3,FeN4/ZnC3,FeN4/FeN3,FeN4/CrN3and FeN4/ZnN3are attractively promising for bifunctional oxygen electrocatalysis due to the small overpotential differenceΔη between oxygen reduction and oxygen evolution that are less than 1 *** functional theory calculations combined with machine learning analysis directly identify the key role played by the interbinding formed between bilayers,that boosts catalytic activity,which establishes a predictable framework for a fast screen for graphene-based bilayer vertical *** work opens up a new path for designing the efficient electrocatalysts via modification of coordination environment.

关键词： Density functional theory Machine learning Oxygen electrocatalysis Thermodynamic analysis

超临界二氧化碳流场作用下线型聚乙烯剪切塑化行为的分子动力学模拟研究

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高分子学报 2024年第10期55卷 1414-1429页

作者：崔文豪顾瑞星米皓阳郑州大学橡塑模具国家工程研究中心郑州450000

通过非平衡分子动力学模拟探讨了聚乙烯(PE)及其与超临界二氧化碳(scCO_(2))共混体系在剪切流下的热力学和构象性质.发现scCO_(2)的增塑作用可显著改变PE的热力学和构象性质,如降低分子间作用力、减少体系剪切应力、降低体系黏度、减少... 详细信息

通过非平衡分子动力学模拟探讨了聚乙烯(PE)及其与超临界二氧化碳(scCO_(2))共混体系在剪切流下的热力学和构象性质.发现scCO_(2)的增塑作用可显著改变PE的热力学和构象性质,如降低分子间作用力、减少体系剪切应力、降低体系黏度、减少分子链构象参数、提高PE链gauche plus构象,从而增加分子链的卷曲和自由体积,减少剪切下的分子取向排列.scCO_(2)还显著降低了体系的弛豫时间,加强了PE分子链抵抗剪切的能力,从而增强了动态性质和热稳定性.这些发现为scCO_(2)在PE体系中的作用提供了微观见解,为调控scCO_(2)辅助聚合物加工工艺,开发高性能聚合物材料提供了理论依据.

关键词：线型聚合物超临界二氧化碳非平衡分子动力学剪切取向剪切流增塑作用

A review of GaN RF devices and power amplifiers for 5G communication applications

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Fundamental Research 2025年第1期5卷 315-331页

作者： Lu, hao Zhang, Meng yang, Ling Hou, Bin Martinez, Rafael Perez mi, minhan Du, Jiale Deng, Longge Wu, Mei Chowdhury, Srabanti Ma, Xiaohua hao, Yue School of microelectronics Xidian University Xi'an 710071 China Department of Electrical Engineering Stanford University Stanford 94305 CA United States

In the emerging 5G and beyond 5G (B5G) era, the spotlight is sharply focused on the power amplifier, a critical component with stringent specification requirements that dictates the performance of the transmitter. The gallium nitride (GaN) device, with its superior inherent properties, is surfacing as a front-runner for power amplifier applications. The increasing demand for high frequency, high linearity, and cost-effective GaN power amplifiers is driven by anticipated traffic surges and the need for extensive 5G deployment. This paper offers a thorough review and future perspective on research developments in RF GaN device technology. It encompasses critical issues in advanced device and circuit technology, with a focus on high frequency, high linearity, cost-effective GaN-on-Si high electron mobility transistors (HEMTs), and compact modeling. This work aims to serve as a guide for the utilization of GaN HEMTs in 5G communication applications. © 2023

关键词： 5G Gallium nitride GaN-on-Si HEMTs High frequency High linearity

The role of sub-continental lithosphere mantle in deep F and Cl cycling:Insight from the Dabeigou basalts,North China Craton

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Science China Earth Sciences 2025年第2期68卷 564-580页

作者： Yadong WU Jinhui yang Jinfeng SUN hao WANG Baoquan ZHOU State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Computational Geodynamics University of Chinese Academy of SciencesBeijing 100049China

The sub-continental lithosphere mantle(SCLM)represents a mechanical barrier that separate the convecting mantle from the exosphere,and possesses the ability to sequester and release volatiles,making it an integral part in deep volatile *** we explore the SCLM in modulating F and Cl cycling through a case study from the Early Cretaceous Dabeigou basalts in the North China Craton(NCC).These lavas are associated with decratonization of the NCC,a process involving significant removal and replacement of the ancient *** Dabeigou basalts,characterized by arc magma-like trace element signatures,evolved initial^(87)Sr/^(86)Sr(0.70574–0.70578),ε_(Nd)(t)(-11.2–-11.1),andε_(Hf)(t)(-13.7–-13.4)values,along with high Fe/Mn ratios,Ni contents,andδ^(18)O values(5.8‰–6.8‰)of olivine phenocrysts,are compatible with their origination from a veined,pyroxene-rich source formed through the infiltration and interaction of hydrous silicate melts from the subducting Pacific slabs with ambient ***-hosted melt inclusions of the Dabeigou basalts have compositions similar to the whole rocks,indicating that they record pre-eruptive melt compositions forming the whole *** melt inclusions exhibit high F(1371–2316 ppm)and moderate Cl(688–900 ppm)contents,with high F/Cl ratios of 2.1±0.3(1σ).The F and Cl signatures of the Dabeigou basalts are different from those of typical arc magmas,which are commonly characterized by high Cl contents(median of~1200 ppm)and low F/Cl ratios(mineral phase for fractionating and preserving F and *** is,amphibole crystallization prefers to retain F rather than Cl,making the metasomes in vein enriched in F and exhibiting elevated F/Cl ratios compared to original metasomatic *** is further suggested that the scenario inferred from the Dabeigou basalts mi

关键词： North China Craton Sub-continental lithosphere mantle Early Cretaceous Dabeigou basalts Melt inclusion F and Cl cycling

Fabric-based all-weather-available photo-electro-thermal steam generator with high evaporation rate and salt resistance

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Science China Materials 2022年第9期65卷 2479-2490页

作者： Shuangjie Sun Qingli Tian hao-yang mi Jun Li Xin Jing Zhanhu Guo Chuntai Liu Changyu Shen National Engineering Research Center for Advanced Polymer Processing Technology The Key Laboratory of Advanced Materials Processing&Mold of Ministry of EducationZhengzhou UniversityZhengzhou 450001China Integrated Composites Laboratory(ICL) Department of Chemical&Biomolecular EngineeringUniversity of TennesseeKnoxville 37996USA Key Laboratory of Advanced Packaging Materials and Technology of Hunan Province Hunan University of TechnologyZhuzhou 412007China

Solar-driven steam generation is a practical strategy to harness solar energy for desalination and production of clean water with a minimized carbon ***,this strategy suffers from a low evaporation rate under weak illumination on cloudy days or at ***,we present a fabric-based all-weather-available photo-electrothermal steam generator(P/ET-SG)capable of regulating the surface temperature and evaporation rate by the coupling effect of photo-thermal and electro-thermal heating depending on the light *** unprecedented high surface temperature of 52℃ in the wet state and an evaporation rate of 2.61 kg m^(-2) h^(-1) were achieved by the P/ET-SG under 1 sun with only 1 V input voltage owing to the uniform heat distribution and the coupled electro-thermal *** oneway fluidic design of the P/ET-SG effectively prevented salt precipitation during continuous desalination in 24 h and was able to remove salt granules from the evaporation ***,the P/ET-SG demonstrated a high evaporation rate of 2.58 kg m^(-2) h^(-1) in the purification of concentrated saline water and dye-contaminated water with high efficiency(>99.9%).This study offers new thoughts for the design of allweather-available solar steam generators with high efficiency and makes a step forward towards fast purification of concentrated saline water and wastewater.

关键词： solar steam generation photo-electro-thermal effect salt resistance desalination fabric

Non-stationarity Characteristics in Dynamic Vehicular ISAC Channels at 28 GHz

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Chinese Journal of Electronics 2025年第1期34卷 73-81页

作者： Zhengyu Zhang Ruisi He mi yang Xuejian Zhang Ziyi Qi Hang mi Guiqi Sun Jingya yang Bo Ai School of Electronic and Information Engineering Beijing Jiaotong University Henan High-Speed Railway Operation and Maintenance Engineering Research Center

Integrated sensing and communications(ISAC) is a potential technology of 6G, aiming to enable end-to-end information processing ability and native perception capability for future communication systems. As an important part of the ISAC application scenarios, ISAC aided vehicle-to-everything(V2X) can improve the traffic efficiency and safety through intercommunication and synchronous perception. It is necessary to carry out measurement,characterization, and modeling for vehicular ISAC channels as the basic theoretical support for system design. In this paper, dynamic vehicular ISAC channel measurements at 28 GHz are carried out and provide data for the characterization of non-stationarity characteristics. Based on the actual measurements, this paper analyzes the time-varying PDPs, RMSDS and non-stationarity characteristics of front, lower front, left and right perception directions in a complicated V2X scenarios. The research in this paper can enrich the investigation of vehicular ISAC channels and enable the analysis and design of vehicular ISAC systems.

关键词： Performance evaluation 6G mobile communication Information processing Integrated sensing and communication Safety Vehicle dynamics Vehicle-to-everything System analysis and design

Genome-wide CRISPR screens identify CLC-2 as a drug target for anti-herpesvirus therapy:tackling herpesvirus drug resistance

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Science China(Life Sciences) 2025年第2期68卷 515-526页

作者： Fayu yang Nan Wei Shuo Cai Jing Liu Qingping Lan hao Zhang Lu Shang Bo Zheng mi Wang Yingchun Liu Lifang Zhang Chenzhong Fei Wu Tong Changlong Liu Ersheng Kuang Guangzhi Tong Feng Gu Shanghai Veterinary Research Institute Chinese Academy of Agricultural SciencesShanghai 200241China Key Laboratory of Veterinary Chemical Drugs and Pharmaceutics Ministry of Agriculture and Rural AffairsShanghai 200241China State Key Laboratory for Animal Disease Control and Prevention College of Veterinary MedicineLanzhou UniversityLanzhou Veterinary Research InstituteChinese Academy of Agricultural SciencesLanzhou 730000China Institute of Human Virology Zhongshan School of MedicineSun Yat-Sen UniversityGuangzhou 510080China School of Medicine Tsinghua UniversityBeijing 100084China

The emergence of drug resistance to virus(i.e.,acyclovir(ACV)to herpesviruses)has been termed one of the common clinical issues,emphasizing the discovery of new antiviral *** address it,a genome-wide clustered regularly interspaced short palindromic repeats(CRISPR)screening was performed in mouse haploid embryonic stem cells infected with pseudorabies virus(PRV),anα-herpesvirus causing human and pig *** results demonstrated that type 2 voltage-gated chloride channels(CLC-2)encoded by one of the identified genes,CLCN2,is a potential drug target for anti-herpesvirus ***-2 inhibitors,omeprazole(OME)and 4,4'-diisothiocyanostilbene-2,2'-disulfonic acid(DIDS),can efficiently inhibit infection of multiple herpesviruses in cellulo(i.e.,PRV,HSV and EBV),and effectively treat murine herpes simplex encephalitis(HSE).Additionally,DIDS was found to inhibit HSV-1 replication by blocking the PI3K/Akt *** importantly,both DIDS and OME were able to inhibit ACV-resistant HSV-1 strain *** study's findings suggest that targeting host-cell factors such as CLC-2 may be a promising approach to tackling herpesvirus drug *** discovery of CLC-2 as a potential drug target for anti-herpesvirus therapy provides a new direction for the development of novel antiviral agents.

关键词： herpesviruses CRISPR host-directed therapy CLC-2 DIDS

Spatial and Temporal Distribution of Metal Elements in the Rivers of Northern Jiangsu Province

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Journal of Ocean University of China 2025年第1期24卷 157-168页

作者： YUAN Liping LIU Qian JIAN Huimin mi Tiezhu yang Fuxia YAO Qingzhen Frontiers Science Center for Deep Ocean Multispheres and Earth System and Key Laboratory of Marine Chemistry Theory and TechnologyMinistry of EducationOcean University of ChinaQingdao 266100China Laboratory of Marine Ecology and Environmental Science Qingdao National Laboratory for Marine Science and TechnologyQingdao 266071China College of Environmental Science and Engineering Ocean University of ChinaQingdao 266100China Key Laboratory of Land and Sea Ecological Governance and Systematic Regulation of the ministry of Ecology and Environment Shandong Academy for Environmental PlanningJinan 250101China

The concentrations of V,Cr,Mn,Fe,Co,Ni,Cu,Zn,As,Mo,Cd,and Pb were determined in Doulonggang River,Xinyanggang River,Huangshagang River,Sheyanghe River,Guangaizongqu River,and Linhonghe River at the North of Jiangsu Province in *** annual average concentrations of V,Cr,Mn,Fe,Co,Ni,Cu,Zn,As,Mo,Cd and Pb in the six rivers were 2.20,1.22,4.53,21.9,0.13,2.79,1.77,4.00,2.97,3.87,0.01,0.19μg L^(-1)*** highest concentration of most trace metals were found in Guangaizongqu River and Linhonghe River,and the lowest concentration were found in Xinyanggang River and Huangshagang *** principal component analysis(PCA)resulted of two factors together explained 91.2%of the variance with>1initial eigenvalue,indicating that both natural and anthropogenic activities were contributing factors as the source of metal abundance in rivers of northern Jiangsu *** first major component represented the influence of anthropogenic activities,including industry and agriculture,with a contribution rate of 54.1%,affected Cr,Fe,Cu,Zn,Mo,Cd and *** second(such as V,Mn,Co,Ni,As)was a mixed source,including the natural processes such as precipitation,erosion and weathering and anthropogenic action like industry and agriculture,with a contribution rate of 37.1%.Seasonal variations in trace metal concentrations were influenced by temperature,salinity,water discharge,and input of external *** highest concentrations were found in wet season and were strongly influenced by rainfall and seasonal industrial and agricultural activities.

关键词： trace metal distribution rivers northern Jiangsu Province