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Nondestructive technique for identifying nuclides using neutron resonance transmission analysis at CSNS Back-n

Nuclear Science and Techniques 2024年第1期35卷 178-187页

作者： Sheng-Da Tang Yong-hao Chen Jing-Yu Tang Rui-Rui fan Qiang Li Gong Li Dong Liu Zheng-Yao Jin Xing-Zhu Cui Tian-Xiang Chen Yi-Wei Yang Rong Liu Han Yi Yang Li Zhen Yang Qi An hao-fan bai Jiang-Bo bai Jie Bao Ping Cao Qi-Ping Chen Zhen Chen Zeng-Qi Cui An-Chuan fan Chang-Qing Feng fan-Zhen Feng Ke-Qing Gao Min-hao Gu Chang-Cai Han Zi-Jie Han Guo-Zhu He Yong-Cheng He Yang Hong Yi-Wei Hu Han-Xiong Huang Wei-Hua Jia hao-yu Jiang Wei Jiang Zhi-jie Jiang Ling Kang Bo Li Chao Li Jia-Wen Li Xiao Li Jie Liu Shu-Bin Liu Guang-Yuan Luan Chang-Jun Ning Bin-Bin Qi Jie Ren Zhi-Zhou Ren Xi-Chao Ruan Zhao-Hui Song Kang Sun Zhi-Xin Tan Li-Jiao Wang Peng-Cheng Wang Zhao-Hui Wang Zhong-Wei Wen Xiao-Guang Wu Xuan Wu Li-Kun Xie Yong-Ji Yu Guo-Hui Zhang Lin-hao Zhang Mo-Han Zhang Qi-Wei Zhang Xian-Peng Zhang Yu-Liang Zhang Yue Zhang Zhi-Yong Zhang Mao-Yuan Zhao Lu-Ping Zhou Zhi-hao Zhou Ke-Jun Zhu Sino-French Institute of Nuclear Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China Institute of High-Energy Physics Chinese Academy of Sciences(CAS)Beijing 100049China Spallation Neutron Source Science Center Dongguan 523803China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Particle Detection and Electronics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China USTC Archaeometry Laboratory University of Science and Technology of ChinaHefei 230026China Institute of Nuclear Physics and Chemistry China Academy of Engineering PhysicsMianyang 621900China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China Northwest Institute of Nuclear Technology Xi’an 710024China University of Chinese Academy of Sciences Beijing 100049China

Nondestructive and noninvasive neutron assays are essential applications of neutron *** resonance transmission analysis(NRTA)is a powerful nondestructive method for investigating the elemental composition of an *** back-streaming neutron line(Back-n)is a newly built time-of-flight facility at the China Spallation Neutron Source(CSNS)that provides neutrons in the eV to 300 MeV range.A feasibility study of the NRTA method for nuclide identification was conducted at the CSNS Back-n via two test *** results demonstrate that it is feasible to identify different elements and isotopes in samples using the NRTA method at *** study reveals its potential future applications.

关键词： CSNS White neutron beam NRTA Nuclide identification Nondestructive method

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10B-doped MCP detector developed for neutron resonance imaging at Back-n white neutron source

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Nuclear Science and Techniques 2024年第8期35卷 58-68页

作者： Qiang Li Li‑Jiao Wang Jing‑Yu Tang Xiang‑Biao Qiu Zhen Chen Mao‑Yuan Zhao Chang‑Jun Ning Kai Pan Wei Xu Tao Li Su‑Peng Lu Han Yi Rui‑Rui fan Chang‑Qing Feng Rong Zhang Xiao‑Yang Sun Qi An hao‑fan bai Jiang‑Bo bai Jie Bao Ping Cao Qi‑Ping Chen Yong‑hao Chen Zeng‑Qi Cui An‑Chuan fan fan‑Zhen Feng Min‑hao Gu Chang‑Cai Han Zi‑Jie Han Guo‑Zhu He Yong‑Cheng He Yang Hong Yi‑Wei Hu Han‑Xiong Huang Wei Jiang Zhi‑Jie Jiang Zheng‑Yao Jin Ling Kang Bo Li Gong Li Xiao Li Yang Li Jie Liu Rong Liu Shu‑Bin Liu Yi‑Na Liu Guang‑Yuan Luan Jie Ren Zhi‑Zhou Ren Xi‑Chao Ruan Zhao‑Hui Song Kang Sun Zhi‑Xin Tan Sheng‑Da Tang Jin‑Cheng Wang Peng‑Cheng Wang Zhao‑Hui Wang Zhong‑Wei Wen Xiao‑Guang Wu Xuan Wu Cong Xia Yong‑Ji Yu Guo‑Hui Zhang Hang‑Chang Zhang Lin‑hao Zhang Qi‑Wei Zhang Xian‑Peng Zhang Yu‑Liang Zhang Yue Zhang Zhi‑Yong Zhang Zhi‑hao Zhou Ke‑Jun Zhu Chong Zou Institute of High Energy Physics Chinese Academy of Sciences(CAS)Beijing 100049China Spallation Neutron Source Science Center Dongguan 523803China State Key Laboratory of Particle Detection and Electronics Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Dongguan Songshan Lake Future School Dongguan 523808China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230027China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China North Night Vision Science and Technology(Nanjing)Research Institute Co.Ltd Nanjing 211106China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China Institute of Modern Physics Fudan UniversityShanghai 200433China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China China Academy of Engineering Physics Institute of Nuclear Physics and ChemistryMianyang 621900China USTC archaeometry lab University of Science and Technology of ChinaHefei 230026China Northwest Institute of Nuclear Technology Xi’an 710024China University of Chinese Academy of Sciences Beijing 100049China China Shipbuilding Trading Co. LtdBeijing 100044China

Neutron resonance imaging(NRI)has recently emerged as an appealing technique for neutron *** complexity surpasses that of conventional transmission imaging,as it requires a high demand for both a neutron source and ***,the progression of NRI technology has been sluggish since its inception in the 1980s,particularly considering the limited studies analyzing the neutron energy range above *** white neutron source(Back-n)at the China Spallation Neutron Source(CSNS)provides favorable beam conditions for the development of the NRI technique over a wide neutron energy range from eV to ***-sensitive microchannel plates(MCP)have emerged as a cutting-edge tool in the field of neutron detection owing to their high temporal and spatial resolutions,high detection efficiency,and low *** this study,we report the development of a 10B-doped MCP detector,along with its associated electronics,data processing system,and NRI experiments at the *** heavy elements such as gold,silver,tungsten,and indium can be easily identified in the transmission images by their characteristic resonance peaks in the 1–100 eV energy range;the more difficult medium-weight elements such as iron,copper,and aluminum with resonance peaks in the 1–100 keV energy range can also be *** particular,results in the neutron energy range of dozens of keV(Aluminum)are reported here for the first time.

关键词： Neutron resonance imaging 10B doped MCP detector White neutron source Sample nuclide identification

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Study of the response of 10B-doped MCP to wide-energy range neutrons from eV to MeV

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Nuclear Science and Techniques 2024年第8期35卷 132-141页

作者： Qiang Li Li‑Jiao Wang Xiang‑Biao Qiu Jing‑Wen Li Wei Xu Tao Li Ze‑Bin Lin Chang‑Jun Ning Yong‑hao Chen Rui‑Rui fan Kang Sun Jing‑Yu Tang Rong Zhang Han‑Tao Jing Bo Mei Qi An hao‑fan bai Jiang‑Bo bai Jie Bao Ping Cao Qi‑Ping Chen Zhen Chen Zeng‑Qi Cui An‑Chuan fan Chang‑Qing Feng fan‑Zhen Feng Ke‑Qing Gao Min‑hao Gu Chang‑Cai Han Zi‑Jie Han Guo‑Zhu He Yong‑Cheng He Yang Hong Yi‑Wei Hu Han‑Xiong Huang Wei‑Hua Jia hao‑Yu Jiang Wei Jiang Zhi‑Jie Jiang Zheng‑Yao Jin Ling Kang Bo Li Chao Li Gong Li Jia‑Wen Li Xiao Li Yang Li Jie Liu Rong Liu Shu‑Bin Liu Guang‑Yuan Luan Bin‑Bin Qi Jie Ren Zhi‑Zhou Ren Xi‑Chao Ruan Zhao‑Hui Song Zhi‑Xin Tan Sheng‑Da Tang Peng‑Cheng Wang Zhao‑Hui Wang Zhong‑Wei Wen Xiao‑Guang Wu Xuan Wu Li‑Kun Xie Yi‑Wei Yang Han Yi Yong‑Ji Yu Guo‑Hui Zhang Lin‑hao Zhang Mo‑Han Zhang Qi‑Wei Zhang Xian‑Peng Zhang Yu‑Liang Zhang Yue Zhang Zhi‑Yong Zhang Mao‑Yuan Zhao Lu‑Ping Zhou Zhi‑hao Zhou Ke‑Jun Zhu Institute of High Energy Physics Chinese Academy of Sciences(CAS)Beijing 100049China Spallation Neutron Source Science Center Dongguan 523803China State Key Laboratory of Particle Detection and Electronics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Dongguan Songshan Lake Future School Dongguan 523808China North Night Vision Science&Technology(Nanjing)Research Institute Co.Ltd. Nanjing 211106China Sino‑French Institute of Nuclear Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230027China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China Institute of Nuclear Physics and Chemistry China Academy of Engineering PhysicsMianyang 621900China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China USTC Archaeometry Lab University of Science and Technology of ChinaHefei 230026China Northwest Institute of Nuclear Technology Xi’an 710024China University of Chinese Academy of Sciences Beijing 100049China

Neutron-sensitive microchannel plates(nMCPs)have applications in neutron detection,including energy spectrum measurements,neutron-induced cross sections,and neutron imaging.10B-doped MCPs(B-MCPs)have attracted significant attention owing to their potential for exhibiting a high neutron detection efficiency over a large neutron energy *** spatial and temporal resolutions are useful for neutron energy-resolved ***,their practical applications still face many technical *** this study,a B-MCP with 10 mol%10B was tested for its response to wide-energy neutrons from eV to MeV at the Back-n white neutron source at the China Spallation Neutron *** neutron detection efficiency was calibrated at 1 eV,which is approximately 300 times that of an ordinary MCP and indicates the success of 10 B *** factors that caused the reduction in the detection efficiency were simulated and *** neutron energy spectrum obtained using B-MCP was compared with that obtained by other measurement methods,and showed very good consistency for neutron energies below tens of *** response is more complicated at higher neutron energy,at which point the elastic and nonelastic reactions of all nuclides of B-MCP gradually become *** is beneficial for the detection of neutrons,as it compensates for the detection efficiency of B-MCP for high-energy neutrons.

关键词： Neutron radiation image 10B-doped MCP Neutron response Wide-energy range neutrons

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Image Inpainting Technique Incorporating Edge Prior and Attention Mechanism

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Computers, Materials & Continua 2024年第1期78卷 999-1025页

作者： Jinxian bai Yao fan Zhiwei Zhao Lizhi Zheng College of Information Engineering Xizang Minzu UniversityXianyang712000China

Recently,deep learning-based image inpainting methods have made great strides in reconstructing damaged ***,these methods often struggle to produce satisfactory results when dealing with missing images with large holes,leading to distortions in the structure and blurring of *** address these problems,we combine the advantages of transformers and convolutions to propose an image inpainting method that incorporates edge priors and attention *** proposed method aims to improve the results of inpainting large holes in images by enhancing the accuracy of structure restoration and the ability to recover texture *** method divides the inpainting task into two phases:edge prediction and image ***,in the edge prediction phase,a transformer architecture is designed to combine axial attention with standard *** design enhances the extraction capability of global structural features and location *** also balances the complexity of self-attention operations,resulting in accurate prediction of the edge structure in the defective *** the image inpainting phase,a multi-scale fusion attention module is *** module makes full use of multi-level distant features and enhances local pixel continuity,thereby significantly improving the quality of image *** evaluate the performance of our *** experiments are conducted on several datasets,including CelebA,Places2,and *** experiments show that our method outperforms the other mainstream ***,it improves Peak Signal-to-Noise Ratio(PSNR)and Structure Similarity Index Measure(SSIM)by 1.141~3.234 db and 0.083~0.235,***,it reduces Learning Perceptual Image Patch Similarity(LPIPS)and Mean Absolute Error(MAE)by 0.0347~0.1753 and 0.0104~0.0402,*** experiments reveal that our method excels at reconstructing images with complete structural information and c

关键词： Image inpainting transformer edge prior axial attention multi-scale fusion attention

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Solvation strategies in various electrolytes for advanced zinc metal anode

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Journal of Energy Chemistry 2024年第7期94卷 740-757页

作者： Zhenxu Wang Lichong bai Hongguang fan Yanpeng Wang Wei Liu School of Materials Science and Engineering Ocean University of ChinaQingdao 266100ShandongChina

Aqueous zinc-ion batteries(AZIBs),known for their high safety,low cost,and environmental friendliness,have a wide range of potential applications in large-scale energy storage ***,the notorious dendrite growth and severe side reactions on the anode have significantly hindered their further practical *** studies have shown that the solvation chemistry in the electrolyte is not only closely related to the barriers to the commercialization of AZIBs,but have also sparked a number of valuable ideas to address the challenges of ***,we systematically summarize and discuss the regulatory mechanisms of solvation chemistry in various types of electrolytes and the influence of the solvation environment on battery *** challenges and future directions for solvation strategies based on the electrolyte environment are proposed to improve their performance and expand their application in AZIBs.

关键词： Solvation strategy Electrolyte Aqueous zinc-ion batteries Zinc dendrite

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Effect of surfactant frequently used in soil flushing on oxygen mass transfer in micro-nano-bubble aeration system

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Chinese Journal of Chemical Engineering 2024年第3期67卷 174-181页

作者： Mei bai Zhibin Liu Zhu Liu Chenfei He Zhanhuang fan Miaoxin Yuan Jiangsu Key Laboratory of Urban Underground Engineering and Environmental Safety Southeast UniversityNanjing 211189China CECEP DADI(Hangzhou)Environmental Remediation Co. Ltd.Hangzhou 310020China

In-site soil flushing and aeration are the typical synergetic remediation technology for contaminated *** surfactant present in flushing solutions is bound to affect the aeration *** purpose of this study is to evaluate the effect of surfactant frequently used in soil flushing on the oxygen mass transfer in micro-nano-bubble(MNB)aeration ***,bio-surfactants and chemical surfactants were used to investigate their effects on Sauter mean diameter of bubble(dBS),gas holdup(ε),volumetric mass-transfer coefficient(kLa)and liquid-side mass-transfer coefficient(kL)in the MNB aeration ***,based upon the experimental results,the Sardeing's and Frossling's models were modified to describe the effect of surfactant on kL in the MNB *** results showed that,for the twenty aqueous surfactant solutions,with the increase in surfactant concentration,the value of dBS,kLa and kL decreased,while the value ofεand gas-liquid interfacial area(a)*** phenomena were mainly attributed to the synergistic effects of immobile bubble surface and the suppression of coalescence in the surfactant *** addition,with the presence of electric charge,MNBs in anionic surfactant solutions were smaller and higher in number than in non-ionic surfactant ***,the accumulation of surfactant on the gas-liquid interface was more conspicuous for small MNB,so the reduction of kL in anionic surfactant solutions was larger than that in non-ionic surfactant ***,the modified Frossling's model predicted the effect of surfactant on kL in MNB aeration system with reasonable accuracy.

关键词： Soil flushing Micro-nano-bubble aeration Bio-surfactant Mass transfer coefficient

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Self-doping active sites in microbe-derived carbonaceous electrocatalysts for the oxygen reduction reaction performance

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Nano Research 2024年第8期17卷 6803-6819页

作者： Xiaofeng Xiao Xiaochun Tian Junpeng Li fan Yang Rui bai Feng Zhao Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China

Microorganisms are rich in heteroatoms,which can be self-doped to form active sites during pyrolysis and loaded on microbederived carbonaceous *** recent years,microbe-derived carbonaceous materials,characterized with abundant selfdoping sites,have been continuously developed as cost-effective electrocatalysts for oxygen reduction reaction(ORR).To fully unlock the catalytic potential of microbe-derived carbonaceous materials,a comprehensive analysis of catalytic sites and mechanisms for ORR is *** paper provides a summary of the ORR catalytic performance of microbe-derived carbonaceous materials reported to date,with a specific focus on the self-doping sites introduced during their pyrolytic *** highlights the mono-or co-doping sites involving nonmetallic elements such as oxygen(O),nitrogen(N),phosphorus(P),and sulfur(S)atoms,as well as covers the doping of metallic iron(Fe)atoms with various coordination configurations in microbe-derived carbonaceous *** the impact of these self-doping sites on ORR catalytic performance can guide the design of doping sites in microbe-derived carbonaceous *** approach has the potential to maximize electrocatalytic activity of microbe-derived carbonaceous materials and contributes to the development of more efficient and cost-effective carbonaceous electrocatalysts.

关键词： electrocatalysis heteroatoms self-doped single atom catalyst microbe-derived carbonaceous material

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FCF-LDH/BiVO4 with synergistic effect of physical enrichment and chemical adsorption for efficient reduction of nitrate

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Green Energy & Environment 2024年第7期9卷 1112-1121页

作者： Yajie bai Zhenyuan fang Yong Lei Lijing Liu Huaiquan Zhao Hongye bai Weiqiang fan Weidong Shi School of Chemistry and Chemical Engineering Jiangsu University School of Chemistry Beihang University Institute of Physics & IMN MacroNano Technische Universit?t Ilmenau

Photoelectrochemical NO3-reduction（PEC NITRR） not only provides a promising solution for promoting the global nitrogen cycle,but also converts NO3-to the important chemicals（NH3）.However,it is still a great challenge to prepare catalysts with excellent NO3-adsorption/activation capacity to achieve high ***,we designed a novel Fe2+～Cu2+Fe3+LDH/BiVO4（FCF-LDH/BVO） catalyst with synergistic effect of chemical adsorption and physical ***2+in FCF-LDH/BVO provides the rich Lewis acid sites for the adsorption of NO3-,and the appropriate layer spacing of FCF-LDH further promotes the physical enrichment of NO3-in its interior,thus realizing the effective contact between NO3-and active sites(Fe2+).FCF-LDH/BVO showed excellent NH3production performance(FENH3=66.1%,rNH3=13.8 μg h-1cm-2) and selectivity(FENO2-=2.5%,rNO2-=4.9 μg h-1cm-2) in 0.5 mol *** addition,FCF-LDH/BVO maintains the desirable PEC stability for six cycle experiments,showing great potential for practical ***14NO3-and15NO3-isotope test provides strong evidence for further verification of the origin of N in the generated *** LDH catalyst has a great potential in PEC removal of NO3-from groundwater.

关键词： LDH Lewis acid sites Physical enrichment Photoelectrochemical NO 3 − Reduction Ammonia

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Experimental and numerical analyses of the effect of fibre content on the close-in blast performance of a UHPFRC beam

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Defence Technology（防务技术） 2024年第1期31卷 242-261页

作者： Junbo Yan Qiyue Zhang Yan Liu Yingliang Xu Zhenqing Shi fan bai Fenglei Huang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

Limited research has been conducted on the influences of fiber content on close-in blasting characteristics for ultrahigh-performance fiber-reinforced concrete(UHPFRC)*** paper aims to address this knowledge gap through experimental and mesoscale numerical *** were conducted on ten UHPFRC beams built with varying steel fiber volumetric fractions subjected to close-in explosive ***,this study considered other parameters,such as the longitudinal reinforcement type and *** the case of UHPFRC beams featuring normal-strength longitudinal reinforcement of diametersΦ12,Φ16,andΦ20,a reduction in maximum displacement by magnitudes of19.6%,19.5%,and 17.4%was observed,respectively,as the volumetric fractions of fiber increased from1.0%to 2.5%.In addition,increasing the longitudinal reinforcement ratio and using high-strength steel longitudinal reinforcement both significantly reduced the deformation characteristics and increase the blasting resistances of UHPFRC ***,the effects on the local crushing and spalling damage were not significant.A mesoscale finite element model,which considers the impacts of fiber parameters on UHPFRC beam behaviors,was also established and well correlated with the test ***,parametric analyses were further conducted to examine the impacts of the steel fiber content and length and the hybrid effects of various types of microfibers and steel fibers on the blasting performance of UHPFRC beams.

关键词： Blast performance Close-in blast Fiber content Mesoscale approach UHPFRC beams

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Design of high-performance and sustainable Co-free Ni-rich cathodes for next-generation lithium-ion batteries

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SusMat 2024年第1期4卷 48-71页

作者： hao Ge Zhiwen Shen Yanhong Wang Zhijia Sun Xiaoman Cao Chaoyue Wang Xinyue fan Jinsong bai Rundong Li Tianhua Yang Gang Wu School of Energy and Environment Shenyang Aerospace UniversityShenyangP.R.China Shenyang Aircraft Airworthiness Certification Center of CAAC ShenyangP.R.China College of Chemistry and Materials Engineering Bohai UniversityJinzhouP.R.China Liaoning General Aviation Academy ShenyangP.R.China Department of Chemical and Biological Engineering University at BuffaloState University of New YorkBuffaloNew YorkUSA

Great attention has been given to high-performance and inexpensive lithiumion batteries(LIBs)in response to the ever-increasing demand for the explosive growth of electric vehicles(EVs).High-performance and low-cost Co-freeNi-rich layered cathodes are considered one of the most favorable candidates for nextgeneration LIBs because the current supply chain of EVs relies heavily on scarce and expensive ***,we review the recent research progress on Co-free Nirich layered cathodes,emphasizing on analyzing the necessity of replacing Co and the popular improvment *** current advancements in the design strategies of Co-free Ni-rich layered cathodes are summarized in *** considerable improvements achieved so far,the main technical challenges contributing to the deterioration of Co-free Ni-rich cathodes such as detrimental phase transitions,crack formation,and severe interfacial side reactions,are difficult to resolve by a single *** cooperation of multiple modification strategies is expected to accelerate the industrialization of Co-free Ni-rich layered cathodes,and the corresponding synergistic mechanisms urgently need to be *** effects will be aroused to explore high-performance Co-free Ni-rich layered cathodes to promote the sustainable development of LIBs.

关键词： Co-free cathodes electrochemical performance lithium-ion batteries modification strategies Ni-rich layered cathodes

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