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There is plenty of room at the top:generation of hot charge carriers and their applications in perovskite and other semiconductor-based optoelectronic devices

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Light(Science & Applications) 2021年第9期10卷 1630-1657页

作者： Irfan Ahmed Lei Shi hannu pasanen Paola Vivo Partha Maity Mohammad Hatamvand Yiqiang Zhan State Key Laboratory of ASIC and System Centre of Micro-Nano SystemSISTFudan University200433ShanghaiChina Department of Physics Government Postgraduate College(Higher Education Department-HED)Khyber Pakhtunkhwa21300MansehraPakistan State Key Laboratory of Surface Physics Key Laboratory of Micro-and Nano-PhotonicsFudan University200433ShanghaiChina Faculty of Engineering and Natural Sciences Tampere UniversityFI-33014TampereFinland KAUST Solar Center Division of Physical Science and EngineeringKing Abdullah University of Science and Technology(KAUST)Thuwal23955-6900RiyadhKingdom of Saudi Arabia

Hot charge carriers(HC)are photoexcited electrons and holes that exist in nonequilibrium high-energy states of photoactive *** cooling time and rapid extraction are the current challenges for the development of future innovative HC-based optoelectronic devices,such as HC solar cells(HCSCs),hot energy transistors(HETs),HC photocatalytic reactors,and lasing *** on a thorough analysis of the basic mechanisms of HC generation,thermalization,and cooling dynamics,this review outlines the various possible strategies to delay the HC cooling as well as to speed up their *** materials with slow cooling behavior,including perovskites and other semiconductors,are thoroughly *** addition,the opportunities for the generation of plasmon-induced HC through surface plasmon resonance and their technological applications in hybrid nanostructures are discussed in *** judiciously designing the plasmonic nanostructures,the light coupling into the photoactive layer and its optical absorption can be greatly enhanced as well as the successful conversion of incident photons to HC with tunable energies can also be ***,the future outlook of HC in optoelectronics is highlighted which will provide great insight to the research community.

关键词： optoelectronic charge plenty

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