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Spatial-temporal Evolution of the Urban-rural Coordination Relationship in Northeast China in 1990-2018

Chinese Geographical Science 2021年第3期31卷 429-443页

作者： wang Ying CHEN Xiaohong SUN Pingjun LIU hang HE Jiaxin College of Geographical Sciences Harbin Normal UniversityHarbin 150025China College of Geographical Sciences Southwest UniversityChongqing 400700China

To comprehensively understand the law of urban-rural relationship and propose scientific measures of urban-rural coordinated development in Northeast China,this study uses the coupling coordination degree model and geographically and temporally weighted regression(GTWR)model to analyze the spatial-temporal patterns and the corresponding driving mechanisms of its urban-rural coordination since *** results are as ***,the urban-rural coupling coordination degree in Northeast China was very low and improved slowly,but its stages of evolution is a good interpretation of the strategic arrangements of China's ***,the urban-rural coupling coordination degree in Northeast China had spatial differences and was characterized by central polarization,converging on urban agglomeration,which was high in the south and low in the ***,the gap between the north and south ***,the spatial-temporal evolution of the urban-rural coordination relationship in Northeast China was influenced by pulling from the central cities,pushing from rural transformation,and government *** influence intensity of the three mechanisms was weak,but the pulling from the central cities was stronger than that of the other two ***,the spatial difference between the three mechanisms determines the spatial pattern and its evolution of the urban-rural coordination relationship in Northeast ***,to promote the development of urban-rural coordination in Northeast China,it is essential to advance urban-rural economic correlation,enhance the government^role in regulating and guiding,and adopt different policies for each region in Northeast China.

关键词： urban-rural coordination relationship spatial-temporal evolution coupling coordination degree model geographically and temporally weighted regression(GTWR) Northeast China

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One-step solution combustion synthesis of micro-nano-scale porous Cu/CeO_(2)with enhanced photocatalytic properties

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Journal of Rare Earths 2023年第2期41卷 250-258页

作者： Zhichao Shang Yong Yu hang Yang Zhongxiang Yang Yang Xiao Xiaohong wang School of Materials Science and Physics China University of Mining and TechnologyXuzhou 221116China School of Chemical Engineering and Technology China University of Mining and TechnologyXuzhou 221116China Davidson School of Chemical Engineering Purdue UniversityWest LafayetteIN47907-2100USA

The Cu/CeO_(2)nanoporous composite material was prepared via a one-step and energy-saving method of solution combustion synthesis(SCS).The phase composition,surface morphology and optical characteristics of Cu/CeO_(2)were *** results show that the SCS products are composed of cubic fluorite CeO_(2)and *** to the generation and escape of gas during the synthetic reaction,the SCS CeO_(2)shows porous structure,in which the mesopores(diameter 10-17 nm)nest in the wall of large pores(diameter80-300 nm).X-ray photoelectron spectroscopy(XPS)outcomes indicate that the oxygen vacancy concentration of CeO_(2)increases(18.97%-30.93%)with the increase of Cu *** decoration of Cu greatly enhances the catalytic activity of CeO_(2)nanomaterials.30 wt%Cu/CeO_(2)composite material shows the best photocatalytic activities for the degradation of methyl orange(MO)(95.99%),which is about 4.3times that of CeO_(2)at the same time(120 min).UV-vis diffuse reflectance spectroscopy(DRS)results show that the semiconductor band gap is reduced with the addition of metallic Cu,which leads to the enhancement of photocatalytic *** free radical trapping experiments demonstrate that·O_(2)-and h+are the main active species in the photocatalytic degradation of *** on the above results,a hypothesized mechanism for enhanced photocatalysis of Cu/CeO_(2)nanomaterials was proposed:the porous structure provides more reactive sites and channels for mass transfer,and the presence of metallic Cu improves the oxygen vacancy concentration of CeO_(2)and then promotes charge-carrier separation,which helps enhance the photocatalytic performance of Cu/CeO_(2).

关键词： Solution combustion synthesis Cu/CeO_(2) Nanoporous material Photocatalyst Rare earths

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Heterocatalytic ethylene methoxycarbonylation via a pseudo-hydride pathway over Pt_(1)/MoS_(2)

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Science China Chemistry 2024年第8期67卷 2427-2428页

作者： Bo-hang Zhao Bin Zhang Institute of Molecular Plus Department of ChemistrySchool of ScienceTianjin UniversityTianjin 300072China

Ethylene (C2H4) methoxycarbonylation (EMC) with CO and methanol (CH3OH) to methyl propanoate (MP) is industrially important due to its 100% atom efficiency [1].However, the heavy reliance on homogeneous Pd-based catalysts and strong acid media over commercial EMC processes still causes economic and environmental concerns [2]. At present, supported single-atom catalysts (SACs) can serve as bridges for accessing homogeneous catalysts in traditional heterogeneous catalytic processes.

关键词： processes. catalytic hydride

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Thiophene-based conjugated microporous polymers:synthesis,characterization and efficient gas storage

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Science China Chemistry 2017年第8期60卷 1067-1074页

作者： Chao-Jing Sun Xue-Qian Zhao Peng-Fei wang Hua wang Bao-hang Han CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in Nanoscience National Center for Nanoseience and Technology Beijing 100190 China

A series of thiophene-based conjugated microporous polymers （ThPOPs） have been synthesized on the basis of ferric chloride-catalyzed oxidative coupling polymerization of muRi-thienyl monomers. The structures of ThPOPs were confirmed via solid-state t3C CP/MAS NMR spectroscopy and Fourier-transform infrared spectroscopy. The ThPOPs possess high porosities and their high Brunauer-Emmett-Teller specific surface area results vary between 350 and 1320mZg . The presence of abundant ultra-micronores at 0.50-0.63 nm allows ThPOPs efficient gas （carbon dioxide, methane, and hydrogen） adsorption.

关键词： conjugated porous organic polymers thiophene gas adsorption oxidative polymerization

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Deformation control criterion of shield tunnel under lateral relaxation of soft soil

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Frontiers of Structural and Civil Engineering 2023年第5期17卷 780-795页

作者： Shimin wang Xiaoyu PENG hang ZHOU Xuhu HE Anqi ZHOU Bing CHEN Key Laboratory of Transportation Tunnel Engineering Ministry of EducationSouthwest Jiaotong UniversityChengdu 610036China Guangdong Provincial Railway Construction Investment Group Co. LtdGuangzhou 510080China

Metro shield tunnels under the lateral relaxation of soil(LRS)are susceptible to significant lateral deformations,which jeopardizes the structural safety and ***,deformation control standards for such situations have not been clearly ***,based on a specific case,a model test is conducted to realize the LRS of a shield tunnel in a sandy stratum to reveal its effect on segment ***,a deformation control criterion is *** LRS is simulated by linearly reducing the loads applied to the lateral sides of the segment *** lateral unloading,the lateral earth pressure coefficient on the segment decreases almost exponentially,and the structural deformation is characterized by horizontal expansion at the arch haunches and vertical shrinkage at the arch vault and arch *** on the mechanical pattern of the segment structure and the acoustic emission,the deformation response of a segment can be classified into three stages:elastic and quasi-elastic,damage,and rapid deformation *** a shield tunnel with a diameter of approximately 6 m and under the lateral relaxation of sandy soil,when the ellipticity of the segment is less than 2.71%,reinforcement measures are not ***,the segment deformation must be controlled when the ellipticity is 2.71%to 3.12%;in this regard,an ellipticity of 3%can be used as a benchmark in similar engineering projects.

关键词： shield tunnel lateral relaxation of soil deformation control criterion of segment structure model test

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Bifunctional LiI additive for poly(ethylene oxide)electrolyte with high ionic conductivity and stable interfacial chemistry

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Journal of Energy Chemistry 2022年第8期31卷 218-224,I0007页

作者： Haonan wang Tianyi Hou hang Cheng Bowen Jiang Henghui Xu Yunhui Huang School of Materials Science and Engineering Huazhong University of Science and TechnologyWuhan 430000HubeiChina

The development of polymer-based solid-state batteries is severely limited by the low ionic conductivity of solid polymer electrolyte and the instable interface between polymer electrolyte and Li-metal *** this work,lithium iodide(LiI)as a bifunctional additive was introduced into the poly(ethylene oxide)(PEO)-based electrolyte to improve the ionic conductivity and to construct a stable interphase at the Li/PEO interface.I-anions offer a strong electrostatic interaction with hydrogen atoms on PEO chains(HPEO)and forming massive I–H bonds that cross-link PEO chains,decrease crystallinity of PEO,and thus improve Li~+interchain *** addition,LiI participates in the formation of an inorganic-rich interphase layer,which decreases the energy barrier of Li+transport across the interface and thus inhibits the growth of lithium *** a result,the composite PEO electrolyte with 2 wt%LiI(PEO-2 LiI)presents a very high ionic conductivity of 2.1×10^(-4) S cm-1 and a critical current density of 2.0 m A cm^(-2) at 45°*** symmetric cell with this PEO-2 LiI electrolyte exhibits a long-term cyclability over 600 h at 0.2 m A cm^(-2).Furthermore,solid-state LiFePO_(4) and LiNi_(0.8)Mn_(0.1)Co_(0.1)O_(2) batteries with the PEO-2 LiI electrolyte show an impressive electrochemical performance with outstanding cycling stability and rate capability at 45°C.

关键词： Solid-state battery LiI Electrostatic interaction Crystallinity Interface

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Generic load regulation strategy for enhancing energy efficiency of chiller plants

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Building Simulation 2024年第8期17卷 1273-1287页

作者： hang Wan Yuyang Gong Shengwei wang Yongjun Sun Tao Xu Gongsheng Huang Department of Architecture and Civil Engineering City University of Hong KongHong KongChina Department of Building Environment and Energy Engineering Hong Kong Polytechnic UniversityHong KongChina School of Civil Engineering Guangzhou UniversityGuangzhouChina Shenzhen Research Institute of City University of Hong Kong ShenzhenChina

In many chiller plants,high coefficient of performance(COP)is only achieved at a few favorable part load ratios(PLRs),while the COP is low at many other non-favorable *** address this issue,this study proposes a generic load regulation strategy that aims to maintain chiller plants operating at high COP,particularly under non-favorable *** is achieved by incorporating thermal energy storage(TES)units and timely optimizing the charging and discharging power of the integrated TES *** optimal charging and discharging power is determined by solving a dynamic optimization problem,taking into account the performance constraints of the TES units and the chiller *** provide an overview of the energy-saving potential of the proposed strategy,a comprehensive analysis was conducted,considering factors such as building load profiles,COP/PLR curves of chillers,and attributes of the TES *** analysis revealed that the proposed load regulation strategy has the potential to achieve energy savings ranging from 5.7%to 10.8%for chiller plants with poor COPs under unfavorable PLRs,particularly in buildings with significant load variations.

关键词： load regulation thermal energy storage chiller plants building energy efficiency

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Evaluating the accuracy of two satellite-based Quantitative Precipitation Estimation products and their application for meteorological drought monitoring over the Lake Victoria Basin,East Africa

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Geo-Spatial Information Science 2022年第3期25卷 500-518页

作者： Priyanko Das Zhenke Zhang hang Ren Center of African Studies Nanjing UniversityNanjingChina and School of Geographic and Oceanographic SciencesNanjing UniversityNanjingChina Center of African Studies Nanjing UniversityNanjingChina and School of Geographic and Oceanographic SciencesNanjing University Nanjing China Institute of Population Studies Nanjing University of Posts and TelecommunicationsNanjingJiangsu provinceChina

This study evaluates the high-resolution satellite estimated long-term precipitation data for monitor-ing the drought condition over the Lake Victoria Basin(LVB)from 1984 to *** Precipitation Indices(SPI)were used to capture the short,medium and long-term meteorological drought conditions at multiple time scales(i.e.3,6,and 12).For these,the following two primaries Quantitative Precipitation Estimation(QPEs)products were employed-1)Climate Hazards group Infra-Red Precipitation with Station(CHIRPS),and 2)the Precipitation Estimation from Remotely Sensed Information using Artificial Neural Network-Climate Data Record(PERSIANN-CDR).This dataset was compared based on the observation data obtained from the Climate Research Unit(CRU)over the nine selected regions surrounding lake *** performance of these two QPEs products was evaluated using seven statistical *** findings of this study indicate that the CHIRPS and PERSIANN-CDR datasets could capture the behavior of drought magnitude based on the time scale of SPI-3,SPI-6,*** results indicate that 2012 and 2017 are significant severe drought years in the recent decade over ***,the CHIRPS datasets provide good agreement(Correlation Coefficient(CC)=0.65)with observation,whereas PERSIANN-CDR present satisfactory results(CC=0.54).In addition,Hurst(H)exponent was used to predict the future drought trend and found that the CHIRPS performed well to predict the degree of drought ***,this study considers the CHIRPS product for near-real-time drought monitoring and PERSIANN-CDR for historical drought ***,the outcome from the H values is greater than 0.5,which indicates the future drought trend would be decreased over *** results are useful for developing the strategies for drought hazards and water resource management in LVB.

关键词： CHIRPS CRU hurst exponent PERSIANN-CDR SPI

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MOF-based materials facilitate efficient anaerobic digestion of organic wastes:integrating substrate bioavailability and microbial syntrophism

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 153-157页

作者： Haoyu Liu Ying Xu Xiang Chen Xiankai wang hang wang Xiaohu Dai State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China YANGTZE Eco-Environment Engineering Research Center China Three Gorges CorporationWuhan 430010China National Engineering Research Center of Eco-Environment Protection for Yangtze River Economic Belt Wuhan 430010China

Anaerobic digestion(AD)of organic waste(OW)for methane production is generally *** of AD systems with traditional materials(e.g.,electroconductive materials)is a current focus of research and has been reported to assist methanogenesis by enhancing the productivity of microbial metabolism among syntrophic *** in the AD of organic wastewater,in which microbial cells come into direct contact with the dissolved substrate,in the complex multiphase AD system of OW,low substrate bioavailability is an inevitable obstacle to microbial syntrophism for ***,we propose that improving substrate bioavailability and microbial syntrophism is a powerful strategy for ensuring material-assisted efficient AD of *** on the above considerations,metal-organic frameworks(MOFs),with their exceptionally high porosity,outstanding multi-functionality,and tuneable structures,have excellent potential for application in multiphase anaerobic systems of OW to integrate substrate bioavailability and microbial syntrophism and drive efficient *** addition,MOFs with designable and tuneable natures have great potential for use in identifying suitable materials for anaerobic systems for different types of OW via machine-learning technologies,thereby effectively enhancing methanogenesis from ***,the sustainable application of MOFs in AD and the corresponding environmental risks warrant further investigation.

关键词： Anaerobic digestion Methane production Biodegradability Functional materials Metal-organic frameworks

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Impact angle constrained fuzzy adaptive fault tolerant IGC method for Ski-to-Turn missiles with unsteady aerodynamics and multiple disturbances

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Journal of Systems Engineering and Electronics 2022年第5期33卷 1210-1226页

作者： GUO hang wang Zheng FU Bin CHEN Kang FU Wenxing YAN Jie Research Center for Unmanned System Strategy Development Northwestern Polytechnical UniversityXi’an 710072China Unmanned System Research Institute Northwestern Polytechnical UniversityXi’an 710072China

An impact angle constrained fuzzy adaptive fault tolerant integrated guidance and control method for Ski-to-Turn(STT)missiles subject to unsteady aerodynamics and multiple disturbances is *** aerodynamics appears when flight vehicles are in a transonic state or confronted with unstable ***,actuator failures and multisource model uncertainties are ***,the boundaries of these multisource uncertainties are assumed *** target is assumed to execute high maneuver movement which is unknown to the ***,impact angle constraint puts forward higher requirements for the interception accuracy of the integrated guidance and control(IGC)*** impact angle constraint and the precise interception are established as the object of the IGC ***,the boundaries of the lumped disturbances are estimated,and several fuzzy logic systems are introduced to compensate the unknown nonlinearities and ***,a series of adaptive laws are developed so that the undesirable effects arising from unsteady aerodynamics,actuator failures and unknown uncertainties could be ***,an impact angle constrained fuzzy adaptive fault tolerant IGC method with three loops is constructed and a perfect hit-to-kill interception with specified impact angle can be ***,the numerical simulations are conducted to verify the effectiveness and superiority of the proposed method.

关键词： integrated guidance and control(IGC) impact angle constraint unsteady aerodynamics fault tolerant control(FTC) actuator failures

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