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Achieving Narrowed Bandgaps and Blue-Light Excitability in Zero-Dimensional Hybrid Metal halide Phosphors via Introducing Cation-Cation Bonding

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Energy & Environmental Materials 2024年第1期7卷 294-300页

作者： Pengfei Fu Shining Geng Ruixiang Mi Ranyun Wu Guangya Zheng Binbin Su Zhiguo xia Guangda Niu jiang Tang Zewen xiao Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China The State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied TechniquesSchool of Materials Science and TechnologySouth China University of TechnologyGuangzhou 510640China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China

Zero-dimensional(0D)hybrid metal halides,which consist of organic cations and isolated inorganic metal halide anions,have emerged as phosphors with efficient broadband ***,these materials generally have too wide bandgaps and thus cannot be excited by blue light,which hinders their applications for efficient white light-emitting diodes(WLEDs).The key to achieving a blue-light-excitable 0D hybrid metal halide phosphor is to reduce the fundamental bandgap by rational chemical *** this work,we report two designed hybrid copper(I)iodides,(Ph_(3)MeP)_(2)Cu_(4)I_(6)and(Cy_(3)MeP)_(2)Cu_(4)I_(6),as blue-light-excitable yellow phosphors with ultrabroadband *** these compounds,the[Cu_(4)I_(6)]^(2-)anion forms an I6 octahedron centered on a cationic Cu_(4)*** strong cation-cation bonding within the unique cationic Cu_(4)tetrahedra enables significantly lowered conduction band minimums and thus narrowed bandgaps,as compared to other reported hybrid copper(I)*** ultrabroadband emission is attributed to the coexistence of free and self-trapped *** WLED using the[Cu_(4)I_(6)]^(2-)anion-based single phosphor shows warm white light emission,with a high luminous efficiency of 65 Im W^(-1)and a high color rendering index of *** work provides strategies to design narrow-bandgap 0D hybrid metal halides and presents two first examples of blue-light-excitable 0D hybrid metal halide phosphors for efficient WLEDs.

关键词： blue-light-excitable cation-cation bonding hybrid metal halide phosphor zero-dimensional

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Paleozoic Multi-Stage Magmatic Events Related to Proto-Tethys and Paleo-Tethys Evolution:Insights from Intrusive Rocks in the Eastern Altyn Orogen,NW China

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Journal of Earth Science 2024年第4期35卷 1130-1148页

作者： Jiyong Li Yanqing xia Xilong Zhang Haoyuan jiang Tianzhu Lei Yongchao Wang Yanhong Liu Shanpin Liu xiaobao Zhang Northwest Institute of Eco-Environment and Resources Chinese Academy of SciencesLanzhou730000China Key Laboratory of Petroleum Resources Gansu ProvinceLanzhou730000China University of Chinese Academy of Sciences Beijing100049China

Abundant mafic-felsic intrusions distributed in the Altyn Orogen record orogenic histories related to Proto-Tethys and Paleo-Tethys *** U-Pb dating of the intrusive rocks in the eastern Altyn Orogen identifies at least three major tectono-magmatic episodes,yielding ages of∼426,∼376–373 and∼269–254 *** first two emplacement episodes correspond to the post-collisional magmatism in the Altyn ***∼426 Ma granitoids possess adakitic characteristics coupled with enriched isotopes,suggesting that they originated from partial melting of thickened lower continental crust induced by upwelling asthenospheric mantle after slab break-off of the South Altyn Ocean ***,the∼376–373 Ma mafic-intermediate rocks and coeval granitoids represent a large thermal event that involved mantle melting with induced new juvenile lower continental crust melting in a post-collisional extensional ***,the∼254 Ma diabase dykes intruded into the∼269 Ma granitoids,which were related to the widespread Late Paleozoic magmatism resulting from Paleo-Tethys Ocean ***-collisional magmatism in the Altyn Orogen significantly enhances understanding of the tectono-magmatic evolution in the northern Tibetan *** penetrative influence of Paleo-Tethys Ocean subduction was more extensive than previously thought.

关键词： Proto-Tethys Paleo-Tethys Altyn Orogen multi-stage magmatic events magnetic cores

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Scheme Based on Multi-Level Patch Attention and Lesion Localization for Diabetic Retinopathy Grading

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Computer Modeling in Engineering & Sciences 2024年第7期140卷 409-430页

作者： Zhuoqun xia Hangyu Hu Wenjing Li Qisheng jiang Lan Pu Yicong Shu Arun Kumar Sangaiah School of Computer and Communication Engineering Changsha University of Science and TechnologyChangshaChina Hunan Province People’s Hospital(The First Affiliated Hospital of Hunan Normal University) ChangshaChina The First Affiliated Hospital of Guangxi Medical University NanningChina International Graduate Institute of AI National Yunlin University of Science and TechnologyYunlinChina Department of Electrical and Computer Engineering Lebanese American UniversityBayrutLebanon

Early screening of diabetes retinopathy(DR)plays an important role in preventing irreversible *** research has failed to fully explore effective DR lesion information in fundus ***,traditional attention schemes have not considered the impact of lesion type differences on grading,resulting in unreasonable extraction of important lesion ***,this paper proposes a DR diagnosis scheme that integrates a multi-level patch attention generator(MPAG)and a lesion localization module(LLM).Firstly,MPAGis used to predict patches of different sizes and generate a weighted attention map based on the prediction score and the types of lesions contained in the patches,fully considering the impact of lesion type differences on grading,solving the problem that the attention maps of lesions cannot be further refined and then adapted to the final DR diagnosis ***,the LLM generates a global attention map based on ***,the weighted attention map and global attention map are weighted with the fundus map to fully explore effective DR lesion information and increase the attention of the classification network to lesion *** paper demonstrates the effectiveness of the proposed method through extensive experiments on the public DDR dataset,obtaining an accuracy of 0.8064.

关键词： DDR dataset diabetic retinopathy lesion localization multi-level patch attention mechanism

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Synergistic effect of carbon nanotube and encapsulated carbon layer enabling high-performance SnS_2-based anode for lithium storage

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Journal of Energy Chemistry 2024年第10期97卷 700-709,I0015页

作者： Chunwei Dong Yongjin xia Zhijiang Su Zhihua Han Yang Dong Jingyun Chen Fei Hao Qiyao Yu Qing jiang Jiaye Ye National Instituteof Clean-and-Low-Carbon Energy Beijing 102209China Key Laboratory of Automobile Materials Ministry of EducationSchool of Materials Science and EngineeringJilin UniversityChangchun 130022JilinChina State Key Laboratory of Explosion Science and Technology School of Mechatronical EngineeringBeijing Institute of TechnologyBeijing 100081China School of Chemistry and Physics Faculty of ScienceQueensland University of Technology2 George StreetBrisbaneQLD 4000Australia Centre for Materials Science Queensland University of Technology2 George StreetBrisbaneQLD 4000Australia

Tin disulfide(SnS_(2)),due to large interlayer spacing and high theoretical capacity,is regarded as a prospective anode material for lithium-ion ***,the poor electron conductivity of SnS_(2) and huge volumetric change during the lithiation/delithiation process lead to a rapid capacity decay of the battery,hindering its *** address these issues,herein,SnS_(2) is in-situ grown on the surface of carbon nanotubes(CNT)and then encapsulated with a layer of porous amorphous carbon(CNT/SnS_(2)@C)by simple solvothermal and further carbonization *** synergistic effect of CNT and porous carbon layer not only enhances the electrical co nductivity of SnS_(2) but also limits the huge volumetric change to avoid the pulverization and detachment of SnS_(2).Density functional theo ry calculations show that CNT/SnS_(2)@C has high Li^(+)adsorption and lithium storage capacity achieving high reaction ***,cells with the CNT/SnS_(2)@C anode exhibit a high lithium storage capacity of 837mAh/g after 100 cycles at 0.1 A/g and retaining a capacity of 529.8 mAh/g under 1.0 A/g after 1000 *** study provides a fundamental understanding of the electrochemical processes and beneficial guidance to design high-performance SnS_(2)-based anodes for LIBs.

关键词： Lithium-ion batteries Porous amorphous carbon Carbon nanotubes SnS_(2)-based anode Density functional theory calculations

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Pathological BBB Crossing Melanin-Like Nanoparticles as Metal-Ion Chelators and Neuroinflammation Regulators against Alzheimer’s Disease

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Research 2024年第1期6卷 687-706页

作者： Qianqian Huang Chaoqing jiang Xue xia Yufan Wang Chenxing Yan xiaorong Wang Ting Lei xiaotong Yang Wenqin Yang Guo Cheng Huile Gao Key Laboratory of Drug-Targeting and Drug Delivery System of the Education Ministry West China School of PharmacySichuan UniversityChengdu 610041P.R.China Laboratory of Molecular Translational Medicine Center for Translational MedicineKey Laboratory of Birth Defects and Related Diseases of Women and Children(Sichuan University)Ministry of EducationDepartment of PediatricsWest China Second University HospitalSichuan UniversityChengdu 610041P.R.China

Inflammatory responses,manifested in excessive oxidative stress and microglia overactivation,together with metal ion-triggered amyloid-beta(Aβ)deposition,are critical hallmarks of Alzheimer’s disease(AD).The intricate pathogenesis causes severe impairment of neurons,which,in turn,exacerbates Aβaggregation and facilitates AD ***,multifunctional melanin-like metal ion chelators and neuroinflammation regulators(named PDA@K)were constructed for targeted treatment of *** this platform,intrinsically bioactive material polydopamine nanoparticles(PDA)with potent metal ion chelating and ROS scavenging effects were decorated with the KLVFF peptide,endowing the system with the capacity of enhanced pathological blood–brain barrier(BBB)crossing and lesion site accumulation via Aβ*** vitro and in vivo experiment revealed that PDA@K had high affinity toward Aβand were able to hitch a ride on Aβto achieve increased pathological BBB *** engineered PDA@K effectively mitigated Aβaggregate and alleviated neuroinflammation.

关键词： oxidative aggregation chelating

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TaCHP encoding C1-domain protein stably enhances wheat yield in saline-alkaline fields

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Journal of Integrative Plant Biology 2024年第2期66卷 169-171页

作者： Guilian xiao Minqin Wang xiaomeng Li Zhengning jiang Hongjian Zhang Derong Gao Boqiao Zhang Guangmin xia Mengcheng Wang The Key Laboratory of Plant Development andEnvironment Adaptation Biology Ministry of Education School of Life ScienceShandong UniversityQingdao 266237China Key Laboratory of Wheat Biology and GeneticImprovement for Low&Middle Yangtze Valley Ministry ofAgriculture Lixiahe Agricultural Institute of Jiangsu ProvinceYangzhou 225007China

Salt and saline-alkaline stress seriously threaten crop production and food security worldwide(Yang and Guo,2018).Identifying genes that confer tolerance to these conditions without yield penalty would help mitigate this problem through molecular breeding(Liang et al.,2023;Sahu and Liu,2023).Although numerous stress-tolerance genes have been identified,their application potential in molecular breeding has rarely been confirmed through multi-year and multi-site field trials.

关键词： breeding fir alkaline

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Highly efficient room temperature phosphorescent liquid crystalline polymer optical waveguides for advanced optoelectronics

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Science China Chemistry 2024年第10期67卷 3450-3457页

作者： Jie Li Yan Guan Wei xia Jin-Kang Chen jiang Huang Yi Chen Qi Lin Er-Qiang Chen He-Lou Xie Key Laboratory of Environmentally Friendly Chemistry and Application of Ministry of Education and Key Laboratory of Advanced Functional Polymer Materials of CollegesUniversities of Hunan Province and College of ChemistryXiangtan UniversityXiangtan 411105China School of Physics and Optoelectronics Xiangtan UniversityXiangtan 411105China Beijing National Laboratory for Molecular Sciences Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Active organic optical waveguide materials(OOWMs)incorporating room temperature phosphorescence(RTP)hold significant promise for diverse applications in photonic and optoelectronic *** this potential,realizing active RTP optical waveguides with large-sized ordered structures and minimal light loss remains a formidable *** address this issue,we present a groundbreaking thermoplastic active OOWM with low light loss,leveraging room temperature phosphorescent liquid crystalline polymer(LCP).This innovative material can be easily synthesized through the copolymerization of phosphorescent and liquid crystalline *** resulting RTP copolymer exhibits a nematic liquid crystal phase with a phosphorescence lifetime of approximately 0.15 ms and an afterglow duration of around 1 *** the excellent processability of LCP,we successfully produce meter-scale fibers via melt *** RTP LCP fibers,characterized by a high orientation of mesogens along the fiber axis,demonstrate superior light confinement and efficient light conduction compared to unoriented samples,resulting in a low optical loss coefficient of 0.13 dB/***,the thermal responsiveness of the RTP LCP optical waveguide enables its use as a photo *** pioneering work paves the way for the design of new OOWMs tailored for advanced photonics and optoelectronics devices.

关键词： room temperature phosphorescence liquid crystalline polymer active optical waveguide

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New Discovery of the Jinshui Tin Deposit in the Middle Section of the East Kunlun Orogenic Belt,Northwestern China:Mineralization Age and Exploration Significance

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Journal of Earth Science 2024年第4期35卷 1373-1377页

作者： Xingkai Zhang Shao-Yong jiang Hui-Min Su Wei Wang Qinglin xia Yunpeng Liu Shien Li State Key Laboratory of Geological Processes and Mineral Resources Collaborative Innovation Center for Exploration of Strategic Mineral ResourcesSchool of Earth ResourcesChina University of GeosciencesWuhan 430074China Third Geological Exploration Institute of Qinghai Nonferrous Geological and Mineral Exploration Bureau Xining 810000China

Tin,as one of the most important critical metals,has at-tracted great attention worldwide(jiang et al.,2023,2020).China has the largest amount of tin resources in the world,ac-counting for nearly one-fourth of the world’s total(jiang et al.,2020;Chen and Sheng,2015).Tin deposits in China mainly occur in the Nanling Range in southern China,the Sanjiang Basin in southwestern China,and the Great Xing’an Range in northeastern China,which account for 98%of the country’s tin resources,whereas tin deposits are relatively rare in north-western China(Ni et al.,2023;Chen et al.,2014,1992).

关键词： Middle northeastern southwestern

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Hydrogel dressings on neurotrophic keratitis in an experimental animal model

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International Journal of Ophthalmology(English edition) 2024年第8期17卷 1396-1402页

作者： Hua-Qin xia xiao-Dan jiang Yi-Fan Song Xue-Min Li Yan-Jie Tian Department of Ophthalmology Peking University Third HospitalBeijing 100191China Beijing Key Laboratory of Restoration of Damaged Ocular Nerve Peking University Third HospitalBeijing 100191China

AIM:To investigate the therapeutic effects of hydrogel dressings on neurotrophic keratitis in ***:Male Wistar rats,aged 42–56d,were randomly divided into control,experimental,and treatment groups,each consisting of five *** experimental and treatment groups underwent neurotrophic keratitis modeling in both *** successful modeling,biomedical hydrogels formed with polyvinyl alcohol and polyvinyl pyrrolidone were used in treatment group for *** irritation response and keratitis index scores,Schirmer’s test,tear film break-up time(BUT),sodium fluorescein staining,and hematoxylin and eosin(HE)staining were used to evaluate the effectiveness of the ***:The neurotrophic keratitis model was successfully established in rats with severe ophthalmic nerve injury,characterized by keratitis,ocular irritation,reduced tear secretion measured by decreased BUT and Schirmer test values,corneal epithelial loss,and disorganized collagen fibers in the stromal *** treatment with hydrogel dressings,significant improvements were observed in keratitis scores and ocular irritation symptoms in model *** the recovery of tear secretion,as measured by the Schirmer’s test,did not show statistical differences,BUT was significantly *** staining confirmed a reduction in the extent of corneal epithelial loss after *** staining revealed the restoration of the structural disorder in both the epithelial and stromal layers to a certain ***:Hydrogel dressing reduces ocular surface irritation,improves tear film stability,and promotes the repair and restoration of damaged epithelial cells by maintaining a moist and clean environment on the ocular surface in the rat model.

关键词： neurotrophic keratitis hydrogel corneal epithelial cells rat

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Improved Unit Commitment with Accurate Dynamic Scenarios Clustering Based on Multi-Parametric Programming and Benders Decomposition

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Energy Engineering 2024年第6期121卷 1557-1576页

作者： Zhang Zhi Haiyu Huang Wei Xiong Yijia Zhou Mingyu Yan Shaolian xia Baofeng jiang Renbin Su Xichen Tian State Grid Corporation of China Beijing100031China Central China Branch State Grid Corporation of ChinaWuhan430077China School of Electric and Electronic Engineering Huazhong University of Science and TechnologyWuhan430074China China Electric Power Research Institute Co. Ltd.Beijing100192China

Stochastic unit commitment is one of the most powerful methods to address uncertainty. However, the existingscenario clustering technique for stochastic unit commitment cannot accurately select representative scenarios,which threatens the robustness of stochastic unit commitment and hinders its application. This paper providesa stochastic unit commitment with dynamic scenario clustering based on multi-parametric programming andBenders decomposition. The stochastic unit commitment is solved via the Benders decomposition, which decouplesthe primal problem into the master problem and two types of subproblems. In the master problem, the committedgenerator is determined, while the feasibility and optimality of generator output are checked in these twosubproblems. Scenarios are dynamically clustered during the subproblem solution process through the multiparametric programming with respect to the solution of the master problem. In other words, multiple scenariosare clustered into several representative scenarios after the subproblem is solved, and the Benders cut obtainedby the representative scenario is generated for the master problem. Different from the conventional stochasticunit commitment, the proposed approach integrates scenario clustering into the Benders decomposition solutionprocess. Such a clustering approach could accurately cluster representative scenarios that have impacts on theunit commitment. The proposed method is tested on a 6-bus system and the modified IEEE 118-bus *** results illustrate the effectiveness of the proposed method in clustering scenarios. Compared withthe conventional clustering method, the proposed method can accurately select representative scenarios whilemitigating computational burden, thus guaranteeing the robustness of unit commitment.

关键词： Stochastic programming unit commitment scenarios clustering Benders decomposition multi-parametric programming

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